International Reference System Research Articles

Update of the BIPM comparison BIPM.RI(II)-K1.Zn-65 of activity measurements of the radionuclide 65Zn to include the 2015 result of the LNMRI-IRD (Brazil) and the 2018 result of the LNE-LNHB (France)

Main textSince 1977, 19 laboratories have submitted 22 samples of 65Zn to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)- K1.Zn-65. The LNMRI-IRD (Brazil) and the LNE-LNHB (France) are the latest participants in the comparison and the key comparison reference value (KCRV) has been updated. The degrees of equivalence between each equivalent activity measured in the SIR and the updated KCRV have been calculated and the results are given in the form of a table. A graphical representation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Cr-51 of activity measurements of the radionuclide 51Cr to include the 2012 result of the KRISS (Rep. of Korea), the 2022 result of the POLATOM (Poland), and to link the 2022 EURAMET.RI(II)-K2.Cr-51 comparison

Main textTwo new participations in the BIPM.RI(II)-K1.Cr-51 comparison have been added to the previous results and this has produced a revised value for the key comparison reference value (KCRV), calculated using the power-moderated weighted mean. A link has been made to the EURAMET.RI(II)-K2.Cr-51 comparison piloted by the POLATOM in 2022, who sent an ampoule from the EURAMET comparison to the International Reference System (SIR). The LNE-LNHB (France) used the EURAMET comparison to update its degree of equivalence. The degrees of equivalence between each equivalent activity measured in the SIR and the KCRV have been calculated and the results are given in the form of a table for the latest results in the BIPM.RI(II)-K1.Cr-51, and the linked EURAMET.RI(II)-K2.Cr-51. A graphical presentation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Ge-68 of activity measurements of the radionuclide 68Ge to include the 2021 result of the NIM (China)

Main textSince 2013, 6 laboratories have submitted 7 samples of 68Ge to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)-K1.Ge-68. Recently, the NIM (China) participated in the comparison and the key comparison reference value (KCRV) has been updated. The degrees of equivalencebetween each equivalent activity measured in the SIR or linked to the SIR from the CCRI(II)-K2.Ge-68 comparison and the updated KCRV have been calculated and the results are given in the form of a table. A graphical representation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Tb-161 of activity measurements of the radionuclide 161Tb to include the 2022 result of the NPL (United Kingdom)

Main textSince 2019, 2 laboratories have submitted 2 samples of 161Tb to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)-K1.Tb-161. Recently, the NPL (United Kingdom) participated in the comparison and the key comparison reference value (KCRV) has been evaluated for the first time. The degrees of equivalence between each equivalent activity measured in the SIR and the updated KCRV have been calculated and the results are given in the form of a table. A graphical representation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Liquid scintillation efficiencies, gamma-ray emission intensities, and half-life for Gd-153

Gadolinium-153 was standardized for activity by live-timed anticoincidence counting and an ampoule was submitted to the international reference system (SIR). Absolute emission intensities for the main γ rays were determined with calibrated high-purity germanium (HPGe) and lithium-drifted silicon (Si(Li)) detectors. A revised decay scheme is indicated, with no probability of direct electron capture to the 153Eu ground state. Triple-to-double coincidence ratio (TDCR) efficiency curves indicate that the revised decay scheme is consistent with experiment. Half-life measurements agree with a previous NIST determination and show no sensitivity to chemical environment.

A first step towards a national realisation of the international height reference system in Sweden with a comparison to RH 2000

Abstract The International Height Reference System (IHRS) was defined by the International Association of Geodesy in 2015. Since then, the international geodetic community has been working on the specification and establishment of its realisation, the International Height Reference Frame (IHRF). This frame will primarily be realised by geopotential numbers (or physical heights) in a sparse global reference network. In Sweden, only one such global station is planned. Regional and national realisations (or densifications) computed in accordance with the IHRS definition are needed to enable the best possible unification of height datums. The main purpose of this article is to make a case study for Sweden regarding the national realisation of IHRS and to investigate in what way preliminary IHRF differs from the current Swedish levelling-based realisation of the European Vertical Reference System, RH 2000. The two different quasigeoid models that we consider best over Sweden at the present time are used to compute the preliminary IHRS realisations in the study. The realisations are compared to each other and to RH 2000. It is shown that a very significant part of the difference to RH 2000 is due to the different postglacial land uplift epochs, permanent tide concepts, and zero levels. The standard deviation for the difference between one of the preliminary national IHRS realisations and RH 2000 is reduced from 75.5 to 19.2 mm after correction of the postglacial land uplift and permanent tide effects. The corresponding mean differences are –208.5 and –454.7 mm, respectively. The magnitude of the mean difference thus increases when the corrections in question are applied.

The international reference system for beta-particle emitting radionuclides: Validation through the pilot study CCRI(II)-P1.Co-60

The Bureau International des Poids et Mesures (BIPM) is developing a new transfer instrument to extend its centralized services for assessing the international equivalence of radioactive standards to new radionuclides. A liquid scintillation counter using the triple/double coincidence ratio method is being studied and tested in the CCRI(II)–P1.Co-60 pilot study. The pilot study, involving 13 participating laboratories with primary calibration capabilities, validated the approach against the original international reference system based on ionization chambers, which has been in operation since 1976. The results are in agreement and an accuracy suitable for purpose, below 5×10−4, is achieved. The pilot study also reveals an issue when impurities emitting low-energy electrons are present in the standard solution, which have a different impact on liquid scintillation counting compared to other primary measurement methods.

Activity standardization of 99mTc by digitizer-based 4πce(LS)-γ and 4πce(PC)-γ coincidence counting

An aqueous solution of 99mTc was standardized by means of 4πce(LS)-γ and 4πce(PC)-γ coincidence counting. The activity concentration was obtained by efficiency extrapolation relying on four different variation techniques. In both setups, fast digitizers were used for data acquisition. Detected events were recorded in list mode format, and their coincidence relationship was analyzed in the subsequent offline analysis. The combined result was used to participate in an international comparison using the Transfer Instrument of the International Reference System.

Determination of Earth rotation parameters by Beidou navigation satellite system

Earth Rotation Parameters (ERP) play an important role in astrometry, geophysics, and space geodesy. Beidou Navigation Satellite System (BDS) has three orbital types of satellites, i.e., Geostationary orbit (GEO), Inclined Geosynchronous Orbit (IGSO), and Medium Earth Orbit (MEO) satellites. The orbital diversity of BDS constellation provides the opportunity to study the influence of system-specific satellite constellation with different orbital characteristic on ERP. In this article, different strategies of ERP estimation are conducted in terms of different solar radiation pressure (SRP) models and different orbital types of satellites. For ERP derived from BDS MEO observations, compared with C04 products from International Earth Rotation and Reference System Service, the results show that the accuracy of ERP with extended Empirical CODE Orbit Model (ECOM) with 9 parameters (ECOM2) outperforms other SRP models (e.g., ECOM with 5 parameters (ECOM1) and ECOM1 with an empirical prior model (EMP + ECOM1)). In EMP + ECOM1 solutions, the application of a prior EMP model would intensify the influence of draconitic year in pole coordinates spectrum, while the visible signal of a period close to 7.4 days with ECOM1 solution can be mitigated. Moreover, the bias of B0 parameter in EMP + ECOM1 would cause a mean offset in Length Of Day (LOD). The accuracy of ERP is also affected by the BDS constellation characteristic. For pole coordinate, MEO-only solution with ECOM2 model shows the best accuracy, while the LOD achieves the best solution when 3 orbital types are employed. Additionally, using the combined constellation of MEO, IGSO, and GEO satellites can decorrelate some of the systematic signals, e.g., the spurious signals of LOD at 2.35-day and 3.5-day in MEO-only solutions are reduced. Likewise, the increase of orbital planes can reduce the amplitude of 3 cycles per draconitic year (close to 121 days) in the pole coordinate spectrum, which is the main error source in pole coordinates estimated from BDS MEO constellation. However, some signals around 10 ∼ 24, 33– and 50-day are found in the Y-pole coordinate and its rate.

Update of the BIPM comparison BIPM.RI(II)-K1.I-131 of activity measurements of the radionuclide 131I to include the 2015 results of the BEV (Austria) and the POLATOM (Poland), the 2017 result of the NMISA (South Africa), and to link the CCRI(II)-S6.I-131 comparison

Main textThree new participations in the BIPM.RI(II)-K1.I-131 comparison have been added to the previous results and this has produced a revised value for the key comparison reference value (KCRV), calculated using the power-moderated weighted mean. A link has been made to the CCRI(II)-S6.I-131 comparison piloted by the International Atomic Energy Agency (IAEA) in 2006, based on the participation of CMI-IIR in both comparisons. One NMI used the S6 comparison to update its degree of equivalence. The results of two NMIs in the CCRI(II)-S6.I-131 comparison were superseded by a more recent APMP.RI(II)-K2.I-131 comparison. The degrees of equivalence between each equivalent activity measured in the International Reference System (SIR) and the KCRV have been calculated and the results are given in the form of a table for the latest results in the BIPM.RI(II)-K1.I-131, and the linked CCRI(II)-S6.I-131, APMP.RI(II)-K2.I-131 and EURAMET.RI(II)-K2.I-131 comparisons. A graphical presentation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Na-22 of activity measurements of the radionuclide 22Na to include the 2022 result of the NMISA (South Africa)

Main textSince 1976, 13 laboratories have submitted 30 samples of 22Na to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)-K1.Na-22. Recently, the NMISA (South Africa) participated in the comparison and the key comparison reference value (KCRV) has been updated. The degrees of equivalence between each equivalent activity measured in the SIR and the updated KCRV have been calculated and the results are given in the form of a table. A graphical representation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Activity measurements of the radionuclides 18F, 64Cu, 99mTc and 11C for the NRC, Canada, in the ongoing comparisons BIPM.RI(II)-K4 series and KCRV update in the corresponding BIPM.RI(II)-K1 comparison

Main textIn 2017, comparisons of activity measurements of 18F, 64Cu, 99mTc and 11C using the Transfer Instrument of the International Reference System (SIRTI) took place at the National Research Council of Canada (NRC, Canada). Ampoules containing 18F, 64Cu, 99mTc and 11C solutions were measured in the SIRTI for about three half-lives (10 half-lives for 11C). The NRC standardized the activity in the ampoules by 4π(PC)β−γ anti-coincidence measurements (CIEMAT/NIST liquid scintillation counting for 11C). The comparisons, identifiers BIPM.RI(II)-K4.F-18, BIPM.RI(II)-K4.Cu-64 and BIPM.RI(II)-K4.Tc-99m are linked to the corresponding BIPM.RI(II)-K1.F-18, BIPM.RI(II)-K1.Cu-64 and BIPM.RI(II)-K1.Tc-99m comparisons. The BIPM.RI(II)-K1 18F and 99mTc key comparison reference values have been updated to include the latest BIPM.RI(II)-K4 linked results and degrees of equivalence for those three comparisons have been evaluated.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Activity measurements of the radionuclides 18F, 64Cu and 99mTc for the ANSTO, Australia, in the ongoing comparisons BIPM.RI(II)-K4 series and KCRV update in the corresponding BIPM.RI(II)-K1 comparison

Main textIn 2017, comparisons of activity measurements of 18F, 64Cu, 99mTc and 11C using the Transfer Instrument of the International Reference System (SIRTI) took place at the Australian Nuclear Science and Technology Organisation (ANSTO, Australia). Ampoules containing 18F, 64Cu and 99mTc solutions were measured in the SIRTI for about 1.7 to 4 half-lives. The ANSTO carried out the primary standardization of the activity in the ampoules by 4π(LS)β—γ coincidence measurements. The comparisons, identifiers BIPM.RI(II)-K4.F-18, BIPM.RI(II)-K4.Cu-64 and BIPM.RI(II)-K4.Tc-99m are linked to the corresponding BIPM.RI(II)-K1.F-18, BIPM.RI(II)-K1.Cu-64 and BIPM.RI(II)-K1.Tc-99m comparisons. The BIPM.RI(II)-K1 18F and 99mTc key comparison reference values have been updated to include the latest BIPM.RI(II)-K4 linked results and degrees of equivalence for those three comparisons have been evaluated.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Co-60 of activity measurements of the radionuclide 60Co to include the 2020 result of the PTB (Germany), the 2020 result of the NIST (United States), the 2020 result of the SMU (Slovakia), the 2021 result of the BARC (India), the 2021 result of the LNE-LNHB (France), the 2021 result of the POLATOM (Poland), the 2021

Main textSince 1976, 30 laboratories have submitted 85 samples of 60Co to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)-K1.Co-60. Recently, the PTB (Germany), the NIST (United States), the SMU (Slovakia), the BARC (India), the LNE-LNHB (France), the POLATOM (Poland), the ENEA-INMRI (Italy), the NPL (United Kingdom), the LNMRI-IRD (Brazil), the NMISA (South Africa) and the ANSTO (Australia) participated in the comparison and the key comparison reference value (KCRV) has been updated. The degrees of equivalence between each equivalent activity measured in the SIR and the updated KCRV have been calculated and the results are given in the form of a table. A graphical representation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Lu-177 of activity measurements of the radionuclide 177Lu to include the 2013 result of the IFIN-HH (Romania), the 2014 result of the LNE-LNHB (France) and the 2022 result of the IRA (Switzerland)

Main text Since 2000, 7 laboratories have submitted 7 samples of 177Lu to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)-K1.Lu-177. Recently, the IFIN-HH (Romania), the LNE-LNHB (France) and the IRA (Switzerland) participated in the comparison. The degrees of equivalence between each equivalent activity measured in the SIR or linked to the SIR from the CCRI(II)-K2.Lu-177 comparison have been calculated. The results are given in the form of a table and a graphical representation is also displayed. To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/. The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Cs-134 of activity measurements of the radionuclide 134Cs to include the 2014 result of the POLATOM (Poland), the 2014 result of the NRC (Canada), the 2015 result of the LNMRI-IRD (Brazil) and the 2016 result of the PTB (Germany)

Main textSince 1976, 23 laboratories have submitted 44 samples of 134Cs to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)-K1.Cs-134. In the last few years, the POLATOM (Poland), the NRC (Canada), the LNMRI-IRD (Brazil) and the PTB (Germany) participated in the comparison and the key comparison reference value (KCRV) has been updated. The degrees of equivalence between each equivalent activity measured in the SIR or linked to the SIR from the APMP.RI(II)-K2.Cs-134 comparison and the updated KCRV have been calculated and the results are given in the form of a table. A graphical representation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Ac-225 of activity measurements of the radionuclide 225Ac to include the 2021 result of the POLATOM (Poland)

Main textSince 2019, 2 laboratories have submitted 2 samples of 225Ac to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)-K1.Ac-225. Recently, the POLATOM (Poland) participated in the comparison and a key comparison reference value (KCRV) has been calculated. For the first time, the degrees of equivalence between each equivalent activity measured in the SIR have been calculated and the results are given in the form of a table. A graphical presentation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Ra-223 of activity measurements of the radionuclide 223Ra to include the 2021 result of the POLATOM (Poland)

Main textSince 2014, 4 laboratories have submitted 4 samples of 223Ra to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)-K1.Ra-223. Recently, the POLATOM (Poland) participated in the comparison and the key comparison reference value (KCRV) has been updated. The degrees of equivalence between each equivalent activity measured in the SIR and the updated KCRV have been calculated and the results are given in the form of a table. A graphical presentation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Update of the BIPM comparison BIPM.RI(II)-K1.Y-88 of activity measurements of the radionuclide 88Y to include the 2016 result of the LNE-LNHB (France) and the 2019 result of the BEV (Austria)

Main textSince 1976, 15 laboratories have submitted 39 samples of 88Y to the International Reference System (SIR) for activity comparison at the Bureau International des Poids et Mesures (BIPM), with comparison identifier BIPM.RI(II)-K1.Y-88. Recently, the LNE-LNHB (France) and the BEV (Austria) participated in the comparison and the key comparison reference value (KCRV) has been updated. The degrees of equivalence between each equivalent activity measured in the SIR and the updated KCRV have been calculated and the results are given in the form of a table. A graphical presentation is also given.To reach the main text of this paper, click on Final Report. Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/.The final report has been peer-reviewed and approved for publication by the CCRI, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

The new international reference system for pure α- and pure β-emitting radionuclides and some electron capture decaying radionuclides by liquid scintillation counting

The new international reference system for pure α- and pure β-emitting radionuclides and some electron capture decaying radionuclides by liquid scintillation counting