Flexible Materials Research Articles

A recyclable, interchangeable optical switch with a PDLC-PVA-PSCLC structure and a low-voltage drive system

ABSTRACT Polymer dispersed liquid crystals (PDLC) and polymer stabilised cholesteric liquid crystals (PSCLC) are an indispensable class of electrically switchable materials, which have been widely applied in the fabrication of efficient and systematic smart windows. And doping nanoparticles in PDLC films can greatly improve their properties. In this study, PDLC films doped with zirconia nanoparticles were prepared by polymerisation-induced phase separation (PIPS) method, PSCLC films with nematic liquid crystals as the main part (reflecting wavelengths in the range of 400–600 nm) were prepared by UV curing method, and a novel optical switch was developed by combining these two liquid crystal films. The optimal bilayer sample was developed through a comparative analysis of properties among samples with varying formulations for each liquid crystal layer. This study represents a novel advancement in PSCLC and nanoparticle-doped PDLC bilayer structures, showcasing fully actuatable properties in the visible wavelength range. These structures exhibit excellent electro-optical properties and demonstrate stable, sustainable performance that can be regenerated. The findings underscore the potential of PDLC and PSCLC for applications in smart curtains and flexible materials, opening up new avenues for innovative technological applications.

A first-principles research on the properties of two-dimensional penta-BP2 as an anode material for both Na and K ion batteries

The escalating demand for large-scale energy storage solutions has sparked significant interest in metal-ion batteries, particularly in the realm of high-performance anode materials. This work explores the potential of penta-BP2 as an anode material for sodium and potassium-ion batteries through first-principles calculations. The two-dimensional metallic structure of penta-BP2 exhibits favorable electrical conductivity, making it an ideal candidate for anode materials. Theoretical analysis reveals that penta-BP2 can adsorb two layers of Na and three layers of K, resulting in high storage capacities of 1105 and 1473 mAh/g, along with low open-circuit voltages of 0.40 and 0.30 V, respectively. These characteristics enable the production of high energy density in sodium and potassium-ion batteries. Additionally, the material's small Young's modulus and low diffusion energy barriers further establish penta-BP2 as a flexible anode material capable of rapid charge/discharge processes.

A Review of Friction in Low-Stress Mechanics of Fibrous Flexible Materials.

The structure of a fabric is a highly complex assembly of fibres, which have order and regularity as well as disorder and randomness. The complexity of the structure poses challenges in defining its mechanical behaviour, particularly at low stress, which is typical to end uses. The coexistence of multiple deformations and the high degree of nonlinearity of the fabric due to fibre friction make its stress-strain relationship complicated. This article reviews the literature on friction related to the low-stress mechanics of fabrics, and it establishes its range and regularity to help with finding a unified reference model, in which although the physical meanings of fabric tensile, shear, and bending vary, they follow consistent mathematical regularities. So, invariably, their disorder and randomness needed in defining them can be obtained from fabric measurement data. It defines the scope and patterns of friction to facilitate the development of a unified reference model. It argues that although the physical interpretations of fabric tensile, shear, and bending characteristics may differ, they adhere to consistent mathematical regularities within this model, and hence extracting disorder and randomness from fabric measurement data may be achievable. This paper concludes with a number of recommendations, postulating that hysteresis caused by friction between fibres in a fabric is an important component of mechanical information, and it coexists with its purely elastic component, but it cannot be obtained directly by measurement. Seeking means to effectively decompose the friction hysteresis and pure elastic components contained in fabric mechanics measurement data will provide an accurate characterization of fabric mechanical properties and hence an accurate modelling and simulation of its behaviour, and will impact many traditional and industrial textile end uses.

Recycling efficiency optimization of tungsten-filled Vinyl-Methyl-Silicone-based flexible gamma ray shielding materials

Tungsten has been widely used for gamma-ray and X-ray radiation shielding, which is one of the main elements of shielding materials. Compared with traditional lead-containing shielding materials, tungsten-containing shielding materials have several advantages, such as good chemical stability, a high melting point and relative environmental friendliness. Considering the recycling of resources, the optimization of pyrolysis temperature and pyrolysis duration of tungsten-filled Vinyl-Methyl-Silicone-based flexible shielding materials needs to be studied. In this paper, these tungsten-filled Vinyl-Methyl-Silicone-based flexible shielding materials were initially recycled using pyrolysis. Subsequently, the crystal structures, surface chemical states and the tungsten concentration after pyrolysis in an argon atmosphere were characterized. In order to increase the tungsten recycling rate, the pyrolyzed samples were further recycled using the ultrasonic cleaning method. Furthermore, the influence of ultrasonic cleaning on tungsten recycling rate and surface morphologies was characterized and analyzed. It is found that the tungsten recycling rate of tungsten-filled Vinyl-Methyl-Silicone based flexible gamma/X-ray shielding material was around 69.9 wt%-81.6 wt% by using the pyrolysis method, while the recycling rate of tungsten can exceed 90.0 wt% by ultrasonic cleaning after pyrolysis.

Nanomaterials used in Flexible Electronics: Recent Trends and Future Approaches

Abstract: The latest research in soft electronics reveals a substantial demand for devices that can fold, bend and stretch to suit the requirements of technological advances. Cellulose, silk, and elastomers are employed in making biodegradable, environmentally benign substrates that accommodate nanofibers, nanoparticles, nanotubes, graphene, and biomaterials in their nano-form. Flexible materials can hold circuits and sensors and can substitute conventional substrates. Transient electronics, e-skin, and biosensors are the most sought-after in medical technology, sensors, energy storage devices, and wearables. These stretchable materials lead the way for developing eco-friendly and sustainable technology to attain sustainable development goals. This research work discusses nano species imbibed in printable and flexible electronics. An analysis of the documents extracted from the Scopus database using VOSviewer and patents in the domain of flexible electronics are presented along with altmetrics.

Highly constrained cooperative guidance for flexible landing on asteroids

Flexible lander, composed of multiple nodes connected by flexible material, can reduce the bouncing and overturning during the asteroid landing. To satisfy the complex constraints in the node cooperation of the flexible landing, an intelligent cooperative guidance method is proposed. The method consists of a double-layer cooperative guidance structure, a guidance parameter determination approach, and an action priority strategy. The double-layer contains a basic guidance used to satisfy the terminal state constraints, and a compensatory guidance used to satisfy the lander’s attitude constraint. For the compensatory guidance, the parameters are determined by multi-agent system, which are trained according to the performance index of flexible landing trajectories. The action priority strategy is used to reduce the detrimental effect of parameter inconsistency on the node cooperation. The simulation of flexible landing shows that the cooperative guidance method is effective in improving the landing accuracy while satisfying the constraints. Meanwhile, the method is robust to the disturbance in the navigation and control.

Evaluation of gamma rays shielding properties of bismuth tungstate with different morphologies

To develop lead-free gamma-ray shielding material, bismuth tungstate (Bi2WO6) nanocrystals were synthesized under different conditions of precursor solution by hydrothermal method and composite material based on polyurethane and bismuth tungstate nanocrystals were prepared and evaluated using gamma ray sources in this study. The effects of crystal structure and morphology on the gamma ray shielding properties of bismuth tungstate were specially investigated. Results indicated that pH value of precursors solution had significant effect on the synthesis of bismuth tungstate: orthorhombic Bi2WO6 were obtained under acidic or neutral conditions while tetragonal Bi0.875W0.125O1.6875 were obtained under strongly alkaline condition. With the increase of pH value, the morphology of bismuth tungstate changed from flower-like microspheres to persimmon-like microstructures, and then to randomly stacked nanosheets. Bismuth tungstate nanocrystals were added to polyurethane to prepare flexible gamma-ray shielding material and the gamma ray shielding properties were also tested with energy of 59.5 keV, 81.0 keV and 121.8 keV. For orthorhombic persimmon-like bismuth tungstate (Bi2WO6) which were produced under weak acidic or neutral condition (pH = 2, 5, 7), it was found that the linear attenuation coefficient of gamma ray grew by about 8 % when pH changing from 2 to 7 for all energy tested. While for tetragonal bismuth tungstate (Bi0.875W0.125O1.6875), weakly alkaline condition (pH = 9) induced significant decrease (9 %@59.5 keV, 17 %@81.0 keV and 11 %121.8 keV) of linear attenuation coefficient compared with neutral condition, which could be explained by the dramatic crystal structure change of bismuth tungstate. More alkaline synthesizing condition would make finer granularity of bismuth tungstate and the linear attenuation coefficient increased when pH change from 9 to 12. In addition, obvious differences of mechanical properties were also observed between the composites prepared using different crystalline bismuth tungstates. The results of this study provide a reference for the development of new flexible radiation shielding materials with non-toxicity, light weight and high efficiency.

A Strategy for Fabricating Ultra-Flexible Thermoelectric Films Using Ag2Se-Based Ink.

Flexible thermoelectric materials have drawn significant attention from researchers due to their potential applications in wearable electronics and the Internet of Things. Despite many reports on these materials, it remains a significant challenge to develop cost-effective methods for large-scale, patterned fabrication of materials that exhibit both excellent thermoelectric performance and remarkable flexibility. In this study, we have developed an Ag2Se-based ink with excellent printability that can be used to fabricate flexible thermoelectric films by screen printing and low-temperature sintering. The printed films exhibit a Seebeck coefficient of -161 μV/K and a power factor of 3250.9 μW/m·K2 at 400 K. Moreover, the films demonstrate remarkable flexibility, showing minimal changes in resistance after being bent 5000 times at a radius of 5 mm. Overall, this research offers a new opportunity for the large-scale patterned production of flexible thermoelectric films.

Strain sensors enhanced by a flexible, conductive hydrogel with superior transparency, frost resistance, and water retention

Flexible hydrogels have received significant attention for their excellent mechanical properties, fast response and good strain sensitivity. However, relatively little research has been conducted on the investigation of hydrogels that exhibit frost resistance, water retention, and transparency characteristics. In this paper, a new flexible strain sensors material was prepared by introducing calcium chloride (CaCl2) and hydrolysed keratin (HK) into the polyvinyl alcohol (PVA) system through complex chemical bond. The PVA/CaCl2/HK hydrogel exhibited excellent mechanical properties, with a tensile strength of 1.578 MPa and a maximum strain of 934 %. Moreover, it showed high transparency, with a transmittance of up to 90 %. The hydrogel demonstrated remarkable water retention properties with about 8 hours of dry resistance under constant temperatures of 40 °C, 60 °C, 80 °C and 100 °C. Additionally, it had excellent frost resistance with a glass transition temperature of −23 °C, making it environmentally tolerant and capable of maintaining long-term stability. Notably, during the experiment, the PVA/CaCl2/HK hydrogel exhibited excellent electrical conductivity and self-powered performance, with a power supply capacity of approximately 14.6 mV. The results of this work provide a promising direction for the development of electronic materials for powered hydrogel strain sensors.

Thermoelectric bismuth telluride nanostructures fabricated by electrodeposition within flexible templates

Bismuth telluride, a highly efficient thermoelectric material, stands out for applications around room temperature in wearable devices. By harnessing the thermal gradient established between the human body and ambient temperature, we can generate useable electricity. Notably, bismuth telluride nanostructures exhibit significantly lower thermal conductivities compared to their bulk counterparts. As a result, the thermoelectric efficiency achieved is notably higher. Our research focuses on developing efficient nanostructured materials based on bismuth telluride inside a flexible substrate made of polyester. We employ scalable methods, such as template-assisted electrochemical deposition, to fabricate these nanostructures. In this study, we present an approach to the development of flexible nanostructured thermoelectric materials. Despite using a reduced quantity of active material, our electrochemically deposited nanostructures inside a flexible template demonstrate a remarkable performance. They exhibit 24 % of the Power Factor reported for conventional electrochemically fabricated Bi2Te3 thin films, and notably, they even surpass the Power Factor reported for flexible Bi2Te3-based inks used in the creation of flexible generators. This achievement underscores the potential of our method in the advancement of efficient, flexible thermoelectric devices.

Application of 3D printing to create an in vitro aneurysm rupture model.

Currently available benchtop (in vitro) aneurysm models are inadequate for testing the efficacy of endovascular device treatments. Specifically, current models do not represent the mechanical instability of giant aneurysms (defined as aneurysms with 25 mm in height or width) and do not predictably rupture under simulated physiological conditions. Hence, in vitro aneurysm models with biomechanically relevant material properties and a predictable rupture timeframe are needed to accurately assess the efficacy of new medical device treatment options. Understanding the material properties of an aneurysm (e.g., shear and compression modulus) as it approaches rupture is a crucial step toward creating a pathologically relevant and sophisticated in vitro aneurysm rupture model. We investigated the change in material properties of a blood vessel, via enzymatic treatment, to simulate the degradation of an aneurysm wall and used this information to create a sophisticated aneurysm rupture model using the latest in additive manufacturing technologies (3D printing) with tissue-like materials. Mechanical properties (shear and compression modulus) of swine carotid vessels were evaluated before and after incubation with collagenase D enzyme (30 min at 37°C) to simulate the effect of biochemical activity on aneurysm wall approaching rupture compared to control vessels (untreated). Mechanical strength of a soft and flexible 3D-printed material (VCA-A30: 30 shore A hardness) was tested for comparison to these arterial vessels. This material was then used to create spherical shaped, giant-sized (25-mm diameter) aneurysm phantoms and were run under neurovascular pressures (120/80 ± 5 mmHg), beats per minute (BPM = 70) and flows representing the middle cerebral artery [MCA: 142.67 (±20.13) mL/min] using a blood analog [3.6 (±0.4) cP viscosity] with non-Newtonian shear-thinning properties. The shear modulus of swine carotid vessel before treatment was 12.2 (±2.7) KPa and compression modulus was 663.5 (±111.6) KPa. After enzymatic treatment by collagenase D, shear modulus of animal tissues reduced by 33% (p-value = .039) while compression modulus remained statistically unchanged (p-value = .615). Control group (untreated vessels) showed minimal reduction (13%, p-value = .226) in shear modulus and 78% increase (p-value = .034) in compression modulus. The shear modulus of the 3D-printed material was 228.59 (±24.82) KPa while its compression modulus was 668.90 (±13.16) KPa. This material was used to prototype a sophisticated in vitro giant aneurysm rupture model. When subjected to physiological pressures and flow rates, the untreated models consistently ruptured at ~12 min. These results indicate that aneurysm rupture can be recreated consistently in a benchtop in vitro model, utilizing the latest 3D-printed materials, connected to a physiologically relevant programmable pump. Further studies will investigate the optimization of various aneurysm dome thickness regions within the aneurysm, with tunable rupture times for comparison of aneurysm device deployment and benchtop controls based on the measurable effects of pressure and flow changes within the aneurysm models. These optimized in vitro rupture models could ultimately be used to test the efficacy of device treatment options and rupture risk by quantifying specific device rupture times and aneurysm rupture position.

Flexible polyurethane-based phase change materials with excellent thermal management for human thermal therapy

Flexible polyurethane-based phase change materials with excellent thermal management for human thermal therapy

Flexible hexagonal boron nitride@liquid metal/polydimethylsiloxane composites with excellent thermal conductivity and superior mechanical properties

AbstractHexagonal boron nitride (h‐BN) has a layered lattice structure, high intrinsic thermal conductivity, and good chemical stability, and it has a promising applications in thermal management materials. However, poor interfacial compatibility and dispersion of BN flakes in the polymer matrix cause thermal contact resistance and gaps, directly impairing the performance of the composites and limiting their thermal conduction applications. Herein, the P‐BN@LM/PDMS thermally conductive composites with superior mechanical properties were fabricated by incorporating dopamine and liquid metal (LM) into BN flakes. The dopamine self‐polymerizes to form polydopamine (PDA) on the BN surface, denoted as P‐BN, which effectively improves interface compatibility and dispersion. The LM attaches to the functionalized P‐BN surface by mechanical grinding, acting as a bridge between adjacent BN flakes to enhance the integrity of the thermal conductive network within the composites. The coordination between P‐BN and LM increases interface strength, effectively improving mechanical performance. Hence, the P‐BN@LM/PDMS composites exhibit excellent thermal conductivity (4.0 W/mK) and an enhancement factor of 1373%, which is 2.22 times that of BN/PDMS composites with the same 30 wt% loading. Additionally, the composite shows superior tensile strength (2.11 MPa) and elongation at break (121%), representing 441% and 203% improvements compared with pure polydimethylsiloxane (PDMS). The P‐BN@LM/PDMS composites, with significant advantages in thermal conductivity and mechanical properties, are promising for future applications as flexible thermal interface materials in thermal management.Highlights The P‐BN@LM/PDMS composites exhibit excellent thermal conductivity (4.0 W/mK) and an enhancement factor of 1373%, making them promising for future applications as flexible thermal interface materials in thermal management. The P‐BN@LM/PDMS composites present a superior tensile strength (2.11 MPa) and elongation at break (121%). PDA formed by the self‐polymerization of dopamine on the BN surface effectively enhances interfacial compatibility and dispersion. LM attaches to the functionalized BN surface through mechanical grinding, acting as a bridge between adjacent BN flakes, thus enhancing the integrity of the thermal conductive network within the composites.

Dynamic loading response of an additively produced bio-inspired nacre structure with foam and acrylic filling

Numerous structures gain inspiration from nature and have been effectively incorporated into different applications such as automobiles and airplanes. In order to effectively withstand impact loads and achieve efficient energy absorption, it is necessary to incorporate appropriate structures along with suitable filler materials. This study examines the energy absorption capacities of a nacre structured core with foam filling at the central nacre cell cavities, as well as an acrylic filling at the top and bottom sides, under low velocity impacts. The design of experiments involved identifying and varying three important design parameters which influence the energy absorption behavior of the composites. Subsequently, fillers were incorporated and the specimens were subjected to drop weight testing. The composite material exhibited minimal deformations while absorbing a maximum energy of 40.87 J. Therefore, it proved that this composite could withstand dynamic impact loads in the absence of fiber face sheets, and adhesion between the PLA-carbon fiber and acrylic fill was also improved under these conditions. The higher energy absorption behavior was obtained due to the intermittent force transfer in the transverse direction due to the presence of the cross webs on the top and bottom of the composite plate. The alternate arrangement of the hard and flexible materials in the composite leads to the suppression of the stress step by step which results in high energy absorption behavior. In order to achieve optimal energy absorption with minimized deformations, the core structure must possess a nacre wall thickness of 2 mm with double cross web design.

Carbon nanomaterials in flexible wearable sensors

Recent remarkable advances in flexible and wearable functional electronics have been achieved due to their advantages of lightweight, convenience to detect complex measured objects, and flexibility, which makes electronic equipment develop from a rigid system to a flexible system. Flexible materials toward wearable devices present a huge market prospect, which demonstrate promise in healthcare, human motion detection, biomedicine, environmental monitoring, and other fields. Unique physical and chemical properties are the critical characteristics of flexible wearable sensors, and the huge surface-to-volume ratio facilitates carbon nanomaterials to be used in various flexible sensors. This review comprehensively introduces the structure, properties, and preparation of carbon nanomaterials like carbon nanotubes, graphene, and MXene. The sensing mechanism of the sensor is outlined, and flexible sensors based on carbon nanomaterials in detecting targets such as pressure, temperature, and gases are proposed. Enhancement of conductivity, sensing factor, and sensitivity of carbon nanomaterials by modifying their structure or preparing composites is presented in detail. Finally, this paper outlines the challenges associated with implementing carbon nanomaterials within the field of flexible wearable sensors and future development.

Flexible Electronics: Advancements and Applications of Flexible Piezoelectric Composites in Modern Sensing Technologies.

The piezoelectric effect refers to a physical phenomenon where piezoelectric materials generate an electric field when subjected to mechanical stress or undergo mechanical deformation when subjected to an external electric field. This principle underlies the operation of piezoelectric sensors. Piezoelectric sensors have garnered significant attention due to their excellent self-powering capability, rapid response speed, and high sensitivity. With the rapid development of sensor techniques achieving high precision, increased mechanical flexibility, and miniaturization, a range of flexible electronic products have emerged. As the core constituents of piezoelectric sensors, flexible piezoelectric composite materials are commonly used due to their unique advantages, including high conformability, sensitivity, and compatibility. They have found applications in diverse domains such as underwater detection, electronic skin sensing, wearable sensors, targeted therapy, and ultrasound diagnostics for deep tissue. The advent of flexible piezoelectric composite materials has revolutionized the design concepts and application scenarios of traditional piezoelectric materials, playing a crucial role in the development of next-generation flexible electronic products. This paper reviews the research progress on flexible piezoelectric composite materials, covering their types and typical fabrication techniques, as well as their applications across various fields. Finally, a summary and outlook on the existing issues and future development of these composite materials are provided.

Terahertz metamaterials for spectrum modulation: structural design, materials and applications

Metamaterials, an artificial electromagnetic (EM) material, have exhibited unique characteristics, enabling innovations in terahertz (THz) wavefront shaping, polarization modulation, surface wave manipulation, and spectrum modulation. In this review, we focus on the advancements in THz metamaterials for spectrum modulation, emphasizing their structural design, special materials, and applications. The review discusses various structural designs, including metal-dielectric composite structures, all-metal structures, and all-dielectric structures, each offering distinct advantages for THz applications. Key special materials such as graphene, vanadium dioxide (VO2), molybdenum disulfide (MoS2), and flexible materials are highlighted for their significant contributions to enhancing the performance and functionality of THz metamaterials. The applications of THz metamaterials in EM stealth and sensing are thoroughly introduced, with a particular focus on biosensing, pesticide detection, and other sensing applications. The review emphasizes the potential of THz metamaterials in developing highly sensitive and selective sensors, as well as efficient THz absorbers and filters. Future perspectives include the continuous development of novel materials, advanced fabrication technologies, and the integration of multifunctional capabilities to further expand the applications and efficiency of THz metamaterials. These advancements are expected to drive significant progress in THz technology, impacting fields such as medical diagnostics, environmental monitoring, food safety, wireless communication, and security.

Tapered fiber optic sensor for arterial pulse wave monitoring

Arterial pulse wave monitoring has been recognized as an effective medical diagnostic tool for various cardiovascular diseases. To overcome the barriers in traditional, complex, and expensive detection configurations, new electronic and optical sensors have been developed with their unique advantages. Particularly, various configurations of fiber-optic sensors have been proposed. This paper demonstrates the use of a tapered optical fiber structure to create a sensitive sensor that can detect carotid arterial pulse waves on the skin surface. The demonstrated fiber sensor probe utilizes an in-line Mach-Zehnder interferometer configuration and liquid-gold film coating on the sensor tip to enhance its sensitivity and demonstrate its use by encapsulating the sensor with a flexible elastomer material for detecting arterial pulse waves with a simple testing configuration. Considering the simple fabrication and high sensitivity without a complex demodulation scheme, the proposed sensor has broad implementation in biomedical health monitoring systems.

Dual conductive network enables mechanically robust polymer composites with highly electrical and thermal conductivities

Thermally and electrically conductive polymer composites (CPCs) have been widely used in smart and flexible electronics; however, huge challenges remain in simultaneously improving the electrical and thermal conductivity of CPCs while maintaining the satisfactory mechanical properties including sufficient strength and toughness. In this study, we propose an effective interfacial regulation approach to fabricate CPCs with a dual conductive network through decoration of Ag nanoparticles (AgNPs) onto the polyurethane (PU) nanofibers containing graphite nanoplatelets (GNPs), followed by hot-pressing. Rigid GNPs expand the PU nanofiber network, facilitating Ag precursor adsorption, while subsequent hot-pressing eliminates the big channels and pores inside nanofiber composite membranes and hence greatly enhance their mechanical properties. After hot-pressing, the synergistic dual conductive network with greatly reduced thermal and electrical contact resistance leads to significant improvements in both thermal and electrical conductivity (up to 27.71 W (m K)−1 and 1.87 × 106 S/m, respectively). Moreover, the mechanically robust CPCs with exceptional durability possess superior Joule heating performance at low voltages and heat dissipation capability. This study provides inspiration for designing highly thermally and electrically conductive CPCs with potential applications as flexible thermal interface materials.

MXene-CNC super performing composite films for flexible and degradable electronics

Flexible electronics have gained significant interest due to their potential applications in wearable devices, biomedical sensors, and flexible displays. This study explores the combination of MXene and cellulose nanocrystals (CNC) for the development of flexible, conductive, and degradable materials. CNC and MXene are high-performance nanomaterials with known degradability. CNC can self-assemble into highly ordered layers and act as an ideal structural companion for enabling large surface MXene-based devices with outstanding performance. Three fabrication routes are explored in this work: self-assembly, drop casting, and dip coating. The mechanical and electrical properties of the CNC-MXene composite films were assessed. Tensile testing revealed that dip-coated films in high-loadings of MXene could exhibit enhanced toughness of up to 1.9 MJ‧m−3, higher than pure MXene or CNC. The electrical conductivity of the films varied depending on MXene concentration and drying, exhibiting superior conductivity in self-assembly with higher MXene loading and rapid drying that prevents oxidation. Self-assembled MXene-CNC with a 1:3 MXene-to-CNC ratio maintained high conductivity of 2.2 × 105 S‧m−1. Zeta potential measurements indicate that CNC enhances the stability of MXene dispersion. These findings demonstrate good synergy between CNC and MXenes for applications in flexible, transparent, and environmentally degradable electronic.