Gimballed Limb Observer For Radiance Imaging Of The Atmosphere Research Articles

Quantification and mitigation of the instrument effects and uncertainties of the airborne limb imaging FTIR GLORIA

Abstract. The Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) is an infrared imaging FTS (Fourier transform spectrometer) with a 2-D infrared detector that is operated on two high-flying research aircraft. It has flown on eight campaigns and measured along more than 300 000 km of flight track. This paper details our instrument calibration and characterization efforts, which, in particular, almost exclusively leverage in-flight data. First, we present the framework of our new calibration scheme, which uses information from all three available calibration sources (two blackbodies and upward-pointing “deep space” measurements). Part of this scheme is a new algorithm for correcting the erratically changing nonlinearity of a subset of detector pixels and the identification of the remaining bad pixels. Using this new calibration, we derive a 1σ bound of 1 % on the instrument gain error and a bound of 30 nW cm−2 sr−1 cm on the instrument offset error. We show how we can examine the noise and spectral accuracy for all measured atmospheric spectra and derive a spectral accuracy of 5 ppm on average. All these errors are compliant with the initial instrument requirements. We also discuss, for the first time, the pointing system of the GLORIA instrument. Combining laboratory calibration efforts with the measurement of astronomical bodies during the flight, we can achieve a pointing accuracy of 0.032∘, which corresponds to one detector pixel. The paper concludes with a brief study of how these newly characterized instrument parameters affect temperature and ozone retrievals. We find that the pointing uncertainty and, to a lesser extent, the instrument gain uncertainty are the main contributors to the error in the result.

Biomass burning pollution in the South Atlantic upper troposphere: GLORIA trace gas observations and evaluation of the CAMS model

Abstract. In this study, we present simultaneous airborne measurements of peroxyacetyl nitrate (PAN), ethane (C2H6), formic acid (HCOOH), methanol (CH3OH), and ethylene (C2H4) above the South Atlantic in September and October 2019. Observations were obtained from the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA), as two-dimensional altitude cross sections along the flight path. The flights were part of the SouthTRAC (Transport and Composition in the Southern Hemisphere Upper Troposphere/Lower Stratosphere) campaign with the German High Altitude and Long Range Research Aircraft (HALO). On two flights (8 September 2019 and 7 October 2019), large enhancements of all these substances were found between 7 and 14 km altitude with maximum volume mixing ratios (VMRs) of 1000 pptv for PAN, 1400 pptv for C2H6, 800 pptv for HCOOH, 4500 pptv for CH3OH, and 200 pptv for C2H4. One flight showed a common filamentary structure in the trace gas distributions, while the second flight is characterized by one large plume. Using backward trajectories, we show that measured pollutants likely reached upper troposphere and lower stratosphere (UTLS) altitudes above South America and central Africa, where elevated PAN VMRs are visible at the surface layer of the Copernicus Atmosphere Monitoring Service (CAMS) model during the weeks before both measurements. In comparison to results of the CAMS reanalysis interpolated onto the GLORIA measurement geolocations, we show that the model is able to reproduce the overall structure of the measured pollution trace gas distributions. For PAN, the absolute VMRs are in agreement with the GLORIA measurements. However, C2H6 and HCOOH are generally underestimated by the model, while CH3OH and C2H4, the species with the shortest atmospheric lifetimes of the pollution trace gases discussed, are overestimated by CAMS. The good agreement between model and observations for PAN suggests that the general transport pathways and emissions locations are well captured by the model. The poorer agreement for other species is therefore most likely linked to model deficiencies in the representation of loss processes and emission strength.

Challenge of modelling GLORIA observations of upper troposphere–lowermost stratosphere trace gas and cloud distributions at high latitudes: a case study with state-of-the-art models

Abstract. Water vapour and ozone are important for the thermal and radiative balance of the upper troposphere (UT) and lowermost stratosphere (LMS). Both species are modulated by transport processes. Chemical and microphysical processes affect them differently. Thus, representing the different processes and their interactions is a challenging task for dynamical cores, chemical modules and microphysical parameterisations of state-of-the-art atmospheric model components. To test and improve the models, high-resolution measurements of the UT–LMS are required. Here, we use measurements taken in a flight of the GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) instrument on HALO (High Altitude and LOng Range Research Aircraft). The German research aircraft HALO performed a research flight on 26 February 2016 that covered deeply subsided air masses of the aged 2015/16 Arctic vortex, high-latitude LMS air masses, a highly textured region affected by troposphere-to-stratosphere exchange and high-altitude cirrus clouds. Therefore, it provides a challenging multifaceted case study for comparing GLORIA observations with state-of-the-art atmospheric model simulations in a complex UT–LMS region at a late stage of the Arctic winter 2015/16. Using GLORIA observations in this manifold scenario, we test the ability of the numerical weather prediction (NWP) model ICON (ICOsahedral Nonhydrostatic) with the extension ART (Aerosols and Reactive Trace gases) and the chemistry–climate model (CCM) EMAC (ECHAM5/MESSy Atmospheric Chemistry – fifth-generation European Centre Hamburg general circulation model/Modular Earth Submodel System) to model the UT–LMS composition of water vapour (H2O), ozone (O3), nitric acid (HNO3) and clouds. Within the scales resolved by the respective model, we find good overall agreement of both models with GLORIA. The applied high-resolution ICON-ART set-up involving an R2B7 nest (local grid refinement with a horizontal resolution of about 20 km), covering the HALO flight region, reproduces mesoscale dynamical structures well. Narrow moist filaments in the LMS observed by GLORIA at tropopause gradients in the context of a Rossby wave breaking event and in the vicinity of an occluded Icelandic low are clearly reproduced by the model. Using ICON-ART, we show that a larger filament in the west was transported horizontally into the Arctic LMS in connection with a jet stream split associated with poleward breaking of a cyclonically sheared Rossby wave. Further weaker filaments are associated with an older tropopause fold in the east. Given the lower resolution (T106) of the nudged simulation of the EMAC model, we find that this model also reproduces these features well. Overall, trace gas mixing ratios simulated by both models are in a realistic range, and major cloud systems observed by GLORIA are mostly reproduced. However, we find both models to be affected by a well-known systematic moist bias in the LMS. Further biases are diagnosed in the ICON-ART O3, EMAC H2O and EMAC HNO3 distributions. Finally, we use sensitivity simulations to investigate (i) short-term cirrus cloud impacts on the H2O distribution (ICON-ART), (ii) the overall impact of polar winter chemistry and microphysical processing on O3 and HNO3 (ICON-ART and EMAC), (iii) the impact of the model resolution on simulated parameters (EMAC), and (iv) consequences of scavenging processes by cloud particles (EMAC). We find that changing the horizontal model resolution results in notable systematic changes for all species in the LMS, while scavenging processes play a role only in the case of HNO3. We discuss the model biases and deficits found in this case study that potentially affect forecasts and projections (adversely) and provide suggestions for further model improvements.

Retrieval of Water Vapour Profiles from GLORIA Nadir Observations

We present the first analysis of water vapour profiles derived from nadir measurements by the infrared imaging Fourier transform spectrometer GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere). The measurements were performed on 27 September 2017, during the WISE (Wave driven ISentropic Exchange) campaign aboard the HALO aircraft over the North Atlantic in an area between 37°–50°N and 20°–28°W. From each nadir recording of the 2-D imaging spectrometer, the spectral radiances of all non-cloudy pixels have been averaged after application of a newly developed cloud filter. From these mid-infrared nadir spectra, vertical profiles of H2O have been retrieved with a vertical resolution corresponding to five degrees of freedom below the aircraft. Uncertainties in radiometric calibration, temperature and spectroscopy have been identified as dominating error sources. Comparing retrievals resulting from two different a priori assumptions (constant exponential vs. ERA 5 reanalysis data) revealed parts of the flight where the observations clearly show inconsistencies with the ERA 5 water vapour fields. Further, a water vapour inversion at around 6 km altitude could be identified in the nadir retrievals and confirmed by a nearby radiosonde ascent. An intercomparison of multiple water vapour profiles from GLORIA in nadir and limb observational modes, IASI (Infrared Atmospheric Sounding Interferometer) satellite data from two different retrieval processors, and radiosonde measurements shows a broad consistency between the profiles. The comparison shows how fine vertical structures are represented by nadir sounders as well as the influence of a priori information on the retrievals.

Orographically induced spontaneous imbalance within the jet causing a large-scale gravity wave event

Abstract. To better understand the impact of gravity waves (GWs) on the middle atmosphere in the current and future climate, it is essential to understand their excitation mechanisms and to quantify their basic properties. Here a new process for GW excitation by orography–jet interaction is discussed. In a case study, we identify the source of a GW observed over Greenland on 10 March 2016 during the POLSTRACC (POLar STRAtosphere in a Changing Climate) aircraft campaign. Measurements were taken with the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) instrument deployed on the High Altitude Long Range (HALO) German research aircraft. The measured infrared limb radiances are converted into a 3D observational temperature field through the use of inverse modelling and limited-angle tomography. We observe GWs along a transect through Greenland where the GW packet covers ≈ 1/3 of the Greenland mainland. GLORIA observations indicate GWs between 10 and 13 km of altitude with a horizontal wavelength of 330 km, a vertical wavelength of 2 km and a large temperature amplitude of 4.5 K. Slanted phase fronts indicate intrinsic propagation against the wind, while the ground-based propagation is with the wind. The GWs are arrested below a critical layer above the tropospheric jet. Compared to its intrinsic horizontal group velocity (25–72 m s−1) the GW packet has a slow vertical group velocity of 0.05–0.2 m s−1. This causes the GW packet to propagate long distances while spreading over a large area and remaining constrained to a narrow vertical layer. A plausible source is not only orography, but also out-of-balance winds in a jet exit region and wind shear. To identify the GW source, 3D GLORIA observations are combined with a gravity wave ray tracer, ERA5 reanalysis and high-resolution numerical experiments. In a numerical experiment with a smoothed orography, GW activity is quite weak, indicating that the GWs in the realistic orography experiment are due to orography. However, analysis shows that these GWs are not mountain waves. A favourable area for spontaneous GW emission is identified in the jet by the cross-stream ageostrophic wind, which indicates when the flow is out of geostrophic balance. Backwards ray-tracing experiments trace into the jet and regions where the Coriolis and the pressure gradient forces are out of balance. The difference between the full and a smooth-orography experiment is investigated to reveal the missing connection between orography and the out-of-balance jet. We find that this is flow over a broad area of elevated terrain which causes compression of air above Greenland. The orography modifies the wind flow over large horizontal and vertical scales, resulting in out-of-balance geostrophic components. The out-of-balance jet then excites GWs in order to bring the flow back into balance. This is the first observational evidence of GW generation by such an orography–jet mechanism.

3-D tomographic observations of Rossby wave breaking over the North Atlantic during the WISE aircraft campaign in 2017

Abstract. This paper presents measurements of ozone, water vapour and nitric acid (HNO3) in the upper troposphere/lower stratosphere (UTLS) over North Atlantic and Europe. The measurements were acquired with the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) during the Wave Driven Isentropic Exchange (WISE) campaign in October 2017. GLORIA is an airborne limb imager capable of acquiring both 2-D data sets (curtains along the flight path) and, when the carrier aircraft is flying around the observed air mass, spatially highly resolved 3-D tomographic data. Here, we present a case study of a Rossby wave (RW) breaking event observed during two subsequent flights 2 d apart. RW breaking is known to steepen tracer gradients and facilitate stratosphere–troposphere exchange (STE). Our measurements reveal complex spatial structures in stratospheric tracers (ozone and nitric acid) with multiple vertically stacked filaments. Backward-trajectory analysis is used to demonstrate that these features are related to several previous Rossby wave breaking events and that the small-scale structure of the UTLS in the Rossby wave breaking region, which is otherwise very hard to observe, can be understood as stirring and mixing of air masses of tropospheric and stratospheric origin. It is also shown that a strong nitric acid enhancement observed just above the tropopause is likely a result of NOx production by lightning activity. The measurements showed signatures of enhanced mixing between stratospheric and tropospheric air near the polar jet with some transport of water vapour into the stratosphere. Some of the air masses seen in 3-D data were encountered again 2 d later, stretched to very thin filament (horizontal thickness down to 30 km at some altitudes) rich in stratospheric tracers. This repeated measurement allowed us to directly observe and analyse the progress of mixing processes in a thin filament over 2 d. Our results provide direct insight into small-scale dynamics of the UTLS in the Rossby wave breaking region, which is of great importance to understanding STE and poleward transport in the UTLS.

Pollution trace gases C<sub>2</sub>H<sub>6</sub>, C<sub>2</sub>H<sub>2</sub>, HCOOH, and PAN in the North Atlantic UTLS: observations and simulations

Abstract. Measurements of the pollution trace gases ethane (C2H6), ethyne (C2H2), formic acid (HCOOH), and peroxyacetyl nitrate (PAN) were performed in the North Atlantic upper troposphere and lowermost stratosphere (UTLS) region with the airborne limb imager GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) with high spatial resolution down to cloud top. Observations were made during flights with the German research aircraft HALO (High Altitude and LOng Range Research Aircraft) in the frame of the WISE (Wave-driven ISentropic Exchange) campaign, which was carried out in autumn 2017 from Shannon (Ireland) and Oberpfaffenhofen (Germany). Enhanced volume mixing ratios (VMRs) of up to 2.2 ppbv C2H6, 0.2 ppbv C2H2, 0.9 ppbv HCOOH, and 0.4 ppbv PAN were detected during the flight on 13 September 2017 in the upper troposphere and around the tropopause above the British Isles. Elevated quantities of PAN were measured even in the lowermost stratosphere (locally up to 14 km), likely reflecting the fact that this molecule has the longest lifetime of the four species discussed herein. Backward trajectory calculations as well as global three-dimensional Chemical Lagrangian Model of the Stratosphere (CLaMS) simulations with artificial tracers of air mass origin have shown that the main sources of the observed pollutant species are forest fires in North America and anthropogenic pollution in South Asia and Southeast Asia uplifted and moved within the Asian monsoon anticyclone (AMA) circulation system. After release from the AMA, these species or their precursor substances are transported by strong tropospheric winds over large distances, depending on their particular atmospheric lifetime of up to months. Observations are compared to simulations with the atmospheric models EMAC (ECHAM5/MESSy Atmospheric Chemistry) and CAMS (Copernicus Atmosphere Monitoring Service). These models are qualitatively able to reproduce the measured VMR enhancements but underestimate the absolute amount of the increase. Increasing the emissions in EMAC by a factor of 2 reduces the disagreement between simulated and measured results and illustrates the importance of the quality of emission databases used in chemical models.

Observation of cirrus clouds with GLORIA during the WISE campaign: detection methods and cirrus characterization

Abstract. Cirrus clouds contribute to the general radiation budget of the Earth and play an important role in climate projections. Of special interest are optically thin cirrus clouds close to the tropopause due to the fact that their impact is not yet well understood. Measuring these clouds is challenging as both high spatial resolution as well as a very high detection sensitivity are needed. These criteria are fulfilled by the infrared limb sounder GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere). This study presents a characterization of observed cirrus clouds using the data obtained by GLORIA aboard the German research aircraft HALO during the WISE (Wave-driven ISentropic Exchange) campaign in September and October 2017. We developed an optimized cloud detection method based on the cloud index and the extinction coefficient retrieved at the microwindow 832.4–834.4 cm−1. We derived macro-physical characteristics of the detected cirrus clouds such as cloud top height, cloud bottom height, vertical extent and cloud top position with respect to the tropopause. The fraction of cirrus clouds detected above the tropopause is on the order of 13 % to 27 %. In general, good agreement with the clouds predicted by the ERA5 reanalysis dataset is obtained. However, cloud occurrence is ≈ 50 % higher in the observations for the region close to and above the tropopause. Cloud bottom heights are also detected above the tropopause. However, considering the uncertainties, we cannot confirm the formation of unattached cirrus layers above the tropopause.

SOUTHTRAC-GW: An Airborne Field Campaign to Explore Gravity Wave Dynamics at the World’s Strongest Hotspot

AbstractThe southern part of South America and the Antarctic peninsula are known as the world’s strongest hotspot region of stratospheric gravity wave (GW) activity. Large tropospheric winds are deflected by the Andes and the Antarctic Peninsula and excite GWs that might propagate into the upper mesosphere. Satellite observations show large stratospheric GW activity above the mountains, the Drake Passage, and in a belt centered along 60°S. This scientifically highly interesting region for studying GW dynamics was the focus of the Southern Hemisphere Transport, Dynamics, and Chemistry–Gravity Waves (SOUTHTRAC-GW) mission. The German High Altitude and Long Range Research Aircraft (HALO) was deployed to Rio Grande at the southern tip of Argentina in September 2019. Seven dedicated research flights with a typical length of 7,000 km were conducted to collect GW observations with the novel Airborne Lidar for Middle Atmosphere research (ALIMA) instrument and the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) limb sounder. While ALIMA measures temperatures in the altitude range from 20 to 90 km, GLORIA observations allow characterization of temperatures and trace gas mixing ratios from 5 to 15 km. Wave perturbations are derived by subtracting suitable mean profiles. This paper summarizes the motivations and objectives of the SOUTHTRAC-GW mission. The evolution of the atmospheric conditions is documented including the effect of the extraordinary Southern Hemisphere sudden stratospheric warming (SSW) that occurred in early September 2019. Moreover, outstanding initial results of the GW observation and plans for future work are presented.

Technical note: Lowermost-stratosphere moist bias in ECMWF IFS model diagnosed from airborne GLORIA observations during winter–spring 2016

Abstract. Numerical weather forecast systems like the ECMWF IFS (European Centre for Medium-Range Weather Forecasts – Integrated Forecasting System) are known to be affected by a moist bias in the extratropical lowermost stratosphere (LMS) which results in a systematic cold bias there. We use high-spatial-resolution water vapor measurements by the airborne infrared limb-imager GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) during the PGS (POLSTRACC/GW-LCYCLE-II/SALSA) campaign to study the LMS moist bias in ECMWF analyses and 12 h forecasts from January to March 2016. Thereby, we exploit the two-dimensional observational capabilities of GLORIA, when compared to in situ observations, and the higher vertical and horizontal resolution, when compared to satellite observations. Using GLORIA observations taken during five flights in the polar sub-vortex region around Scandinavia and Greenland, we diagnose a systematic moist bias in the LMS exceeding +50 % (January) to +30 % (March) at potential vorticity levels from 10 PVU (∼ highest level accessed with suitable coverage) to 7 PVU. In the diagnosed time period, the moist bias decreases at the highest and driest air masses observed but clearly persists at lower levels until mid-March. Sensitivity experiments with more frequent temporal output, and lower or higher horizontal and vertical resolution, show the short-term forecasts to be practically insensitive to these parameters on timescales of < 12 h. Our results confirm that the diagnosed moist bias is already present in the initial conditions (i.e., the analysis) and thus support the hypothesis that the cold bias develops as a result of forecast initialization. The moist bias in the analysis might be explained by a model bias together with the lack of water vapor observations suitable for assimilation above the tropopause.

Pollution trace gas distributions and their transport in the Asian monsoon upper troposphere and lowermost stratosphere during the StratoClim campaign 2017

Abstract. We present the first high-resolution measurements of pollutant trace gases in the Asian summer monsoon upper troposphere and lowermost stratosphere (UTLS) from the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) during the StratoClim (Stratospheric and upper tropospheric processes for better climate predictions) campaign based in Kathmandu, Nepal, 2017. Measurements of peroxyacetyl nitrate (PAN), acetylene (C2H2), and formic acid (HCOOH) show strong local enhancements up to altitudes of 16 km. More than 500 pptv of PAN, more than 200 pptv of C2H2, and more than 200 pptv of HCOOH are observed. Air masses with increased volume mixing ratios of PAN and C2H2 at altitudes up to 18 km, reaching to the lowermost stratosphere, were present at these altitudes for more than 10 d, as indicated by trajectory analysis. A local minimum of HCOOH is correlated with a previously reported maximum of ammonia (NH3), which suggests different washout efficiencies of these species in the same air masses. A backward trajectory analysis based on the models Alfred Wegener InsTitute LAgrangian Chemistry/Transport System (ATLAS) and TRACZILLA, using advanced techniques for detection of convective events, and starting at geolocations of GLORIA measurements with enhanced pollution trace gas concentrations, has been performed. The analysis shows that convective events along trajectories leading to GLORIA measurements with enhanced pollutants are located close to regions where satellite measurements by the Ozone Monitoring Instrument (OMI) indicate enhanced tropospheric columns of nitrogen dioxide (NO2) in the days prior to the observation. A comparison to the global atmospheric models Copernicus Atmosphere Monitoring Service (CAMS) and ECHAM/MESSy Atmospheric Chemistry (EMAC) has been performed. It is shown that these models are able to reproduce large-scale structures of the pollution trace gas distributions for one part of the flight, while the other part of the flight reveals large discrepancies between models and measurement. These discrepancies possibly result from convective events that are not resolved or parameterized in the models, uncertainties in the emissions of source gases, and uncertainties in the rate constants of chemical reactions.

Superposition of gravity waves with different propagation characteristics observed by airborne and space-borne infrared sounders

Abstract. Many gravity wave analyses, based on either observations or model simulations, assume the presence of only a single dominant wave. This paper shows that there are much more complex cases with gravity waves from multiple sources crossing each others' paths. A complex gravity wave structure consisting of a superposition of multiple wave packets was observed above southern Scandinavia on 28 January 2016 with the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA). The tomographic measurement capability of GLORIA enabled a detailed 3-D reconstruction of the gravity wave field and the identification of multiple wave packets with different horizontal and vertical scales. The larger-scale gravity waves with horizontal wavelengths of around 400 km could be characterised using a 3-D wave-decomposition method. The smaller-scale wave components with horizontal wavelengths below 200 km were discussed by visual inspection. For the larger-scale gravity wave components, a combination of gravity-wave ray-tracing calculations and ERA5 reanalysis fields identified orography as well as a jet-exit region and a low-pressure system as possible sources. All gravity waves are found to propagate upward into the middle stratosphere, but only the orographic waves stay directly above their source. The comparison with ERA5 also shows that ray tracing provides reasonable results even for such complex cases with multiple overlapping wave packets. Despite their coarser vertical resolution compared to GLORIA measurements, co-located AIRS measurements in the middle stratosphere are in good agreement with the ray tracing and ERA5 results, proving once more the validity of simple ray-tracing models. Thus, this paper demonstrates that the high-resolution GLORIA observations in combination with simple ray-tracing calculations can provide an important source of information for enhancing our understanding of gravity wave propagation.

Nitrification of the lowermost stratosphere during the exceptionally cold Arctic winter 2015–2016

Abstract. The Arctic winter 2015–2016 was characterized by exceptionally low stratospheric temperatures, favouring the formation of polar stratospheric clouds (PSCs) from mid-December until the end of February down to low stratospheric altitudes. Observations by GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) on HALO (High Altitude and LOng range research aircraft) during the PGS (POLSTRACC–GW-LCYCLE II–SALSA) campaign from December 2015 to March 2016 allow the investigation of the influence of denitrification on the lowermost stratosphere (LMS) with a high spatial resolution. Two-dimensional vertical cross sections of nitric acid (HNO3) along the flight track and tracer–tracer correlations derived from the GLORIA observations document detailed pictures of wide-spread nitrification of the Arctic LMS during the course of an entire winter. GLORIA observations show large-scale structures and local fine structures with enhanced absolute HNO3 volume mixing ratios reaching up to 11 ppbv at altitudes of 13 km in January and nitrified filaments persisting until the middle of March. Narrow coherent structures tilted with altitude of enhanced HNO3, observed in mid-January, are interpreted as regions recently nitrified by sublimating HNO3-containing particles. Overall, extensive nitrification of the LMS between 5.0 and 7.0 ppbv at potential temperature levels between 350 and 380 K is estimated. The GLORIA observations are compared with CLaMS (Chemical Lagrangian Model of the Stratosphere) simulations. The fundamental structures observed by GLORIA are well reproduced, but differences in the fine structures are diagnosed. Further, CLaMS predominantly underestimates the spatial extent of HNO3 maxima derived from the GLORIA observations as well as the overall nitrification of the LMS. Sensitivity simulations with CLaMS including (i) enhanced sedimentation rates in case of ice supersaturation (to resemble ice nucleation on nitric acid trihydrate (NAT)), (ii) a global temperature offset, (iii) modified growth rates (to resemble aspherical particles with larger surfaces) and (iv) temperature fluctuations (to resemble the impact of small-scale mountain waves) slightly improved the agreement with the GLORIA observations of individual flights. However, no parameter could be isolated which resulted in a general improvement for all flights. Still, the sensitivity simulations suggest that details of particle microphysics play a significant role for simulated LMS nitrification in January, while air subsidence, transport and mixing become increasingly important for the simulated HNO3 distributions towards the end of the winter.

Unusual chlorine partitioning in the 2015/16 Arctic winter lowermost stratosphere: observations and simulations

Abstract. The Arctic winter 2015/16 was characterized by cold stratospheric temperatures. Here we present a comprehensive view of the temporal evolution of chlorine in the lowermost stratosphere over the course of the studied winter. We utilize two-dimensional vertical cross sections of ozone (O3) and chlorine nitrate (ClONO2), measured by the airborne limb imager GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) during the POLSTRACC/GW-LCYCLE II/GWEX/SALSA campaigns, to investigate the tropopause region in detail. Observations from three long-distance flights in January, February, and March 2016 are discussed. ClONO2 volume mixing ratios up to 1100 pptv were measured at 380 K potential temperature in mesoscale structures. Similar mesoscale structures are also visible in O3 measurements. Both trace gas measurements are applied to evaluate simulation results from the chemistry transport model CLaMS (Chemical Lagrangian Model of the Stratosphere) and the chemistry–climate model EMAC (ECHAM5/MESSy Atmospheric Chemistry). These comparisons show agreement within the expected performance of these models. Satellite measurements from Aura/MLS (Microwave Limb Sounder) and SCISAT/ACE-FTS (Atmospheric Chemistry Experiment – Fourier Transform Spectrometer) provide an overview over the whole winter and information about the stratospheric situation above the flight altitude. Time series of these satellite measurements reveal unusually low hydrochloric acid (HCl) and ClONO2 at 380 K from the beginning of January to the end of February 2016, while chlorine monoxide (ClO) is strongly enhanced. In March 2016, unusually rapid chlorine deactivation into HCl is observed instead of deactivation into ClONO2, the more typical pathway for deactivation in the Arctic. Chlorine deactivation observed in the satellite time series is well reproduced by CLaMS. Sensitivity simulations with CLaMS demonstrate the influence of low abundances of O3 and reactive nitrogen (NOy) due to ozone depletion and sedimentation of NOy-containing particles, respectively. On the basis of the different altitude and time ranges of these effects, we conclude that the substantial chlorine deactivation into HCl at 380 K arose as a result of very low ozone abundances together with low temperatures. Additionally, CLaMS estimates ozone depletion of at least 0.4 ppmv at 380 K and 1.75 ppmv at 490 K, which is comparable to other extremely cold Arctic winters. We have used CLaMS trajectories to analyze the history of enhanced ClONO2 measured by GLORIA. In February, most of the enhanced ClONO2 is traced back to chlorine deactivation that had occurred within the past few days prior to the GLORIA measurement. In March, after the final warming, air masses in which chlorine has previously been deactivated into ClONO2 have been transported in the remnants of the polar vortex towards the location of measurement for at least 11 d.

Mesoscale fine structure of a tropopause fold over mountains

Abstract. We report airborne remote-sensing observations of a tropopause fold during two crossings of the polar front jet over northern Italy on 12 January 2016. The GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) observations allowed for a simultaneous mapping of temperature, water vapour, and ozone. They revealed deep, dry, and ozone-rich intrusions into the troposphere. The mesoscale fine structures of dry filaments at the cyclonic shear side north of the jet and tongues of moist air entraining tropospheric air into the stratosphere along the anticyclonic shear side south of the jet were clearly resolved by GLORIA observations. Vertically propagating mountain waves with recorded temperature residuals exceeding ±3 K were detected above the Apennines. Their presence enhanced gradients of all variables locally in the vicinity of the tropopause. The combination of H2O−O3 correlations with potential temperature reveals an active mixing region and shows clear evidence of troposphere-to-stratosphere and stratosphere-to-troposphere exchange. High-resolution short-term deterministic forecasts of ECMWF's integrated forecast system (IFS) applying GLORIA's observational filter reproduce location, shape, and depth of the tropopause fold very well. The fine structure of the mixing region, however, cannot be reproduced even with the 9 km horizontal resolution of the IFS, used here. This case study demonstrates convincingly the capabilities of linear limb-imaging observations to resolve mesoscale fine structures in the upper troposphere and lower stratosphere, validates the high quality of the IFS data, and suggests that mountain wave perturbations have the potential to modulate exchange processes in the vicinity of tropopause folds.

Airborne limb-imaging measurements of temperature, HNO<sub>3</sub>, O<sub>3</sub>, ClONO<sub>2</sub>, H<sub>2</sub>O and CFC-12 during the Arctic winter 2015/2016: characterization, in situ validation and comparison to Aura/MLS

Abstract. The Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) was operated on board the German High Altitude and Long Range Research Aircraft (HALO) during the PGS (POLSTRACC/GW-LCYCLE/SALSA) aircraft campaigns in the Arctic winter 2015/2016. Research flights were conducted from 17 December 2015 until 18 March 2016 within 25–87∘ N, 80∘ W–30∘ E. From the GLORIA infrared limb-emission measurements, two-dimensional cross sections of temperature, HNO3, O3, ClONO2, H2O and CFC-12 are retrieved. During 15 scientific flights of the PGS campaigns the GLORIA instrument measured more than 15 000 atmospheric profiles at high spectral resolution. Dependent on flight altitude and tropospheric cloud cover, the profiles retrieved from the measurements typically range between 5 and 14 km, and vertical resolutions between 400 and 1000 m are achieved. The estimated total (random and systematic) 1σ errors are in the range of 1 to 2 K for temperature and 10 % to 20 % relative error for the discussed trace gases. Comparisons to in situ instruments deployed on board HALO have been performed. Over all flights of this campaign the median differences and median absolute deviations between in situ and GLORIA observations are -0.75K±0.88 K for temperature, -0.03ppbv±0.85 ppbv for HNO3, -3.5ppbv±116.8 ppbv for O3, -15.4pptv±102.8 pptv for ClONO2, -0.13ppmv±0.63 ppmv for H2O and -19.8pptv±46.9 pptv for CFC-12. Seventy-three percent of these differences are within twice the combined estimated errors of the cross-compared instruments. Events with larger deviations are explained by atmospheric variability and different sampling characteristics of the instruments. Additionally, comparisons of GLORIA HNO3 and O3 with measurements of the Aura Microwave Limb Sounder (MLS) instrument show highly consistent structures in trace gas distributions and illustrate the potential of the high-spectral-resolution limb-imaging GLORIA observations for resolving narrow mesoscale structures in the upper troposphere and lower stratosphere (UTLS).

Limited angle tomography of mesoscale gravity waves by the infrared limb-sounder GLORIA

Abstract. Three-dimensional measurements of gravity waves are required in order to quantify their direction-resolved momentum fluxes and obtain a better understanding of their propagation characteristics. Such 3-D measurements of gravity waves in the lowermost stratosphere have been provided by the airborne Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) using full angle tomography. Closed flight patterns of sufficient size are needed to acquire the full set of angular measurements for full angle tomography. These take about 2 h and are not feasible everywhere due to scientific reasons or air traffic control restrictions. Hence, this paper investigates the usability of limited angle tomography for gravity wave research based on synthetic observations. Limited angle tomography uses only a limited set of angles for tomographic reconstruction and can be applied to linear flight patterns. A synthetic end-to-end simulation has been performed to investigate the sensitivity of limited angle tomography to gravity waves with different wavelengths and orientations with respect to the flight path. For waves with wavefronts roughly perpendicular to the flight path, limited angle tomography and full angle tomography can derive wave parameters like wavelength, amplitude, and wave orientation with similar accuracy. For waves with a horizontal wavelength above 200 km and vertical wavelength above 3 km, the wavelengths can be retrieved with less than 10 % error, the amplitude with less than 20 % error, and the horizontal wave direction with an error below 10∘. This is confirmed by a comparison of results obtained from full angle tomography and limited angle tomography for real measurements taken on 25 January 2016 over Iceland. The reproduction quality of gravity wave parameters with limited angle tomography, however, depends strongly on the orientation of the waves with respect to the flight path. Thus, full angle tomography might be preferable in cases in which the orientation of the wave cannot be predicted or waves with different orientations exist in the same volume and thus the flight path cannot be adjusted accordingly. Also, for low-amplitude waves and short-scale waves full angle tomography has advantages due to its slightly higher resolution and accuracy.

First tomographic observations of gravity waves by the infrared limb imager GLORIA

Abstract. Atmospheric gravity waves are a major cause of uncertainty in atmosphere general circulation models. This uncertainty affects regional climate projections and seasonal weather predictions. Improving the representation of gravity waves in general circulation models is therefore of primary interest. In this regard, measurements providing an accurate 3-D characterization of gravity waves are needed. Using the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA), the first airborne implementation of a novel infrared limb imaging technique, a gravity wave event over Iceland was observed. An air volume disturbed by this gravity wave was investigated from different angles by encircling the volume with a closed flight pattern. Using a tomographic retrieval approach, the measurements of this air mass at different angles allowed for a 3-D reconstruction of the temperature and trace gas structure. The temperature measurements were used to derive gravity wave amplitudes, 3-D wave vectors, and direction-resolved momentum fluxes. These parameters facilitated the backtracing of the waves to their sources on the southern coast of Iceland. Two wave packets are distinguished, one stemming from the main mountain ridge in the south of Iceland and the other from the smaller mountains in the north. The total area-integrated fluxes of these two wave packets are determined. Forward ray tracing reveals that the waves propagate laterally more than 2000 km away from their source region. A comparison of a 3-D ray-tracing version to solely column-based propagation showed that lateral propagation can help the waves to avoid critical layers and propagate to higher altitudes. Thus, the implementation of oblique gravity wave propagation into general circulation models may improve their predictive skills.

Denitrification, dehydration and ozone loss during the 2015/2016 Arctic winter

Abstract. The 2015/2016 Arctic winter was one of the coldest stratospheric winters in recent years. A stable vortex formed by early December and the early winter was exceptionally cold. Cold pool temperatures dropped below the nitric acid trihydrate (NAT) existence temperature of about 195 K, thus allowing polar stratospheric clouds (PSCs) to form. The low temperatures in the polar stratosphere persisted until early March, allowing chlorine activation and catalytic ozone destruction. Satellite observations indicate that sedimentation of PSC particles led to denitrification as well as dehydration of stratospheric layers. Model simulations of the 2015/2016 Arctic winter nudged toward European Centre for Medium-Range Weather Forecasts (ECMWF) analysis data were performed with the atmospheric chemistry–climate model ECHAM5/MESSy Atmospheric Chemistry (EMAC) for the Polar Stratosphere in a Changing Climate (POLSTRACC) campaign. POLSTRACC is a High Altitude and Long Range Research Aircraft (HALO) mission aimed at the investigation of the structure, composition and evolution of the Arctic upper troposphere and lower stratosphere (UTLS). The chemical and physical processes involved in Arctic stratospheric ozone depletion, transport and mixing processes in the UTLS at high latitudes, PSCs and cirrus clouds are investigated. In this study, an overview of the chemistry and dynamics of the 2015/2016 Arctic winter as simulated with EMAC is given. Further, chemical–dynamical processes such as denitrification, dehydration and ozone loss during the 2015/2016 Arctic winter are investigated. Comparisons to satellite observations by the Aura Microwave Limb Sounder (Aura/MLS) as well as to airborne measurements with the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) performed aboard HALO during the POLSTRACC campaign show that the EMAC simulations nudged toward ECMWF analysis generally agree well with observations. We derive a maximum polar stratospheric O3 loss of ∼ 2 ppmv or 117 DU in terms of column ozone in mid-March. The stratosphere was denitrified by about 4–8 ppbv HNO3 and dehydrated by about 0.6–1 ppmv H2O from the middle to the end of February. While ozone loss was quite strong, but not as strong as in 2010/2011, denitrification and dehydration were so far the strongest observed in the Arctic stratosphere in at least the past 10 years.

New calibration noise suppression techniques for the GLORIA limb imager

Abstract. The Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) presents new opportunities for the retrieval of trace gases in the upper troposphere and lower stratosphere. The radiometric calibration of the measured signal is achieved using in-flight measurements of reference blackbody and upward-pointing "deep space" scenes. In this paper, we present techniques developed specifically to calibrate GLORIA data exploiting the instrument's imaging capability. The algorithms discussed here make use of the spatial correlation of parameters across GLORIA's detector pixels in order to mitigate the noise levels and artefacts in the calibration measurements. This is achieved by combining a priori and empirical knowledge about the instrument background radiation with noise-mitigating compression methods, specifically low-pass filtering and principal component analysis (PCA). In addition, a new software package for the processing of GLORIA data is introduced which allows us to generate calibrated spectra from raw measurements in a semi-automated data processing chain.