High Terahertz Research Articles

Design and error analysis of simple terahertz high birefringence microstructured fiber

Abstract High birefringence fibers are significant in the terahertz technology field, serving as waveguides for terahertz transmission. They are applicable in various fields such as communication, imaging. Integrating metal microstructures into polymer microstructured optical fibers can effectively modulate the transmission characteristics of the fiber, enhancing birefringence and reducing loss, thereby achieving better performance compared to traditional single-material fibers. This paper presents a structurally simple terahertz high birefringence microstructured fiber, where the introduction of gold microstructures enhances the birefringence of fiber, with a maximum birefringence of up to 1.089 × 10-2. We also discuss several manufacturing errors that may occur during the fiber fabrication process. The results indicate that the designed fiber exhibits significant manufacturing tolerance. Variations in the thickness and angle of the gold microstructures, as well as the angular offset of the elliptical cladding wall, peak-to-valley errors, and changes in the aspect ratio of the elliptical tube, have relatively minor effects on the overall transmission performance. The research findings provide insights for designing subsequent high birefringence terahertz fibers, thereby propelling advancements in this field. They offer a theoretical basis for the preparation of related microstructured fiber structures and provide valuable understanding for optimizing fiber manufacturing processes.

High brightness terahertz quantum cascade laser with near-diffraction-limited Gaussian beam

High-power terahertz (THz) quantum cascade laser, as an emerging THz solid-state radiation source, is attracting attention for numerous applications including medicine, sensing, and communication. However, due to the sub-wavelength confinement of the waveguide structure, direct beam brightness upscaling with device area remains elusive due to several mode competition and external optical lens is normally used to enhance the THz beam brightness. Here, we propose a metallic THz photonic crystal resonator with a phase-engineered design for single mode surface emission over a broad area. The quantum cascade surface-emitting laser is capable of delivering an output peak power over 185 mW with a narrow beam divergence of 4.4° × 4.4° at 3.88 THz. A high beam brightness of 1.6 × 107 W sr−1m−2 with near-diffraction-limited M2 factors of 1.4 in both vertical and lateral directions is achieved from a large device area of 1.6 × 1.6 mm2 without using any optical lenses. The adjustable phase shift between the lattices enables a stable and high-intensity surface emission over a broad device area, which makes it an ideal light extractor for large-scale THz emitters. Our research paves the way to high brightness solid-state THz lasers and facilitates new applications in standoff THz imaging, detection, and diagnosis.

Design and simulation of a high sensitivity terahertz metamaterial sensor based on plasmon-induced transparency

Design and simulation of a high sensitivity terahertz metamaterial sensor based on plasmon-induced transparency

Mechanism of the Terahertz Wave-MXene Interaction and Surface/Interface Chemistry of MXene for Terahertz Absorption and Shielding.

ConspectusOver the past two decades, terahertz (THz) technology has undergone rapid development, driven by advancements and the growing demand for THz applications across various scientific and technological domains. As the cornerstone of THz technology, strong THz-matter interactions, especially realized as high THz intrinsic absorption in nanometer-thick materials, play a highly important role in various applications including but not limited to THz absorption/shielding, detection, etc. The rigorous electromagnetic theory has posited a maximum intrinsic absorption of 50% for electromagnetic waves by thin films, and the succinct impedance matching condition has also been formulated to guide the design of highly intrinsically absorbing materials. However, these theories face challenges when applied to the THz spectrum with an ultrabroad bandwidth. Existing thin films typically achieve a maximum intrinsic absorption within a narrow frequency range, significantly limiting the performance of THz absorbers and detectors. To date, both theoretical frameworks and experimental solutions are lacking in overcoming the challenge of achieving broadband maximum intrinsic absorption in the THz regime.In this Account, we describe how two-dimensional (2D) transition-metal carbide and/or nitride (MXene) films with nanometer thickness can realize the maximum intrinsic absorption in the ultrabroad THz band, which successfully addresses the forementioned longstanding issue. Surprisingly, traditional DC impedance matching theory fails to explain this phenomenon, while we instead propose a novel theory of AC impedance matching to provide a satisfactory explanation. By delving into the microscopic transport behavior of free electrons in MXene, we discover that intraflake transport dominates terahertz conductivity under THz wave excitation, while interflake transport primarily dictates DC conductivity. This not only elucidates the significant disparities between DC and AC impedance in MXenes but also underscores the suitability of AC impedance matching for achieving broadband THz absorption limits. Furthermore, we identify a high electron concentration and short relaxation time as crucial factors for achieving broadband maximum absorption in the THz regime. Although approaching the THz intrinsic absorbing limits, it still faces hurdles to the use of MXene in practical applications. First, diverse and uncontrollable terminations exist on the surface of MXene stemming from the synthesis process, which largely influence the electron structure and THz absorbing property of MXene. Second, MXene suffers from poor stability in the presence of oxygen and water. To address the above issues, we have undertaken distinctive works to precisely control the terminations and suppress the oxidation of MXene even at high temperature through surface and interface chemistry, such as low-temperature Lewis basic halide treatment and building a Ti3C2Tx/extracted bentonite (EB) interface. For practical application consideration, we proposed a copolymer-polyacrylic latex (PAL)-based MXene waterborne paint (MWP) with a strong intermolecular polar interaction between MWP and the substrate provided by the cyano group in PAL. This not only has strong THz EMI shielding/absorption efficiency but also can easily adhere to various substrates that are commonly used in the THz band. These studies may have significant implications for future applications of MXene nanofilms in THz optoelectronic devices.

Absorption dominated broadband terahertz electromagnetic shielding properties of ultrathin rGO paper

The demand for absorption-dominated terahertz (THz) electromagnetic shielding materials is critical in THz devices or components for electromagnetic compatibility and protection. However, it is challenging to find out an ultrathin, absorption-dominated shielding material with high absorptivity in a broad range. Herein, we demonstrate the hydrogen iodine (HI) acid reduced graphene oxide (rGO) ultrathin paper as a promising candidate for absorption-dominated electromagnetic interference (EMI) shielding. By optimizing the conductivity and layered structures, rGO paper with thickness of only 13 μm exhibited an absorption-dominated EMI shielding effectiveness (SE) of 21.09 dB in a broad band from 0.2 to 1.2 THz. Simple stacking of the rGO papers further improved the EMI SE up to 42.53 dB with a total thickness of 40 μm. rGO papers can also be integrated into structured substrates for applications in different scenarios. Covering a single rGO paper onto the wedge structure array, a broadband THz absorption over 99 % can be achieved. Similarly, combining rGO papers and arrays of zinc pyramids, and the average SE and the max THz absorption were enhanced to 54.83 dB and 99.986 %, respectively. We believe this absorption-dominated THz shielding rGO paper paves an efficient avenue towards high performance THz shielding/absorption devices for diverse applications.

A quad-port triple-band high isolation terahertz MIMO antenna for short-distance THz communication links

This paper introduces an arrangement of a Multiple-Input Multiple-Output antenna array implemented specifically for operating within the THz frequency bands. The antenna is designed for short-distance THz communication links. A quad-port MIMO antenna configuration has been chosen to function across three frequency bands. Each cell element is situated on top of a silicon substrate. The combined cross-sectional surface of the MIMO antenna is 70 × 50 µm². The proposed MIMO antenna device reaches the following three frequency bands: 2.6–7.9 THz, 9.66–10.3 THz and 11.5–14.1 THz. In addition, the mutual coupling coefficient is less than − 20 dB, indicating strong isolation between antenna elements. This high isolation is obtained by using a defected sibstrat structure and a specifique distance between antenna elements. The MIMO array antenna attains peak gains of 11.88 dBi, 8.78 dBi and 10.65 dBi when operating over the three cited bandwidth. Furthermore, the suggested MIMO structure exhibits favorable characteristics with CCL < 0.5 bps/Hz/sec, MEG ≤ –3.0 dB, ECC < 0.01, and DG ≈ 10 dB, over the operating bands. Based on the results obtained and compared to several works reported in the literature, the proposed implementation maintains a good size-performance compromise which allows better adaptation to applications requiring versatile performance in various communication scenarios.

Enhancement of terahertz fields in LiTaO3 waveguides using a conical pulse front.

The development of methods for the generation of strong ultrafast electromagnetic pulses in the terahertz (THz) spectral range has led to a surge of progress in nonlinear THz spectroscopy and THz control of molecular and collective responses. For spectroscopy in the 1-THz range, the submillimeter wavelengths and associated large spot sizes, large optical elements, and short distances between final focusing elements and samples can lead to cumbersome experimental setups that are incompatible with some sample environments. Here, we introduce a novel terahertz ring excitation (TREx) optical pumping geometry to generate superposing, focusing fields in planar THz waveguides made out of the electro-optic material lithium tantalate. High THz fields, >175 kV/cm, are generated and measured optically with no free-space THz propagation. The field level achieved by pumping with a sequence of concentric rings of excitation light exceeds by about 20× the result of a single cylindrically focused line of pump light that has been used routinely in previous work. The technique opens new prospects for compact waveguide-based linear and nonlinear THz spectroscopy and signal processing.

THz vs NIR laser-assisted atom probe tomography of LaB6 samples

Terahertz (THz) radiation with low-energy photons (meV) is used in a wide range of applications, such as microscopy, sensing, and spectroscopy. However, recently, high amplitude THz pulses of MV/cm have been generated and used for electron emission and ion evaporation from field emitters, opening up the possibility of using high amplitude THz pulses for material imaging by THz-assisted atom probe tomography (APT). In this work, we compare the APT analyses of lanthanum hexaboride (LaB6) samples using a femtosecond near-infrared laser with those obtained using high-amplitude single-cycle THz pulses. The atomic-scale characterization of stoichiometric LaB6 is challenging in laser-assisted APT due to the detection losses of boron ions. Here, we show that the THz radiation reduces the emission of molecular ions and multiple detection events, and it increases the charge state of the emitted ions. All these effects result in an improvement in boron detection. Furthermore, the emission dynamics of boron and lanthanum ions differ in their evaporation times when using THz radiation. This work emphasizes the ability of high-amplitude, single-cycle THz pulses to well control material analysis in APT, leading to better results on chemical composition. It also paves the way for the use of this radiation for material manipulation.

High performance THz metasurface sensor based on modified-SWCNTs film for femtomolar protein detection

Terahertz (THz) metasurface sensor plays an important role in environmental monitoring, biomedical diagnostics, and materials science. However, most traditional THz metasurfaces for trace biological substance detection either suffer from high ohmic loss, or cannot achieve ultra-low concentration detection at the femtomolar level, which limits the application range of THz metasurfaces. Here, we propose a novel metasurface based on modified single-walled carbon nanotubes (SWCNTs) film for specific detection of SAA protein in femtomolar concentration. By modifying the SWCNTs film with concentrated sulfuric acid and introducing functionalized gold nanoparticles (Au-NPs), not only the non-resonant loss of the SWCNTs film was greatly reduced, but also the specific selection of trace SAA proteins was achieved. We experimentally demonstrated that the sensitivity of this THz metasurface sensor for SAA protein detection is 37.5 GHz/fM. In contrast to conventional metal or dielectric metasurfaces, because the unique mesh-like structure of the SWCNTs film can greatly increase the interaction between trace substances and the sensor, this new modifiable metasurface can achieve the lowest detection limit of 0.1 fM, which has increased by an order of magnitude. Our results provide a new and promising method for THz metasurfaces to realize high-performance biosensors.

High sensitivity terahertz biomedical sensing with graphene metamaterial

Identification of biomedical molecules by terahertz (THz) sensing is a quite promising noninvasive technique. Here, we present a THz graphene metamaterial with plasmon-induced transparency (PIT) for high sensitivity biosensing. The strong PIT effect is generated by the destructive interference between the plasmon modes excited by two graphene strips. For testing different biomedical analytes, a distinct frequency shift at PIT resonance can be observed due to the effect of surrounding refractive index variation. The metamaterial scheme for noninvasive biomedical sensing can achieve the sensitivity as high as 2.6 THz/RIU. Particular, it can not only detect the phase of red blood cell infected by malaria but also the concentration of ethanol aqueous solution. The underlying mechanism is discussed for understanding the THz sensing operation.

High repetition rate coherent terahertz synchrotron radiation via self-amplified energy modulation

Coherent terahertz (THz) radiation sources based on a storage ring hold a significant future for generating high average power terahertz radiation, as the electron beam possesses a high revolution frequency. We propose a novel scheme to generate a high repetition rate coherent THz radiation leveraging the energy modulation self-amplification technology. In this scheme, utilizing the interaction of external intensity-modulated laser pulses with the electron beam can lead to a customized manipulation of the electron beam, such as a periodic longitudinal density modulation with a submillimeter scale for coherent THz radiation. Positively, it can propel the repetition rate when the peak power requirement of an external laser system is decreased. Thus, we employ a self-modulation method to enhance the initial weak energy modulation induced by the laser directly. In the meanwhile, the use of self-modulation can bypass the limitation that the bandwidth of a long modulator should be smaller than that of the external wideband laser source, which is necessary to shape the intensity envelope flexibly. The one-dimensional analytical description of electron longitudinal dynamic during the self-modulation process is given, which confirms the effective enhancement of the modulation at THz band. Three-dimensional time-dependent simulation results based on the parameters of Hefei light source-II show that the coherent THz radiation pulses with a repetition rate of 10 kHz can be generated. Published by the American Physical Society 2024

Extreme terahertz magnon multiplication induced by resonant magnetic pulse pairs

Nonlinear interactions of spin-waves and their quanta, magnons, have emerged as prominent candidates for interference-based technology, ranging from quantum transduction to antiferromagnetic spintronics. Yet magnon multiplication in the terahertz (THz) spectral region represents a major challenge. Intense, resonant magnetic fields from THz pulse-pairs with controllable phases and amplitudes enable high order THz magnon multiplication, distinct from non-resonant nonlinearities such as the high harmonic generation by below-band gap electric fields. Here, we demonstrate exceptionally high-order THz nonlinear magnonics. It manifests as 7th-order spin-wave-mixing and 6th harmonic magnon generation in an antiferromagnetic orthoferrite. We use THz two-dimensional coherent spectroscopy to achieve high-sensitivity detection of nonlinear magnon interactions up to six-magnon quanta in strongly-driven many-magnon correlated states. The high-order magnon multiplication, supported by classical and quantum spin simulations, elucidates the significance of four-fold magnetic anisotropy and Dzyaloshinskii-Moriya symmetry breaking. Moreover, our results shed light on the potential quantum fluctuation properties inherent in nonlinear magnons.

Characterization of High Sensitivity Terahertz Metasurface Resonance With Application to Tumor Cell Detection

Characterization of High Sensitivity Terahertz Metasurface Resonance With Application to Tumor Cell Detection

A metasurface structure-assisted terahertz negative curvature fiber

Negative curvature fibers have the benefits of high bandwidth, low loss, and provide higher transmission performances. Birefringence of the fiber is particularly important, with potential application value in communication, imaging and other fields. In this paper, a metasurface structure-assisted terahertz negative curvature fiber is designed to improve the birefringence characteristic. This work breaks through the conditional design ideas, and theoretically analyzes the effect of adding gold microstructures in the cladding structures on the transmission characteristics of negative curvature fibers. The investigation results show that the birefringence of the designed fiber exhibits a significant increase in most frequency range between 1.75–2.4 THz compared to the results before adding gold microstructures. The maximum birefringence reaches as high as 0.00216 when the frequency is 2.175 THz and θ is 90°. Compared to the original frequency, the birefringence has increased by nearly an order of magnitude. The highest birefringence has been increased to 3.5 times. In addition, the influences of the gold microstructures on the confinement loss, waveguide dispersion, and effective mode field area are also investigated. This fiber provides a reference for the design of high birefringence terahertz fibers in the future.

Super-resolution terahertz imaging based on a meta-waveguide.

A terahertz metamaterial waveguide (meta-waveguide) and a meta-waveguide-based lens-free imaging system are presented. The meta-waveguide not only inherits the low-loss transmission performance of a waveguide but also breaks through the diffraction limit under the action of the metamaterial, achieving subwavelength focusing. The focusing distance is far greater than the Rayleigh length, thus enabling far-field scanning imaging. For verification, a metal ring-based meta-waveguide was fabricated by 3D printing and metal cladding technology. Then, a transmission scanning imaging system working at 0.1 THz was built. High quality terahertz images with a resolution of 1/3 of the wavelength were obtained by placing the imaging targets at the focus and performing two-dimensional scanning. The focusing and transmission of terahertz wave in the meta-waveguide were simulated and analyzed.

An Ultra-high Quality Factor Terahertz Photonic Crystal Cavity

High quality factor Terahertz (THz) cavities are highly desired for many THz applications. This paper presents an ultra-high quality factor terahertz planar photonic crystal cavity at 300 GHz range. Two approaches are employed to reduce the losses in the cavity increasing the quality factor of the cavity. Firstly, short embedded photonic crystal waveguides are employed to reduce the in – plane loss. Secondly, a novel way of hole displacement is adopted for four edged holes of the L3 – type photonic crystal cavity to decrease the radiation loss. An ultra – high quality factor of 65000 at a resonant frequency of 315.3 GHz was achieved for the designed cavity. This result could enable promising applications such as THz sensing.

Hollow metal tubes for efficient electron manipulation using terahertz surface waves.

Compact electron sources have been instrumental in multidiscipline sciences including fundamental physics, oncology treatments, and advanced industries. Of particular interest is the terahertz-driven electron manipulation that holds great promise for an efficient high gradient of multi-GeV/m inside a regular dielectric-lined waveguide (DLW). The recent study relying on terahertz surface waves has demonstrated both high terahertz energy and improved coupling efficiency with the DLW. However, the large energy spread pertaining to the laser-induced electron pulse impedes the practical use of the system. Here, we propose a scheme for extending the idea of surface-wave-driven electron manipulation to mature electron sources such as commercial direct-current and radio-frequency electron guns. By using a simple hollow cylinder tube for electron transmission, we show that the electron energy modulation can reach up to 860 keV, or compress the electron pulse width to 15 fs using a 2.9 mJ single-cycle terahertz pulse. The trafficability of the hollow tube also allows for a cascade of the system, which is expected to pave the way for compact and highly efficient THz-driven electron sources.

Temperature-Dependent Electromagnetic Surface Wave Supported by Graphene-Loaded Indium Antimonide Planar Structure

In this study, the propagation characteristics of EM surface waves supported by the graphene-coated indium antimonide (InSb) planar waveguide have been investigated theoretically and numerically. The modeling of graphene has been performed by use of Kubo formalism whereas the relative permittivity of indium antimonide has been calculated using Drude’s model. The results for transverse electric (TE) and transverse magnetic (TM) polarized surface waves have been computed analytically and numerically. The major challenge is to model the atomically thick graphene sheet over the InSb grounded slab. To get the temperature-dependent characteristic equation for the electromagnetic surface waves, the surface current boundary conditions’ approach has been employed. The numerical results have been computed for both the TE and TM polarization states and reported that the TE does not support the propagation of surface waves. The dispersion relation, effective mode index, phase speed, propagation length, and field profile have been computed in Mathematica under TM polarization. The graphene and indium antimonide have been found active for low and high Terahertz regions, respectively. As temperature increases, the plasma frequency of the InSb increases due to this reason with the increase of temperature and the resonance frequency, leading to a shift in the dispersion curve. Moreover, with the increase of temperature, the effective wave number of transverse magnetic polarized surface waves also increases. Resultantly, the confinement of such surface waves supported by graphene-loaded InSb increases. It is shown that with the variation of temperature of indium antimonide, the surface waves propagating across the interface can be tuned in the Terahertz region and can be exploited for thermo-optical sensing, near-field communications waveguides, and graphene-based temperature sensor designing.

Terahertz Conductivity of Free-Standing 3D Covalent Organic Framework Membranes Fabricated via Triple-Layer-Dual Interfacial Approach.

Processable covalent organic framework membranes (COFM) are emerging as potential semiconducting materials for device applications. Nevertheless, the fabrication of crystalline and free-standing 3D COFMs is challenging. In this work, a unique time and solvent-efficient triple-layer-dual interfacial (TLDI) approach for the simultaneous synthesis of two 3D COFMs from a single system is developed. Besides, for the first time, the optical conductivity of these free-standing 3D COFMs is analyzed using terahertz (THz) spectroscopy in transmission mode. Interestingly, these membranes show excellent transmittance at THz frequencies with very high intrinsic THz conductivities. The evaluated scattering time and plasma frequency of the free carriers of the COFMs are highly promising for future applications in optoelectronic devices in THz frequencies.

Recent progress of THz source at the SXFEL

Coherent, wide-tunable frequency and high intensity terahertz (THz) source is under preparation at the Shanghai Soft X-ray free-electron laser facility (SXFEL). The electron bunches modulated by frequency beating light can generate coherent, wide-tunable, high intensity THz radiation from 0.1 to 30 THz through wigglers. The electromagnetic wiggler with peak magnetic field up to 1.75 T is adopted and the parameters of the wiggler are optimized to ensure the generation of strong field THz radiation. Due to the limitation of layout space of the SXFEL, the length of wiggler is limited within 5 meters. By properly increasing the charge of the electron beam, the THz pulse energy can be kept at sub mJ level under the proposed different parameters of the wiggler. In this article, we will present the possible layout of THz source on the SXFEL and the S2E simulation of THz radiation of sub mJ magnitude within the 5-meter wiggler.