Source Of Femtosecond Pulses Research Articles

Widely wavelength-tunable high-repetition-rate femtosecond pulse source with highest average power up to 28 W

We have proposed and demonstrated a high-repetition-rate ultrashort pulse fiber amplification system based on a wavelength-tunable oscillator. This fiber amplification system produces an average power exceeding 20 W in bursts of 200 pulses with a 578 MHz intra-burst pulse repetition rate and a 1 MHz burst repetition rate. The center wavelength of the amplified pulses can be tuned from 1030 to 1080 nm. By utilizing pre-chirp management nonlinear amplification technique, the achieved shortest pulse duration is 27 fs with an average power of 25 W at 1032 nm. For all the amplified pulses with different wavelengths, the pulse duration after optimal compression is below 60 fs. To the best of our knowledge, this is the first time that a widely wavelength-tunable high-power laser with a repetition rate exceeding 100 MHz and a pulse duration of several tens of femtoseconds has been realized. Additionally, using only common double-cladding Yb-doped fiber as the gain fiber, without any large-mode-area Yb-doped photonic crystal fiber or rod-type Yb-doped fiber, makes the system compact and reliable due to the simple fusion operation.

165 MHz highly stable femtosecond Er:ZBLAN fiber laser operating at 2.8 µm.

Three-micrometer mid-infrared (MIR) femtosecond pulse sources with a high repetition rate (HRR) have potential applications in a number of fields such as biological imaging, optical frequency combs, and gas detection. In this paper, by optimizing the fiber length and the cavity structure, we demonstrated a highly stable, self-starting mode-locked fluoride fiber laser (MLFFL) with a fundamental repetition rate of ∼165 MHz and a signal-to-noise ratio (SNR) of 90 dB. As far as we know, this stands as the highest fundamental repetition rate ever acquired directly from an ultrafast MLFFL in the >2.5 µm MIR region. Stable 352-fs pulses at 2795 nm with an average output power of 392 mW and a low integrated relative intensity noise (RIN) of 0.018% [10 Hz, 10 MHz] were generated. The root mean square (RMS) power fluctuation is 0.17% over 2 h, which indicates excellent oscillator stability. This high-performance laser offers a practicable scheme both for scaling the repetition frequency in MIR MLFFLs and high-precision ultrafast applications at longer wavelengths.

Plasma electron acceleration driven by a long-wave-infrared laser

Laser-driven plasma accelerators provide tabletop sources of relativistic electron bunches and femtosecond x-ray pulses, but usually require petawatt-class solid-state-laser pulses of wavelength λL ~ 1 μm. Longer-λL lasers can potentially accelerate higher-quality bunches, since they require less power to drive larger wakes in less dense plasma. Here, we report on a self-injecting plasma accelerator driven by a long-wave-infrared laser: a chirped-pulse-amplified CO2 laser (λL ≈ 10 μm). Through optical scattering experiments, we observed wakes that 4-ps CO2 pulses with < 1/2 terawatt (TW) peak power drove in hydrogen plasma of electron density down to 4 × 1017 cm−3 (1/100 atmospheric density) via a self-modulation (SM) instability. Shorter, more powerful CO2 pulses drove wakes in plasma down to 3 × 1016 cm−3 that captured and accelerated plasma electrons to relativistic energy. Collimated quasi-monoenergetic features in the electron output marked the onset of a transition from SM to bubble-regime acceleration, portending future higher-quality accelerators driven by yet shorter, more powerful pulses.

Integrated femtosecond pulse generator on thin-film lithium niobate.

Integrated femtosecond pulse and frequency comb sources are critical components for a wide range of applications, including optical atomic clocks1, microwave photonics2, spectroscopy3, optical wave synthesis4, frequency conversion5, communications6, lidar7, optical computing8 and astronomy9. The leading approaches for on-chip pulse generation rely on mode-locking inside microresonators with either third-order nonlinearity10 or with semiconductor gain11,12. These approaches, however, are limited in noise performance, wavelength and repetition ratetunability10,13. Alternatively, subpicosecond pulses can be synthesized without mode-locking, by modulating a continuous-wave single-frequency laser using electro-optic modulators1,14-17. Here we demonstrate a chip-scale femtosecond pulse source implemented on an integrated lithium niobate photonic platform18, using cascaded low-loss electro-optic amplitude and phase modulators and chirped Bragg grating, forming a time-lens system19. The device is driven by a continuous-wave distributed feedback laser chipand controlled by a single continuous-wave microwave source without the need for any stabilization or locking. We measure femtosecond pulse trains (520-femtosecond duration) with a 30-gigahertz repetition rate, flat-top optical spectra with a 10-decibel optical bandwidth of 12.6 nanometres, individual comb-line powers above 0.1 milliwatts, and pulse energies of 0.54 picojoules. Our results represent a tunable, robust and low-cost integrated pulsed light source with continuous-wave-to-pulse conversion efficiencies an order of magnitude higher than those achieved with previous integrated sources. Our pulse generator may find applications in fields such as ultrafast optical measurement19,20 or networks of distributed quantum computers21,22.

High-efficiency and broadband on-chip electro-optic frequency comb generators

Developments in integrated photonics have led to stable, compact, and broadband comb generators that support a wide range of applications. Current on-chip comb generators, however, are still limited by low optical pump-to-comb conversion efficiencies. Here, we demonstrate an integrated electro-optic frequency comb with a conversion efficiency of 30% and an optical bandwidth of 132 nm, featuring a 100-times higher conversion efficiency and 2.2-times broader optical bandwidth compared with previous state-of-the-art integrated electro-optic combs. We further show that, enabled by the high efficiency, the device acts as an on-chip femtosecond pulse source (336 fs pulse duration), which is important for applications in nonlinear optics, sensing, and computing. As an example, in the ultra-fast and high-power regime, we demonstrate the observation of a combined EO-\chi^(3) nonlinear frequency comb. Our device paves the way for practical optical frequency comb generators enabling energy-efficient computing, communication, and metrology, and provides a platform to investigate new regimes of optical physics that simultaneously involve multiple nonlinearities.

Frequency-multiplexed entanglement for continuous-variable quantum key distribution

Quantum key distribution with continuous variables already uses advantageous high-speed single-mode homodyne detection with low electronic noise at room temperature. Together with continuous-variable information encoding to nonclassical states, the distance for secure key transmission through lossy channels can approach 300 km in current optical fibers. Such protocols tolerate higher channel noise and also limited data processing efficiency compared to coherent-state protocols. The secret key rate can be further increased by increasing the system clock rates, and, further, by a suitable frequency-mode-multiplexing of optical transmission channels. However, the multiplexed modes couple together in the source or any other part of the protocol. Therefore, multiplexed communication will experience cross talk and the gain can be minuscule. Advantageously, homodyne detectors allow solving this cross-talk problem by proper data processing. It is a potential advantage over protocols with single-photon detectors, which do not enable similar data processing techniques. We demonstrate the positive outcome of this methodology on the experimentally characterized frequency-multiplexed entangled source of femtosecond optical pulses with natural cross talk between eight entangled pairs of modes. As the main result, we predict the almost 15-fold higher secret key rate. This experimental test and analysis of frequency-multiplexed entanglement source open the way for the field implementation of high-capacity quantum key distribution with continuous variables.

Fiber source of femtosecond pulses at 910–940 nm based on a Mamyshev pulse oscillator and wavelength conversion in a photonic crystal fiber

In this work, we present a fiber-based setup for femtosecond pulse generation at ∼ 910 − 940 n m wavelength. Pump pulses from a Mamyshev oscillator with center wavelength at 1036 nm 1 ps duration are amplified and coupled into a photonic crystal fiber forming a soliton at 1051 nm. Due to the nonlinear four-wave mixing process, soliton pulses are converted to 910–940 nm with a few hundred femtosecond pulses with energy up to 0.7 nJ. The proposed design utilizes features of the Mamyshev oscillator, enabling a robust way of generating femtosecond pulses at ∼ 910 − 940 n m .

Femtosecond pulse generation from external cavity diode laser based on self-mode-locking.

In this Letter, we report optical pulse generation from a single-section diode gain chip, employed in an external cavity geometry based on the self-mode-locking regime. The gain chip emits light at 1550 nm wavelength range. The external cavity is operated at various repetition rates, ranging from 1 to 2.5 GHz. An optical pulse width of approximately 650 fs is obtained by fitting a Lorentzian distribution. A low RF spectral width of 78.875 kHz is measured corresponding to a low pulse-to-pulse RMS timing jitter of 1.273 ps. This system paves the way towards ultra-compact, cost-effective, and chirp-compensated femtosecond laser pulse sources with adjustable repetition rates.

Broadband and Tunable 920-nm Femtosecond Pulse Generated by an All-Fiber Er:Fiber Laser System

Fiber-optic Cherenkov radiation (FOCR) is a promising nonlinear process that is widely used for nonlinear wavelength conversion. In this study, an all-fiber 920-nm femtosecond pulse source is experimentally demonstrated by using Cherenkov radiation. The 4-nJ 150-fs 1550-nm amplified seed pulse source ensures highly efficient 920-nm pulse generation. Cherenkov radiation is stimulated by inputting the high-energy ultrashort pulse to a highly nonlinear fiber. The dispersion values of the highly nonlinear fiber (HNLF) are carefully chosen to generate CR pulses at 920 nm. The generated pulse has a 150-pJ single pulse energy and a 232-fs pulse duration. The typical 30-nm bandwidth can support a sub-50-fs transform-limited pulse duration. The pump current can be adjusted to tune the central wavelength of the pulse source over 905–930 nm. This very simple approach can generate 920-nm femtosecond pulses. The wavelength range is useful for a wide range of applications, such as two-photon microscopy (TPM) in bio-imaging and so on.

Longwave mid-IR femtosecond pulse sources driven by ultrafast fiber lasers (Invited)

Longwave mid-IR femtosecond pulse sources driven by ultrafast fiber lasers (Invited)

Retrieving intracycle interference in angle-resolved laser-assisted photoemission from argon

We report on a combined experimental and theoretical study of XUV ionization of atomic argon in the presence of a near-infrared (NIR) laser field. Using a table-top source of wavelength-selected femtosecond XUV pulses in combination with a velocity map imaging spectrometer we record angle- and energy-resolved photoelectron distributions and simulate the experimental data by solving the time-dependent Schrödinger equation ab initio. In order to compare with the experimental data we average the calculated energy-angle probability distributions over the experimental focal volume for different values of the magnetic quantum number of the photoelectron. This averaging procedure washes out the intracycle interference pattern, which would otherwise be observed in the form of angular modulations of the photoelectron spectra. We recover these modulations experimentally and in the simulations by evaluating the difference between two averaged distributions that are obtained for slightly different NIR laser field intensities.

Mode-locked dysprosium fiber laser: Picosecond pulse generation from 2.97 to 3.30 μm

Mode-locked fiber laser technology to date has been limited to sub-3 μm wavelengths despite significant application-driven demand for compact picosecond and femtosecond pulse sources at longer wavelengths. Erbium-doped and holmium-doped fluoride fiber lasers incorporating a saturable absorber are emerging as promising pulse sources for 2.7–2.9 μm, yet it remains a major challenge to extend this coverage. Here, we propose a new approach using a dysprosium-doped fiber with frequency shifted feedback (FSF). Using a simple linear cavity with an acousto-optic tunable filter, we generate ∼33 ps pulses with up to 2.7 nJ energy and 330 nm tunability from 2.97 to 3.30 μm (∼3000–3400 cm−1)—the first mode-locked fiber laser to cover this spectral region and the most broadly tunable pulsed fiber laser to date. Numerical simulations show excellent agreement with experiments and also offer new insights into the underlying dynamics of FSF pulse generation. This highlights the remarkable potential of both dysprosium as a gain material and FSF for versatile pulse generation, opening new opportunities for mid-IR laser development and practical applications outside the laboratory.

Mid-Infrared Self-Similar Pulse Compression in a Tapered Tellurite Photonic Crystal Fiber and Its Application in Supercontinuum Generation

In this paper, we design a tapered tellurite photonic crystal fiber (TTPCF) with nonlinear coefficient increasing along the propagation direction, and demonstrate the mid-infrared self-similar pulse compression of the fundamental soliton in such a TTPCF. When the variation of group-velocity dispersion, higher-order dispersion, higher-order nonlinearity, and linear loss are considered, a 1 ps pulse at wavelength 2.5 μm can be compressed to 62.16 fs after a 1.63-m long propagation, along with the negligible pedestal, compression factor F c of 16.09, and quality factor Q c of 83.16%. Then the compressed pulse is launched into another uniform tellurite PCF, where highly coherent and octave-spanning supercontinuum (SC) is generated. Compared to the initial picosecond pulse, the compressed pulse has much larger tolerance of noise level for the SC generation. Our research results provide a promising solution to realize the fiber-based mid-infrared femtosecond pulse source for nonlinear photonics and spectroscopy.

High-order harmonic generations in intense MIR fields by cascade three-wave mixing in a fractal-poled LiNbO3 photonic crystal.

We report on the generation of harmonic-like photon upconversion in a LiNbO3-based nonlinear photonic crystal by mid-infrared (MIR) femtosecond laser pulses. We study below bandgap harmonics of various driver wavelengths, reaching up to the 11th order at 4μm driver with 13% efficiency. We compare our results to numerical simulations based on two mechanisms: cascade three-wave mixing and non-perturbative harmonic generation, both of which include quasi-phase matching. The cascade model reproduces well the general features of the observed spectrum, including a plateau-like harmonic distribution and the observed efficiency. This has the potential for providing a source of tabletop few femtosecond ultraviolet pulses.

Kerr-lens mode-locked 2.3-μm Tm3+:YLF laser as a source of femtosecond pulses in the mid-infrared.

We report what is to our knowledge a new source of femtosecond pulses in the mid-infrared, based on a Kerr-lens mode-locked (KLM) Tm3+:YLF laser at 2303nm. An undoped ZnSe substrate was included in the resonator to provide enhanced nonlinear phase modulation during KLM operation. The Tm3+:YLF laser was end-pumped with a continuous-wave Ti3+ : sapphire laser at 780nm. With 880mW of pump power, we generated 514-fs pulses at a pulse repetition rate of 41.5MHz with an average power of 14.4mW. The spectral width (full width at half-maximum) was measured as 15.4nm, giving a time-bandwidth product of 0.44. We foresee that the wide availability of this gain medium, as well as the straightforward pumping scheme near 800nm, will make 2.3-μm, mode-locked Tm3+:YLF lasers versatile sources of ultrashort pulses in the mid-infrared.

Tunable time-resolved tick-tock pulsed digital holographic microscopy for ultrafast events.

This study presents a time-resolved imaging technique for detecting ultrafast events in the sample with tunable tick-tock pulses in common-path digital holographic microscopy. The tick-tock pulses are generated from the same single femtosecond pulse source and manipulated through a spatial-multiplexing encoding/decoding scheme with two complementary binary codes for digital hologram recording and reconstruction. The spatial-multiplexing encoding/decoding scheme with compressive sensing on the Fresnel digital hologram is used to recover missing data and achieve high-fidelity wavefront reconstruction. The elapsed time of tick-tock pulses can be adjusted by changing the optical path difference between the pulse pair arms for dynamic observation at various timescales. The proposed method is applied to explore the ultrafast physical phenomenon by quantitative phase imaging with a stopwatch-like tunable timescale ranging from nanoseconds to femtoseconds.

Controlling single harmonic enhancement in laser-produced plasmas

We compare the plasma emission and harmonic generation spectra in the cases of resonance enhancement of single harmonic using various laser-produced plasmas. The analysis of these spectra showed that the enhancement of harmonics depended on the oscillator strengths of the nearby ionic transitions rather than the plasma emission transitions. To prove it, we used the tunable source of mid-infrared radiation from an optical parametric amplifier (1200–1600 nm) and the fixed wavelength source (810 nm) of femtosecond pulses. The comparison of resonantly enhanced and featureless plateaulike harmonic spectra from different laser-produced plasmas, as well as their plasma emissions, confirmed this assumption.

Undulators and generation of X-ray pulses in free-electron lasers with self-amplified spontaneous emission

The results of theoretical examination and comparative analysis of synchrotron radiation sources (specifically, undulators and X-ray free-electron lasers (FELs)) are presented. The problem of generation of shorter radiation pulses is prioritized; undulator systems and their corresponding FELs, which are considered to be the most promising in terms of generation of high-frequency ultrashort pulses of such radiation (in particular, in the X-ray range) are studied. The possibility of generation of higher harmonics is explored. The advantages and disadvantages of single-pass (with no reflecting elements) and multi-pass (with mirrors) FEL lasing schemes are revealed. The potential to reduce the duration of laser pulses produced by undulators and FELs and use them as sources of femtosecond pulses is investigated. The prospects for further development of X-ray free-electron lasers and the ways to improve the quality of their radiation with the given parameters are discussed.

All-Fiber Generation of Sub-30 fs Pulses at 1.3-μm via Cherenkov Radiation With Entire Dispersion Management

An all-fiber 1.3-μm femtosecond pulse source has been demonstrated via Cherenkov radiation in highly nonlinear fiber seeded by an ultrafast Er-doped fiber laser. Through the dispersion management in total process, the generated pulses can be as short as 29 fs. This pulse source has a 15% conversion efficiency accounting for the input power and the single pulse energy reaches 76 pJ. Furthermore, a simulation has been carried out to illustrate the pulse evolution on the spectral and temporal progress in fibers. To the best of our knowledge, this is the first report of all-fiber 1.3 μm ultrashort pulse source with the duration below 30 fs.

Ways of development of compact coherent femtosecond X-ray sources for applications in nano- and biophotonics

Ways of the development of compact coherent sources of soft X-ray femtosecond pulses are discussed, which meet the requirements for the implementation of the “diffraction-before-destruction” approach in the lensless X-ray Coherent Diffractive Imaging (CDI) technique enabling quantitative 3D mapping of material structure with the nanoscale spatial resolution. An innovative hybrid (solid/gas) approach to produce ultra-intense femtosecond laser pulses in the visible is described in the context of its applications for laser driven high harmonic generation (HHG) and soft X-ray generation in laser plasmas due to recombination mechanism of excitation.