High-power Sources Research Articles

What is Multi-extreme THz ESR? Developments and its Applications

AbstractThis review explores the multi-extreme THz ESR system in Kobe, Japan, with a focus on pulsed magnetic fields, mechanical detection, and high pressure as central elements of multi-extreme THz ESR. Initially, it discusses the advantages of multi-frequency THz ESR using mini-pulsed and 55 T‒pulsed magnetic fields, with typical examples featuring the finite Haldane chain substance Y2BaNi0.96Mg0.04O5 and the deformed diamond chain antiferromagnet Cu3(CO3)2(OH)2 (Azurite). The measurement efficiency and the measurement beyond the magnetic phase transition, in contrast to the conventional superconducting magnet, are discussed. Second, the high sensitivity obtained from the use of a nano-membrane for mechanical detection is shown. Also shown are the high-temperature (280 K) THz ESR results for DPPH powder and a Cu(C4H4N2)(NO3)2 (CuPzN) single crystal, with the combination of a nano-membrane device and a high-power source, a gyrotron. Finally, the high-pressure THz ESR results for KCuCl3 using a transmission-type double-layered pressure cell are shown, along with the application of the thermally detected high-pressure THz ESR.

Blacklight sintering of BaZrO3-based proton conductors

Acceptor-doped BaZrO3, a ceramic proton conductor, is well researched for use in solid oxide fuel cells due to its proton conductivity and chemical stability. A major drawback of the material is the difficulty of sintering as it requires high sintering temperatures and long heating times (> 1600 °C, 24 h). An emerging sintering technology to mitigate this challenge is blacklight sintering, which uses a high-powered blue or UV light source to heat ceramics extremely fast leading to short sintering times and reduced energy demand. In this work, BaZr0.8Y0.2O3-δ (BZY20) and BaZr0.8Y0.1Sc0.1O3-δ (BZY10Sc10) were blacklight-sintered with a high-power blue laser in under four minutes. Even though the resulting samples have a gradient from large to small grains and structurally disordered grain boundaries, the proton conductivity is comparable to conventionally sintered samples. Hence, blacklight sintering is a promising technology with the potential to sinter BaZrO3 much faster, while saving energy.

Research on mid-infrared quantum cascade lasers spectral beam combining

Quantum cascade lasers (QCLs) in the mid-infrared (MIR) hold significant potential for widespread applications in both military and civilian contexts. However, the utility of present single-chip QCLs is hampered by issues such as low output power and subpar beam quality. This study addresses these limitations by employing spectral beam combining (SBC) based on a diffraction grating, with an aim to enhance both power and beam quality of MIR QCLs. Coaxial power synthesis of three single-chip QCLs (around 4.75 μm) is achieved experimentally, importantly, the beam quality did not decrease after combining, essentially maintaining the same quality as before combining. It is proposed that there are four main factors affecting the combining efficiency, namely operating optical power (or driving current) of the chips, individual differences in QCL chips, diffraction grating, and reflectivity of feedback mirror, and their effects on the combining efficiency are discussed separately. This study confirms that SBC is an effective way to obtain high-power and high-beam quality MIR QCL sources, and lays a research foundation for more beam spectral combining.

Roadmap on basic research needs for laser technology

Abstract Motivated by the profound impact of laser technology on science, arising from an increase in focused light intensity by seven orders of magnitude and flashes so short electron motion is visible, this roadmap outlines the paths forward in laser technology to enable the next generation of science and applications. Despite remarkable progress, the field confronts challenges in developing compact, high-power sources, enhancing scalability and efficiency, and ensuring safety standards. Future research endeavors aim to revolutionize laser power, energy, repetition rate and precision control; to transform mid-infrared sources; to revolutionize approaches to field control and frequency conversion. These require reinvention of materials and optics to enable intense laser science and interdisciplinary collaboration. The roadmap underscores the dynamic nature of laser technology and its potential to address global challenges, propelling progress and fostering sustainable development. Ultimately, advancements in laser technology hold promise to revolutionize myriad applications, heralding a future defined by innovation, efficiency, and sustainability.

Modeling the hundreds-of-nanoseconds-long irradiation of tin droplets with a 2 µm-wavelength laser for future EUV lithography

Abstract The properties of an extreme ultraviolet (EUV) source driven by hundreds-of-nanoseconds-long laser pulses of λ laser = 2 µm wavelength are investigated through radiation-hydrodynamic simulations. We show that single-pulse irradiation of 30 µm-diameter tin droplets can generate in-band energies ∼ 30 mJ directed in the 2π sr solid angle subtended by the collector mirror, yielding energies ∼100 mJ produced from 45 µm-diameter droplets. Time-integrated in-band EUV emission profiles, generated by taking Abel transforms of the local net in-band emissivity, reveal EUV source sizes in the axial (laser) direction × radial direction of ∼600 (1000) × 100 (150) µm2 for 30 (45) µm-diameter droplets. We find that approximately 74% of the total in-band emission is produced during the first half of the total propulsion distance irrespective of droplet size or laser intensity. Furthermore, we propose a one-dimensional analytical propulsion model to qualitatively explain the simulated droplet trajectory and to predict the time taken for the droplet to vaporize. These findings offer motivation for the development of high-power EUV sources based on single-pulse, hundreds-of-nanoseconds-long irradiation of tin droplets.

Plasma discharge experiments of a Faraday shieldless driver for high-power and long-pulse radio frequency ion source for NBI application.

Due to the high stability and less maintenance, the radio frequency (RF) driven ion source is preferred for the neutral beam injection (NBI) system. In a popular design of the RF ion source for NBI application, a Faraday shield (FS) is installed inside the RF plasma driver to protect the discharge tube. However, the FS also brings some drawbacks, such as lowering the RF power transfer and increasing the processing difficulty. A prototype of the RF plasma driver without FS and with mature manufacturing technology has been developed by using a water-cooled discharge tube. After basic testing, this prototype was further tested under the RF plasma discharge experiments in views of high power, long pulse, and long term. The reliability and its plasma characteristics were the focus of these experiments, also for the hidden issues. The results show that the prototype could generate stable and high-density plasma without any damage or sputtering mark. An RF plasma discharge of 50 kW and 20s has been achieved. The expected frequency tuning was equally effective on the prototype. Moreover, compared to the RF plasma driver with FS, the prototype could produce higher electron density in the extraction region under the same RF power. Of course, some of the shortcomings of the prototype have also been exposed in the experiments and will be improved in subsequent experiments.

Research on a broad-band X-band high power relativistic klystron amplifier

This paper introduces a high-power broadband X-band klystron amplifier that achieves an output power of 157 MW and a 3 dB operating bandwidth of 6.7%. The amplifier employs an explosive emission diode with high impedance, which balances the requirements of high power and broadband. The multi-gap input and output cavities are designed to operate at two different longitudinal modes within the operating frequency band, resulting in a flat absorption rate and output efficiency. Moreover, an eight-stage stagger-tuned bunching section is implemented to achieve a uniform fundamental harmonic current modulation depth across the frequency band. Simulation results indicate that when the diode voltage is 550 kV and the beam current is 550 A, the amplifier can achieve a maximum power of 157 MW with an efficiency of 51.9% at the central frequency of 9.8 GHz. Furthermore, within the 3 dB operating bandwidth of 6.7% (670 MHz), the power output remains higher than 80 MW. This novel klystron amplifier structure exhibits exceptional performance in terms of bandwidth, power, and efficiency, thus validating the effectiveness of the design in enhancing bandwidth and providing a solid foundation for the broadband design of high-power microwave sources.

Conductive Li2S‐NbSe2 Cathode Material Capable of Bidirectional Self‐Activation for High‐Performance All‐Solid‐State Lithium Metal Batteries

AbstractAll‐solid‐state lithium metal batteries (ASSLBs) offer an alternative route to safe and high energy density power sources. Sulfur‐based cathodes with high theoretical specific capacity and low cost are crucial for advancing ASSLBs. However, the electronic insulation and sluggish kinetics of sulfide materials like Li2S severely limit battery performance. Herein, the strategy is proposed that a highly electronic conductive Li2S‐NbSe2 material enhances the electrochemical performance through bidirectional self‐activation. The chemical interaction between Li2S and NbSe2 induces NbSe2‐xSx and Li2Se derivatization, serving as the basis for activation. The carrier transport properties, chemical evolution and self‐activation mechanism of Li2S‐NbSe2 during the oxidation–reduction process are revealed. The chemical activation of NbSe2‐xSx is explored to accelerate the electrochemical processes by modifying the conductivity of sulfur species and the conversion pathways without insulating Li2S and S aggregation. Therefore, ASSLBs using Li2S‐NbSe2 as cathode active material achieve an electrode‐level energy density of 394 Wh kg−1 and a power density of 524 W kg−1 at 1 C (4.35 mA cm−2) and 25 °C. The capacity retention after 100 cycles at 0.5 C is ≈99.3% with almost no degradation. This work provides new options and insights for the rational design and development of chalcogenide cathode active materials for high‐performance ASSLBs.

Experimental study on plasma characteristics in the extraction region of a high-power RF negative ion source based on electrostatic probe

Abstract The plasma characteristics of the extraction region in high-power RF negative ion source have a significant impact on the production and extraction of negative hydrogen ions. This study utilized electrostatic probe to investigate the effect of RF power, source pressure, magnetic filter field and bias voltage on the plasma parameters of the extraction region (without cesium), and also studied the variation of plasma parameters with position and time. The results indicate that as RF power increases, the plasma density in the extraction region significantly rises, but it also leads to an increase in the electron temperature ( T e ) of the extraction region (which increases the loss of negative hydrogen ions); increasing the source pressure can effectively increase the electron density ( N e ) in the extraction region and reduce T e as expected; increasing the magnetic filter field can effectively reduce the T e in the extraction region, but after the plasma grid current exceeds 1900 A, the change in T e is not significant; although increasement of the bias voltage can effectively suppress the N e in the extraction region, it causes T e to rise; moreover, the distribution of plasma parameters in the extraction region is relatively uniform; in addition, the variation of plasma parameters with time is not obvious. These findings not only deepen the understanding of the physical mechanisms of plasma behavior in the extraction region of negative ion sources, but also provide important theoretical and experimental bases for the optimization of high-power RF negative ion sources.

Determination of the electron temperature and electron density in reduced pressure hydrogen peroxide (H2O2) discharge.

A reduced pressure glow discharge is produced by passing a high-power pulsed DC source of 0-500W with a frequency of 50Hz across two parallel disk electrodes. A hydrogen peroxide aqueous solution is used as a flowing gas for discharge generation. Optical emission spectroscopy is employed to diagnose the discharge generated at a reduced pressure of 0.2mbar with an electrode gap of 4cm. The spectra are recorded at a power density of 9.4 mW/cm3 and typically lie in the visible wavelength range of 380-880nm. The spectra are analyzed using the line intensity ratio method to estimate electron temperature and density. The results indicated that the electron temperature and density are, respectively, 0.87eV and 6.4 × 1014cm-3.

Calculations for preemptive surface adsorbate drive-off to minimize plasma formation during operation of high-power microwave sources

Thermal driven desorption of surface impurities is probed based on coupled Monte Carlo–heat flow–molecular dynamics simulations. Such adsorbates can lead to plasma formation during the operation of high-power microwave systems with various negative outcomes and so need to be curtailed. Our study attempts to obtain temperature thresholds for desorbing different surface contaminants such as C2, O2, CO, and CO2. The results show that carbon-based adsorbates on copper (chosen as an example anode material) could be ejected at a relatively modest surface temperature of 650 K. On the other hand, reactive species such as oxygen are very stable due to their large cohesive energies. Our calculations further suggest the benefit of using a platinum coating layer, as the noble metal is robust with strong resistance to oxidation.

Power over fiber using a multimode optical power with a core diameter of 50 µm

We report on the properties of the Power over Fiber (PoF) transmission link using a High-Power Laser Source operating at 976 nm and using three types of optical fiber with a core diameter of 50 µm. Two step-index profile multimode optical fibers and one fiber with a gradient index were used for optical power transmission. Optical light was converted to electricity using commercially available Photovoltaic Power Convertors (PPCs) with a maximal optical input power of 1.5 W and experimental PPCs with a maximal optical input power of 4.0 W. We experimentally proved optical power transmission up to a distance of 300 m. In the case of the commercially available working PPC and using the gradient index fiber we achieved a result of 0.534 W of electrical power and using the experimental PPC we achieved 0.645 W. In the case of the step-index optical fiber, the result was 1.3 W.

15.5 W, pulsed 630 nm generation based on Raman fiber laser and second-harmonic generation

We present a high-power, nanosecond 630 nm beam generation based on Raman conversion and second-harmonic generation (SHG). 116.2 W, single-mode 1080 nm fiber laser based on 10/125 µm optical fiber is used as a pump source for Raman conversion and the 1260 nm seed laser diode helps the amplification of third-order Raman conversion, which results in 63.7 W at 1260 nm with 54.8% Raman conversion efficiency. SHG to 630 nm is based on type-I noncritical phase-matching conditions with bismuth triborate (BIBO) nonlinear crystal. The average power of 630 nm is 15.5 W at a repetition rate of 9.26 MHz, a pulse width of 16.0 ns, and a SHG efficiency of 24.4%. This result can facilitate the generation of a high-power visible light source with good beam quality at a specific wavelength.

Efficient extreme ultraviolet emission by multiple laser pulses

We demonstrated an efficient extreme ultraviolet (EUV) source at a wavelength of 13.5 nm using spatially separated multiple solid-state-laser pulse irradiation. The maximum conversion efficiency (CE) achieved was 3.8% for ±30° oblique laser pulse injection, which was about twice as high as that for single laser pulse irradiation of 1.7%, with an EUV source size of about 100 μm for two spatially separated laser pulses with a total laser energy of 500 mJ at a laser intensity of 2×1011 W/cm2. In addition, we achieved an EUV CE of 4.7% for ±60° oblique laser pulse injection, which was one of the highest values ever reported, in the case of a 1-μm solid-state laser-produced planar Sn target plasma by multiple laser pulse irradiation. This result suggests that multiple laser-pulse irradiation at high repetition rate operation could credibly provide the next technology for future high-power EUV sources and exposure tools toward future EUV technology nodes.

A Vision for the Future of Neutron Scattering and Muon Spectroscopy in the 2050s.

Neutron scattering and muon spectroscopy are techniques that use subatomic particles to understand materials across a wide range of energy (μeV to tens of eV), length (Å to cm) and time (attosecond to hour) scales. The methods are widely used to study condensed phase materials in areas that span physics, chemistry, biology, engineering and cultural heritage. In this Perspective we consider three questions: (i) will neutron scattering and muon spectroscopy still be needed in the 2050s? (ii) What might the technology to produce neutron and muon beams look like in the 2050s? (iii) What will be the applications in the 2050s? Overall, the neutron/muon ecosystem in the 2050s will have less capacity than now, but greater capability because of the somewhat higher power sources, better instrumentation and data analysis.

Postfilament-Induced Two-Photon Fluorescence of Dyed Liquid Aerosol Enhanced by Structured Femtosecond Laser Pulse

Laser-induced fluorescence spectroscopy (LIFS) is actively used for remote sensing of atmospheric aerosols and is currently one of the most sensitive and selective techniques for determining small concentrations of substances inside particles. The use of high-power femtosecond laser sources for LIFS-based remote sensing of aerosols contributes to the development of new-generation fluorescence atmospheric lidars since it makes it possible to overcome the energy threshold for the nonlinear-optical effects of multiphoton absorption in particles and receive the emission signal at long distances in the atmosphere. Our study is aimed at the development and experimental demonstration of the technique of nonlinear laser-induced fluorescence spectroscopy (NLIFS) based on the remote excitation of aerosol fluorescent emission stimulated by a spatially structured high-power femtosecond laser pulse. Importantly, for the first time to our knowledge, we demonstrate the advances in using stochastically structured plasma-free intense light channels (postfilaments) specially formed by the propagation of femtosecond laser radiation through a turbulent air layer to improve NLIFS efficiency. A multiple increase in the received signal of two-photon-excited fluorescence of polydisperse-dyed aqueous aerosols by the structured postfilaments is reported.

Nonlinear optical physics at terahertz frequency

Abstract Terahertz (THz) waves have exhibited promising prospects in 6G/7G communications, sensing, nondestructive detection, material modulation, and biomedical applications. With the development of high-power THz sources, more and more nonlinear optical effects at THz frequency and THz-induced nonlinear optical phenomena are investigated. These studies not only show a clear physics picture of electrons, ions, and molecules but also provide many novel applications in sensing, imaging, communications, and aerospace. Here, we review recent developments in THz nonlinear physics and THz-induced nonlinear optical phenomena. This review provides an overview and illustrates examples of how to achieve strong THz nonlinear phenomena and how to use THz waves to achieve nonlinear material modulation.

Structural Design and Optimization of Low-Frequency High-Power Electromagnetic Transducer

Crucial equipment for marine engineering and research, high-power ultra-low frequency sound sources have become necessary with the rapid development of seabed resource exploration, marine environment monitoring, underwater remote target detection, and communication technology. The current ultra-low frequency sound source cannot meet the requirements of practical applications. In this paper, both the finite element method and equivalent circuit method are used to improve the electromagnetic acoustic transducer, focusing on solving the structural design of the functional parts of the transducer, as well as the mechanical, electrical, magnetic parametrization of the transducer and other key technologies. The structural parameters and material parameters in the transducer that affect the final performance response are obtained through the optimization of the genetic algorithm. The results show that the electromagnetic acoustic transducer studied in this paper can emit low-frequency sound waves below 50~Hz, and the maximum sound pressure level reaches 138~dB, which meets the requirements of general low-frequency high-power acoustic wave transducers in practical work.

Microstructured large-area photoconductive terahertz emitters driven at high average power

Emitters based on photoconductive materials excited by ultrafast lasers are well-established and popular devices for THz generation. However, so far, these emitters – both photoconductive antennas and large area emitters - were mostly explored using driving lasers with moderate average powers (either fiber lasers with up to hundreds of milliwatts or Ti:Sapphire systems up to few watts). In this paper, we explore the use of high-power, MHz repetition rate Ytterbium (Yb) based oscillator for THz emission using a microstructured large-area photoconductive emitter, consist of semi-insulating GaAs with a 10 × 10 mm2 active area. As a driving source, we use a frequency-doubled home-built high average power ultrafast Yb-oscillator, delivering 22 W of average power, 115 fs pulses with 91 MHz repetition rate at a central wavelength of 516 nm. When applying 9 W of average power (after an optical chopper with a duty cycle of 50%) on the structure without optimized heatsinking, we obtain 65 µW THz average power, 4 THz bandwidth; furthermore, we safely apply up to 18 W of power on the structure without observing damage. We investigate the impact of excitation power, bias voltage, optical fluence, and their interplay on the emitter performance and explore in detail the sources of thermal load originating from electrical and optical power. Optical power is found to have a more critical impact on large area photoconductive emitter saturation than electrical power, thus optimized heatsinking will allow us to improve the conversion efficiency in the near future towards much higher emitter power. This work paves the way towards achieving hundreds of MHz or even GHz repetition rates, high-power THz sources based on photoconductive emitters, that are of great interest for example for future THz imaging applications.

Numerical investigation of a THz-driven dielectric accelerator with a Bragg-reflector for accelerating sub-relativistic electron beams

Structure-based novel accelerators exhibit significant potential for substantial reduction in size and associated costs of future accelerators. Utilizing high-power THz sources in dielectric accelerator structures presents a favorable compromise for achieving elevated gradients and alleviating beam injection requirements. We conducted numerical investigations on an energy-efficient dielectric single grating structure accompanied by a Bragg-reflector, employing THz pulses to generate a phase-modified field for accelerating sub-relativistic electron beams. The structural parameters were optimized to enhance the strength of the acceleration field. The simulation results demonstrate that the side-coupling single grating structure, accompanied by a Bragg-reflector, designed for sub-relativistic electron beam acceleration, can increase the relative structural energy efficiency by more than 50% compared to a dual-grating accelerator structure. Moreover, it offers an available maximum acceleration gradient of up to 400 MeV m−1.