The Yangtze (Changjiang River) Delta serves as a prominent depocenter for siliciclastic sediments from the Tibetan Plateau and Yangtze Craton, providing essential data on sediment source-to-sink dynamics and geomorphological evolution of large river drainage systems. This study presents the detrital zircon geochronology of Plio–Pleistocene sediments in the Yangtze Delta, alongside the data from modern river sediments, to elucidate provenance evolution since the Pliocene. The zircon geochronology reveals a considerable shift in sediment provenance during the Pliocene–Pleistocene transition. The Pliocene sediments exhibit a straightforward and predominant zircon age spectrum characterized by a typical peak age of 100–200 Ma. This spectrum markedly differs from the modern upper–middle Yangtze River sediments but closely resembles those of local rivers in the lower Yangtze River region. This demonstrates that the Pliocene sediments originated from local mountainous rivers, indicating the paleo-Yangtze River channelization prior to the Quaternary. In contrast, the zircon age spectra of Pleistocene sediments in the present-day delta reveal several dominant age groups ranging from 11.9 ± 1 to 3643 ± 30 Ma, similar to those found in present-day upper–middle Yangtze River sediments. This implies that the Pleistocene sediments were mainly derived from the upper–middle Yangtze River, showing a diversity of source rocks with varying geological ages and origins. The presence of the upper Yangtze River provenance signal, characterized by Cenozoic (<65 Ma) zircons, in early Pleistocene strata (ca. 1.6 Ma) of the delta suggests that the paleo-Yangtze River transported Tibet-sourced sediments into the modern delta area no later than that time. These findings indicate the geomorphological evolution of the Yangtze River Delta from an intermontane basin in the Pliocene to an alluvial–fluvial plain during the Quaternary. This geomorphological and geographic evolution, along with changes in sediment source, directly reflect extensive tectonic subsidence in eastern China since the late Cenozoic.