Fiber-based Quantum Communication Research Articles

Numerical investigation of plasmon-enhanced emission from a nanofiber coupled single photon emitter

This study explores the enhancement of emission from a single photon emitter in a quantum communication network by coupling the source with an optical nanofiber and leveraging gold nanoparticles for Purcell enhancement. Large Purcell enhancements of more than 50 times were recently reported experimentally, but the understanding of important issues, including the maximum Purcell factor and limits to quantum efficiency due to ohmic losses, is still lacking. Our findings reveal that the reported experimental results are reasonable, and confirm that such composite devices provide a promising route for high-efficiency single photon sources coupled to an optical fiber-based quantum communication network.

Nonorthogonal coding in spectrally-entangled photons

Controlling and engineering continuous spectral modes of entangled photons represents one of the promising approaches toward secure quantum communications. By using the telecom bandwidth generated from a cascade-emitted biphoton in atomic ensembles, a fiber-based long-distance quantum communication can be feasible owing to its low transmission loss. With multiplexed photon pairs, we propose to implement a nonorthogonal coding scheme in their spectral modes and present an architecture of multiple channels enabling a high-capacity transfer of codewords. Using the measures of the second-order correlations and associated visibility and contrast, we further quantify the performance of the proposed nonorthogonal coding scheme. Our results demonstrate the capability to encode and decode quantum information beyond the orthogonal coding scheme, and in particular, the multi-channel setup manifests a resilience and an advantage in a design with multiple channel errors. The proposed scheme here can be applicable to a large-scale and multiuser quantum communication and pave the way toward an efficient and functional quantum information processing.

Telecom C-band photon emission from (In,Ga)As quantum dots generated by filling nanoholes in In0.52Al0.48As layers

We present the fabrication of strain-free quantum dots in the In0.53Ga0.47As/In0.52Al0.48As-system lattice matched to InP, as future sources for single and entangled photons for long-haul fiber-based quantum communication in the optical C-band. We achieved these quantum dots by local droplet etching via InAl droplets in an In0.52Al0.48As layer and subsequent filling of the holes with In0.53Ga0.47As. Here, we present detailed investigations of the hole morphologies measured by atomic force microscopy. Statistical analysis of a set of nanoholes reveals a high degree of symmetry for nearly half of them when etched at optimized temperatures. Overgrowth with 50–150 nm In0.52Al0.48As increases their diameter and elongates the holes along the [01̄1]-direction. By systematically scanning the parameter space, we were able to fill the holes with In0.53Ga0.47As, and by capping the filled holes and performing photoluminescence measurements, we observe photoluminescence emission in the O-band up into the C-band depending on the filling height of the nanoholes.

Local defects in two-dimensional gallium sulfide as potential single-photon emitters: First-principles evaluation

The single-photon emitters (SPEs) are essential components of emerging quantum communication technology. It has been shown that the local defects in the wide-bandgap semiconductors can be sources of sharp zero-phonon lines (ZPLs) of emission, which is favorable for applications. Most of the reported SPEs emit photons in the visible light region, while fiber-based quantum communication applications require sources of near-infrared (NIR) emission. Therefore, the purpose of this paper is to search for defects which are promising candidates for SPEs in the NIR region by applying computational methods. To this end, based on an educated guess, 12 local doping substitutional defects in two-dimensional (2D) gallium sulfide were selected for consideration. The selected defects are ${Y}_{X}$, where $X=\mathrm{Ga}$ or S, and $Y=\mathrm{C}$, Si, Ge, N, P, As. Here, $X$ stands for a substituted element and $Y$ for a dopant. To evaluate the stability of the defects, their formation energy, binding energy of the dopants, and phonon spectra were calculated within the density functional theory (DFT) approximation. Three defects, ${\mathrm{Ge}}_{\mathrm{Ga}}, {\mathrm{N}}_{\mathrm{Ga}}$, and ${\mathrm{P}}_{\mathrm{Ga}}$, are found to have imaginary-frequency vibration modes, indicating their dynamical instability. They were removed from further consideration. A preliminary analysis of the DFT densities of electronic states (DOS) revealed six remaining defects, ${\mathrm{As}}_{\mathrm{Ga}}, {\mathrm{Ge}}_{\mathrm{S}}, {\mathrm{Si}}_{\mathrm{S}}, {\mathrm{C}}_{\mathrm{S}}, {\mathrm{N}}_{\mathrm{S}}$, and ${\mathrm{P}}_{\mathrm{S}}$, with DOS favorable for formation of local optical excitations in the NIR region. Next, for these six defects, the state-of-the-art linear response GW and the Bethe-Salpeter equation (BSE) methods were used to obtain their electronic structures, in terms of the independent quasiparticle (IQP) states, and optical excitation spectra, in terms of the frequency-dependent dielectric function and the dipole optical transition oscillator strength. The calculation results indicate that the ${\mathrm{C}}_{\mathrm{S}}, {\mathrm{N}}_{\mathrm{S}}$, and ${\mathrm{P}}_{\mathrm{S}}$ defects have intense sharp excitation peaks in the NIR region. The analysis of the contributions of the IQP states to the corresponding BSE eigenstates brings us to the conclusion that these excitations can result in emission with dominating narrow ZPL peaks. I thus propose here the ${\mathrm{C}}_{\mathrm{S}}, {\mathrm{N}}_{\mathrm{S}}$, and ${\mathrm{P}}_{\mathrm{S}}$ defects in 2D GaS as promising candidates for SPEs in the NIR emission region.

Hyperentangled Time-Bin and Polarization Quantum Key Distribution

Fiber-based quantum communication networks are currently limited without quantum repeaters. Satellite-based quantum links have been proposed to extend the network domain. We have developed a quantum communication system, suitable for realistic satellite-to-ground communication. With this system, we have executed an entanglement-based quantum key distribution (QKD) protocol developed by Bennett, Brassard, and Mermin in 1992 (BBM92), achieving quantum bit error rates (QBER) below 2$\%$ in all bases. More importantly, we demonstrate low QBER execution of a higher dimensional hyperentanglement-based QKD protocol, using photons simultaneously entangled in polarization and time-bin, leading to significantly higher secure key rates, at the cost of increased technical complexity and system size. We show that our protocol is suitable for a space-to-ground link, after incorporating Doppler shift compensation, and verify its security using a rigorous finite-key analysis. Additionally, We discuss system engineering considerations relevant to those and other quantum communication protocols, and their dependence on what photonic degrees of freedom are utilized.

Bright single-photon sources in the telecom band by deterministically coupling single quantum dots to a hybrid circular Bragg resonator

High-performance solid-state quantum sources in the telecom band are of paramount importance for long-distance quantum communications and the quantum Internet by taking advantage of a low-loss optical fiber network. Here, we demonstrate bright telecom-wavelength single-photon sources based on In(Ga)As/GaAs quantum dots (QDs) deterministically coupled to hybrid circular Bragg resonators (h-CBRs) by using a wide-field fluorescence imaging technique. The QD emissions are redshifted toward the telecom O-band by using an ultra-low InAs growth rate and an InGaAs strain reducing layer. Single-photon emissions under both continuous wave (CW) and pulsed operations are demonstrated, showing high brightness with count rates of 1.14 MHz and 0.34 MHz under saturation powers and single-photon purities of g ( 2 ) ( 0 ) = 0.11 ± 0.02 (CW) and g ( 2 ) ( 0 ) = 0.087 ± 0.003 (pulsed) at low excitation powers. A Purcell factor of 4.2 with a collection efficiency of 11.2 % ± 1 % at the first lens is extracted, suggesting efficient coupling between the QD and h-CBR. Our work contributes to the development of highly efficient single-photon sources in the telecom band for fiber-based quantum communication and future distributed quantum networks.

Concurrent efficient entanglement routing for quantum wireless networks

Due to the unconditional security of quantum communication and flexible and economical implementation of wireless communication, quantum wireless networks (QWNs) have attracted wide attention. Different from fiber-based or satellite-based quantum communication, quantum wireless networks have the characteristics of high dynamics, limited node energy, and quantum resource competition. We have found that the existing quantum wireless network routing protocols suffer from path collision, high energy consumption, and low utilization of quantum resources. In this paper, a more practical and efficient entanglement routing protocol, which can find contention-free paths for concurrent source destination pairs, is proposed. Simulation results show that the proposed protocol can not only greatly improve the throughput and success rate of the network, but also significantly prolong the network lifetime. The research developed by this work may stimulate more investigations of entanglement routing problems in QWNs.

Strain-Controlled Quantum Dot Fine Structure for Entangled Photon Generation at 1550 nm.

Entangled photon generation at 1550 nm in the telecom C-band is of critical importance as it enables the realization of quantum communication protocols over long distance using deployed telecommunication infrastructure. InAs epitaxial quantum dots have recently enabled on-demand generation of entangled photons in this wavelength range. However, time-dependent state evolution, caused by the fine-structure splitting, currently limits the fidelity to a specific entangled state. Here, we show fine-structure suppression for InAs quantum dots using micromachined piezoelectric actuators and demonstrate generation of highly entangled photons at 1550 nm. At the lowest fine-structure setting, we obtain a maximum fidelity of 90.0 ± 2.7% (concurrence of 87.5 ± 3.1%). The concurrence remains high also for moderate (weak) temporal filtering, with values close to 80% (50%), corresponding to 30% (80%) of collected photons, respectively. The presented fine-structure control opens the way for exploiting entangled photons from quantum dots in fiber-based quantum communication protocols.

Metamorphic Buffer Layer Platform for 1550 nm Single-Photon Sources Grown by MBE on (100) GaAs Substrate.

We demonstrate single-photon emission with a low probability of multiphoton events of 5% in the C-band of telecommunication spectral range of standard silica fibers from molecular beam epitaxy grown (100)-GaAs-based structure with InAs quantum dots (QDs) on a metamorphic buffer layer. For this purpose, we propose and implement graded In content digitally alloyed InGaAs metamorphic buffer layer with maximal In content of 42% and GaAs/AlAs distributed Bragg reflector underneath to enhance the extraction efficiency of QD emission. The fundamental limit of the emission rate for the investigated structures is 0.5 GHz based on an emission lifetime of 1.95 ns determined from time-resolved photoluminescence. We prove the relevance of a proposed technology platform for the realization of non-classical light sources in the context of fiber-based quantum communication applications.

Long-lived and multiplexed atom-photon entanglement interface with feed-forward-controlled readouts

Quantum interfaces (QIs) that generate entanglement between photonic and spin-wave (atomic memory) qubits are basic building block for quantum repeaters. Realizing ensemble-based repeaters in practice requires quantum memory providing long lifetimes and multimode capacity. Significant progress has been achieved on these separate goals. The remaining challenge is to combine the two attributes into a single QI. Here, by establishing spatial multimode, magnetic-field-insensitive and long-wavelength spin-wave storage in laser-cooled atoms inside a phase-passively-stabilized polarization interferometer, we constructed a multiplexed QI that stores up to three long-lived spin-wave qubits. Using a feed-forward-controlled system, we demonstrated that a multiplexed QI gives rise to a 3-fold increase in the atom–photon (photon–photon) entanglement-generation probability compared with single-mode QIs. For our multiplexed QI, the measured Bell parameter is 2.51±0.01 combined with a memory lifetime of up to 1 ms. This work represents a key step forward in realizing fiber-based long-distance quantum communications.

Thermal stability of emission from single InGaAs/GaAs quantum dots at the telecom O-band

Single-photon sources are key building blocks in most of the emerging secure telecommunication and quantum information processing schemes. Semiconductor quantum dots (QD) have been proven to be the most prospective candidates. However, their practical use in fiber-based quantum communication depends heavily on the possibility of operation in the telecom bands and at temperatures not requiring extensive cryogenic systems. In this paper we present a temperature-dependent study on single QD emission and single-photon emission from metalorganic vapour-phase epitaxy-grown InGaAs/GaAs QDs emitting in the telecom O-band at 1.3 μm. Micro-photoluminescence studies reveal that trapped holes in the vicinity of a QD act as reservoir of carriers that can be exploited to enhance photoluminescence from trion states observed at elevated temperatures up to at least 80 K. The luminescence quenching is mainly related to the promotion of holes to higher states in the valence band and this aspect must be primarily addressed in order to further increase the thermal stability of emission. Photon autocorrelation measurements yield single-photon emission with a purity of {g}_{50K}^{(2)}left(0right)=0.13 up to 50 K. Our results imply that these nanostructures are very promising candidates for single-photon sources at elevated (e.g., Stirling cryocooler compatible) temperatures in the telecom O-band and highlight means for improvements in their performance.

Optimal photon pairs for quantum communication protocols

We theoretically investigate the problem of finding optimal characteristics of photon pairs, produced in the spontaneous parametric down-conversion (SPDC) process, for fiber-based quantum communication protocols. By using the accessible setup parameters, the pump pulse duration and the extended phase-matching function width, we minimize the temporal width of SPDC photons within the general scenario. This allows one to perform more effectively the temporal filtering procedure, which aims at reducing the noise acquired by the measurement devices. Moreover, we compare the obtained results with the achievable parameter values for SPDC sources based on beta-Barium Borate crystal. We also investigate the influence of non-zero detection timing jitter. Finally, we apply our optimization strategy to a simple quantum key distribution scheme to show that the full optimization of an SPDC source can potentially extend the maximal security distance by several tens of kilometres, which is around 30% more as compared to previous approaches.

Optimizing up-conversion single-photon detectors for quantum key distribution.

High-performance single-photon detectors (SPDs) at 1550-nm band are critical for fiber-based quantum communications. Among many types of SPDs, the up-conversion SPDs based on periodically poled lithium niobate waveguides are of great interest. Combined with a strong pump laser, the telecom single-photons are converted into short wavelength ones and detected by silicon-based SPDs. However, due to the difficulty of precise controlling waveguide profile, the direct coupling between a single-mode fiber and the waveguide is not efficient. Here by utilizing fiber taper with proper diameter, optimal mode-matching is achieved and coupling efficiency up to 93% is measured. With an optimized design, a system detection efficiency of 36% and noise counting rate of 90 cps are realized. The maximum detection efficiency is characterized as 40% with a noise counting rate of 200 cps. Numerical simulation results indicate that our device can significantly improve the performance of QKD and extend the communication distance longer than 200 km.

Quantum dot-based broadband optical antenna for efficient extraction of single photons in the telecom O-band.

Long-distance fiber-based quantum communication relies on efficient non-classical light sources operating at telecommunication wavelengths. Semiconductor quantum dots are promising candidates for on-demand generation of single photons and entangled photon pairs for such applications. However, their brightness is strongly limited due to total internal reflection at the semiconductor/vacuum interface. Here we overcome this limitation using a dielectric antenna structure. The non-classical light source consists of a gallium phosphide solid immersion lens in combination with a quantum dot nanomembrane emitting single photons in the telecom O-band. With this device, the photon extraction is strongly increased in a broad spectral range. A brightness of 17% (numerical aperture of 0.6) is obtained experimentally, with a single photon purity of g(2)(0)=0.049±0.02 at saturation power. This brings the practical implementation of quantum communication networks one step closer.

Drone-based entanglement distribution towards mobile quantum networks.

Satellites have shown free-space quantum-communication ability; however, they are orbit-limited from full-time all-location coverage. Meanwhile, practical quantum networks require satellite constellations, which are complicated and expensive, whereas the airborne mobile quantum communication may be a practical alternative to offering full-time all-location multi-weather coverage in a cost-effective way. Here, we demonstrate the first mobile entanglement distribution based on drones, realizing multi-weather operation including daytime and rainy nights, with a Clauser-Horne-Shimony-Holt S-parameter measured to be 2.41 ± 0.14 and 2.49 ± 0.06, respectively. Such a system shows unparalleled mobility, flexibility and reconfigurability compared to the existing satellite and fiber-based quantum communication, and reveals its potential to establish a multinode quantum network, with a scalable design using symmetrical lens diameter and single-mode-fiber coupling. All key technologies have been developed to pack quantum nodes into lightweight mobile platforms for local-area coverage, and arouse further technical improvements to establish wide-area quantum networks with high-altitude mobile communication.

Orbital Angular Momentum States Enabling Fiber-based High-dimensional Quantum Communication

Quantum networks are the ultimate target in quantum communication, where many connected users can share information carried by quantum systems. The keystones of such structures are the reliable generation, transmission and manipulation of quantum states. Two-dimensional quantum states, qubits, are steadily adopted as information units. However, high-dimensional quantum states, qudits, constitute a richer resource for future quantum networks, exceeding the limitations imposed by the ubiquitous qubits. The generation and manipulation of such $D$-level systems have been improved over the last ten years, but their reliable transmission between remote locations remains the main challenge. Here, we show how a recent air-core fiber supporting orbital angular momentum (OAM) modes can be exploited to faithfully transmit $D$-dimensional states. Four OAM quantum states and their superpositions are created, propagated in a 1.2 km long fiber and detected with high fidelities. In addition, three quantum key distribution (QKD) protocols are implemented as concrete applications to assert the practicality of our results. This experiment enhances the distribution of high-dimensional quantum states, attesting the orbital angular momentum as vessel for the future quantum network.

Spectrally entangled biphoton state of cascade emissions from a Doppler-broadened atomic ensemble

We theoretically investigate the spectral property of biphoton state from the cascade emissions from a Doppler-broadened atomic ensemble. This biphoton state is spontaneously created in the four-wave-mixing process. The upper transition of the emissions lies in telecom bandwidth, which prevails in fiber-based quantum communication for low-loss transmission. We obtain the spectral function of the biphoton state in terms of superradiant decay rates of the lower transition, excitation pulse durations, and temperature of the medium. We quantify their frequency entanglement by Schmidt decomposition and find that more entangled source can be generated with longer excitation pulses, enhanced decay rates, and significant Doppler broadening. A minimally entangled biphoton source can also be located at some optimal temperature of the atoms. By tuning these parameters, this biphoton source allows spectral shaping of continuous frequency entanglement, which is useful in multimode long-distance quantum communication.

Two-photon interference in the telecom C-band after frequency conversion of photons from remote quantum emitters.

Efficient fibre-based long-distance quantum communication via quantum repeaters relies on deterministic single-photon sources at telecom wavelengths, potentially exploiting the existing world-wide infrastructures. For upscaling the experimental complexity in quantum networking, two-photon interference (TPI) of remote non-classical emitters in the low-loss telecom bands is of utmost importance. Several experiments have been conducted regarding TPI of distinct emitters, for example, using trapped atoms1, ions2, nitrogen vacancy centres3,4, silicon vacancy centres5, organic molecules6 and semiconductor quantum dots7,8. However, the spectral range was far from the highly desirable telecom C-band. Here, we exploit quantum frequency conversion to realize TPI at 1,550 nm with single photons stemming from two remote quantum dots. We thereby prove quantum frequency conversion9-11 as a bridging technology and a precise and stable mechanism to erase the frequency difference between independent emitters. On resonance, a TPI visibility of 29 ± 3% has been observed, limited only by the spectral diffusion processes of the individual quantum dots12,13. The local fibre network used covers several rooms between two floors of the building. Even the addition of up to 2 km of fibre channel shows no influence on the TPI visibility, proving the photon wavepacket distortion to be negligible. Our studies pave the way to establish long-distance entanglement distribution between remote solid-state emitters including interfaces with various quantum hybrid systems14-16.

Compact frequency-stabilized pump laser for wavelength conversion in long-distance quantum communication

We demonstrate a compact frequency-stabilized laser at 1064 nm using Doppler-free saturation absorption spectroscopy of molecular iodine. The achieved laser frequency stability and linewidth are 5.7 10-12 (corresponding to an uncertainty of the laser frequency of 1.6 kHz) and 400 kHz, respectively. The developed frequency-stabilized laser can be used as a pump laser for wavelength conversion from visible to telecom (or vice versa) to connect quantum memories utilizing nitrogen-vacancy centers in diamond at remote nodes in fiber-based quantum communication.

A stable wavelength-tunable triggered source of single photons and cascaded photon pairs at the telecom C-band

The implementation of fiber-based long-range quantum communication requires tunable sources of single photons at the telecom C-band. Stable and easy-to-implement wavelength-tunability of individual sources is crucial to (i) bring remote sources into resonance, (ii) define a wavelength standard, and (iii) ensure scalability to operate a quantum repeater. So far, the most promising sources for true, telecom single photons are semiconductor quantum dots, due to their ability to deterministically and reliably emit single and entangled photons. However, the required wavelength-tunability is hard to attain. Here, we show a stable wavelength-tunable quantum light source by integrating strain-released InAs quantum dots on piezoelectric substrates. We present triggered single-photon emission at 1.55 μm with a multi-photon emission probability as low as 0.097, as well as photon pair emission from the radiative biexciton–exciton cascade. We achieve a tuning range of 0.25 nm which will allow us to spectrally overlap remote quantum dots or tuning distant quantum dots into resonance with quantum memories. This opens up realistic avenues for the implementation of photonic quantum information processing applications at telecom wavelengths.