This study reports the first experimental demonstration of surface contamination cleaning from a high-repetition supply of thin-tape targets for laser-driven carbon-ion acceleration. The adsorption of contaminants containing protons, mainly water vapor and hydrocarbons, on the surface of materials exposed to low vacuum (>10−3 Pa) suppresses carbon-ion acceleration. The newly developed contamination cleaner heats a 5-μm-thick nickel tape to over 400 °C in 100 ms by induction heating. In the future, this heating method could be scaled to laser-driven carbon-ion acceleration at rates beyond 10 Hz. The contaminant hydrogen is eliminated from the heated nickel surface, and a carbon source layer—derived from the contaminant carbon—is spontaneously formed by the catalytic effect of nickel. The species of ions accelerated from the nickel film heated to various temperatures have been observed experimentally. When the nickel film is heated beyond ∼150 °C, the proton signal considerably decreases, with a remarkable increase in the number and energy of carbon ions. The Langmuir adsorption model adequately explains the temperature dependence of desorption and re-adsorption of the adsorbed molecules on a heated target surface, and the temperature required for proton-free carbon-ion acceleration can be estimated.