Extrusion-based metal direct writing is a promising metal additive manufacturing technology due to its high efficiency and low cost. However, fabricating parts with high integrity and complex geometry remains challenging. The most critical factor is the unavailable of semi-solid slurries with uniform and nearly spherical solid particles, resulting in uncontrollable extrusion and printing. Currently, mixed powder remelting (MPR) is reported to preset the features of the solid phases, including volume fraction, morphology, and size distribution. Specifically, the semi-solid slurries of hypoeutectic AlSi alloys were obtained by preheating and shearing the mixed powder composed of eutectic AlSi alloy powder and pure aluminum powder. Their microstructural characteristics and rheological behavior were investigated, demonstrating the microstructure tailoring (controllable solid fraction and size distribution, high shape factor of about 0.9) and the reduced viscosity fluctuation by a factor of 7 compared with traditional processes. MPR shows unparalleled advantages for further engineering applications of metal direct writing.