Explosion Of Clusters Research Articles

Transition from Surface to Volume Expansion in Argon Clusters Coulomb Explosion.

The intensity-difference spectrum technique is applied to record charge-state resolved ion energy spectra from the Coulomb explosion of small Ar clusters under well-resolved laser intensity conditions. The far-reaching control of the experimental parameters permits us to identify a striking change in the expansion pattern of the nanoplasma beyond a given intensity. The simultaneous characterization of ion charge state and energy uncovers that a reduction of the laser intensity leads to a development of low energy cuts in the ion yields, not present at higher fluence. The complex interplay of outer ionization, recombination, ion screening, and the phenomenon of ionization saturation favors a surface-driven expansion at low plasma electron temperatures. With increasing laser intensity a transition into a volume-driven Coulomb explosion is observed.

Numerical simulation of deflagration fracturing in shale gas reservoirs considering the effect of stress wave impact and gas drive

Methane deflagration fracturing is a new reservoir stimulation method that serves the efficient development of shale gas reservoirs. However, the propagation law of deflagration fractures is still unclear. In this paper, a numerical model considering the effect of stress wave impact and gas drive of deflagration fracturing was established based on the continuum–discontinuum element method (CDEM). The correctness of the numerical model was verified by comparing it with a laboratory experiment, the steady and unsteady analytical solutions of gas flow, and the approximate solution of fracture propagation. Then, numerical simulations of methane deflagration fracturing in vertical wells and horizontal wells under different factors were carried out to analyze the fracture mechanism. The results indicate that deflagration fracturing in vertical wells can break through the stress concentration around the borehole; the initial radial fractures are formed under the action of stress wave impact and then propagate substantially under the driving action of high-pressure gas. The in-situ stress difference affects the deflagration fracture propagation and makes the half-fracture length in the direction of maximum principal stress larger than that in the direction of minimum principal stress. The more significant the stress difference is, the more noticeable this deviation will be. When the deflagration peak pressure is high, the reservoir burst degree is large, which is conducive to enlarging the stimulation range of deflagration fracturing. Staged deflagration fracturing in horizontal wells can form 5–8 obvious fractures perpendicular to the horizontal borehole in each explosion section. A large cluster spacing and explosion section length are conducive to expanding the stimulation scope. Moreover, the propagation of deflagration fractures will be induced by the natural fractures, and the natural fracture with a considerable length or a slight angle between the dip angle and the propagation direction of deflagration fractures is more likely to be activated.

Surface explosion and subsequent core expansion of laser-heated clusters probed by time-resolved photoelectron spectroscopy

The dynamics of nanoplasma produced by an intense near-infrared pulse was investigated by time-resolved soft x-ray photoelectron spectroscopy. The pump-probe electron spectra indicate transient evolution of the electronic states of the constituent atoms and ions during plasma formation and disintegration. The delay dependence of photoelectron yields supports two-step fragmentation of laser-heated clusters, i.e., rapid explosion of surface ions followed by slow expansion of neutral atoms. The speed of the neutral core expansion was evaluated by comparing the experimental data with a model of uniform neutral core expansion.

Limited Formation of CO3+ through Strong-Field Ionization and Coulomb Explosion of Formic Acid Clusters.

Femtosecond laser pulses are utilized to drive multiple ionization in gas-phase formic acid clusters (FA)n. Experimental measurements of the kinetic energy release (KER) of the ions through Coulomb explosion are studied using time-of-flight mass spectrometry and compared to the values recorded from molecules. Upon interacting with 200 fs linearly polarized laser pulses of 400 nm, formic acid clusters facilitate the formation of higher charge states than the formic acid dimer, reaching both C3+ and O3+ and also increasing the KER values to several hundred electronvolts in magnitude for such ions. At a lower laser intensity (3.8 × 1014 W/cm2), we record an enhancement in the signal of the (FA)5(H2O)H+ cluster, which suggests that it has a higher stability, in agreement with previous studies. A molecular dynamics simulation of the Coulomb explosion shows that the highly charged atomic ions arise from larger clusters, whereas the production of CO3+ is more likely to arise from the molecular case. Thus, the relative production of CO3+ is reduced in comparison to the highly charged ions upon clustering and is likely due to the higher ionization levels achieved, which facilitate dissociation.

Simulating fusion reactions from Coulomb explosions within a transport approach

We have studied nuclear fusion reactions from the Coulomb explosion of deuterium clusters induced by high-intensity laser beams within a transport approach. By incorporating the D+D $\rightarrow$ n + He$^3$ channel as inelastic collisions based on the stochastic method, we have calibrated the neutron yield from the simulation in a box system with that from the reaction rate equation. After justifying the Coulomb explosion of a single cluster by comparing results with available theoretical limits, we have then investigated the dynamics from Coulomb explosions of systems with different cluster numbers and different deuteron numbers in clusters. We find that the kinetic energy spectrum of deuterons at the final stage is different from that when neutrons are abundantly produced, corresponding to significantly different reaction rates. We also extrapolate the neutron yield result from small systems to large systems based on an intuitive parameterized form and compare with the available experimental result. The present framework can be extended by incorporating more channels, and useful for further studies of nuclear fusion reactions in plasma systems at higher energies reached in more recent experiments.

Development of ion recoil energy distributions in the Coulomb explosion of argon clusters resolved by charge-state selective ion energy spectroscopy

The laser intensity dependence of the recoil energies from the Coulomb explosion of small argon clusters has been investigated by resolving the contributions of the individual charge states to the ion recoil energy spectra. Between 10^{14} and 10^{15} W/cm^2, the high-energy tail of the ion energy spectra changes its shape and develops into the well-known knee feature, which results from the cluster size distribution, laser focal averaging, and ionization saturation. Resolving the contributions of the different charge states to the recoil energies, the experimental data reveal that the basic assumption of an exploding homogeneously charged sphere cannot be maintained in general. In fact, the energy spectra of the high-q show distinct gaps in the yields at low kinetic energies, which hints at more complex radial ion charge distributions developing during the laser pulse impact.

Generation of Multiply Charged Argon Ions in Nanosecond Laser Field Ionization of Argon Clusters.

Zhang and co-workers ( J. Phys. Chem. Lett. 2020, 11, 1100-1105) have recently reported results of experiments involving irradiation of argon clusters doped with bromofluorene chromophores by nanosecond-long pulses of 532 nm laser light. Multiply charged ions of atomic argon (Arn+, 1 ≤ n ≤ 7) and carbon (Cn+, 1 ≤ n ≤ 4) are observed, which are sought to be rationalized using an evaporation model. The distinguishing facet of exploding clusters being progenitors of energetic ions and electrons constitutes the key driver for contemporary research in laser-cluster interactions; it is, therefore, important to point out inconsistencies that are intrinsic to the model of Zhang and co-workers. In light of similar reports already in the literature, we show that their model is of limited utility in describing the dynamics that govern how fast, multiply charged atomic ions result from laser irradiation of gas-phase clusters. We posit that it is plasma behavior that underpins cluster heating and cluster explosion dynamics.

Coulomb cluster explosion boosted by an electrical pulse—neutron source, diagnostic tool, and test of nuclear fusion efficiency

To greatly enhance output of fusion-produced neutrons in a laser-initiated Coulomb explosion (CE) of D clusters, we propose to accelerate D+ ions by an electrical pulse to the energies where the collision cross-section is the highest. With ions bombarding a D-rich cathode, this solves a few problems simultaneously by (a) removing the electron cloud hindering the CE, (b) utilizing up to 100% of the ions to hit the high-density packed nuclei, and (c) reaching the highly increased cross-section of neutron production in a single collision, by using a multi-layered target. We show that neutron output can reach up to 1015 per shot, which provides a powerful and compact neutron source. We also consider the use of E-pulse acceleration for diagnostic purposes.

Frustrated Coulomb explosion of small helium clusters

Almost ten years ago, energetic neutral hydrogen atoms were detected after a strong-field double ionization of H$_2$. This process, called 'frustrated tunneling ionization', occurs when an ionized electron is recaptured after being driven back to its parent ion by the electric field of a femtosecond laser. In the present study we demonstrate that a related process naturally occurs in clusters without the need of an external field: we observe a charge hopping that occurs during a Coulomb explosion of a small helium cluster, which leads to an energetic neutral helium atom. This claim is supported by theoretical evidence. As an analog to 'frustrated tunneling ionization', we term this process 'frustrated Coulomb explosion'.

A New Hyper-runaway Star Discovered from LAMOST and Gaia: Ejected Almost in the Galactic Rotation Direction

Abstract In this paper, we report the discovery of a new late-B-type unbound hyper-runaway star (LAMOST-HVS4) from the LAMOST spectroscopic surveys. According to its atmospheric parameters, it is either a B-type main-sequence (MS) star or a blue horizontal branch (BHB) star. Its Galactocentric distance and velocity are 30.3 ± 1.6 kpc and 586 ± 7 km s−1 if it is an MS star, and they are 13.2 ± 3.7 kpc and 590 ± 7 km s−1 if a BHB star. We track its trajectories back and find that the trajectories intersect with the Galactic disk, and the Galactic center lies outside of the intersection region at the 3σ confidence level. We investigate a number of mechanisms that could be responsible for the ejection of the star and find that it is probably ejected from the Galactic disk by supernova explosion or multiple-body interactions in dense young stellar clusters.

Oblique Propagation of Electrostatic Waves in a Magnetized Electron-Positron-Ion Plasma in the Presence of Heavy Particles

Abstract A theoretical investigation is carried out to understand the basic features of nonlinear propagation of heavy ion-acoustic (HIA) waves subjected to an external magnetic field in an electron-positron-ion plasma that consists of cold magnetized positively charged heavy ion fluids and superthermal distributed electrons and positrons. In the nonlinear regime, the Korteweg-de Vries (K-dV) and modified K-dV (mK-dV) equations describing the propagation of HIA waves are derived. The latter admits a solitary wave solution with both positive and negative potentials (for K-dV equation) and only positive potential (for mK-dV equation) in the weak amplitude limit. It is observed that the effects of external magnetic field (obliqueness), superthermal electrons and positrons, different plasma species concentration, heavy ion dynamics, and temperature ratio significantly modify the basic features of HIA solitary waves. The application of the results in a magnetized EPI plasma, which occurs in many astrophysical objects (e.g. pulsars, cluster explosions, and active galactic nuclei) is briefly discussed.

Highly Charged Rydberg Ions from the Coulomb Explosion of Clusters.

Ion emission from a nanoplasma produced in the interaction of intense optical laser pulses with argon clusters is studied resolving simultaneously charge states and recoil energies. By applying appropriate static electric fields we observe that a significant fraction of the ions Ar^{q+} (q=1-7) has electrons with binding energies lower than 150meV; i.e., n_{Ryd}≥15 levels are populated. Charge state changes observed on a μs time scale can be attributed to electron emission due to autoionizing Rydberg states, indicating that high-ℓ Rydberg levels are populated as well. The experiments support theoretical predictions that a significant fraction of delocalized electrons, which are bound with hundreds of eV to the nanoplasma after the laser exposure, fill up meV bound ion states in the adiabatic expansion. We expect the process to be relevant for the long-term evolution of expanding laser-induced dense plasmas in general.

Micron-size hydrogen cluster target for laser-driven proton acceleration

As a new laser-driven ion acceleration technique, we proposed a way to produce impurity-free, highly reproducible, and robust proton beams exceeding 100 MeV using a Coulomb explosion of micron-size hydrogen clusters. In this study, micron-size hydrogen clusters were generated by expanding the cooled high-pressure hydrogen gas into a vacuum via a conical nozzle connected to a solenoid valve cooled by a mechanical cryostat. The size distributions of the hydrogen clusters were evaluated by measuring the angular distribution of laser light scattered from the clusters. The data were analyzed mathematically based on the Mie scattering theory combined with the Tikhonov regularization method. The maximum size of the hydrogen cluster at 25 K and 6 MPa in the stagnation state was recognized to be 2.15 ± 0.10 μm. The mean cluster size decreased with increasing temperature, and was found to be much larger than that given by Hagena’s formula. This discrepancy suggests that the micron-size hydrogen clusters were formed by the atomization (spallation) of the liquid or supercritical fluid phase of hydrogen. In addition, the density profiles of the gas phase were evaluated for 25 to 80 K at 6 MPa using a Nomarski interferometer. Based on the measurement results and the equation of state for hydrogen, the cluster mass fraction was obtained. 3D particles-in-cell (PIC) simulations concerning the interaction processes of micron-size hydrogen clusters with high power laser pulses predicted the generation of protons exceeding 100 MeV and accelerating in a laser propagation direction via an anisotropic Coulomb explosion mechanism, thus demonstrating a future candidate in laser-driven proton sources for upcoming multi-petawatt lasers.

Role of the vibrational contribution in Coulomb explosion of dicationic neon gas clusters: a parallel tempering based study.

The problem of Coulomb explosion in dicationic neon gas clusters has been investigated with special emphasis on the role of the vibrational contribution. The problem has been handled by describing the dicationic neon gas system with an adequate potential energy surface comprising dispersive interaction, Coulombic and polarizability containing terms. This potential energy surface, if explored for various sizes of the clusters, shows Coulombic explosion features below a certain threshold size. However this classical treatment fails to account for the correct threshold predicted from other studies including experiments. This signifies that quantum effects play an important role. With the incorporation of the vibrational contribution as the quantum effect, it is seen that reduction in the threshold value indeed occurs and the amount of decrease significantly varies with temperature. The whole study has been done using the stochastic search strategy or parallel tempering to explore the potential energy surface of the system. The stochastic strategy guarantees the achievement of a low energy solution as it is not stuck in local energy basins.

Predicting stability limits for pure and doped dicationic noble gas clusters undergoing coulomb explosion: A parallel tempering based study.

We have used a replica exchange Monte-Carlo procedure, popularly known as Parallel Tempering, to study the problem of Coulomb explosion in homogeneous Ar and Xe dicationic clusters as well as mixed Ar-Xe dicationic clusters of varying sizes with different degrees of relative composition. All the clusters studied have two units of positive charges. The simulations reveal that in all the cases there is a cutoff size below which the clusters fragment. It is seen that for the case of pure Ar, the value is around 95 while that for Xe it is 55. For the mixed clusters with increasing Xe content, the cutoff limit for suppression of Coulomb explosion gradually decreases from 95 for a pure Ar to 55 for a pure Xe cluster. The hallmark of this study is this smooth progression. All the clusters are simulated using the reliable potential energy surface developed by Gay and Berne (Gay and Berne, Phys. Rev. Lett. 1982, 49, 194). For the hetero clusters, we have also discussed two different ways of charge distribution, that is one in which both positive charges are on two Xe atoms and the other where the two charges are at a Xe atom and at an Ar atom. The fragmentation patterns observed by us are such that single ionic ejections are the favored dissociating pattern. © 2017 Wiley Periodicals, Inc.

Neutron enhancement from laser interaction with a critical fluid

We discuss experimentally and theoretically neutron production from the laser driven explosion of gas clusters prepared near the liquid-gas critical point. We let deuterated methane that was prepared very close to its critical temperature and pressure expand through a conical nozzle to create clusters, and then irradiated those clusters with a high intensity pulse from the Texas Petawatt Laser. After ionization, the clusters explode producing energetic ions, some of which fuse with resultant neutron emission. We show that the critical fluctuations present in the nozzle before the expansion influence the dynamics of neutron production. Neutron production near the critical point follows a power law, which is a signature of a second order phase transition and it is consistent with the Fisher model. This result might be relevant for energy production from fusion reactions.

Optimal control with nonadiabatic molecular dynamics: Application to the Coulomb explosion of sodium clusters

We present an implementation of optimal control theory for the first-principles non-adiabatic Ehrenfest Molecular Dynamics model, which describes a condensed matter system by considering classical point-particle nuclei, and quantum electrons, handled in our case with time-dependent density-functional theory. The scheme is demonstrated by optimizing the Coulomb explosion of small Sodium clusters: the algorithm is set to find the optimal femtosecond laser pulses that disintegrate the clusters, for a given total pulse duration, fluence, and cut-off frequency. We describe the numerical details and difficulties of the methodology.

Interaction of xenon clusters with intense sub-cycle laser pulses

In this work, we have studied the interaction dynamics of the intense sub-cycle laser with the Xe2600 (Xenon) cluster by using a molecular dynamic code. The code is benchmarked against a couple of experimental works on Xe clusters. In the sub-cycle regime, the plane wave prescription of the laser pulse is not adequate, giving unrealistic field profiles, and hence in this study, we have relied on complex-source based sub-cycle pulsed beam model, which is an exact solution of Maxwell's equations. In order to see the effect of the sub-cycle pulses, the laser pulse duration is varied from 0.2 to 1 laser cycle while keeping the pulse energy conserved (by varying the peak amplitude with pulse duration). It has been observed that for the same laser energy the more energetic ions are obtained for sub-cycle pulses. Although the cluster explosion is symmetric, higher charge states are observed along the direction of laser polarization. The conversion efficiency of the energy absorbed per atom to average kinetic energy is found to be maximum for the shortest pulse duration of 0.2 laser cycle. The scaling law for maximum ion energy, total energy absorbed, and average kinetic energy of the ions with laser pulse duration is also deduced.

Comparative study of energy of particles ejected from coulomb explosion of rare gas and metallic clusters irradiated by intense femtosecond laser field

We present our study of high intensity femtosecond laser field interaction with large cluster of Kr and Na (contained 2.103 to 2.107 atoms). When laser intensity is above a critical value, it blows off all of electrons from the cluster and forms a non neutral ion cloud. The irradiation of these clusters by the intense laser field leads to highly excitation energy which can be the source of energetic electrons, electronic emission, highly charge, energetic ions and fragmentation process. During the Coulomb explosion of the resulting highly ionized, high temperature nanoplasma, ions acquire again their energy. It is shown that ultra fast ions are produced. The goal of our study is to investigate in detail a comparative study of the expansion and explosion then the ion energy of metallic and rare gas clusters irradiated by an intense femtosecond laser field. We have found that ions have a kinetic energy up to 105 eV and the Coulomb pressure is little than the hydrodynamic pressure. The Coulomb explosion of a cluster may provide a new high energy ion source.

Thermal and log-normal distributions of plasma in laser driven Coulomb explosions of deuterium clusters

In this work, we explore the possibility that the motion of the deuterium ions emitted from Coulomb cluster explosions is highly disordered enough to resemble thermalization. We analyze the process of nuclear fusion reactions driven by laser–cluster interactions in experiments conducted at the Texas Petawatt laser facility using a mixture of D2+3He and CD4+3He cluster targets. When clusters explode by Coulomb repulsion, the emission of the energetic ions is “nearly” isotropic. In the framework of cluster Coulomb explosions, we analyze the energy distributions of the ions using a Maxwell–Boltzmann (MB) distribution, a shifted MB distribution (sMB), and the energy distribution derived from a log-normal (LN) size distribution of clusters. We show that the first two distributions reproduce well the experimentally measured ion energy distributions and the number of fusions from d–d and d-3He reactions. The LN distribution is a good representation of the ion kinetic energy distribution well up to high momenta where the noise becomes dominant, but overestimates both the neutron and the proton yields. If the parameters of the LN distributions are chosen to reproduce the fusion yields correctly, the experimentally measured high energy ion spectrum is not well represented. We conclude that the ion kinetic energy distribution is highly disordered and practically not distinguishable from a thermalized one.