Infrared Stimulated Luminescence Research Articles

Towards accurate modelling of rock surface exposure dating using luminescence to estimate post-exposure erosion rate

Depth-dependent luminescence in the top few millimetres of rock surface emerges as a potential tool to estimate rock surface exposure age and post-exposure erosion rate. It relies on the principle that the luminescence depth profile (LDP) propagates deeper with the time of sunlight exposure and moves to shallower depth with the erosion rate. The propagation of LDP is generally assumed to follow the first-order kinetic (FOK) model, except for a few recent studies. The FOK model predicts an exponential decay of infrared stimulated luminescence (IRSL) signal with light exposure time, which rarely corroborates experimental observation; IRSL signal decay is much slower than exponential decay. The faster decay of IRSL, predicted by the FOK model, results in faster propagation of LDP and thus always underestimates the exposure age and translates into a higher erosion rate. Interestingly, the slower-than-exponential decay of the IRSL signal can be better explained by general order kinetics (GOK). Thus, recent studies on rock surface luminescence dating have employed the GOK model. However, the GOK model is yet to be explored to predict post-exposure erosion rates. Here, we apply the GOK model and theoretically demonstrate the impact of the order of kinetics on the calibration and propagation of LDP in the presence of erosion and how the LDP's transient to steady state transition depends on the order of kinetics. We have performed a series of synthetic tests to assess the impact of selecting an incorrect model on the prediction of erosion rate. Finally, using the revised rate equation, the erosion rates are recalculated for natural samples (data available in the literature: Lehmann et al. (2019b)) and the impact of GOK on the predicted erosion rate is discussed.

Single grain K-feldspar MET-IRSL sediment transport determination: bleaching patterns and rates

This paper describes ways that Infra-Red Stimulated Luminescence (IRSL) signals from K-feldspar grains can be used to determine patterns and rates of sediment transport. In particular, it focusses on the potential provided by single grains to reveal their individual exposure and burial histories by the application of multiple elevated temperature (MET) IRSL measurements. We examine similarities and differences in bleaching behaviour with different light sources and introduce the concept of an equilibrium bleach. We present data on the variability of bleaching parameters for grains from single sediment samples, and discuss different analysis approaches to best determine individual grain histories. We describe a single grain “bleach recovery” experiment, and the application of a combined growth-bleach protocol designed to allow optimal data collection of both aspects of grain behaviour. We discuss the development of a burial-bleach model using numerical simulations based on direct observations of sample characteristics.

Late Quaternary glacial maxima in southern Patagonia: insights from the Lago Argentino glacier lobe

Abstract. Determining the timing and extent of Quaternary glaciations around the globe is critical to understanding the drivers behind climate change and glacier fluctuations. Evidence from the southern mid-latitudes indicates that local glacial maxima preceded the global Last Glacial Maximum (LGM), implying that feedbacks in the climate system or ice dynamics played a role beyond the underlying orbital forcings. To shed light on these processes, we investigated the glacial landforms shaped and deposited by the Lago Argentino glacier (50° S), an outlet lobe of the former Patagonian Ice Sheet, in southern Argentina. We mapped geomorphological features on the landscape and dated moraine boulders and outwash sediments using 10Be cosmogenic nuclides and feldspar infrared stimulated luminescence (IRSL) to constrain the chronology of glacial advance and retreat. We report that the Lago Argentino glacier lobe reached more extensive limits prior to the global LGM, advancing during the middle to late Pleistocene between 243–132 ka and during Marine Isotope Stage 3 (MIS 3), culminating at 44.5 ± 8.0 and at 36.6 ± 1.0 ka. Our results indicate that the most extensive advance of the last glacial cycle occurred during MIS 3, and we hypothesize that this was a result of longer and colder winters, as well as increased precipitation delivered by a latitudinal migration of the Southern Westerly Winds belt, highlighting the role of local and regional climate feedbacks in modulating ice mass changes in the southern mid-latitudes.

Presence and implications of petrogenic organic carbon in High Himalayan Crystalline lake sediment

AbstractTwelve lacustrine sediment samples from a relict lake in the Kalla Glacier valley were co-dated using AMS radiocarbon (14C) and infrared stimulated luminescence (IRSL) dating methods. In general, the radiocarbon ages of bulk organic matter were older by a minimum of 1500 years compared to (age depth) modeled luminescence ages after fading corrections. This is observed for the first time in the lake sediments of High Himalayan Crystalline zone. A combination of lipid n-alkane data, Raman spectra and geochemical proxies suggested that this was due to ancient organic carbon (OCancient) that is a mixture of pre-aged (OCpre-aged) and petrogenic (OCpetro) organic carbon within older glacial moraine debris that served as sediment source to the lake. Raman spectra suggest the presence of moderate to highly graphitized OCpetro in all the profile samples. The OCpetro contributed 0.064 ± 0.032% to the sediment and the lake stored 2.5 ± 0.7 Gg OCpetro at variable rates during the last 16 kyr, with the mean burial flux 160 kg OCpetro yr−1. This study implies (1) employing another independent dating method in addition to radiocarbon method using bulk sediment organic matter, if the carbon content is low, to observe any discrepancy, and (2) a need to investigate on the fate of OCpetro as many such small lakes become relict in this region.

How old are the Mojave topographic dunes? The implications of new luminescence dating analyses from the Cady Mountains, Mojave Desert, southwest USA

The aeolian landforms of the Mojave Desert in the SW USA have been studied in detail over the last three decades, particularly in terms of their relationship to the region's topography and Pleistocene climate / sediment supply histories, as well as wider developments, such as the aeolian “sediment state” concept. In this context, the evolution of the Mojave River and its associated palaeolakes is thought to have been a key control on long-term sediment supply to aeolian systems, and luminescence dating chronologies for a range of (resulting) aeolian landforms have been related to these hydrological changes. Here we argue that at least some of these aeolian chronologies need to be re-assessed.We focus on luminescence chronologies for aeolian landforms within and marginal to the Cady Mountains, a mountain block adjacent to the Mojave River and palaeolake Manix, east of Barstow, California. We demonstrate that quartz in this locale exhibits several malign luminescence properties, and that low temperature K-feldspar infrared stimulated luminescence (IRSL) consistently exhibits high anomalous fading rates. Both contribute to age underestimation. We address these issues via post-infrared IRSL (pIRIR) and post-isothermal post-IR (pIt-IR) analyses of K-feldspars. The resulting ages span the last ~120 ka and imply phases of aeolian activity of a substantially greater antiquity than previously inferred. Notably, at one well-studied site – the Soldier Mountain sand ramp – the new ages suggest a landform dating not to Marine Isotope Stage (MIS) 1 or 2, as previously suggested, but more likely to MIS 5. The Cady Mountain record indicates that the only period of the last glacial cycle lacking evidence for aeolian sedimentation is ~40–9 ka, broadly consistent with expectations of increased regional humidity. These results also suggest that site topographic context may influence the age structure of aeolian deposits. In this instance, sand ramps consistently represent the oldest type of deposit (range ~ 40–120 ka), while early-mid Holocene dune accumulation is associated with sandsheets and valley-fill sands. Based on these findings, we argue that there is a need to critically re-assess the existing regional luminescence age database, and that there is potential to significantly revise our understanding of the region's aeolian system responses, and associated paleoenvironmental interpretations.

Multi-method luminescence dating of young aeolian dunes in the central Tibetan plateau

The environment of the Tibetan Plateau (TP) is extremely sensitive to global climate change, and the frequent aeolian activity on the central TP generates large amounts of dust with the result that the region has a major impact on regional and global environmental change. The extensive aeolian dunes on the central TP provide a direct and valuable archive of aeolian activity; however, the age and sediment deposition processes of these dunes are still poorly understood. Optically stimulated luminescence (OSL) dating, an effective method for dating aeolian sediments, has been used sparingly in the region. In this study, we applied quartz single-aliquot regenerative-dose (SAR) OSL, K-feldspar post-infrared infrared-stimulated luminescence (pIRIR), and single-grain K-feldspar pIRIR methods to determine the ages of two well-preserved sand dunes in the Lunpola (LD) and Tuotuohe (TTH) river basins in the central TP. Our results showed that the quartz OSL signal of the TTH dune was dim, while the LD dune quartz exhibited a higher OSL sensitivity than that of the TTH dune. The high recuperation observed could be attributed to the low signal-to-noise ratio of the OSL signals. The K-feldspar signal was bright and the pIR50IR170 signal could be used to date young dune samples in the central TP, whereas it could be affected by the residual dose, or incomplete bleaching in the TTH profile, resulting in age overestimation. The single-grain K-feldspar protocol had a good potential for dating the young TP dunes. Multi-method luminescence dating is recommended for the cross-checking of young dune samples with low OSL sensitivity in the TP. Our luminescence dating reveals that aeolian dunes in the central TP formed approximately 385 to 330 a and persisted to the present, possibly in response to climate change since the late stage of Little Ice Age (1400−1850 CE).

New data on tributary terraces and a reappraisal of the incision history of the Jinshan Gorge, middle Yellow River

River channel profiles and river terraces are two typical landscape features to investigate river incision history. However, incision history inferred from the two markers can be inconsistent. For example, along the Jinshan Gorge in the middle Yellow River, pseudo-terraces (a virtual metric derived from channel profile modelling) suggest a recent acceleration in incision rates only in the southern gorge, and the northern keeps steady, while river terraces in the trunk channel indicate recently increased incision rates all along the gorge. To mitigate these discrepancies, we investigate six tributaries along the Jinshan Gorge by mapping and dating several strath terraces at various distances from the confluence to the trunk channel. By comparing tributary terraces of similar age, we find generally increasing incision rates towards the confluence with the trunk river in the southern Jinshan Gorge. North to south increasing incision rates along the gorge are also observed from coeval tributary terraces. In addition, two different landscapes between the southern and northern tributaries near the confluence are recognized, one with a deeply incised gorge and another one with floodplains, suggesting incision rate in the northern gorge is steady through time. Integrating the new infrared stimulated luminescence (IRSL) and Accelerator Mass Spectrometry (AMS) 14C data from tributaries with the abundant literature data of terrace samples mostly in the Jinshan Gorge dated with various methods, we suggest published ages from optically stimulated luminescence (OSL) might be too young. The methodological limitation associated to the dating method can explain the observed mismatch of incision history in the northern gorge inferred from pseudo-terraces and from river terraces in the trunk channel, and reconcile some contradicting patterns in published trunk terrace data.

Influence of Na-feldspar grains within the K-feldspar fraction on sediments IRSL dating

The post-Infrared Infrared Stimulated Luminescence (pIRIR) protocol has been successfully applied to date Quaternary sediments using the K-rich feldspar fraction (density ＜2.58 g/cm3). However, during the extraction of K-feldspar grains, Na-feldspar particles (density 2.58–2.62 g/cm3) may be included, especially within the medium grained fraction. However, the possible influence of Na-feldspar contamination on K-feldspar IRSL dating results has not been investigated in detail. In this study, we applied the pIRIR dating protocol to measure the coarse- and medium-grained K-and Na-feldspar fractions of eight aeolian samples from various regions. Blue-violet and yellow-green detection windows were used for derived the signals of K- and Na-feldspar, respectively, and we attempted to evaluate the influence of the contamination by Na-feldspar grains on feldspar pIRIR dating. Comparison of the three signals (K-feldspar blue, Na-feldspar blue, Na-feldspar yellow) from each sample showed that the influence of the IRSL blue signal from Na-feldspar grains on the signal of the K-feldspar fraction was < 1–3%. Because of high fading rates, the Des or pIRIR ages obtained from the Na-feldspar yellow signal were underestimated. The Na-feldspar blue pIRIR Des and ages were nevertheless consistent with their corresponding K-feldspar blue De values and ages. This is because the few K-feldspar grains included within the Na-feldspar fraction emitted the greater part of the blue signals. From these observations, we conclude that the influence of Na-feldspar grains within the K-feldspar fraction on K-feldspar IRSL dating results can be ignored.

Multi-method geochronological approach to reconstruct post-1800 floodplain sedimentation in the upper Rhine plain, France

The precise dating of sedimentary archives covering the last 200 years in floodplains massively impacted by human activities is a major challenge. A combination of geochronological approaches is necessary to accurately date post-1800 sedimentary deposits. Here, we use a combination of a wide range of methods to unravel floodplain sedimentary dynamics, through the example of the Upper Rhine which is a highly regulated river. This comprises short--lived radionuclides (137Cs, 210Pbxs) and Infrared Stimulated Luminescence (IRSL) single-grain dating. Luminescence profiling methods (IRSL screening, portable luminescence reader) were also used to further characterise sedimentation dynamics. These were combined with a hydrogeomorphological approach based on historical planimetric and hydrological data, the knowledge of engineering works as well as the morpho-sedimentary adjustments they induced. Our study demonstrates the value of historic maps as well as historical hydrological data, which provide precise time markers for dating the sedimentary archive under study. We illustrate different assumptions, validity domains and limitations inherent to each method, especially the complexity of 137Cs to date floodplain sediments and the potential of luminescence methods for dating and estimating sedimentation continuity. We finally show the advantage of combining geochronological approaches in the construction of robust age models for young floodplain sedimentary archives in highly anthropized fluvial environments.

Not too old to rock: ESR and OSL dating reveal Quaternary activity of the Periadriatic Fault in the Alps

The Periadriatic Fault system (PAF) ranks among the largest post-collisional structures of the European Alps. Recent geodetic data suggest that a fraction of the Adria–Europe convergence is still being accommodated in the Eastern Alps. However, the historical seismicity records along the easternmost segment of the PAF are ambiguous, and instrumental records indicate that seismotectonic deformation is mostly concentrated in the adjacent Southern Alps and Dinarides. Both electron spin resonance (ESR) and optically stimulated luminescence (OSL) dating methods can be used to date coseismic slip (with a combined range covering a few decades to a couple of million years) in slowly deforming fault zones, such as the PAF. Since the saturation doses of the quartz ESR signals are larger than quartz and feldspar OSL, ESR enables establishing a maximum age of the last resetting event of the system, while OSL allows constraining their minimum age when the signal is in saturation. We collected fault gouge samples from three localities along the easternmost segment of the PAF. For ESR, we measured the signals from the Al center in quartz comparing the results from the single aliquot additive dose (SAAD) and single aliquot regenerative (SAR) dose protocols. For OSL, we recorded the infrared stimulated luminescence signal at 50°C (IR50) and post-infrared infrared-stimulated luminescence signal at 225 °C (pIRIR225). Our dating results indicate that the studied segment of the PAF system accommodated seismotectonic deformation during the Quaternary, with a maximum age for the last resetting event of the system ranging from 1075 ± 48 to 552 ± 26 ka (ESR SAR) and minimum ages in the range from 196 ± 12 to 281 ± 16 ka (saturation of pIRIR225). The obtained ages suggest that the studied segment of the PAF could be considered at least as a potentially active fault.Graphical abstract

IRSL properties of HfO2 obtained by the precipitation method and its correlation to ESR centres

Infrared-stimulated luminescence (IRSL) emission and its characterisation are reported for the first time for HfO2 synthesised by the precipitation method and its electron spin resonance (ESR) centres properties are shown in this study. IRSL spectrum has a broad emission band in the blue region, which is centred at about 2.49 eV. A similar emission was observed for the radiofluorescence (RF) with a band centred at 2.52 eV. RF signal intensity decreases with the readout temperature, which might indicate a thermal quenching process.IRSL signal is strongly affected by the readout temperature, as part of its emission is related to the presence of shallow traps (<100 °C). The IRSL shine-down curve is composed of two components with decay times of 15.7 and 800 s, and photoionisation cross-section values of about 1.20 × 10−19 and 2.35 × 10−21 cm2, respectively, based on IRSL carried out at 100 °C after 2 Gy of beta irradiation dose, using a general-order kinetic model. Dosimetric analyses indicated that there is a reproducible signal in IRSL, with a coefficient of variation lower than 9 % for repeatability and 3 % for reproducibility measurements. The dose-response curve has a linear trend in the dose range of 0.3–2.0 Gy. Regarding the photon energy study, it shows an overresponse for photo energy values below 200 keV. Fading of about 40 % after one day of storage was observed.Bleaching measurements indicated that the TL peaks located between 100 and 250 °C share the same trap levels as the IRSL ones. In addition, a possible charge transference is observed from the peak at 330 °C to lower temperature peaks. ESR analyses identified that oxygen vacancies of V+ type in a four-coordinated arrangement are induced by irradiation and are temperature-sensitive. Based on the bleaching and ESR measurements, it is reasonable to infer that V+ type vacancies are likely responsible for the IRSL, and its blue emission.

Luminescence and thermometry studies of plant opal phytoliths

We have investigated the luminescence properties of plant opal phytoliths to assess their suitability for determination of age and/or thermometric information from soil and sediment sequences. This study examined a <2.37 gcm−3 density fraction in parallel with quartz grains from samples collected from alluvial terraces. We observed comparable optically stimulated luminescence (OSL) from the phytolith fraction to the quartz, and thermoluminescence (TL) with broader peaks and continuum to higher temperatures. Scanning electron microscopy (SEM) data suggested the presence of opal clasts and contaminant minerals. To better understand the luminescence from opal phytoliths we analyzed a suite of biogenic materials including very pure diatoms, phytoliths, and quartz reference materials. We observe low sensitivity but measurable OSL signals in all the materials analyzed, and infrared stimulated luminescence (IRSL) signals with fast decay rates exceeding those of more typical feldspars in some of the purer materials. TL signals are similar to those observed for glasses and suggests dose response might extend beyond quartz saturation levels. Preliminary investigations of OSL dose response show very promising growth characteristics for opal phytolith samples and all other biogenic silica materials analyzed.

Regional beryllium-10 production rate for the mid-elevation mountainous regions in central Europe, deduced from a multi-method study of moraines and lake sediments in the Black Forest

Abstract. Beryllium-10 cosmic-ray exposure (CRE) dating has revolutionized our understanding of glacier fluctuations around the globe. A key prerequisite for the successful application of this dating method is the determination of regional production rates of in situ accumulated 10Be, usually inferred at independently dated calibration sites. Until now, no calibration site has been available for the mid-elevation mountain ranges of central Europe. We fill this gap by determining in situ 10Be concentrations in large boulders on moraines and by applying radiocarbon and infrared-stimulated luminescence (IRSL) dating to stratigraphically younger lake sediments in the southern Black Forest, SW Germany. The dating methods yielded concordant results, and, based on age–depth modelling with 14C ages, the age of a cryptotephra, and IRSL ages, we deduced a regional 10Be production rate in quartz. Calibrating the Black Forest production rate (BFPR) in the Cosmic-Ray Exposure program (CREp) resulted in a spallogenic sea-level and high-latitude (SLHL) production rate of 3.64±0.11 atoms 10Be g−1 quartz a−1 when referring to time-dependent Lal–Stone scaling, the European Reanalysis (ERA)-40 atmosphere model, and the atmospheric 10Be-based geomagnetic database in CREp. The BFPR turned out to be ∼11 % lower than both those at the nearest calibration site in the Alps (4.10±0.10 atoms 10Be g−1 quartz a−1 at SLHL) and the canonical global 10Be production rate (4.11±0.19 atoms 10Be g−1 quartz a−1 at SLHL) in CREp. A stronger weathering and snow cover bias and a higher impact of forest, soil, moss, and shrub cover at the study site likely explain this discrepancy.

Effect of IRSL-BLSL-TSL reading modes combination on thermoluminescence (TL) response of BeO dosimeter.

The ultimate goal of this work is the study of the effect of luminescence stimulations and signals reading modes combinations on the thermoluminescence intensity and glow curve behaviour for the same X-ray irradiation dose. Three interesting stimulating and reading modes are considered, namely, infrared stimulated luminescence (IRSL), blue light-emitting diode stimulated luminescence (BLSL) and thermally stimulated luminescence (TSL). The studied stimulation and reading modes combination protocols are (Protocol 1) IRSL-TSL, (Protocol 2) IRSL-BLSL-TSL and (Protocol 3) BLSL-IRSL-TSL. Experiments are performed on beryllium oxide (BeO) dosimeter. Results demonstrate well that the combination of reading modes have direct impact on the TL signal in terms of intensity and glow curve shape. It was also found that when reading modes are correctly combined, particularly when IRSL is applied first, then BLSL and TL, it is possible to collect two or more exploitable signals of different stimulation types for the same irradiation that can be used for different purposes and final applications.

Infrared stimulated luminescence properties of highly sensitive K2SO4:Cu phosphor

The objective of this work is to investigate the dosimetric properties of a newly developed phosphor, which is potassium sulfate doped with copper. K2SO4:Cu exhibits high sensitivity as a radiation detector in the infrared stimulated luminescence (IRSL) method. The phosphor allows for dose measurements of the order of μGy using an appropriately sensitive luminescence reader. Basic dosimetric properties were examined, including: detection limit, dose-response over a wide dose range (eight orders of magnitude), reproducibility, reusability, signal bleaching and signal stability (fading) during a long time after irradiation (up to six months). The results showed dose linearity in the range of at least 1 mGy - 10 Gy, minimum detectable dose in the order of μGy and no signal loss several days after irradiation. At longer intervals after exposure, the signal begins to fade. Due to the high sensitivity of the material, despite fading, the IRSL signal still remains at a sufficient level after several months. In addition to fading, signal regeneration was noticed in the material and preliminarily studied.

Insight into the dynamics of a long-runout mass movement using single-grain feldspar luminescence in the Pokhara Valley, Nepal

Abstract. Mass movements play an important role in landscape evolution of high mountain areas such as the Himalayas. Yet, establishing numerical age control and reconstructing transport dynamics of past events is challenging. To fill this research gap, we bring luminescence dating to the test in an extremely challenging environment: the Pokhara Valley in Nepal. This is challenging for two reasons: (i) the optically stimulated luminescence (OSL) sensitivity of quartz, typically the mineral of choice for dating sediments younger than 100 ka, is poor, and (ii) highly rapid and turbid conditions during mass movement transport hamper sufficient OSL signal resetting prior to deposition, which eventually results in age overestimation. Here, we first assess the applicability of single-grain feldspar dating of medieval mass movement deposits catastrophically emplaced in the Pokhara Valley. Second, we exploit the poor bleaching mechanisms to get insight into the sediment dynamics of this paleo-mass movement through bleaching proxies. The Pokhara Valley is a unique setting for our case study, considering the availability of an extensive independent radiocarbon dataset as a geochronological benchmark. Single-grain infrared stimulated luminescence (IRSL) signals were measured at 50 ∘C (IRSL-50) and post-infrared infrared stimulated luminescence signals at 150 ∘C (pIRIR-150). Our results show that the IRSL-50 signal is better bleached than the pIRIR-150 signal. A bootstrapped minimum age model (bMAM) is applied to retrieve the youngest subpopulation to estimate the paleodose. However, burial ages calculated with this paleodose overestimate the radiocarbon ages by an average factor of ∼23 (IRSL-50) and ∼72 (pIRIR-150), showing that dating of the Pokhara Formation with a single-grain approach was not successful for most samples. Some samples, however, only slightly overestimate the true emplacement age and thus could be used for a rough age estimation. Large inheritances in combination with the scatter in the single-grain dose distributions show that the sediments have been transported under extremely limited light exposure prior to deposition, which is consistent with the highly turbid nature of the sediment-laden flood and debris flows depositing the Pokhara gravels. To investigate the sediment transport dynamics in more detail, we studied three bleaching proxies: the percentage of grains in saturation 2D0 criteria, the percentage of best-bleached grains (2σ range of bMAM-De) and the overdispersion (OD). None of the three bleaching proxies indicate a spatial relationship with runout distance of the mass movement deposits. We interpret this as evidence for the lack of bleaching during transport, which reflects the catastrophic nature of the event. While not providing reliable burial ages of the Pokhara mass movement deposits, single-grain feldspar dating can potentially be used as an age range finder method. Our approach shows the potential of luminescence techniques to provide insights in sediment transport dynamics of extreme and rare mass movement events in mountainous regions.

Implications and hydrographs for two Pre-Bonneville pluvial lakes and double geosols from 14 OSL-IRSL ages in Cache Valley, NE Bonneville Basin

In the northeastern Great Basin, USA, thirteen new optically stimulated luminescence (OSL) ages and one infrared stimulated luminescence (IRSL) age show that two deep pluvial lakes preceded the Bonneville lake cycle in Cache Valley during marine oxygen-isotope stages (MIS) 6 (123-191 ka) and 4 (56-71 ka), respectively. Our new data define quantitative hydrographs of the Little Valley and Cutler Dam lake cycles in both Cache Valley and the main Bonneville basin. In western Cache Valley, excavation of a faulted, east-plunging spit has sequentially exposed these deposits and overlying MIS 3 Fielding humid-over-arid double geosols that end westward at a strand of the east-dipping Dayton-Oxford normal-fault zone. Lithologically identical double paleosols in eastern Cache Valley overlie a variety of deposits, including dated Little Valley lake beds, and persist above the Bonneville shoreline. Six new ages show that the Little Valley lake cycle in Cache Valley began before 169 ka and ended after 143 ka, and its highest shoreline was above 1493 m. The &gt;25 kyr duration of this pluvial lake cycle rivals the combined durations of the two subsequent lake cycles, during MIS 4 and MIS 2. The Cutler Dam lake rose at least to ~1450 m by ~67 ka in Cache Valley. In the type area in the main Bonneville basin, west of Cutler Narrows, four averaged IRSL dates from Cutler Dam lake beds show that the lake level there had dropped to ~1340 m by ~59 ka. The Little Valley lake rose at least 40 to 50 m above the local Provo shoreline whereas the Cutler Dam lake missed reaching the Provo shoreline by ~13 m. Beneath central Cache Valley, southeast of the study area, there are two laterally extensive, confining layers of silty clay with an intervening sandy gravel layer, all overlying thick gravelly sediment. Both confining layers enclose additional thin and discontinuous gravel layers with adjacent oxidized clays. These alternating coarse and fine sediments are probably correlative with the exposed MIS 6 to MIS 1 deposits and, possibly, older lake cycles.

Integrated uplift, subsidence, erosion and deposition in a tightly coupled source‐to‐sink system, Pagliara basin, northeastern Sicily, Italy

AbstractHow tectonic forcing, expressed as base level change, is encoded in the stratigraphic and geomorphic records of coupled source‐to‐sink systems remains uncertain. Using sedimentological, geochronological and geomorphic approaches, we describe the relationship between transient topographic change and sediment deposition for a low‐storage system forced by rapid rock uplift. We present five new luminescence ages and two terrestrial cosmogenic nuclide paleo‐erosion rates for the late Pleistocene Pagliara fan‐delta complex and we model corresponding base level fall history and erosion of the source catchment located on the Ionian flank of the Peloritani Mountains (NE‐Sicily, Italy). The Pagliara delta complex is part of the broader Messina Gravel‐and‐Sands lithostratigraphic unit that outcrops along the Peloritani coastal belt as extensional basins have been recently inverted by both normal faults and regional uplift at the Messina Straits. The deltas exposed at the mouth of the Pagliara River have constructional tops at ca. 300 m a.s.l. and onlap steeply east‐dipping bedrock at the coast to thickness between ca. 100 and 200 m. Five infrared‐stimulated luminescence (IRSL) ages collected from the delta range in age from ca. 327 to 208 ka and indicate a vertical long‐term sediment accumulation rate as rapid as ca. 2.2 cm/yr during MIS 7. Two cosmogenic 10Be concentrations measured in samples of delta sediment indicate paleo‐erosion rates during MIS 8–7 near or slightly higher than the modern rates of ca. 1 mm/yr. Linear inversion of Pagliara fluvial topography indicates an unsteady base level fall history in phase with eustasy that is superimposed on a longer, tectonically driven trend that doubled in rate from ca. 0.95 to 1.8 mm/yr in the past 150 ky. The combination of footwall uplift rate and eustasy determines the accommodation space history to trap the fan‐deltas at the Peloritani coast in hanging wall basins, which are now inverted, uplifted and exposed hundreds of metres above the sea level.

Pulsed infrared stimulated luminescence measurements for defect pair model studies in feldspars

We present a time-resolved experimental study of feldspar infrared stimulated luminescence (IRSL) as part of a defect pair model investigation of the underlying mechanisms. Within our investigation we recorded ultraviolet emissions that covered a diverse range of alkali feldspars together with a limited selection of plagioclase feldspars. In analysing our measurements, we find that each IRSL pulse response is characterised by a combination of fast and slow components, the relative proportions of which vary across the range of feldspars we tested. We interpret the presence of the components as providing evidence as to the dual roles played by high mobility electrons and by the less mobile alkali ions that are released during the underlying physical processes. Consistent with earlier data, we find further that the luminescent sensitivities vary widely across the range of feldspars we tested.

Testing new kinetic models and calibration methods for Rock Surface Luminescence Exposure dating using controlled experiments

Rock surface luminescence exposure dating (RSLED) is an evolving tool in dating prehistoric rock surfaces. In this study, we explore and compare current and new models and calibration methods using optically stimulated luminescence (OSL) depth profiles from quartz grains and Infrared Stimulated Luminescence (IRSL; IR50, pIRIR225, and MET290) from feldspar grains found in granite and sandstone samples.This study shows that, although correct model assumptions improve the quality of exposure age estimates, significant discrepancies between observed and expected fitting parameter values remain, and these discrepancies leads to inaccurate age estimation. This is particularly the case when post-IR signals from feldspar are used. Here, the spectral dependency of luminescence signals is examined to better understand these problems. The demonstrated depth dependency of fitting parameters, previously assumed to be constant with depth, also gives rise to discrepancies in parameter values. The surprising observation that, in rocks, the IR50 signal is apparently more easily bleached than the quartz fast-component OSL signal is explained in terms of the wavelength dependence of light attenuation increasing the effective path length for shorter wavelengths, and so changing the shape of the light spectrum with penetration depth. This complicates parameter estimates in exposure dating even more.Alternative approaches (rather than parameter estimation) for estimating how long a rock surface has been exposed to light are considered, based on modelling the shape and position of the measured luminescence-depth profile. It is concluded that the most accurate exposure age is derived by interpolating the depth of an unknown profile onto a curve of profile depths from known age profiles (the Exposure Response Curve, or ERC, approach).