Devonian–Carboniferous strata in the Hida Gaien belt, Southwest Japan, are characterized by a change in the dominant lithology from clastic rocks and limestones to volcanic rocks. The sandstone compositions and detrital zircon U–Pb ages indicate that the Devonian sedimentary rocks were derived from various basement rocks, including granite and basalt, that were uplifted, exposed, and eroded during the Early–Middle Devonian (398–383 Ma). The source of sediment to these strata changed to basalts and rhyolites in the early Carboniferous (∼346 Ma). Early Carboniferous bimodal volcanic rocks are present in the Hida Gaien and South Kitakami belts, the southeastern margin of the South China block (Hainan), and the Jilin area (NE China) of the eastern Central Asian Orogenic Belt (CAOB). The Cambrian–Silurian zircon grains (540–480 Ma and 460–420 Ma) in the Hida Gaien belt were derived from arc basement of a similar age to the South Kitakami and Kurosegawa belts, the Jiamusi–Khanka–Bureya (NE China and the Russian Far East) and Songliao–Xilinhot (Inner Mongolia) blocks in the eastern CAOB, and the eastern South China and Indochina blocks. The Devonian strata also contain Precambrian zircon grains derived from Mesoarchean basement (∼3000 Ma) and the Grenvillian tectonothermal event (∼1000 Ma), suggesting sediment supply from NE Gondwana (the Thomson and Lachlan orogens of eastern Australia) or related continental remnants. Detrital zircon U–Pb age spectra similar to those of the Devonian strata of the Hida Gaien belt are also observed in Silurian–Devonian metasedimentary rocks in the Jilin area. During the early Paleozoic, the Hida Gaien belt, the eastern margin of the South China block, and the magmatic arcs and microcontinents in the eastern CAOB were located close to NE Gondwana along the western margin of the Paleo-Pacific Ocean.