Icelandic Dust Research Articles

Investigation of Icelandic Dust Presence in the Aerosols Collected at Hornsund (Svalbard, Norwegian Arctic) in Spring 2019

Investigation of Icelandic Dust Presence in the Aerosols Collected at Hornsund (Svalbard, Norwegian Arctic) in Spring 2019

Complex refractive index and single scattering albedo of Icelandic dust in the shortwave part of the spectrum

Abstract. Icelandic dust can impact the radiative budget in high-latitude regions directly by affecting light absorption and scattering and indirectly by changing the surface albedo after dust deposition. This tends to produce a positive radiative forcing. However, the limited knowledge of the spectral optical properties of Icelandic dust prevents an accurate assessment of these radiative effects. Here, the spectral single scattering albedo (SSA) and the complex refractive index (m=n-ik) of Icelandic dust from five major emission hotspots were retrieved between 370–950 nm using online measurements of size distribution and spectral absorption (βabs) and scattering (βsca) coefficients of particles suspended in a large-scale atmospheric simulation chamber. The SSA(λ) estimated from the measured βabs and βsca increased from 0.90–0.94 at 370 nm to 0.94–0.96 at 950 nm in Icelandic dust from the different hotspots, which falls within the range of mineral dust from northern Africa and eastern Asia. The spectral complex refractive index was retrieved by minimizing the differences between the measured βabs and βsca and those computed using the Mie theory for spherical and internally homogeneous particles, using the size distribution data as input. The real part of the complex refractive index (n(λ)) was found to be 1.60–1.61 in the different samples and be independent of wavelength. The imaginary part (k(λ)) was almost constant with wavelength and was found to be around 0.004 at 370 nm and 0.002–0.003 at 950 nm. The estimated complex refractive index was close to the initial estimates based on the mineralogical composition, also suggesting that the high magnetite content observed in Icelandic dust may contribute to its high absorption capacity in the shortwave part of the spectrum. The k(λ) values retrieved for Icelandic dust are at the upper end of the reported range for low-latitude dust (e.g., from the Sahel). Furthermore, Icelandic dust tends to be more absorbing towards the near-infrared. In Icelandic dust, k(λ) between 660–950 nm was 2–8 times higher than most of the dust samples sourced in northern Africa and eastern Asia. This suggests that Icelandic dust may have a stronger positive direct radiative forcing on climate that has not been accounted for in climate predictions.

Fully Dynamic High–Resolution Model for Dispersion of Icelandic Airborne Mineral Dust

Icelandic topsoil sediments, as confirmed by numerous scientific studies, represent the largest and the most important European source of mineral dust. Strong winds, connected with the intensive cyclonic circulation in the North Atlantic, induce intense emissions of mineral dust from local sources all year and carry away these fine aerosol particles for thousands of kilometers. Various impacts of airborne mineral dust particles on local air quality, human health, transportation, climate and marine ecosystems motivated us to design a fully dynamic coupled atmosphere–dust numerical modelling system in order to simulate, predict and quantify the Icelandic mineral dust process including: local measurements and source specification over Iceland. In this study, we used the Dust Regional Atmospheric Model (DREAM) with improved Icelandic high resolution dust source specification and implemented spatially variable particle size distribution, variable snow cover and soil wetness. Three case studies of intense short- and long-range transport were selected to evaluate the model performance. Results demonstrated the model’s capability to forecast major transport features, such as timing, and horizontal and vertical distribution of the processes. This modelling system can be used as an operational forecasting system, but also as a reliable tool for assessing climate and environmental Icelandic dust impacts.

Potential Source Contribution Function Analysis of High Latitude Dust Sources over the Arctic: Preliminary Results and Prospects

The results of a preliminary investigation of the dust sources in the Arctic based on their geochemical properties by potential source contribution function (PSCF) analysis are presented in this paper. For this purpose, we considered one year of aerosol geochemical data from Ny-Ålesund, Svalbard, and a short list of chemical elements (i.e., Al, Fe, Mn, Ti, Cr, V, Ni, Cu, and Zn) variably related to the dust fraction. Based on PSCF analysis: (i) four different dust source areas (i.e., Eurasia, Greenland, Arctic-Alaska, and Iceland) were characterized by distinguishing geochemical ranges and seasonal occurrence; and (ii) a series of typical dust days from the distinct source areas were identified based on the corresponding back trajectory patterns. Icelandic dust samples revealed peculiar but very variable characteristics in relation to their geographical source regions marked by air mass back trajectories. The comparison between pure and mixed Icelandic dust samples (i.e., aerosols containing Icelandic dust along with natural and/or anthropogenic components) revealed the occurrence of different mixing situations. Comparison with Icelandic soils proved the existence of dilution effects related to the emission and the transport processes.

Particle‐scale characterization of volcaniclastic dust sources within Iceland

AbstractVolcaniclastic dust particles are characterized by unique physical properties, which are speculated to influence their rates of entrainment, emission and deposition within the atmospheric boundary layer. Few detailed particle‐scale measurements exist, so that natural particles often are idealized as solid glass spheres in the parameterization of dust dispersion models. This study shows that volcaniclastic dust particles from Iceland contain substantial quantities of amorphous glass, large internal voids and copious dustcoats comprised of nano‐scale flakes. Their high porosity, found to increase with particle diameter, generates particle densities that can be substantially lower than expected for a solid sphere. An abundance of volcanic glass also seems to increase particle porosity and roughness, and thereby strongly correlates with the Brunauer Emmett Teller surface area. An analysis based on Stokes' law further suggests that Icelandic dust with a standardized geometric diameter (10 μm or PM10), but with varying density, shape and origin, may have settling velocities in still air that are up to 20% lower than for a reference glass sphere. As a first approximation, neglecting complex particle interactions and wind speed, which also affect the deposition rate in the atmosphere, their low density and large surface area could increase the expected residence time by a factor of five. Model parameterization should be refined to incorporate these particle‐scale factors in order to improve on the estimation of volcaniclastic dust dispersion.

Wind Tunnel‐Based Comparison of PM10 Emission Rates for Volcanic Ash and Glaciogenic Aerosol Sources Within Iceland

AbstractIceland contributes 30–40 million tons of mineral dust to the atmosphere each year. Emission events are linked to exceedingly high concentrations of PM10, poor air quality, and respiratory disease, particularly in Reykjavík. Volcaniclastic aerosols have unique microphysical properties, and usually are porous and highly angular, with large surface areas bearing ultrafine, nanoscale dustcoats. The large internal void space contributes to low particle density, believed to affect emission and deposition rates in the atmospheric boundary layer, as well as the range of transport. However, the aerodynamic and sedimentological factors that govern dust entrainment in these high‐latitude settings are not well constrained empirically, providing little guidance for the parameterization of aerosol dispersion models. A series of laboratory wind tunnel simulations were carried out under full climate control to evaluate these effects for Icelandic samples collected from five active dust sources, inclusive of volcanic ash and glaciofluvial sediments. PM10 emission rates measured in this study are similar in magnitude to those obtained in a small number of field studies within selected high‐latitude regions, and for volcanic ash using a PI‐SWERL. The scaling with friction velocity is well described by the 1988 dust emission model of Gillette and Passi, while the parameterization appears to be strongly dependent on the median particle size. Sediments from the coarsest Icelandic dust sources were found to be most emissive, owing to the importance of particle impact, while the proportionate amount of PM10 within the test bed was not found to correlate with the emission rate.

Distinct chemical and mineralogical composition of Icelandic dust compared to northern African and Asian dust

Abstract. Iceland is a highly active source of natural dust. Icelandic dust has the potential to directly affect the climate via dust–radiation interaction and indirectly via dust–cloud interaction, the snow/ice albedo effect and impacts on biogeochemical cycles. The impacts of Icelandic dust depend on its mineralogical and chemical composition. However, a lack of data has prevented an accurate assessment of the role of Icelandic dust in the Earth system. Here, we collected surface sediment samples from five major Icelandic dust hotspots. Dust aerosols were generated and suspended in atmospheric chambers, and PM10 and PM20 fractions were collected for further analysis. We found that the dust samples primarily consist of amorphous basaltic materials ranging from 8 wt % (from the Hagavatn hotspot) to 60 wt %–90 wt % (other hotspots). Samples had relatively high total Fe content (10 wt %–13 wt %). Sequential extraction of Fe to determine its chemical form shows that dithionite Fe (Fe oxides such as hematite and goethite) and ascorbate Fe (amorphous Fe) contribute respectively 1 %–6 % and 0.3 %–1.4 % to the total Fe in Icelandic dust. The magnetite fraction is 7 %–15 % of total Fe and 1 %–2 wt % of PM10, which is orders of magnitude higher than in mineral dust from northern Africa. Nevertheless, about 80 %–90% of the Fe is contained in pyroxene and amorphous glass. The initial Fe solubility (ammonium acetate extraction at pH 4.7) is from 0.08 % to 0.6 %, which is comparable to low-latitude dust such as that from northern Africa. The Fe solubility at low pH (i.e. pH 2) is significantly higher than typical low-latitude dust (up to 30 % at pH 2 after 72 h). Our results revealed the fundamental differences in composition and mineralogy of Icelandic dust from low-latitude dust. We attribute these differences to the low degree of chemical weathering, the basaltic composition of the parent sediments and glacial processes. Icelandic dust contributes to the atmospheric deposition of soluble Fe and can impact primary productivity in the North Atlantic Ocean. The distinct chemical and mineralogical composition, particularly the high magnetite content (1 wt %–2 wt %), indicates a potentially significant impact of Icelandic dust on the radiation balance in the subpolar and polar regions.

Properties of dust source material and volcanic ash in Iceland

AbstractThe volcanic origin, primarily basaltic, of most of the surface material in Iceland influences its physical properties and appearance. Size distributions, shape analyses and melting experiments were made for surface material collected in high‐erosion dust source areas and fresh volcanic ash deposits to determine whether they differ from one another and from dust from other major dust sources. The major differences found between Icelandic dust and dust from other major dust sources in the world, such as the Sahara, are in the particle shapes, lower density and darker colour. Icelandic dust particles greater than 20 μm retain volcanic morphological properties that are also found in fresh volcanic ash. Dust and fresh volcanic ash particles less than 20 μm are crystalline and blocky in nature, similar to the dust from other global source regions. The finer grained (<20 μm) Icelandic particles will have similar suspension and transport behaviours and be similarly hazardous to health and infrastructure as non‐Icelandic dust. The coarser particles (>20 μm) will have different suspension and transport behaviours than other dusts due to the volcanic morphology. Icelandic surface material has between 5% and 30% glassy particles compared to fresh volcanic ash which has more than 50% glassy particles. Glassy particles were observed to melt at a lower temperature than the mineral grains; and, as a result, volcanic ash is found to be more threatening to aircraft engines than the typical dust from Iceland. Icelandic dust was observed to be blocky, or plate‐like in the respirable size fraction, suggesting similar health hazards as dust from other regions.

Can Volcanic Dust Suspended From Surface Soil and Deserts of Iceland Be Transferred to Central Balkan Similarly to African Dust (Sahara)?

In this work we use chemical fingerprints as characteristics ratios of specific crustal elements Ca/Al, Fe/Al, K/Al, Mg/Al, Mn/Al, Ca/Fe and Mg/Fe to investigate the long-range transport of volcanic aerosols which are entering the atmosphere in suspended and resuspended processes from Icelandic deserts and hot spots in remote areas in Iceland and transmitted to the central Balkan area (Belgrade). For this purpose, backward trajectories from Belgrade (=44°48’; =20°28’) in 2012 and 2013, simultaneous with atmospheric aerosols measurements, were calculated by using the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model. We found that about 17% of air masses passed over Icelandic territory and arrived to Balkan area. In almost all of these episodes ratios of some investigated elements in suburban aerosols of Balkan area corresponded to the ratios of elements investigated in surface soil of the Rangárvellir area - South Iceland in the vicinity of volcanoes. We identified several episodes, such as 6 – 8 August 2012, 2 – 6 June 2013, 26 – 28 June 2013, and 18 – 20 September 2013, with the characteristic ratios of the highest number of investigated elements in atmospheric aerosol of central Balkan corresponding to ratios from Icelandic soil material. This study provides evidence that Icelandic dust can travel long distances showing the importance of High Latitude Dust sources.

Aerosol optical properties in the Arctic: The role of aerosol chemistry and dust composition in a closure experiment between Lidar and tethered balloon vertical profiles

A closure experiment was conducted over Svalbard by comparing Lidar measurements and optical aerosol properties calculated from aerosol vertical profiles measured using a tethered balloon. Arctic Haze was present together with Icelandic dust. Chemical analysis of filter samples, aerosol size distribution and a full set of meteorological parameters were determined at ground. Moreover, scanning electron microscopy coupled with energy-dispersive X-ray (SEM-EDS) data were at disposal showing the presence of several mineralogical phases (i.e., sheet silicates, gypsum, quartz, rutile, hematite).The closure experiment was set up by calculating the backscattering coefficients from tethered balloon data and comparing them with the corresponding lidar profiles. This was preformed in three subsequent steps aimed at determining the importance of a complete aerosol speciation: (i) a simple, columnar refractive index was obtained by the closest Aerosol Robotic Network (AERONET) station, (ii) the role of water-soluble components, elemental carbon and organic matter (EC/OM) was addressed, (iii) the dust composition was included.When considering the AERONET data, or only the ionic water-soluble components and the EC/OM fraction, results showed an underestimation of the backscattering lidar signal up to 76, 53 and 45% (355, 532 and 1064 nm). Instead, when the dust contribution was included, the underestimation disappeared and the vertically-averaged, backscattering coefficients (1.45 ± 0.30, 0.69 ± 0.15 and 0.34 ± 0.08 Mm−1 sr−1, at 355, 532 and 1064 nm) were found in keeping with the lidar ones (1.60 ± 0.22, 0.75 ± 0.16 and 0.31 ± 0.08 Mm−1 sr−1). Final results were characterized by low RMSE (0.36, 0.08 and 0.04 Mm−1 sr−1) and a high linear correlation (R2 of 0.992, 0.992 and 0.994) with slopes close to one (1.368, 0.931 and 0.977, respectively). This work highlighted the importance of all the aerosol components and of the synergy between single particle and bulk chemical analysis for the optical property characterization in the Arctic.

A 60 Year Examination of Dust Day Activity and Its Contributing Factors From Ten Icelandic Weather Stations From 1950 to 2009

High latitude dust is an important contributor to the global dust cycle, which affects the radiative balance of the atmosphere. The frequency and severity of dust events are driven by variables such as wind speed, precipitation, temperature, surface cover type, and volcanic activity. The extent of impact of glacial retreat is yet to be determined, but glacial outburst floods, known as jokulhlaups, have been suggested to be a significant factor in the seasonal pattern of dust activity, with major jokulhlaups being attributed as a cause for an increase in dust activity in their subsequent year. However, in examination of ten meteorological stations from 1950 to 2009, there does not appear to be sufficient evidence that jokulhlaups are a significant driver of Iceland’s dust activity. Additionally, taking into account a larger range of dust codes, contributions from Icelandic dust plumes are found to be greater than previously assumed, with an average of 128 dust days per year as compared to a previously determined average of 34 dust days annually.

Mineralogical and Chemical Records of Icelandic Dust Sources Upon Ny-Ålesund (Svalbard Islands)

This work aims to identify the geochemical and mineralogical markers of Icelandic dust and to differentiate it from the dust of local origin deposited at the Ny-Alesund station. We characterized representative sediment samples from Iceland and Svalbard and compared them to a set of aerosol samples collected in Ny-Alesund to check the existence and type of the mineralogical markers. The sediment samples were analyzed by X-ray diffraction (XRD) to detect the mineralogical constrain of the geochemical markers. Both aerosol and sediment samples were examined by scanning electron microscopy coupled with EDS microanalysis (SEM-EDS) and image analysis to detect and to provide a morpho-chemical characterization of the mineralogical markers of dust provenance. Comparison between local and Icelandic sediments reveals the metal oxide particles as the most representative and distinguishing mineralogical/phase markers for Iceland dust sources. In particular, we have considered the magnetite-chromite and the magnetite-ulvospinel associations as marker facies of the tholeiitic magmatic series and the presence of volcanic glass as a further indicator of provenance from Iceland. The morphochemical characteristics of the metal oxide particles in the aerosol samples compared to those of the sediment samples have proved to be a powerful tool to separate Icelandic dust from other sources for dust. In particular, the small size, higher grain boundary complexity and lower Fe/Cr ratios suggest the influence of anthropogenic sources, well in accordance with the results of air mass backward trajectories which reveal a main contribution from industrialized areas in Eurasia. This study shows the reliability of the geochemical characterization of the metal oxide particles for the identification of the source regions of dust. In addition it provides an evidence that Icelandic dust can be transported long range to Svalbard confirming the importance of High Latitude Dust sources.

Temporal and spatial variability of Icelandic dust emissions and atmospheric transport

Abstract. Icelandic dust sources are known to be highly active, yet there exist few model simulations of Icelandic dust that could be used to assess its impacts on the environment. We here present estimates of dust emission and transport in Iceland over 27 years (1990–2016) based on FLEXDUST and FLEXPART simulations and meteorological re-analysis data. Simulations for the year 2012 based on high-resolution operational meteorological analyses are used for model evaluation based on PM2. 5 and PM10 observations in Iceland. For stations in Reykjavik, we find that the spring period is well predicted by the model, while dust events in late fall and early winter are overpredicted. Six years of dust concentrations observed at Stórhöfði (Heimaey) show that the model predicts concentrations of the same order of magnitude as observations and timing of modelled and observed dust peaks agrees well. Average annual dust emission is 4.3 ± 0.8 Tg during the 27 years of simulation. Fifty percent of all dust from Iceland is on average emitted in just 25 days of the year, demonstrating the importance of a few strong events for annual total dust emissions. Annual dust emission as well as transport patterns correlate only weakly to the North Atlantic Oscillation. Deposition amounts in remote regions (Svalbard and Greenland) vary from year to year. Only limited dust amounts reach the upper Greenland Ice Sheet, but considerable dust amounts are deposited on Icelandic glaciers and can impact melt rates there. Approximately 34 % of the annual dust emission is deposited in Iceland itself. Most dust (58 %), however, is deposited in the ocean and may strongly influence marine ecosystems.

Long-term dust aerosol production from natural sources in Iceland

Iceland is a volcanic island in the North Atlantic Ocean with maritime climate. In spite of moist climate, large areas are with limited vegetation cover where >40% of Iceland is classified with considerable to very severe erosion and 21% of Iceland is volcanic sandy deserts. Not only do natural emissions from these sources influenced by strong winds affect regional air quality in Iceland (“Reykjavik haze”), but dust particles are transported over the Atlantic ocean and Arctic Ocean >1000 km at times. The aim of this paper is to place Icelandic dust production area into international perspective, present long-term frequency of dust storm events in northeast Iceland, and estimate dust aerosol concentrations during reported dust events.Meteorological observations with dust presence codes and related visibility were used to identify the frequency and the long-term changes in dust production in northeast Iceland. There were annually 16.4 days on average with reported dust observations on weather stations within the northeastern erosion area, indicating extreme dust plume activity and erosion within the northeastern deserts, even though the area is covered with snow during the major part of winter. During the 2000s the highest occurrence of dust events in six decades was reported. We have measured saltation and Aeolian transport during dust/volcanic ash storms in Iceland, which give some of the most intense wind erosion events ever measured.Icelandic dust affects the ecosystems over much of Iceland and causes regional haze. It is likely to affect the ecosystems of the oceans around Iceland, and it brings dust that lowers the albedo of the Icelandic glaciers, increasing melt-off due to global warming. The study indicates that Icelandic dust may contribute to the Arctic air pollution.Implications: Long-term records of meteorological dust observations from Northeast Iceland indicate the frequency of dust events from Icelandic deserts. The research involves a 60-year period and provides a unique perspective of the dust aerosol production from natural sources in the sub-Arctic Iceland. The amounts are staggering, and with this paper, it is clear that Icelandic dust sources need to be considered among major global dust sources. This paper presents the dust events directly affecting the air quality in the Arctic region.

Pathways of high-latitude dust in the North Atlantic

The contribution of mineral dust from high-latitude sources has remained an under-examined feature of the global dust cycle. Dust events originating at high latitudes can provide inputs of aeolian sediment to regions lying well outside the subtropical dust belt. Constraining the seasonal variability and preferential pathways of dust from high-latitude sources is important for understanding the potential impacts that the dust may have on wider environmental systems, such as nearby marine or cryospheric domains. This study quantifies dust pathways from two areas exhibiting different emission dynamics in the north and south of Iceland, which is a prominent Northern Hemisphere dust source. The analysis uses air parcel trajectory modelling, and for the first time for high-latitude sources, explicitly links all trajectory simulations to time-specific (meteorological) observations of suspended dust. This approach maximises the potential for trajectories to represent dust, and illustrates that trajectory climatologies not limited to dust can grossly overestimate the potential for dust transport.Preferential pathways emerge that demonstrate the role of Iceland in supplying dust to the Northern Atlantic and sub-Arctic oceans. For dust emitted from northern sources, a dominant route exists to the northeast, into the Norwegian, Greenland and Barents Seas, although there is also potential for delivery to the North Atlantic in summer months. From the southern sources, the primary pathway extends into the North Atlantic, with a high density of trajectories extending as far south as 50°N, particularly in spring and summer. Common to both southern and northern sources is a pathway to the west-southwest of Iceland into the Denmark Strait and towards Greenland. For trajectories simulated at ≤500 m, the vertical development of dust plumes from Iceland is limited, likely due to the stable air masses of the region suppressing the potential for vertical motion. Trajectories rarely ascend high enough to reach the central portions of the Greenland Ice Sheet. The overall distribution of trajectories suggests that contributions of Icelandic dust are relatively more important for neighbouring marine environments than the cryosphere.

The Spatial Variation of Dust Particulate Matter Concentrations during Two Icelandic Dust Storms in 2015

Particulate matter mass concentrations and size fractions of PM1, PM2.5, PM4, PM10, and PM15 measured in transversal horizontal profile of two dust storms in southwestern Iceland are presented. Images from a camera network were used to estimate the visibility and spatial extent of measured dust events. Numerical simulations were used to calculate the total dust flux from the sources as 180,000 and 280,000 tons for each storm. The mean PM15 concentrations inside of the dust plumes varied from 10 to 1600 µg·m−3 (PM10 = 7 to 583 µg·m−3). The mean PM1 concentrations were 97–241 µg·m−3 with a maximum of 261 µg·m−3 for the first storm. The PM1/PM2.5 ratios of >0.9 and PM1/PM10 ratios of 0.34–0.63 show that suspension of volcanic materials in Iceland causes air pollution with extremely high PM1 concentrations, similar to polluted urban areas in Europe or Asia. Icelandic volcanic dust consists of a higher proportion of submicron particles compared to crustal dust. Both dust storms occurred in relatively densely inhabited areas of Iceland. First results on size partitioning of Icelandic dust presented here should challenge health authorities to enhance research in relation to dust and shows the need for public dust warning systems.

Insulation effects of Icelandic dust and volcanic ash on snow and ice

In the Arctic region, Iceland is an important source of dust due to ash production from volcanic eruptions. In addition, dust is resuspended from the surface into the atmosphere as several dust storms occur each year. During volcanic eruptions and dust storms, material is deposited on the glaciers where it influences their energy balance. The effects of deposited volcanic ash on ice and snow melt were examined using laboratory and outdoor experiments. These experiments were made during the snow melt period using two different ash grain sizes (1 ϕ and 3.5 ϕ) from the Eyjafjallajokull 2010 eruption, collected on the glacier. Different amounts of ash were deposited on snow or ice, after which the snow properties and melt were measured. The results show that a thin ash layer increases the snow and ice melt but an ash layer exceeding a certain critical thickness caused insulation. Ash with 1 ϕ in grain size insulated the ice below at a thickness of 9–15 mm. For the 3.5 ϕ grain size, the insulation thickness is 13 mm. The maximum melt occurred at a thickness of 1 mm for the 1 ϕ and only 1–2 mm for 3.5 ϕ ash. A map of dust concentrations on Vatnajokull that represents the dust deposition during the summer of 2013 is presented with concentrations ranging from 0.2 up to 16.6 g m−2.

Quantification of iron-rich volcanogenic dust emissions and deposition over the ocean from Icelandic dust sources

Abstract. Iceland has extremely active dust sources that result in large-scale emissions and deposition on land and at sea. The dust has a volcanogenic origin of basaltic composition with about 10% Fe content. We used two independent methods to quantify dust emission from Iceland and dust deposition at sea. Firstly, the aerial extent (map) of deposition on land was extended to ocean areas around Iceland. Secondly, surveys of the number of dust events over the past decades and calculations of emissions and sea deposition for the dust storms were made. The results show that total emissions range from 30.5 (dust-event-based calculation) to 40.1 million t yr−1 (map calculation), which places Iceland among the most active dust sources on Earth. Ocean deposition ranges between 5.5 (dust event calculations) and 13.8 million tons (map calculation). Calculated iron deposition from Icelandic dust ranges between 0.567 and 1.4 million tons, which are distributed over wide areas (>370 000 km2) and consist of fine reactive volcanic materials. The paper provides the first quantitative estimate of total dust emissions and oceanic deposition from Iceland. Iron is a limiting nutrient for primary production in the oceans around Iceland, and the dust is likely to affect Fe levels in Icelandic ocean waters.

Snow–Dust Storm: Unique case study from Iceland, March 6–7, 2013

Iceland is an active dust source in the high-latitude cold region. About 50% of the annual dust events in the southern part of Iceland take place at sub-zero temperatures or in winter, when dust may be mixed with snow. We investigated one winter dust event that occurred in March 2013. It resulted in a several mm thick dark layer of dust deposited on snow. Dust was transported over 250 km causing impurities on snow in the capital of Iceland, Reykjavik. Max one-minute PM10 concentration measured in Kirkjubæjarklaustur (20–50 km from the dust source) exceeded 6500 μg m−3 while the mean (median) PM10 concentration during 24-h storm was 1281 (1170) μg m−3. Dust concentrations during the dust deposition in Reykjavik were only about 100 μg m−3, suggesting a rapid removal of the dust particles by snow during the transport. Dust sample taken from the snow top layer in Reykjavik after the storm showed that about 75% of the dust deposit was a volcanic glass with SiO2 ∼45%, FeO ∼14.5%, and TiO2 ∼3.5. A significant proportion of organic matter and diatoms was also found. This case study shows that severe dust storms are related also to meteorological conditions, such as winter snow storms, and moist conditions. Small volcanic dust particles deposited on snow tend to form larger particles (“clumping mechanism”) resulting in stronger light absorbance. This is one of the first reports on the “clumping mechanism” observed in natural conditions. The deposition of Icelandic dust on snow, glaciers and sea ice may accelerate the thaw, with the potential to increase the anthropogenic Arctic warming.

Long-term frequency and characteristics of dust storm events in Northeast Iceland (1949–2011)

Long-term records of meteorological dust observations from Northeast Iceland were analysed and frequency of dust events from Icelandic deserts calculated. A total of 1033 dust days were reported during the period 1949–2011 with an annual mean of 16.4 dust days year−1, placing the area among the dustiest areas in the world. The most active decades were the 2000s, 1990s and 1950s. Monthly dust event frequency is bimodal with primary and secondary maxima in June and September. A total of 14 severe dust storms (visibility < 500 m) occurred during the period. Median dust event concentration was calculated as 106 μg m−3 from the visibility observations. The frequency and severity of dust events depend on Sea Level Pressure (SLP) oscillation which controls the southerly winds in NE Iceland. The availability of fine sediments susceptible to dust production in outwash plains controlled by the flow rate of glacial river is also important. Volcanic ash from eruptions in 2010 and 2011 barely affected the dust event frequency in NE Iceland. Icelandic dust may be substantial source for large scale air pollution in the Arctic.