First-order Quantum Phase Transition Research Articles

Quantum phase transitions and cat states in cavity-coupled quantum dots

We study double quantum dots coupled to a quasistatic cavity mode with high mode-volume compression allowing for strong light-matter coupling. Besides the cavity-mediated interaction, electrons in different double quantum dots interact with each other via dipole-dipole (Coulomb) interaction. There is a first-order cavity-induced ferroelectric quantum phase transition when the attractive dipolar interaction is smaller than the critical value defined by the energy splitting in DQDs and a smooth transition, otherwise. We show that, in the smooth transition region, both the ground and the first excited states of an array of double quantum dots are cat states. Such states are actively discussed as high-fidelity qubits for quantum computing, and thus our proposal provides a platform for semiconductor implementation of such qubits. We also calculate gauge-invariant observables such as the net dipole moment, the optical conductivity, and the absorption spectrum beyond the semiclassical approximation. The results are robust against cavity losses and variations of system parameters. Published by the American Physical Society 2024

Quantum scaling of the spin lattice relaxation rate in the checkerboard J-Q model

Motivated by recent progress on the experimental realization of proximate deconfined quantum critical point in a frustrated quantum magnet, we study the low-energy spin dynamics of a related checkerboard J-Q model by using quantum Monte Carlo simulations. The ground state of this model undergoes a weakly first-order quantum phase transition with an emergent O(4) symmetry between an antiferromagnetic state and a plaquette valence bond solid. The calculated spin lattice relaxation rate of nuclear magnetic resonance, 1/T1 , exhibits distinct low-temperature behaviors depending on the ground states. With decreasing the temperature, 1/T1 rises up on the antiferromagnetic side, characterizing a crossover to the renormalized classical regime, whereas 1/T1 drops exponentially on the side of valence bond solid, reflecting the gap opening in the plaquette ordered phase. The extracted spin gap scales with the distance to the transition point as a power-law with an exponent φ ≈ 0.3, consistent with the scaling ansatz ϕ=νz with ν ≈ 0.3 and z = 1. Near the quantum phase transition, the temperature dependent 1/T1 shows a broad crossover regime where a universal scaling 1/T1∼Tη with η ≈ 0.6 is found. Our results suggest a quantum scaling regime associated with the emergent enhanced symmetry near this first-order quantum phase transition.

Analytical solution and spectral structure of the two-photon anisotropic Rabi-Stark model

Since the realization of the strong coupling between light and matter in experimental setups, the quantum Rabi model and its generalized models describing the interaction between the boson field and the two-level system have attracted extensive interest again. The study of anisotropic generalized Rabi models enables us to better understand the novel physical properties of the interaction between light and matter in the ultra-strong and deep-strong coupling regions. In this work, the two-photon anisotropic Rabi-Stark model (tpARSM) is analytically solved by using the Bogoliubov operator approach and the su(1, 1) Lie algebra. We derive the G-function, whose zeros give the regular spectrum of the system. By studying the pole structure of the G-function and the coefficients in the function, exceptional solutions, including the first-order quantum phase transition points, doubly degenerate exceptional solutions and nondegenerate exceptional solutions, are obtained. By discussing the spectral structure, we give the conditions for the first-order quantum phase transition of tpARSM. Furthermore, we find that the property that all of the lowest doubly degenerate crossing points in the two-photon Rabi-Stark model have the same energy only holds for the special case of the tpARSM in which the anisotropy parameter is equal to 1. Finally, from the perspective of first-order quantum phase transitions, concise conditions for the ground state energy level to collapse to or escape from the collapse point for the tpARSM are presented. A good understanding of the tpARSM will lay a good foundation for studying the extended two-photon systems involving multiple levels and multiple bosonic modes, and even the relevant open quantum systems.

First-order quantum phase transition in the two-qubit squeezed Rabi model

We study the ground state of the two-qubit squeezed Rabi model. Two special transformations are found to diagonalize the system Hamiltonian when each qubit’s frequency is close to the field frequency, where both the squeezing and counterrotating-wave interactions are removed, leading to an effective integrable Hamiltonian. The analytical ground state is determined and matches with numerical solutions well for a range of squeezing strengths and qubit-field detunings in the ultrastrong-coupling regime. We demonstrate that the ground state exhibits a first-order quantum phase transition at a phase boundary linearly induced by the squeezed light. We characterize the two-qubit negativity analytically and find that its two-qubit entanglement increases with the increasing squeezing strength nonlinearly. The average photon numbers of the field mode and variances of position and momentum quadratures are also analyzed and discovered to have a nonlinear relation with the squeezing strength. Finally, we discuss the experimental scheme and realization possibility of the predicted results.

Exploring global symmetry-breaking superradiant phase via phase competition.

Superradiant phase transitions play a fundamental role in understanding the mechanism of collective light-matter interaction at the quantum level. Here we investigate multiple superradiant phases and phase transitions with different symmetry-breaking patterns in a two-mode V-type Dicke model. Interestingly, we show that there exists a quadruple point where one normal phase, one global symmetry-breaking superradiant phase, and two local symmetry-breaking superradiant phases meet. Such a global phase results from the phase competition between two local superradiant phases and cannot occur in the standard Λ- and Ξ-type three-level configurations in quantum optics. Moreover, we exhibit a sequential first-order quantum phase transition from one local to the global again to the other local superradiant phase. Our study opens up a perspective of exploring multilevel quantum critical phenomena with global symmetry breaking.

First-order localization and quantum phase transition induced by quasicrystal imaginary domain

First-order localization and quantum phase transition induced by quasicrystal imaginary domain

Bounding first-order quantum phase transitions in adiabatic quantum computing

Bounding first-order quantum phase transitions in adiabatic quantum computing

First-order quantum phase transition in the hybrid metal-Mott insulator transition metal dichalcogenide 4Hb-TaS2.

Coupling together distinct correlated and topologically nontrivial electronic phases of matter can potentially induce novel electronic orders and phase transitions among them. Transition metal dichalcogenide compounds serve as a bedrock for exploration of such hybrid systems. They host a variety of exotic electronic phases, and their Van der Waals nature enables to admix them, either by exfoliation and stacking or by stoichiometric growth, and thereby induce novel correlated complexes. Here, we investigate the compound 4Hb-TaS2 that interleaves the Mott-insulating state of 1T-TaS2 and the putative spin liquid it hosts together with the metallic state of 2H-TaS2 and the low-temperature superconducting phase it harbors using scanning tunneling spectroscopy. We reveal a thermodynamic phase diagram that hosts a first-order quantum phase transition between a correlated Kondo-like cluster state and a depleted flat band state. We demonstrate that this intrinsic transition can be induced by an electric field and temperature as well as by manipulation of the interlayer coupling with the probe tip, hence allowing to reversibly toggle between the Kondo-like cluster and the depleted flat band states. The phase transition is manifested by a discontinuous change of the complete electronic spectrum accompanied by hysteresis and low-frequency noise. We find that the shape of the transition line in the phase diagram is determined by the local compressibility and the entropy of the two electronic states. Our findings set such heterogeneous structures as an exciting platform for systematic investigation and manipulation of Mott-metal transitions and strongly correlated phases and quantum phase transitions therein.

Generalized phase-space techniques to explore quantum phase transitions in critical quantum spin systems

We apply the generalized Wigner function formalism to detect and characterize a range of quantum phase transitions in several cyclic, finite-length, spin-12 one-dimensional spin-chain models, viz., the Ising and anisotropic XY models in a transverse field, and the XXZ anisotropic Heisenberg model. We make use of the finite system size to provide an exhaustive exploration of each system’s single-site, bipartite and multi-partite correlation functions. In turn, we are able to demonstrate the utility of phase-space techniques in detecting and characterizing first-order, second-order and infinite-order quantum phase transitions, while also enabling an in-depth analysis of the correlations present within critical systems. We also highlight the method’s ability to capture other features of spin systems such as ground-state factorization and critical system scaling. Finally, we demonstrate the generalized Wigner function’s utility for state verification by determining the state of each system and their constituent sub-systems at points of interest across the quantum phase transitions, enabling interesting features of critical systems to be readily analyzed.

Observation of First-Order Quantum Phase Transitions and Ferromagnetism in Twisted Double Bilayer Graphene

Observation of First-Order Quantum Phase Transitions and Ferromagnetism in Twisted Double Bilayer Graphene

Phases of the spin- 12 Heisenberg antiferromagnet on the diamond-decorated square lattice in a magnetic field

The spin-1/2 Heisenberg antiferromagnet on the frustrated diamond-decorated square lattice is known to feature various zero-field ground-state phases, consisting of extended monomer-dimer and dimer-tetramer ground states as well as a ferrimagnetic regime. Using a combination of analytical arguments, density matrix renormalization group (DMRG), exact diagonalization as well as sign-problem-free quantum Monte Carlo (QMC) calculations, we investigate the properties of this system and the related Lieb lattice in the presence of a finite magnetic field, addressing both the ground-state phase diagram as well as several thermodynamic properties. In addition to the zero-field ground states, we find at high magnetic field a spin-canted phase with a continuously rising magnetization for increasing magnetic field strength as well as the fully polarized paramagnetic phase. At intermediate field strength, we identify a first-order quantum phase transition line between the ferrimagnetic and the monomer-dimer regime. This first-order line extends to finite temperatures, terminating in a line of critical points that belong to the universality class of the two-dimensional Ising model.

Spectral structure of two-mode Rabi–Stark model

The analytical solutions of the two-mode Rabi–Stark model (tmRSM) are obtained by using the Bogoliubov operators approach in Lie algebra space, which fit the exact numerical results well. The structure of the energy spectra is related to many fundamental physics characters such as symmetry, quantum phase transition (QPT), spectral collapse etc. In this paper, the spectral structure of tmRSM is discussed analytically. The regular energy spectra are given by the zeros of the G-function, and the poles appearing in the G-function are responsible for the exceptional solutions. The double degenerate exceptional solutions could be predicted by discussing the divergence of the coefficients in the G-function. If the numerator and denominator of vanish, the lowest double degenerate exceptional solutions for the nth energy levels would be located, including the first-order QPT point, the corresponding energy () is independent of the coupling strength and the energy level, even independent of the Bargmann index q. While, the nondegenerate exceptional solutions can be reproduced by the nondegenerate exceptional G-functions, the results show that more nondegenerate exceptional solutions would be found in the subspace with larger q. Then, the regular solution and two kinds of exceptional Juddian solutions of tmRSM are accurately located. The spectral collapse energy are dependent on the strength of Stark coupling and the frequency of two-level system, and Stark coupling could results in the limit of E 0 pole line is higher than that of E n pole lines, which may cause more energy levels separate from the collapse energy.

First-order quantum phase transition in the squeezed Rabi model

Quantum phase transition and entanglement in the Rabi model with a squeezed light are investigated. We find a special unitary-transformation method that removes the nonintegrable squeezing and counterrotating-wave interactions when the qubit frequency is close to the field frequency. The analytical ground state agrees well with the numerical solution. We demonstrate that the ground state exhibits a first-order quantum phase transition at a critical point induced linearly by the squeezed light. This quantum phase transition requires neither multiple qubits nor an infinite ratio of qubit frequency to field frequency, which solves a critical problem for the theory and experiment in Rabi model. As the qubit-field coupling strength increases, the ground-state entanglement reaches its maximum value at the critical point.

First-order quantum phase transition and entanglement in the Jaynes–Cummings model with a squeezed light

We study the quantum phase transition and entanglement in the Jaynes–Cummings model with squeezed light, utilize a special transformation method to obtain the analytical ground state of the model within the near-resonance regime, and numerically verify the validity of the analytical ground state. It is found that the ground state exhibits a first-order quantum phase transition at the critical point linearly induced by squeezed light, and the ground state entanglement reaches its maximum when the qubit-field coupling strength is large enough at the critical point.

Quantum Phase Transitions for an Integrable Quantum Rabi-like Model with Two Interacting Qubits.

A two-interacting-qubit quantum Rabi-like model with vanishing transverse fields on the qubit pair is studied. Independently of the coupling regime, this model can be exactly and unitarily reduced to two independent single-spin quantum Rabi models, where the spin-spin coupling plays the role of the transverse field. This transformation and the analytical treatment of the single-spin quantum Rabi model provide the key to prove the integrability of our model. The existence of different first-order quantum phase transitions, characterized by discontinuous two-spin magnetization, mean photon number, and concurrence, is brought to light.

Superradiant Quantum Phase Transition for an Exactly Solvable Two-Qubit Spin-Boson Model.

A spin-boson-like model with two interacting qubits is analysed. The model turns out to be exactly solvable since it is characterized by the exchange symmetry between the two spins. The explicit expressions of eigenstates and eigenenergies make it possible to analytically unveil the occurrence of first-order quantum phase transitions. The latter are physically relevant since they are characterized by abrupt changes in the two-spin subsystem concurrence, in the net spin magnetization and in the mean photon number.

Finite temperature quantum condensations in the space of states: general proof

We formalize and prove the extension to finite temperature of a class of quantum phase transitions, acting as condensations in the space of states, recently introduced and discussed at zero temperature (Ostilli and Presilla 2021 J. Phys. A: Math. Theor. 54 055005). In details, we find that if, for a quantum system at canonical thermal equilibrium, one can find a partition of its Hilbert space into two subspaces, and , such that, in the thermodynamic limit, and the free energies of the system restricted to these subspaces cross each other for some value of the Hamiltonian parameters, then, the system undergoes a first-order quantum phase transition driven by those parameters. The proof is based on an exact probabilistic representation of quantum dynamics at an imaginary time identified with the inverse temperature of the system. We also show that the critical surface has universal features at high and low temperatures.

Thermal critical points from competing singlet formations in fully frustrated bilayer antiferromagnets

We examine the ground-state phase diagram and thermal phase transitions in a plaquettized fully frustrated bilayer spin-1/2 Heisenberg model. Based on a combined analysis from sign-problem free quantum Monte Carlo simulations, perturbation theory, and free-energy arguments, we identify a first-order quantum phase transition line that separates two competing quantum-disordered ground states with dominant singlet formations on interlayer dimers and plaquettes, respectively. At finite temperatures, this line extends to form a wall of first-order thermal transitions, which terminates in a line of thermal critical points. From a perturbative approach in terms of an effective Ising model description, we identify a quadratic suppression of the critical temperature scale in the strongly plaquettized region. Based on free-energy arguments we furthermore obtain the full phase boundary of the low-temperature dimer-singlet regime, which agrees well with the quantum Monte Carlo data.

Implication of giant photon bunching on quantum phase transition in the dissipative anisotropic quantum Rabi model

We investigate quantum phase transition in the dissipative anisotropic quantum Rabi model in the framework of quantum dressed master equation. From perspectives of both numerical and analytical analysis, we unravel the implication of the giant photon-bunching behavior on the first-order quantum phase transition. The observed two-photon statistics can be well described analytically within a few lowest eigenstates at the low temperature. Moreover, such significant photon-bunching feature is generally exhibited at the deep-strong qubit–photon coupling, which is however lacking in the dissipative isotropic quantum Rabi model. Therefore, we suggest that the photon-bunching measurement is helpful to characterize quantum phase transition of the qubit–photon hybrid systems.

Tunable quantum criticalities in an isospin extended Hubbard model simulator

Studying strong electron correlations has been an essential driving force for pushing the frontiers of condensed matter physics. In particular, in the vicinity of correlation-driven quantum phase transitions (QPTs), quantum critical fluctuations of multiple degrees of freedom facilitate exotic many-body states and quantum critical behaviours beyond Landau’s framework1. Recently, moiré heterostructures of van der Waals materials have been demonstrated as highly tunable quantum platforms for exploring fascinating, strongly correlated quantum physics2–22. Here we report the observation of tunable quantum criticalities in an experimental simulator of the extended Hubbard model with spin–valley isospins arising in chiral-stacked twisted double bilayer graphene (cTDBG). Scaling analysis shows a quantum two-stage criticality manifesting two distinct quantum critical points as the generalized Wigner crystal transits to a Fermi liquid by varying the displacement field, suggesting the emergence of a critical intermediate phase. The quantum two-stage criticality evolves into a quantum pseudo criticality as a high parallel magnetic field is applied. In such a pseudo criticality, we find that the quantum critical scaling is only valid above a critical temperature, indicating a weak first-order QPT therein. Our results demonstrate a highly tunable solid-state simulator with intricate interplay of multiple degrees of freedom for exploring exotic quantum critical states and behaviours.