Integrated Quantum Optics Research Articles

Topological and conventional nanophotonic waveguides for directional integrated quantum optics

Directionality in integrated quantum photonics has emerged as a promising route towards achieving scalable quantum technologies with nonlinearities at the single-photon level. Topological photonic waveguides have been proposed as a novel approach to harnessing such directional light-matter interactions on-chip. However, uncertainties remain regarding the strength of the directional coupling of embedded quantum emitters to topological waveguides in comparison to conventional line defect waveguides. In this work we present an investigation of directional coupling in a range of waveguides using a combination of experimental, theoretical, and numerical analyses. We quantitatively characterize the position dependence of the light-matter coupling on several topological photonic waveguides and benchmark their directional coupling performance against conventional line defect waveguides. We conclude that topological waveguides underperform in comparison to conventional line defect waveguides, casting their directional optics credentials into doubt. To demonstrate this is not a question of the maturity of the field; we show that state-of-the-art inverse design methods, while capable of improving the directional emission of these topological waveguides, still place them significantly behind the operation of a conventional (glide-plane) photonic crystal waveguide. Our results and conclusions pave the way towards improving the implementation of quantitatively predicted quantum nonlinear effects on-chip. Published by the American Physical Society 2024

Superconducting nanowire single-photon detectors with saturated quantum efficiency at 1550 nm on single-crystal diamond substrates

Single-crystal diamond possesses exceptional physical and optical properties, rendering it an ideal platform for integrated quantum optics. The direct integration of broadband-sensitive and high-performance single-photon detectors on diamond holds significant implications for the realization of integrated diamond quantum optical circuits. In this study, we polished the diamond surface with RMS (root mean square) below 0.6 nm suitable for the deposition and patterning of NbN thin films through ion beam etching. Subsequently, we fabricated superconducting nanowire single-photon detectors directly on the polished diamond substrates and characterized for their electrical and optical properties. The NbN-SNSPD exhibited a high critical current density (2 MA cm−2), a saturated quantum efficiency (QE) below 2.5 K, and a maximum value of QE up to 88% at 4 K. These findings offer a promising solution for fully integrated quantum optical chips on single-crystal diamond substrates.

Pyroelectric influence on lithium niobate during the thermal transition for cryogenic integrated photonics

Lithium niobate has emerged as a promising platform for integrated quantum optics, enabling efficient generation, manipulation, and detection of quantum states of light. However, integrating single-photon detectors requires cryogenic operating temperatures, since the best performing detectors are based on narrow superconducting wires. While previous studies have demonstrated the operation of quantum light sources and electro-optic modulators in LiNbO3 at cryogenic temperatures, the thermal transition between room temperature and cryogenic conditions introduces additional effects that can significantly influence device performance. In this paper, we investigate the generation of pyroelectric charges and their impact on the optical properties of lithium niobate waveguides when changing from room temperature to 25 K, and vice versa. We measure the generated pyroelectric charge flow and correlate this with fast changes in the birefringence acquired through the Sénarmont-method. Both electrical and optical influence of the pyroelectric effect occur predominantly at temperatures above 100 K.

The Influence of Deposition Temperature and Material Stress on Low-Loss Silicon Nitride Films for Integrated Quantum Optics

The Influence of Deposition Temperature and Material Stress on Low-Loss Silicon Nitride Films for Integrated Quantum Optics

Demonstration of Hong-Ou-Mandel interference in an LNOI directional coupler.

Interference between single photons is key for many quantum optics experiments and applications in quantum technologies, such as quantum communication or computation. It is advantageous to operate the systems at telecommunication wavelengths and to integrate the setups for these applications in order to improve stability, compactness and scalability. A new promising material platform for integrated quantum optics is lithium niobate on insulator (LNOI). Here, we realise Hong-Ou-Mandel (HOM) interference between telecom photons from an engineered parametric down-conversion source in an LNOI directional coupler. The coupler has been designed and fabricated in house and provides close to perfect balanced beam splitting. We obtain a raw HOM visibility of (93.5 ± 0.7) %, limited mainly by the source performance and in good agreement with off-chip measurements. This lays the foundation for more sophisticated quantum experiments in LNOI.

Robust Directional Couplers for State Manipulation in Silicon Photonic-Integrated Circuits

Photonic integrated circuits play a central role in current and future applications such as communications, sensing, ranging, and information processing. Photonic quantum computing will also likely require an integrated optics architecture for improved stability, scalability, and performance. Fault-tolerant quantum computing mandates very accurate and robust quantum gates. In this work, we demonstrate high-fidelity directional couplers for single-qubit gates in photonic integrated waveguides, utilizing a novel scheme of detuning-modulated composite segments. Specific designs for reduced sensitivity to wavelength variations and real-world geometrical fabrication errors in waveguides width and depth are presented. Enhanced wavelength tolerance is demonstrated experimentally. The concept shows great promise for scaling high fidelity gates as part of integrated quantum optics architectures.

Direct Observation of Dynamically Localized Quantum Optical States.

Quantum-correlated biphoton states play an important role in quantum communication and processing, especially considering the recent advances in integrated photonics. However, it remains a challenge to flexibly transport quantum states on a chip, when dealing with large-scale sophisticated photonic designs. The equivalence between certain aspects of quantum optics and solid-state physics makes it possible to utilize a range of powerful approaches in photonics, including topologically protected boundary states, graphene edge states, and dynamic localization. Optical dynamic localization allows efficient protection of classical signals in photonic systems by implementing an analogue of an external alternating electric field. Here, we report on the observation of dynamic localization for quantum-correlated biphotons, including both the generation and the propagation aspects. As a platform, we use sinusoidal waveguide arrays with cubic nonlinearity. We record biphoton coincidence count rates as evidence of robust generation of biphotons and demonstrate the dynamic localization features in both spatial and temporal space by analyzing the quantum correlation of biphotons at the output of the waveguide array. Experimental results demonstrate that various dynamic modulation parameters are effective in protecting quantum states without introducing complex topologies. Our Letter opens new avenues for studying complex physical processes using photonic chips and provides an alternative mechanism of protecting communication channels and nonclassical quantum sources in large-scale integrated quantum optics.

Cryogenic electro-optic modulation in titanium in-diffused lithium niobate waveguides

Lithium niobate is a promising platform for integrated quantum optics. In this platform, we aim to efficiently manipulate and detect quantum states by combining superconducting single photon detectors and modulators. The cryogenic operation of a superconducting single photon detector dictates the optimisation of the electro-optic modulators under the same operating conditions. To that end, we characterise a phase modulator, directional coupler, and polarisation converter at both ambient and cryogenic temperatures. The operation voltage of these modulators increases, due to the decrease in the electro-optic effect, by 74% for the phase modulator, 84% for the directional coupler and 35% for the polarisation converter below 8.5. The phase modulator preserves its broadband nature and modulates light in the characterised wavelength range. The unbiased bar state of the directional coupler changed by a wavelength shift of 85 while cooling the device down to 5. The polarisation converter uses periodic poling to phasematch the two orthogonal polarisations. The phasematched wavelength of the utilised poling changes by 112 when cooling to 5.

C-shaped chiral waveguide for spin-dependent unidirectional propagation

Spin-dependent unidirectional propagation is one of the most intriguing features of the Quantum spin-Hall effect, which was studied intensively in electronic systems and led to the discovery of topological insulators. Recently, it was proven that evanescent waves intrinsically possess transverse spin that is dependent on the direction of propagation. This has enabled new applications in unidirectional waveguiding and integrated quantum optics. In this work, we study via numerical simulations a waveguide design consisting of C-shaped metallic particles characterized by extrinsic chirality and strong transverse spin. The design supports confined, spin-dependent unidirectional propagation with a high directionality ratio reaching 95%. We also study the effect of placing different local defects on the directionality of the supported guided mode.

Photonic-crystal optical parametric oscillator

The first demonstration of an optical parametric oscillator using a photonic crystal microcavity is promising for the future development of on-chip light sources for applications in integrated quantum optics.

Broadband detection of multiple spin and orbital angular momenta via dielectric metasurface.

Light beams carrying spin angular momentum (SAM) and orbital angular momentum (OAM) have created novel opportunities in the areas of optical communications, imaging, micromanipulation and quantum optics. However, complex optical setups are required to simultaneously manipulate, measure and analyze these states, which significantly limits system integration. Here, we introduce a novel detection approach for measuring multiple SAM and OAM modes simultaneously through a planar nanophotonic demultiplexer based on an all-dielectric metasurface. Coaxial light beams carrying multiple SAM and OAM states of light upon transmission through the demultiplexer are spatially separated into a range of vortex beams with different topological charge, each propagating along a specific wavevector. The broadband response, material dispersion and momentum conservation further enable the demultiplexer to achieve wavelength demultiplexing. We envision the ultracompact multifunctional architecture to enable simultaneous manipulation and measurement of polarization and spin encoded photon states with applications in integrated quantum optics and optical communications.

Tunable Linear Polarization-State Generator of Single Photons on a Lithium Niobate Chip

Controlling the polarization state of light at a fast speed is important in both classical and quantum regimes. Here, we present an easily integrated compact tunable linear polarization-state generator of single photons in the telecom wavelength band on a periodically poled lithium niobate on insulator (PPLNOI) chip. The linear polarization of single photons can be continuously rotated by applying a transverse electric field utilizing the electro-optic (EO) effect. With strong light confinement and the large EO coefficient in the PPLNOI ridge waveguide, dramatically reduced driving voltage and fast-speed modulation is realized. Moreover, quantum entanglement is well maintained during the switching of polarization states, as proved in the time-energy entanglement measurement. The scheme holds promise for realizing integrated quantum optics.

On-chip quantum opticsand integrated optomechanics

Recent developments in quantum computing and the growing interest in optomechanics and quantum optics need platforms that enable rapid prototyping and scalability. This can be fulfilled by on-chip integration, as we present here. The different nanofabrication steps are explained, and our automated measurement setup is discussed. We present an opto-electromechanical device, the H-resonator, which enables optomechanical experiments such as electrostatic springs and nonlinearities and thermomechanical squeezing. Moreover, it also functions as an optomechanical phase shifter, an essential element for our integrated quantum optics efforts. Besides this, the equivalent of a beam splitter in photonics-the directional coupler-is shown. Its coupling ratio can be reliably controlled, as we show with experimental data. Several directional couplers combined can realize the CNOT operation with almost ideal fidelity.

Scalable in operando strain tuning in nanophotonic waveguides enabling three-quantum-dot superradiance.

The quest for an integrated quantum optics platform has motivated the field of semiconductor quantum dot research for two decades. Demonstrations of quantum light sources, single photon switches, transistors and spin-photon interfaces have become very advanced. Yet the fundamental problem that every quantum dot is different prevents integration and scaling beyond a few quantum dots. Here, we address this challenge by patterning strain via local phase transitions to selectively tune individual quantum dots that are embedded in a photonic architecture. The patterning is implemented with in operando laser crystallization of a thin HfO2 film 'sheath' on the surface of a GaAs waveguide. Using this approach, we tune InAs quantum dot emission energies over the full inhomogeneous distribution with a step size down to the homogeneous linewidth and a spatial resolution better than 1 µm. Using these capabilities, we tune multiple quantum dots into resonance within the same waveguide and demonstrate a quantum interaction via superradiant emission from three quantum dots.

Near-Unity Indistinguishability Single Photon Source for Large-Scale Integrated Quantum Optics.

Integrated single photon sources are key building blocks for realizing scalable devices for quantum information processing. For such applications highly coherent and indistinguishable single photons on a chip are required. Here we report on a triggered resonance fluorescence single photon source based on In(Ga)As/GaAs quantum dots coupled to single- and multimode ridge waveguides. We demonstrate the generation of highly linearly polarized resonance fluorescence photons with 99.1% (96.0%) single photon purity and 97.5% (95.0%) indistinguishability in case of multimode (single mode) waveguide devices fulfilling the strict requirements imposed by multi-interferometric quantum optics applications. Our integrated triggered single photon source can be readily scaled up, promising a realistic pathway for on-chip linear optical quantum simulation, quantum computation, and quantum networks.

Spin‐Selective and Wavelength‐Selective Demultiplexing Based on Waveguide‐Integrated All‐Dielectric Metasurfaces

AbstractA novel approach for the design of a spin‐selective directional coupler and spin‐selective wavelength demultiplexing device by integrating an all‐dielectric metasurface into a silicon nitride waveguide is proposed and demonstrated. Taking advantage of the intrinsic chirality of the electromagnetic field inside the waveguide, the propagation direction of the excited waveguide mode can be easily controlled by the spin and wavelength of the incident light. The coupling efficiency of the spin‐selective directional coupler toward one side can reach ≈51.6% at 1836 nm. In addition, the working wavelengths, coupling efficiency, peak width, and mode type can be easily tailored by adjusting the geometric parameters of the waveguide and the antenna arrays. This study may provide a further step in the development of photonic integrated circuits, integrated quantum optics, chiral optics, and high‐bit‐rate telecommunication applications.

High-efficiency broadband light coupling between optical fibers and photonic integrated circuits

Abstract Efficient light energy transfer between optical waveguides has been a critical issue in various areas of photonics and optoelectronics. Especially, the light coupling between optical fibers and integrated waveguide structures provides essential input-output interfaces for photonic integrated circuits (PICs) and plays a crucial role in reliable optical signal transport for a number of applications, such as optical interconnects, optical switching, and integrated quantum optics. Significant efforts have been made to improve light coupling properties, including coupling efficiency, bandwidth, polarization dependence, alignment tolerance, as well as packing density. In this review article, we survey three major light coupling methods between optical fibers and integrated waveguides: end-fire coupling, diffraction grating-based coupling, and adiabatic coupling. Although these waveguide coupling methods are different in terms of their operating principles and physical implementations, they have gradually adopted various nanophotonic structures and techniques to improve the light coupling properties as our understanding to the behavior of light and nano-fabrication technology advances. We compare the pros and cons of each light coupling method and provide an overview of the recent developments in waveguide coupling between optical fibers and integrated photonic circuits.

Minimum resources for versatile continuous-variable entanglement in integrated nonlinear waveguides

In a recent paper [Phys. Rev. A {\bf 96}, 053822 (2017)], we proposed a strategy to generate bipartite and quadripartite continuous-variable entanglement of bright quantum states based on degenerate down-conversion in a pair of evanescently coupled nonlinear $\chi^{(2)}$ waveguides. Here, we show that the resources needed for obtaining these features can be optimized by exploiting the regime of second harmonic generation: the combination of depletion and coupling among pump beams indeed supplies all necessary wavelengths and appropriate phase mismatch along propagation. Our device thus entangles the two fundamental classical input fields without the participation of any harmonic ancilla. Depending on the propagation distance, the generated harmonics are entangled in bright or vacuum modes. We also evidence two-color bipartite and quadripartite entanglement over the interacting modes. The proposed device represents a boost in continuous-variable integrated quantum optics since it enables a broad range of quantum effects in a very simple scheme, which optimizes the resources and can be easily realized with current technology.

Invited Article: Time-bin entangled photon pairs from Bragg-reflection waveguides

Semiconductor Bragg-reflection waveguides are well-established sources of correlated photon pairs as well as promising candidates for building up integrated quantum optics devices. Here, we use such a source with optimized non-linearity for preparing time-bin entangled photons in the telecommunication wavelength range. By taking advantage of pulsed state preparation and efficient free-running single-photon detection, we drive our source at low pump powers, which results in a strong photon-pair correlation. The tomographic reconstruction of the state's density matrix reveals that our source exhibits a high degree of entanglement. We extract a concurrence of $88.9\pm 1.8\%$ and a fidelity of $94.2 \pm 0.9\%$ with respect to a Bell state.

Large-scale integrated quantum optics

Quantum Optics The ability to pattern optical circuits on-chip, along with coupling in single and entangled photon sources, provides the basis for an integrated quantum optics platform. Wang et al. demonstrate how they can expand on that platform to fabricate very large quantum optical circuitry. They integrated more than 550 quantum optical components and 16 photon sources on a state-of-the-art single silicon chip, enabling universal generation, control, and analysis of multidimensional entanglement. The results illustrate the power of an integrated quantum optics approach for developing quantum technologies. Science , this issue p. [285][1] [1]: /lookup/doi/10.1126/science.aar7053