Utilizing high-efficiency electrostatic assembly and a scalable freeze-drying technique followed by carbonization, we have developed a series of unique, lightweight, hierarchically porous 1D+2D aerogels containing carbon nanotubes (CNTs) and reduced graphene oxide (rGO). By manipulating the interaction between CNTs and graphene oxide perjurer in cellulose nanofiber (CNF), CNTs can uniformly distribute along the graphene cell walls via an exceptional cross-linking interface in the resultant rGO/CNT aerogels. This arrangement enables abundant heterogeneous interfaces, endowing the aerogels with high conductivity and polarization loss capacity. Moreover, the 1D+2D microstructure of CNT/rGO and the hierarchical pore architecture of the aerogels facilitate multiple scattering, further enhancing their loss capacity toward electromagnetic wave absorption (EMW). Coupled with the optimized impedance matching derived from the adjustable dielectric properties, the aerogels exhibit outstanding EMW absorption with a filling ratio of merely 2 wt%. Specifically, a minimum reflection loss (RLmin) of −49.61 dB and an effective absorption bandwidth (EAB) of 4.16 GHz are achieved. With a filling ratio of 3 wt%, the RLmin reaches −77.51 dB, accompanied by an EAB of 3.84 GHz, surpassing the reported carbon or graphene-based aerogel EMW absorbers. In this work, the ultra-low filling ratio resulting from high conductivity confers a practical design for fabricating lightweight carbon-based aerogels suitable for high-efficiency EMW absorption, manifesting multiple applications in electromagnetic compatibility and aerospace contexts.