The primitive sea that occupied the Central South Atlantic (CSA), part of the intra-Gondwana rift during the Early Cretaceous, allowed precipitation of an extensive and thick layer of evaporites, the Ibura Salt, followed by the deposition of a prominent Albian carbonate package. Although the shallow platform facies do not contain classical benthic Tethys markers, the pelagic open sea carbonates are essentially dominated by planktonic elements coming from the Tethys Realm. This condition led some researchers to think that Tethys waters also contributed to salt formation, an idea that clashes with the geotectonic model of northward separation of Africa and South America and ingression of predominantly Austral marine waters. Now, a new controversy arises as to the age of this salt layer when trying to position bio-events and lithological and chemostratigraphic markers from these rocks with respect to established data for the Global Boundary Stratotype Section and Point for the Aptian/Albian boundary (GSSP-Alb). Biochronostratigraphic information on planktonic foraminifera points to an Aptian age as opposed to the earliest Albian traditionally accepted for the carbonate section that overlies the giant salt layer. On the other hand, stratigraphic and geochronological data suggest an age of 113 Ma for the base of the salt, very near to the 113.2 ± 0.1 Ma arbitrated for the GSSP-Alb. In this study, we adopt the base of the evaporite bed as the Aptian/Albian boundary in the CSA, Equatorial South Atlantic (ESA), and northeastern Brazilian interior basins (BNE) as well. Based on these criteria, a broad review and the integration of available information have led to new interpretations regarding the earliest phase of these segments of the South Atlantic and adjacent areas. Initially, during the Aptian-Albian transition, an ephemeral interior sea within Brazil, drawing its waters from the north, would have contributed to salt deposition in the intra-Gondwana rift (evaporitic stage of the CSA). Afterward, but still within the earliest Albian, the evaporitic system evolved into a carbonate gulf when the northern barrier, the Exception Zone (EZ), disappeared. The lagoonal circulation pattern that then formed in the CSA created a hypersaline and warm outflow plume that swept across the marine bottom of the ESA and part of the Tethys Sea. Paleoceanographic events registered at Site 545, Mazagan Plateau, support this new hypothesis and illustrate the potential complexity of correlation of organic-rich deposits in which local influences have been greater than global ones. This long, narrow, and continuous carbonate gulf disappeared at the end of the Albian with the arrival of southern waters from the Meridional South Atlantic (MSA), and the South Atlantic became consolidated as a proto-ocean.