Integration Of Quantum Emitters Research Articles

Top-down integration of an hBN quantum emitter in a monolithic photonic waveguide

Integrated quantum photonics, with potential applications in quantum information processing, relies on the integration of quantum emitters into on-chip photonic circuits. Hexagonal boron nitride (hBN) is recognized as a material that is compatible with such implementations, owing to its relatively high refractive index and low losses in the visible range, together with advantageous fabrication techniques. Here, we combine hBN waveguide nanofabrication with the recently demonstrated local generation of quantum emitters using electron irradiation to realize a fully top-down elementary quantum photonic circuit in this material, operating at room temperature. This proof of principle constitutes a first step toward deterministic quantum photonic circuits in hBN.

Chiral topological add–drop filter for integrated quantum photonic circuits

The integration of quantum emitters within topological nanophotonic devices enables the control of light–matter interactions at the single photon level. Here, we experimentally realize an integrated topological add–drop filter and observe multiport chiral emission from single photon emitters (quantum dots) embedded within the device. The filter is imprinted within a valley-Hall photonic crystal membrane and comprises a resonator evanescently coupled to a pair of access waveguides. We show that the longitudinal modes of the resonator enable the filter to perform wavelength-selective routing of light, protected by the underlying topology. Furthermore, we demonstrate that for a quantum dot located at a chiral point in the resonator, selective coupling occurs between well-defined spin states and specific pairs of the filter output ports. The combination of multiport routing, allied with the inherent nonreciprocity of the device at the single photon level, presents opportunities for the formation of complex quantum optical devices, such as an on-chip quantum optical circulator.

(Invited) Opportunities and Challenges for Quantum Emitters in One and Two Dimensional Materials

The last five years have witnessed dramatic advances in realization of quantum emitters (QEs) in one dimensional carbon nanotubes and two dimensional layered semiconductors. These novel QEs offer exciting opportunities for not only storing, processing and transducing of quantum information but also sensing physical phenomena beyond classical detection limits. Realization of these opportunities also present multiple challenges including: (1) realizing room temperature, telecommunication wavelength operation; (2) controlling fundamental as well as quantum optical properties such as QE emission wavelengths, linewidths, polarization, coherent times, single photon purity and indistinguishability; (3) deterministic placement and integration of QEs into photonic, plasmonic, and mangnonic platforms for quantum sensing and transduction applications. Here in this talk I will present recent efforts toward meeting these challenges. In 1D carbon nanotubes, we recently demonstrated that chemical binding configuration of covalent quantum defects can be controlled through the spin multiplicity of photoexcited intermediates. This enable us to control the emission wavelength of QEs by creating previously inaccessible chemical configuration. In 2D semiconductor, we have successfully created the telecommunication wavelength quantum emitters by local strain engineering of MoTe2. We have also realized chiral quantum emitters via exploit of magnetic proximity interaction between quantum emitters of WSe2 monolayer and localized magnetization crated in NiPS3 anti-ferromagnetic insulator by nanoscale stain engineering.

Hybridization of epsilon-near-zero modes via resonant tunneling in layered metal-insulator double nanocavities

Abstract The coupling between multiple nanocavities in close vicinity leads to the hybridization of their modes. Stacked metal-insulator-metal (MIM) nanocavities constitute a highly versatile and very interesting model system to study and engineer such mode coupling, as they can be realized by lithography-free fabrication methods with fine control on the optical and geometrical parameters. The resonant modes of such MIM cavities are epsilon-near-zero (ENZ) resonances, which are appealing for nonlinear photophysics and a variety of applications. Here, we study the hybridization of ENZ resonances in MIMIM nanocavities, obtaining a very large mode splitting reaching 0.477 eV, Q-factors of the order of 40 in the visible spectral range, and fine control on the resonance wavelength and mode linewidth by tuning the thickness of the dielectric and metallic layers. A semiclassical approach that analyzes the MIMIM structure as a double quantum well system allows to derive the exact analytical dispersion relation of the ENZ resonances, achieving perfect agreement with numerical simulations and experiments. Interestingly, the asymmetry of the mode splitting in a symmetric MIMIM cavity is not reflected in the classical model of coupled oscillators, which can be directly related to quantum mechanical tunneling for the coupling of the two cavities. Interpreting the cavity resonances as resonant tunneling modes elucidates that they can be excited without momentum matching techniques. The broad tunability of high-quality ENZ resonances together with their strong coupling efficiency makes such MIMIM cavities an ideal platform for exploring light-matter interaction, for example, by the integration of quantum emitters in dielectric layers.

Integration of quantum dots with lithium niobate photonics

The integration of quantum emitters with integrated photonics enables complex quantum photonic circuits that are necessary for photonic implementation of quantum simulators, computers, and networks. Thin-film lithium niobate is an ideal material substrate for quantum photonics because it can tightly confine light in small waveguides and has a strong electro-optic effect that can switch and modulate single photons at low power and high speed. However, lithium niobate lacks efficient single-photon emitters, which are essential for scalable quantum photonic circuits. We demonstrate deterministic coupling of single-photon emitters with a lithium niobate photonic chip. The emitters are composed of InAs quantum dots embedded in an InP nanobeam, which we transfer to a lithium niobate waveguide with nanoscale accuracy using a pick-and-place approach. An adiabatic taper transfers single photons emitted into the nanobeam to the lithium niobate waveguide with high efficiency. We verify the single photon nature of the emission using photon correlation measurements performed with an on-chip beamsplitter. Our results demonstrate an important step toward fast, reconfigurable quantum photonic circuits for quantum information processing.

Direct laser written polymer waveguides with out of plane couplers for optical chips

Optical technologies call for waveguide networks featuring high integration densities, low losses, and simple operation. Here, we present polymer waveguides fabricated from a negative tone photoresist via two-photon-lithography in direct laser writing, and show a detailed parameter study of their performance. Specifically, we produce waveguides featuring bend radii down to 40 μm, insertion losses of the order of 10 dB, and loss coefficients smaller than 0.81 dB mm−1, facilitating high integration densities in writing fields of 300 μm×300 μm. A novel three-dimensional coupler design allows for coupling control as well as direct observation of outputs in a single field of view through a microscope objective. Finally, we present beam-splitting devices to construct larger optical networks, and we show that the waveguide material is compatible with the integration of quantum emitters.

Tunable negative permeability in a quantum plasmonic metamaterial

We consider the integration of quantum emitters into a negative permeability metamaterial design in order to introduce tunability as well as nonlinear behavior. The unit cell of our metamaterial is a ring of metamolecules, each consisting of a metal nanoparticle and a two-level semiconductor quantum dot (QD). Without the QDs, the ring of the unit cell is known to act as an artificial optical magnetic resonator. By adding the QDs we show that a Fano interference profile is introduced into the magnetic field scattered from the ring. This induced interference is shown to cause an appreciable effect in the collective magnetic resonance of the unit cell. We find that the interference provides a means to tune the response of the negative permeability metamaterial. The exploitation of the QD's inherent nonlinearity is proposed to modulate the metamaterial's magnetic response with a separate control field.