Elevated Radon Concentrations Research Articles

Fractal discrete fracture network modeling of radon gas concentration in underground tunnels under Książ Castle in Poland

The numerical modeling of radon concentrations in the fault zone of the underground excavations at Książ Castle was conducted using a stochastic Discrete Fracture Network (DFN) model. Due to the difficulties related with obtaining the exact fractures in a rock mass, the novel approach used in this study incorporates the stochastic model with known site data. The analysis utilized a dataset comprising long-term measurements of 222Rn activity concentration and geodetic measurements for twelve faults in the Książ unit. The parameters considered in the DFN model are: fracture length, Peclet number (Pe = 0.1 and 1.0, respectively), advection velocities (from 10–8 m/s to 10–6 m/s and from range from 10–7 m/s to 10–4 m/s, respectively), radon diffusion (D = 2.1 × 10–61/s), radon decay constant (λ = 1/s), and radon gas generation (q) along the fractures within the range of 1.5 × 10–3 Bq/m3·s to 3.5 × 10–3 Bq/m3·s. The calibration process obtained the best fit when the radon generation rate was uniformly distributed through the rock mass in addition to incorporating a higher value of radon generation rate (q = 3.0 × 10–3 Bq/m3·s) where elevated radon concentrations have been measured. The modeling results also confirmed that the radon generation rate should always be higher where elevated radon activity concentrations were measured regardless of the measurement period. For the indicated “area” the radon generation rate should be higher from 25% to 37.5% between May–October and 18.5% to 40% between November–April. The influence of fracture zones on the recorded radon activity concentrations was noticeable up to a depth of 15 m. Within this range, the highest values of 222Rn activity concentration, ranging from 1,600 Bq/m3 to 2,000 Bq/m3, were consistently observed regardless of the season. However, as the depth increased, the values of 222Rn activity concentration decreased from 800 Bq/m3 to 400 Bq/m3 and became more dispersed.

Assessment of Radon and Naturally Occurring Radionuclides in the Vredefort Meteorite Crater in South Africa

The concentric impact rings of the Vredefort Crater contain rocks with elevated uranium concentrations resulting from the geological signature of a meteoric impact. The decay of this uranium was estimated to lead to elevated indoor radon concentrations in the Crater, but such a study has never been carried out. This study explores the relationship between the natural radionuclides found in the geology of the Vredefort Crater and indoor radon concentrations. This was achieved through soil sampling and radionuclide surveys conducted on three impact rings, supplemented by indoor radon measurements in dwellings found in the area. In situ measurements revealed that one impact ring had higher-than-average uranium concentrations at 50 Bq/kg. Surprisingly, the measured indoor radon levels were lower than expected (113 Bq/m3). These measurements were taken during the COVID-19 pandemic and colder months, conditions that would typically result in elevated indoor radon levels. Soil samples indicated uranium activity of 30 Bq/kg, comparable to the world average of 35 Bq/kg. However, defunct mine tunnels in the area exhibited elevated radon concentrations, averaging 364 Bq/m3. The disparity between expected and measured indoor radon levels was attributed to the composition of surficial deposits, bedrock, and architectural features of the dwellings preventing radon accumulation.

Preliminary study of chromosome aberrations using Giemsa, two-colour fish, and micronucleus assays in lymphocytes of individuals living in elevated radon concentration areas.

The frequencies of unstable and stable chromosome aberrations and micronuclei were examined in peripheral blood samples from 10 individuals living in elevated radon concentration areas (Takandeang Village, Mamuju, Indonesia). Blood samples from 10 people living in Topoyo Village were used as a control group. For unstable chromosome aberration analysis, a dicentric chromosome assay was conducted using conventional Giemsa staining. Chromosomal painting of chromosomes 1 and 4 using the fluorescence in situ hybridisation technique was also applied to four subjects to assess the stable chromosome aberration. Our study showed no significant increases across all groups in dicentric and other unstable chromosome aberrations, such as rings and acentric fragments. Translocations were found in one person from Takandeang Village and two Topoyo Village inhabitants. The translocations found in the subjects from Takandeang Village were due more to aging factors than to radon exposure. The number of micronuclei per 1000 binucleus cells in Takandeang Village inhabitants was not significantly different than that in the control group (p=0.943). A more comprehensive analysis should be conducted in a subsequent study by increasing the number of study donors and the number of metaphases to be analysed in both dicentric chromosome assay and fluorescence in situ hybridisation assays. Such research could provide valid information on the cytogenetic effects of elevated indoor radon exposure.

TIME SERIES ANALYSIS OF RADON CONCENTRATION AT DIFFERENT DEPTHS IN AN UNDERGROUND GOLDMINE

Indoor radon concentrations were collected monthly over a period of one year in 10 different levels in an underground goldmine and the data was analysed using a four moving average time series to determine the relationship between depths of the underground mine and the indoor radon concentration. The detectors were installed in batches within four quarters. The measurements were carried out using LR115 solid state nuclear track detectors. Statistical models are applied in the prediction and analysis of the radon concentration at various depths. The time series model predicted a positive relationship between the depth of the underground mine and the indoor radon concentration. Thus, elevated radon concentrations are expected at deeper levels of the underground mine, but the relationship was insignificant at the 5% level of significance with a negative adjusted R 2 (R 2 = – 0.021) due to an appropriate engineering and adequate ventilation rate in the underground mine. Keywords : LR115, Radon Concentration, Time Series, Underground goldmine, DOI: 10.7176/APTA/87-03 Publication date: April 30 th 2023

Long-Term Monitoring of Bioaerosols in an Environment without UV and Desiccation Stress, an Example from the Cave Postojnska Jama, Slovenia

A natural cave environment subject to regular human visitation was selected for aerobiological study to minimize the effects of severe temperature fluctuations, UV radiation, and desiccation stress on the aerobiome. The longer sampling period of bioaerosols, up to 22 months, was generally not associated with a proportionally incremental and cumulative increase of microbial biomass. The culture-independent biomass indicator ATP enabled quick and reliable determination of the total microbial biomass. Total airborne microbial biomass was influenced by human visitation to the cave, as confirmed by significantly higher concentrations being observed along tourist footpaths (p < 0.05). Airborne beta-glucans (BG) and lipopolysaccharide (LPS) are present in cave air, but their impact on the cave remains to be evaluated. Staphylococcus spp., as an indicator of human presence, was detected at all sites studied. Their long-term survival decrease is likely due to high relative humidity, low temperature, the material to which they adhere, and potentially natural elevated radon concentration. The most commonly recorded species were: S. saprophyticus, which was identified in 52% of the studied sites, S. equorum in 29%, and S. warneri in 24% of the studied sites. Only a few isolates were assigned to Risk group 2: S. aureus, S. epidermidis, S. haemolyticus, S. pasteuri, and S. saprophyticus.

RADON-PRONE AREAS IN SLOVAKIA PREDICTED BY RESCALED RADON POTENTIAL MAPS.

Several scientific studies have shown that high content of radon in the soil environment can be a precursor of increased indoor radon levels. Inhabited areas where elevated indoor radon concentration appears for natural (geogenic) reasons are commonly referred to as radon-prone areas. In this study, radon-prone areas in the Slovak Republic were predicted on the basis of radon potential maps after its specific rescaling. In total, 99 municipalities have been identified in Slovakia where the annual average indoor radon concentration is expected to exceed the reference level of 300Bqm-3; five of those are even expected to exceed 1000Bqm-3. In these municipalities it is then required to conduct a survey of indoor radon measurements. Compared with a nationwide survey, the proposed approach of searching for houses with potentially high radon exposure is more efficient.

The Effect of the Coal Industry on Indoor Radon Concentrations in eMalahleni, Mpumalanga Province of South Africa.

South Africa has rich coal deposits concentrated in the northeast of the country, and as a result, most of the country's coal mining is located in this region. Two of the principal coalfields exploited are the Witbank and Highveld coalfields, located in the Mpumalanga province. Coal contains trace quantities of the naturally occurring radionuclides whose mass concentration can be enhanced by anthropogenic activity. The radioactive fallout from these activities could lead to elevated radon concentrations indoors. Two towns, Secunda and eMalahleni, were identified due to their proximity to coal-based industries. A previous study investigated whether these industries caused elevated radon levels in Secunda homes but found a lower-than-expected average concentration of 76.4 ± 7.6 Bq m-3. This was attributed to either the prevailing wind depositing the radioactive fallout to neighboring towns, such as eMalahleni, or the type of industrial activity. This paper builds on this study by investigating whether elevated radon levels are found in homes in eMalahleni. Measurements were performed in 22 homes during December 2019, and the average indoor radon concentration was calculated as 122.1 ± 8.5 Bq m-3. The cause of these elevated levels was then investigated, and it was found that even though the coal industry contributes to elevated radon levels, the town's underlying geology seems to be the primary contributor.

Origin of the chemical composition of São Francisco ultra-fresh thermal water (Itabira region, Minas Gerais, Brazil)

Geochemical studies documented the composition of ultra-fresh thermal water in the Fazenda Giráu, near Itabira (Minas Gerais state, Brazil) for the first time. The studied water is characterized by temperature of 35 °C, very low electric conductivity (approx. 20 μS/cm), uncommon Mg–Ca–HCO3–NO3 hydrochemical type, and an elevated radon concentration (about 500 Bq/L). The presence of tritium suggests the modern age of studied water, contained in highly resistant quartzite-dominated aquifer rocks. Application of a geothermometric approach gave an estimation of the equilibrium temperature in the geothermal system at about 42 °C. Inverse geochemical modelling quantified water-rock reactions responsible for the observed groundwater chemistry. Decomposition of soil organic matter and decay of primary (feldspars, biotites, muscovite) and secondary (montmorillonites, illite) aluminosilicate minerals accompanied by kaolinite and gibbsite formation are the dominant processes forming chemical composition of water. The investigated water has balneotherapeutic potential due its elevated temperature and high concentrations of radon and silicic acid.

Occupational Radon Assessment in Underground Storage Facilities in Saudi Arabia.

An occupational radon assessment was conducted at five underground storage facilities in the Kingdom of Saudi Arabia to evaluate the radon concentration and determine if remedial action is required to ameliorate conditions and ensure compliance with international guidance on acceptable radon levels in working environments. The assessment was carried out in four operational areas in the underground storage facilities routinely occupied or visited by workers. Initial radon concentrations were obtained using 293 passive CR-39 Nuclear Track Detector (NTD) radon dosimeters installed in the four operational areas for all the underground storage facilities. The detectors were left in place for 12 mo. As some of the radon measurements exceeded the International Atomic Energy Agency reference level of 1,000 Bq m-3 for radon in workplaces, a follow-up assessment was conducted using a real-time monitoring device in locations where high radon levels were observed. The measured radon concentrations in the four operational areas in three of the five underground storage facilities were below the reference level, and in the remaining two storage facilities, low ventilation rates in one operational area were identified as the principal cause of elevated radon concentrations. Notwithstanding, the potential radiation dose from radon exposure was determined to be well below the International Commission on Radiation Protection reference annual dose level of 10 mSv in all five underground storage facilities. Radon exposure to workers in all the underground storage facilities was found to be within the reference dose level for workplaces and does not pose an acute health risk.

Soil Gas Measurements of Radon, CO2 and Hydrocarbon Concentrations as Indicators of Subsurface Hydrocarbon Accumulation and Hydrocarbon Seepage

Soil gas measurements of radon (222Rn), CO2, and hydrocarbon concentrations, as well as gamma-ray spectrometry, were conducted at two separate locations to estimate the measurement results for known locations of hydrocarbon accumulations in the subsurface and oil seepage on the surface. The aim of the study was to confirm the applicability of the method for identifying migration pathways (e.g., faults) and to detect possible seepages of hydrocarbons to the surface as well as to investigate possible health issue potential about the soil gas analysis results. Site A investigations were performed with a large number of sampling points to provide sufficient spatial coverage to capture the influence of subsurface lithologic variability as well as the influence of the migration pathway on the measured parameters. For the investigation of site B, sampling points were positioned to reflect the situation between the area above producing hydrocarbon fields and areas with no confirmed accumulation. The results presented show that it is possible to distinguish the near-surface lithology (gamma-ray spectrometry), characterize the migration pathway, and indicate the area of oil seepage at the surface. Areas above the known hydrocarbon accumulations generally have elevated radon concentrations and detectable heavier hydrocarbons with sporadic methane in soil gas, which contrasts with the lower radon levels and lack of detectable heavier hydrocarbons in soil gas in the area with no confirmed hydrocarbon accumulation in the subsurface.

The analysis of results of radon/thoron measurements performed with the use of nuclear track detectors

Radon has been identified as one of the most important hazards, causing lung cancer. The most important isotope of radon is 222Rn (3.83 d), while thoron 220Rn (55 s) is treated as the less important isotope due to its short half-life. The radon/thoron hazard for people is related to inhalation of their decay products, but usually, only measurements of radon gas are done in dwellings. For such a purpose nuclear track detectors are used in most of the cases. Since several years simultaneous measurements are done to estimate thoron contribution to indoor radon and thoron exposure with the use of track detectors, too. Typically, a set of two detectors are applied and thoron concentrations are calculated on the basis of discriminative calculations. Unfortunately, very often results of these surveys are not accurate due to underestimation of the lower limit of detection (LLD) for thoron in the presence of elevated radon concentrations. Therefore an analysis of thoron LLDs in relationship to radon concentrations is presented.

Australian action to reduce health risks from radon.

In Australia, worker exposure to radon in underground uranium mines has been a focus of policy makers and regulators, and has been well controlled in the industry sector. That cannot be said for public exposure to radon. Radon exposure studies in the late 1980s and early 1990s demonstrated that the levels of radon in Australian homes were some of the lowest in the world. The International Basic Safety Standards, published by the International Atomic Energy Agency, requires the government to establish and implement an action plan for controlling public exposure due to radon indoors. When considering different policy options, it is important to develop radon prevention and mitigation programmes reflecting elements that are unique to the region or country. The Australian Radon Action Plan is being considered at a national level, and presents a long-range strategy designed to reduce radon-induced lung cancer in Australia, as well as the individual risk for people living with high concentrations of radon. In Australia, workers who are not currently designated as occupationally exposed are also considered as members of the public. In the Australian context, there are only a limited set of scenarios that might give rise to sufficiently high radon concentrations that warrant mitigation. These include highly energy efficient buildings in areas of high radon potential, underground workplaces, workplaces with elevated radon concentrations (e.g. spas using natural spring waters), and enclosed workspaces with limited ventilation. The key elements for a successful plan will rely on collaboration between government sectors and other health promotion programmes, cooperative efforts involving technical and communication experts, and partnering with building professionals and other stakeholders involved in the implementation of radon prevention and mitigation.

Changes in groundwater radon concentrations caused by the 2016 Kumamoto earthquake

This study examined radon concentrations in springs in Kumamoto and Aso regions following the 2016 Kumamoto earthquake, in addition to monitoring springs near the Futagawa-Hinagu fault zone for more than two years following the earthquake to investigate the relationship between crustal deformation and the radon concentration variation. We compared these radon concentrations with those obtained prior to the earthquake. The springs that showed elevated radon concentrations were located within the compressive strain quadrant of the earthquake. The post-seismic concentration variations of the monitored springs can be explained by rock porosity changes. These results suggest that the radon concentration in spring water is affected by porosity changes caused by stress changes derived from earthquake deformation and subsequent post-seismic relaxation. Our results are consistent with the previously inferred permeability enhancement model. Mass conservation calculations for radon release yielded porosity changes ranging from 30% to 70% for some aquifer systems. This study explores the possibility of radon monitoring as a tool to investigate not only seismic precursors but also post-seismic crustal deformation and aquifer property changes due to large earthquakes on a regional scale.

Water velocity and groundwater upwelling influence benthic algal biomass in a sandy tropical river: implications for water-resource development

Benthic algae are a major source of carbon supporting aquatic food webs in northern Australia, but little is known about the factors that regulate algal production. We surveyed benthic algal biomass in mainstem habitats of an unregulated sandy tropical river (the Fitzroy River) during a base-flow period. We used predictive models to reveal the physical and chemical parameters controlling algal biomass in mainstem habitats. We found that water velocity was an important driver—algal biomass was lower at higher water velocities. Subsurface flow was also influential—algal biomass increased in locations where groundwater upwelling occurred, as evident by a positive relationship between algal biomass and elevated radon and ammonium concentrations. In this sand-bed river, it is likely that high water velocity destabilises the sandy substrate reducing the establishment of algal biofilms. However, where water velocity is low enough for algal establishment, groundwater upwelling likely promotes algal growth by delivering limiting resources and/or creating stable conditions that promote algal production. The importance of surface and subsurface-flow conditions to benthic algal biomass means that any modification to the Fitzroy River catchment that alters dry-season longitudinal flows (via river regulation) or groundwater levels (via groundwater extraction) may directly influence river algal production.

Screen printed electrostatic concentrator with origami-inspired design for low-cost radon detection

There is an increasing awareness of the dangers posed by elevated radon concentration in indoor spaces. This has led to demand for improved measurement solutions which enable low-cost, accurate, and practical measurement of radon concentration. In this work, the use of screen printing to fabricate an electrostatic concentrator for radon detection is demonstrated. An origami-inspired design enables the use of printed electronics as a manufacturing technology with a resulting reduction in component cost and weight. A new metric for such electrostatic concentrators known as the ‘active volume’ was defined, taking into account the time of flight to the sensor and residence time of the radon progeny. This metric was utilised in a genetic algorithm in order to optimise the concentrator design, resulting in a 62% improvement in radon progeny concentration, enabling more rapid and accurate understanding of radon risk.

Radon concentration in groundwater sources of the Baikal region (East Siberia, Russia)

In this study, we conduct a systematic study of groundwater radioactivity in the territories around Lake Baikal in Siberia, including Pribaikalie and Transbaikalia. The database includes more than 200 measurements of 222Rn from monitored water sources in the study region. We classify the groundwater sources in the Baikal region into seven groups (I–VII) that differ in radon concentration in space and time. The spatial distribution of water sources belonging to certain groups depend on geochemical and structural factors. In Transbaikalia, intrusive rocks with elevated contents of uranium are abundant. In Pribaikalie, many water sources are classified into Groups I and II (Q < 100 Bq/L). Group I includes groundwater with background concentrations, and Group II includes groundwater with anomalous concentrations of radon. Water sources belonging to elevated radon concentration Groups III to VI are considered as anomalies. Faulting is one of the main causes of radon anomalies as groundwater in the fault zones is enriched with 222Rn due to the increased permeability of rocks and rock crushing resulting from displacements of the fault walls.Monitoring of water sources in Pribaikalie shows that 222Rn concentrations vary also in time mainly within the range of values corresponding to a particular group. The oscillatory pattern of the temporal variations is clearly revealed by radon measurements conducted every two weeks and depends mainly on meteorological factors. Seasonal variations in air temperature and atmospheric pressure lead to changes in groundwater temperature, dilution of groundwater due to precipitation, freezing the top layer of soil, and other phenomena. As a result, the concentration regularly increases in winter and decreases in summer. In this study, seismic activity has not been revealed as significant factor of impact on the concentration of radon in groundwater, since strong earthquakes did not occur during the monitoring period.

Influences of meteorological parameters on indoor radon concentrations (222Rn) excluding the effects of forced ventilation and radon exhalation from soil and building materials

Elevated indoor radon concentrations (222Rn) in dwellings pose generally a potential health risk to the inhabitants. During the last decades a considerable number of studies discussed both the different sources of indoor radon and the drivers for diurnal and multi day variations of its concentration. While the potential sources are undisputed, controversial opinions exist regarding their individual relevance and regarding the driving influences that control varying radon indoor concentrations. These drivers include (i) cyclic forced ventilation of dwellings, (ii) the temporal variance of the radon exhalation from soil and building materials due to e.g. a varying moisture content and (iii) diurnal and multi day temperature and pressure patterns. The presented study discusses the influences of last-mentioned temporal meteorological parameters by effectively excluding the influences of forced ventilation and undefined radon exhalation. The results reveal the continuous variation of the indoor/outdoor pressure gradient as key driver for a constant “breathing” of any interior space, which affects the indoor radon concentration with both diurnal and multi day patterns. The diurnally recurring variation of the pressure gradient is predominantly triggered by the day/night cycle of the indoor temperature that is associated with an expansion/contraction of the indoor air volume. Multi day patterns, on the other hand, are mainly due to periods of negative air pressure indoors that is triggered by periods of elevated wind speeds as a result of Bernoulli's principle.

RADON SAFETY OF MODERN MULTI-STOREY BUILDINGS WITH DIFFERENT ENERGY EFFICIENCY CLASSES

According to results of the survey in Ekaterinburg, Russia, indoor radon concentrations above the city average level have been found in each of the studied buildings with high energy efficiency class. Measures to increase energy efficiency were confirmed to decrease the air exchange rate and accumulation of high radon concentrations indoors. Despite of recommendations to use mechanical ventilation with heat recovery as the main scenario for reducing elevated radon concentrations in energy-efficient buildings, the use of such systems did not show an obvious advantage. In real situation, mechanical ventilation system is not used properly both in the automatic and manual mode, which does not give an obvious advantage over the natural ventilation in the climate of the Middle Urals in Ekaterinburg.

Assessment of radon concentration and heavy metal contamination in groundwater of Udhampur district, Jammu & Kashmir, India.

Radon concentration was measured in water samples of 41 different locations from Udhampur district of Jammu & Kashmir, India, by using RAD7 and Smart RnDuo monitor. The variation of radon concentration in water ranged from 1.44±0.31 to 63.64±2.88 BqL-1, with a mean value of 28.73 BqL-1 using RAD7 and 0.64±0.28 to 52.65±2.50 BqL-1, with a mean value of 20.30 BqL-1 using Smart RnDuo monitor, respectively. About 17.07% of the studied water samples recorded to display elevated radon concentration above the reference range suggested by United Nation Scientific Committee on the Effects of Atomic Radiations (UNSCEAR). The mean annual effective dose of these samples was determined, and 78.95% samples were found to be within the safe limits set by World Health Organisation (WHO) and European Council (EU). The study revealed good agreement between the values obtained with two methods. Heavy metals (Zn, Cd, Fe, Cu, Ni, As, Hg, Co, Pb and Cr) were determined in water samples by microwave plasma atomic emission spectrometer, and their correlation with radon content was also analysed.

Distribution of 222Rn in groundwater and estimation of resulting radiation dose to different age groups: A case study from Bangalore City

ABSTRACTIngesting waters holding high levels of natural occurring radioactive element like Radon would contribute to increase in the effective dose received by people followed by an increased prevalence of cancer. The current study is an attempt to describe the extent of contribution of 222Rn to natural background radiation and the resultant effective dose to public of different age groups. In order to do so, 65 groundwater samples from selected parts of Bangalore city were collected and analyzed for radon activity using RAD7 radon monitor coupled with RAD H2O accessories. The radon activity was in the range of 3.05–696 Bq/L (mean: 91.39 Bq/L) and 92.31% of the groundwater samples recorded elevated radon concentration above the United States environmental protection agency (USEPA's) Maximum Contaminant Level (MCL) value of 300 pCi/L, corresponding to 11.1 Bq/L. The mean annual effective dose contribution of people falling under different age groups (viz., infants, children, teens: males and females, adults: males and females, pregnant and lactating women) due to ingestion of water-borne 222Rn ranged from 0.082 to 0.444 mSv/y and was found to be higher in all the age groups of males compared to respective female age groups, but well within the United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) and World Health Organization (WHO) proposed limit of 1 mSv/y.