Entangled Source Research Articles

Orchestrating time and color: a programmable source of high-dimensional entanglement

High-dimensional encodings based on temporal modes (TMs) of photonic quantum states provide the foundations for a highly versatile and efficient quantum information science (QIS) framework. Here, we demonstrate a crucial building block for any QIS applications based on TMs: a programmable source of maximally entangled high-dimensional TM states. Our source is based on a parametric downconversion process driven by a spectrally shaped pump pulse, which facilitates the generation of maximally entangled TM states with a well-defined dimensionality that can be chosen programmatically. We characterize the effective dimensionality of the generated states via measurements of second-order correlation functions and joint spectral intensities, demonstrating the generation of bi-photon TM states with a controlled dimensionality in up to 20 dimensions.

Entanglement source and quantum memory analysis for zero-added-loss multiplexing

Entanglement source and quantum memory analysis for zero-added-loss multiplexing

Fabrication of hydrothermal PPKTP and its spontaneous parametric down-conversion characteristics

High-voltage electric field polarization, selective corrosion, current monitoring, and other methods are used to develop hydrothermal PPKTP. It is found that the reversal domain nucleation of hydrothermal-grown KTP crystals has four kinds of microscopic morphology, namely, strip shape, spindle shape, bullet shape and irregular shape, in the process of high voltage electric field polarization. Compared with the leakage current in the process of polarization of flux-grown KTP crystals, the hydrothermal-grown KTP crystals only exist when the applied electric field is much larger than the coercive field. The leakage current can be suppressed by multiple loading of short pulses, and the PPKTP with a poled period of 10 μm and 46 μm were fabricated, respectively. Subsequently, based on the fabricated PPKTP, the SPDC characteristics are studied. To the PPKTP with a poled period of 10 μm, the quantum entanglement source whose brightness exceeds 2.1 kHz @ 810 nm is prepared by the SPDC technique. Otherwise, the PPKTP with a poled period of 46 μm is used for SPDC, and the brightness of entangled photon pairs in channel 1 and channel 2 are 3.21 kHz @ 1560 nm and 5.31 kHz @ 1560 nm, respectively.

Quantum Entanglement between Optical and Microwave Photonic Qubits

Entanglement is an extraordinary feature of quantum mechanics. Sources of entangled optical photons were essential to test the foundations of quantum physics through violations of Bell’s inequalities. More recently, entangled many-body states have been realized via strong nonlinear interactions in microwave circuits with superconducting qubits. Here, we demonstrate a chip-scale source of entangled optical and microwave photonic qubits. Our device platform integrates a piezo-optomechanical transducer with a superconducting resonator which is robust under optical illumination. We drive a photon-pair generation process and employ a dual-rail encoding intrinsic to our system to prepare entangled states of microwave and optical photons. We place a lower bound on the fidelity of the entangled state by measuring microwave and optical photons in two orthogonal bases. This entanglement source can directly interface telecom wavelength time-bin qubits and gigahertz frequency superconducting qubits, two well-established platforms for quantum communication and computation, respectively. Published by the American Physical Society 2024

Comparative analysis of quantum two-way time transfer and quantum round-trip time transfer in consistent spatiotemporal settings

In this study, we conducted experiments using a single energy-time entangled biphoton source to compare the performance of quantum two-way time transfer (Q-TWTT) and quantum round-trip time transfer (Q-RTTT) under consistent spatiotemporal conditions. By conducting experiments with different fiber links of 11.3 km, 22.4 km, and 55.6 km, while ensuring uniform photon counts received by the single-photon detectors, we measured standard deviations (SDs) and stabilities of the time offsets. The measured SDs for Q-TWTT and Q-RTTT were 0.46 ps and 0.65 ps over the 11.3 km fiber, 1.14 ps and 1.3 ps over the 22.4 km fiber, 3.98 ps and 4.39 ps over the 55.6 km fiber, respectively. These results show good agreement with theoretical predictions, and the smaller SDs for Q-TWTT can be directly attributed to protocol-specific factors related to system symmetry. The long-term time stabilities of Q-TWTT and Q-RTTT were evaluated in terms of time deviation (TDEV). At an average time of 12680 s, the measured TDEVs were 0.49 ps and 0.63 ps for the 11.3 km fiber, 0.59 ps and 0.7 ps for the 22.4 km fiber, 1.01 ps and 1.36 ps for the 55.6 km fiber, respectively. The results validate that Q-TWTT exhibits superior time transfer performance compared to Q-RTTT, highlighting the advantages of Q-TWTT in practical applications.

Deterministic photon source of genuine three-qubit entanglement

Deterministic photon sources allow long-term advancements in quantum optics. A single quantum emitter embedded in a photonic resonator or waveguide may be triggered to emit one photon at a time into a desired optical mode. By coherently controlling a single spin in the emitter, multi-photon entanglement can be realized. We demonstrate a deterministic source of three-qubit entanglement based on a single electron spin trapped in a quantum dot embedded in a planar nanophotonic waveguide. We implement nuclear spin narrowing to increase the spin dephasing time to T2*≃33\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${T}_{2}^{*}\\simeq 33$$\\end{document} ns, which enables high-fidelity coherent optical spin rotations, and realize a spin-echo pulse sequence for sequential generation of spin-photon and spin-photon-photon entanglement. The emitted photons are highly indistinguishable, which is a key requirement for scalability and enables subsequent photon fusions to realize larger entangled states. This work presents a scalable deterministic source of multi-photon entanglement with a clear pathway for further improvements, offering promising applications in photonic quantum computing or quantum networks.

SNR analysis of a multi-channel temporal correlation scheme in quantum-enhanced target detection.

In lossy and noisy environments, quantum-enhanced target detection based on temporal quantum correlation encounters low signal-to-noise ratio (SNR), resulting in poor detection performance. To address these challenges, we propose a multi-channel temporal correlation scheme. In this scheme, signal photons from multiple independent entangled sources illuminate the target and arrive at the same detector. Coincidences are obtained by correlation measurements of the entangled photons on one signal path and different reference paths. We then propose a weighted average processing method for fusing the coincidences to obtain higher SNR. The relationship between the SNR and the number of sources is analyzed for different background noise levels. It is shown that the SNR increases as the number of sources increases, but eventually approaches a limit. Experimental results verify the correction of our theoretical analysis.

Enhancing quantum time transfer security: detecting intercept-resend attacks with energy-time entanglement

Abstract Quantum time transfer has emerged as a powerful technique, offering sub-picosecond precision and inherent security through the nonlocal temporal correlation property of energy-time entangled biphoton sources. In this paper, we demonstrate the inherent security advantage of quantum time transfer, and the utilization in detecting potential intercept-resend attacks. By investigating the impact of these attacks on the nonlocality identifier associated with nonlocal dispersion cancellation of energy-time entanglement, we establish a security threshold model for detecting intercept-resend attacks. Experimental verification on a 102 km fiber-optic link confirms that even a malicious delay as small as 25 ps can be identified. This investigation serves as a compelling illustration of secure two-way time transfer, safeguarding against intercept-resend attacks, and showcasing its potential applications in fields reliant on authentic time distribution between remote parties.

A tunable transition metal dichalcogenide entangled photon-pair source

Entangled photon-pair sources are at the core of quantum applications like quantum key distribution, sensing, and imaging. Operation in space-limited and adverse environments such as in satellite-based and mobile communication requires robust entanglement sources with minimal size and weight requirements. Here, we meet this challenge by realizing a cubic micrometer scale entangled photon-pair source in a 3R-stacked transition metal dichalcogenide crystal. Its crystal symmetry enables the generation of polarization-entangled Bell states without additional components and provides tunability by simple control of the pump polarization. Remarkably, generation rate and state tuning are decoupled, leading to equal generation efficiency and no loss of entanglement. Combining transition metal dichalcogenides with monolithic cavities and integrated photonic circuitry or using quasi-phasematching opens the gate towards ultrasmall and scalable quantum devices.

Scalable determination of multipartite entanglement in quantum networks

Quantum networks comprised of entangled end nodes serve stronger than the classical correlation for unparalleled quantum internet applications. However, practical quantum networking is affected by noise, which at its worst, causes end nodes to be described by pre-existing classical data. In such untrusted networks, determining quantum network fidelity and genuine multi-node entanglement becomes crucial. Here, we show that determining quantum network fidelity and genuine N-node entanglement in an untrusted star network requires only N + 1 measurement settings. This method establishes a semi-trusted framework, allowing some nodes to relax their assumptions. Our network determination method is enabled by detecting genuine N-node Einstein-Podolsky-Rosen steerability. Experimentally, using spontaneous parametric down-conversion entanglement sources, we demonstrate the determinations of genuine 3-photon and 4-photon quantum networks and the false positives of the widely used entanglement witness, the fidelity criterion of 1/2. Our results provide a scalable method for the determination of multipartite entanglement in realistic quantum networks.

Loophole-Free Test of Local Realism via Hardy's Violation.

Bell's theorem states that the quantum mechanical description of physical quantities cannot be fully explained by local realistic theories, laying a solid basis for various quantum information applications. Hardy's paradox is celebrated as the simplest form of Bell's theorem concerning its "All versus Nothing" approach to test local realism. However, due to experimental imperfections, existing tests of Hardy's paradox require additional assumptions of the experimental systems, and these assumptions constitute potential loopholes for faithfully testing local realistic theories. Here, we experimentally demonstrate Hardy's nonlocality through a photonic entanglement source. By achieving a detection efficiency of 82.2%, a quantum state fidelity of 99.10%, and applying high-speed quantum random number generators for the measurement setting switching, the experiment is implemented in a loophole-free manner. During 6h of running, a strong violation of P_{Hardy}=4.646×10^{-4} up to 5 standard deviations is observed with 4.32×10^{9} trials. A null hypothesis test shows that the results can be explained by local realistic theories with an upper bound probability of 10^{-16348}. These testing results provide affirmative evidence against local realism, and establish an advancing benchmark for quantum information applications based on Hardy's paradox.

A source of entangled photons based on a cavity-enhanced and strain-tuned GaAs quantum dot

A quantum-light source that delivers photons with a high brightness and a high degree of entanglement is fundamental for the development of efficient entanglement-based quantum-key distribution systems. Among all possible candidates, epitaxial quantum dots are currently emerging as one of the brightest sources of highly entangled photons. However, the optimization of both brightness and entanglement currently requires different technologies that are difficult to combine in a scalable manner. In this work, we overcome this challenge by developing a novel device consisting of a quantum dot embedded in a circular Bragg resonator, in turn, integrated onto a micromachined piezoelectric actuator. The resonator engineers the light-matter interaction to empower extraction efficiencies up to 0.69(4). Simultaneously, the actuator manipulates strain fields that tune the quantum dot for the generation of entangled photons with corrected fidelities to a maximally entangled state up to 0.96(1). This hybrid technology has the potential to overcome the limitations of the key rates that plague QD-based entangled sources for entanglement-based quantum key distribution and entanglement-based quantum networks.

A Probability-Based Optimization Approach for Entanglement Distribution and Source Position in Quantum Networks

A Probability-Based Optimization Approach for Entanglement Distribution and Source Position in Quantum Networks

Efficient source-independent quantum conference key agreement

Quantum conference key agreement (QCKA) enables the unconditional secure distribution of conference keys among multiple participants. Due to challenges in high-fidelity preparation and long-distance distribution of multi-photon entanglement, entanglement-based QCKA is facing severe limitations in both key rate and scalability. Here, we propose a source-independent QCKA scheme utilizing the post-matching method, feasible within the entangled photon pair distribution network. We introduce an equivalent distributing virtual multi-photon entanglement protocol for providing unconditional security proof even in the case of coherent attacks. For the symmetry star network, compared with the previous n-photon entanglement protocol, the conference key rate is improved from O(η n ) to O(η2), where η is the transmittance from the entanglement source to one participant. Simulation results show that the performance of our protocol has multiple orders of magnitude advantages in the intercity distance. We anticipate that our approach will demonstrate its potential in the implementation of quantum networks.

Keep an open mind on faster-than-light 'tachyons' as the source of quantum entanglement.

Keep an open mind on faster-than-light 'tachyons' as the source of quantum entanglement.

Error correction based artificial neural network in multi-modes CV-QKD with simultaneous type-I and type-II parametric-down conversion entangled photon source

We model simultaneous type-I and type-II phase matching in a single non-linear crystal (NLC), based on a double periodically poled lithium niobate crystal. We also discuss entanglement based continuous variable quantum key distribution (CV-QKD), and the security of such scheme is analyzed considering an eavesdropper being capable of individual attacks. We further demonstrate efficiency of the artificial neural network (ANN) algorithm during post-processing or errors correction in such CV-QKD protocols. Results show that employing simultaneous type-I and type-II SPDC process in single NLC is a potential source to generate high dimensional (or hyper-entangled) states, strongly required for quantum information processing tasks, an example of CV-QKD. Security analysis of such a CV-QKD protocol shows a strong advantage of employing the above entangled photon state source, given that it provides a higher secure key rate and thus a secure communication within a larger distance. In addition, the suggested error correction algorithm is less time consuming and highly efficient, since full synchronization is achieved just after a few number of updates of trusted parties’ tree-parity-machines. Our results sufficiently demonstrate that the suggested CV-QKD is able to distribute secure keys in nearby inter-city areas, and therefore allows lower-cost secure communication networks.

Spatio‐Temporal Nonlinear Theory in Birefringent Microrings

AbstractFrequency‐dependent nonlinear process in microresonators is widely acknowledged, but there is no theory available to calculate the conversion efficiency for each resonance of the ring, except for the phase‐matching one. Similarly for azimuth‐dependent nonlinear process in birefringent rings, there is a lack of theory to analysis the conversion efficiency for each azimuth of the ring. Consequently, it leads to old‐fashioned or ill‐considered coupling position and inefficient energy conversion in birefringent microrings. Here, the study introduces spatio‐temporal coupled‐mode equation to describe mode spatial properties in the cavity, compensating for the deficiency of temporal coupled‐mode equation in describing sophisticated responses. By this equation, it is found that over a wide frequency range, the extremely strong second‐harmonic generation of TE modes can be achieved at different azimuth under different pumps in an X‐cut lithium niobate microring, as proved by a 440 000%/W conversion efficiency in a non‐poling ring recently. This theory is important for realizing an efficient entangled quantum light source, for example. Meanwhile, it will provide new ideas and guidelines for design and applications of monolithic birefringent photonic integrated circuits with high energy efficiency.

High-rate multiplexed entanglement source based on time-bin qubits for advanced quantum networks

Entanglement distribution based on time-bin qubits is an attractive option for emerging quantum networks. We demonstrate a 4.09-GHz repetition rate source of photon pairs entangled across early and late time bins separated by 80 ps. Simultaneous high rates and high visibilities are achieved through frequency multiplexing the spontaneous parametric down conversion output into eight time-bin entangled channel pairs. We demonstrate entanglement visibilities as high as 99.4%, total entanglement rates up to 3.55×106 coincidences/s, and predict a straightforward path towards achieving up to an order of magnitude improvement in rates without compromising visibility. Finally, we resolve the density matrices of the entangled states for each multiplexed channel and express distillable entanglement rates in ebit/s, thereby quantifying the trade-off between visibility and coincidence rates that contributes to useful entanglement distribution. This source is a fundamental building block for high-rate entanglement-based quantum key distribution systems or advanced quantum networks.

Cooperative properties of multiple quantum scattering: I quantum nutation

The cooperative models of the bimodal field in the multiple quantum scattering nutations are discussed and proposed for possible detections in open cavities. We proposed two types of cooperation between the converted photon processes in these multiple steps of scattering nutation in the cavity. One of them takes into consideration the cooperative process between the photons of each step of the multiple steps of Raman conversion. The second cooperative process takes place between the photons belonging to different steps of multiple scattering conversions. The proposed novel bimodal entangled sources take into consideration both the coherence and collective phenomena between the photons belonging to the system of the bimodal field obtained in multiple scattering emissions. The application of higher-order multiple Raman bimodal coherent field in quantum information is proposed.

Linear and Nonlinear Optical Properties of All-cis and All-trans Poly(p-phenylenevinylene).

Poly(p-phenylenevinylene) (PPV) is a staple of the family of conjugated polymers with desirable optoelectronic properties for applications including light-emitting diodes (LEDs) and photovoltaic devices. Although the significant impact of olefin geometry on the steady-state optical properties of PPVs has been extensively studied, PPVs with precise stereochemistry have yet to be investigated using nonlinear optical spectroscopy for quantum sensing, as well as light harvesting for biological applications. Herein, we report our investigation of the influence of olefin stereochemistry on both linear and nonlinear optical properties through the synthesis of all-cis and all-trans PPV copolymers. We performed two-photon absorption (TPA) using a classical and entangled light source and compared both classical TPA and entangled two-photon absorption (ETPA) cross sections of these stereodefined PPVs. Whereas the TPA cross section of the all-trans PPV was expectedly higher than that of all-cis PPV, presumably because of the larger transition dipole moment, the opposite trend was measured via ETPA, with the all-cis PPV exhibiting the highest ETPA cross section. DFT calculations suggest that this difference might stem from the interaction of entangled photons with lower-lying electronic states in the all-cis PPV variant. Additionally, we explored the photoinduced processes for both cis and trans PPVs through time-resolved fluorescence upconversion and femtosecond transient absorption techniques. This study revealed that the sensitivity of PPVs in two-photon absorption varies with classical versus quantum light and can be modulated through the control of the geometry of the repeating alkenes, which is a key stepping stone toward their use in quantum sensing, bioimaging, and the design of polymer-based light-harvesting systems.