Boundary recognition visually delineates the horizontal extent of subsurface anomalies, providing a foundational basis for interpreting gravity data. Compared to gravity observations, gravity gradient data offers the benefits of multiple components and the enhancement of shortwave information in graphical representations. In our study, we investigated the delineation of geological structure boundaries in the lunar Oceanus Procellarum region using gravity gradient techniques. First, based on the observations from the Gravity Recovery and Interior Laboratory (GRAIL) mission, we obtained high-precision synthetic full tensor values of the gravity gradient as our primary research data. Moreover, to reduce curvature errors during large-scale terrain forward modeling, we applied the spherical prism of tesseroid to eliminate the effects of near-surface topography. Grounded on the Bouguer anomalies of gravity gradient, four distinct boundary recognition methods have been employed to explore the geological structure of the lunar Oceanus Procellarum region. It includes the Theta map method, the directional Theta map method, the combination of total horizontal derivative and the modulus of full tensor gravity gradient, and the improved edge detection method based on the Theta map method.The common feature of these methods is the utilization of the multi-component data combination from gravity gradient tensors, which can enhance the accuracy of edge detection. From the investigation results presented in the paper, we have found the following: 1) The improved edge detection method, based on the Theta map principle, enables better identification of the center of subsurface anomaly bodies during boundary recognition, utilizing a consistent single color in graphic displays. 2) According to the results of boundary recognition, numerous strip anomalies exist in the Oceanus Procellarum area that show less correlation with topographic relief. One possible explanation for these graphical anomalies of gravity gradient is that they serve as channels for the upwelling of mantle material during lunar evolution.