This study aimed to develop teaching, learning, and assessment materials emphasizing the use of technological tools in the revised 2022 mathematics curriculum. To achieve the aim, this research reviewed previous studies to list technological tools applicable to the curriculum, analyzed achievement standards related to the use of technological tools, and developed 20 teaching, learning, and assessment materials based on these achievement standards. This process was conceptualized using the LED model, which consists of the List-up, Elaboration, and Development stages, allowing for systematic relations with technological tools, mathematics curriculum, and teaching, learning, and assessment. To ensure the quality of the developed materials, validity was secured through Delphi surveys, expert consultation, and field trials. The research findings are expected to provide assistance to teachers who aim to design and implement student-centered inquiry-based classes using technological tools, and to offer insights for developing relevant educational policies.