The development of a dual-mode sensing method for lead ions (Pb2+) is crucial and desirable. Herein, a single component-based bifunctional signal probe (perylene derivative-modified MOFs-gold nanoclusters, PTC-NH2@MOFs-AuNCs), which was capable of simultaneously generating an electrochemiluminescence (ECL) signal and exhibiting nanoenzyme activity, was prepared to fabricate a novel ratiometric ECL/colorimetry dual-mode platform for the visual, reliable, and sensitive analysis of Pb2+. Specifically, the PTC-NH2@MOFs-AuNCs were firstly synthesized via the electrostatic adsorption of AuNCs on the surface of PTC-NH2@MOFs. Upon the addition of Pb2+, the ECL signal of PTC-NH2@MOFs-AuNCs, which had been quenched by the adsorbed aptamer, could be restored at both the anode and cathode. Simultaneously, the peroxidase-like activity of PTC-NH2@MOFs-AuNCs was also recovered, accompanied by a distinct color transition from light blue to dark blue. The linear ranges of ratiometric ECL/colorimetric dual-modal assay for Pb2+ were 1 pM ∼ 5 nM and 1 nM ∼ 2 μM, with the limits of detection of 0.1 pM and 0.31 nM, respectively. More importantly, by introducing the screen-printed electrode and paper chip as sensing platform, a portable sensor for the convenient detection of Pb2+ was further established, demonstrating its promising practicability of rapid visual screening and accurate quantitative analysis in farmland soils.