A series of (Ba2Zn2Fe12O22)1−x(NiFe2O4)x ferrites (x = 0.0, 0.2, 0.4, 0.6, 0.8 and 1.0) were successfully synthesized by one-pot coprecipitation route. XRD analysis reveals the formation of Ba2Zn2Fe12O22 and NiFe2O4 composite after sintering calcined precursor powder at 1200 °C/4 h. Densification behaviour was evaluated by Archimedes’ principle. Field emission scanning electron microscopy was used to study morphological characteristics. Room temperature magnetization behaviour was evaluated using a vibrating sample magnetometer. In composite, it was observed that the saturation magnetization (Ms) and coercivity (Hc) increased with increasing NiF content. With the increase of NiF in the composite, the permittivity (ε) decreased from 28.6 (for x = 0.2) to 13.6 (for x = 0.8) with the corresponding decrease in dielectric loss (tanδε) at 100 MHz. The permeability (μ) also decreased from 21.3 (x = 0.2) to 17.9 (x = 0.8) with the associated decrease of the magnetic losses (tanδμ) at 100 MHz. Miniaturization factor (n) of 19.2 and characteristic impedance of 1.1 were obtained for x = 0.4 composition at 100 MHz along with low dielectric loss factor (tan δε/ε) and magnetic loss factor (tan δµ/µ). The ferrite resonator antenna was fabricated using FR4 as substrate and ferrite pellet as magneto-dielectric resonator material. The antenna characteristics parameters reflection loss S (1,1) and voltage standing wave ratio (VSWR) were measured by vector network analyser (VNA).
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