Elucidating the effect of local strain on the mechanical properties is of great significance for the design of high-performance layered metals. For this purpose, we conceived the present study, featured by tailoring the local strain by layer thickness design, and simultaneous monitoring of local strain and geometrically necessary dislocations (GNDs) via coupling in-situ electron backscatter diffraction (EBSD) and high-resolution digital image correlation (DIC). In addition, synchrotron X-ray micro-computed tomography (μCT) was employed to analyze the microcracks that serve as another form of strain localization. Such detailed experimental studies revealed that the interfacial strain gradient was rapidly elevated, and the strain localization band was effectively dispersed as the layer thickness decreased. This leads to two typical transitions, from grain-boundary-related to layer-interface-related plastic deformation mode, and from macroscopic shear to zig-zag fracture mode. Their influences on the mechanical properties, as well as underlying mechanisms, were discussed based on the relationship among the layer thickness, strain gradient, strain localization, GND density, and microcracks. Our work not only contributes to the fundamental understanding of the mechanical behavior of multilayered metals but also offers guidance for the structural design of high-performance metals aimed at achieving superior strength-ductility combinations.
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