Efficient THz Pulse Generation Research Articles

Enhancement of THz Generation by Two-Color TW Laser Pulses in a Low-Pressure Gas

We identify experimental conditions for efficient generation of THz pulses by high power near IR laser radiation: 2 TW, 30 fs, 800-nm laser pulses with their second harmonic were slightly focused in a low-pressure gas cell in such a way to avoid multiple filamentation and excessive ionization. This two-color scheme yields a microjoule level of THz pulses which is two orders of magnitude higher than the signal generated in the atmosphere of ambient air.

High-energy terahertz pulses from semiconductors pumped beyond the three-photon absorption edge.

A new route to efficient generation of THz pulses with high-energy was demonstrated using semiconductor materials pumped at an infrared wavelength sufficiently long to suppress both two- and three-photon absorption and associated free-carrier absorption at THz frequencies. For pumping beyond the three-photon absorption edge, the THz generation efficiency for optical rectification of femtosecond laser pulses with tilted intensity front in ZnTe was shown to increase 3.5 times, as compared to pumping below the absorption edge. The four-photon absorption coefficient of ZnTe was estimated to be β4=(4±1)×10-5 cm5/GW3. THz pulses with 14 μJ energy were generated with as high as 0.7% efficiency in ZnTe pumped at 1.7 µm. It is shown that scaling the THz pulse energy to the mJ level by increasing the pump spot size and pump pulse energy is feasible.

Efficient generation of THz pulses with 04 mJ energy

Efficient generation of THz pulses with high energy was demonstrated by optical rectification of 785-fs laser pulses in lithium niobate using tilted-pulse-front pumping. The enhancement of conversion efficiency by a factor of 2.4 to 2.7 was demonstrated up to 186 μJ THz energy by cryogenic cooling of the generating crystal and using up to 18.5 mJ/cm2 pump fluence. Generation of THz pulses with more than 0.4 mJ energy and 0.77% efficiency was demonstrated even at room temperature by increasing the pump fluence to 186 mJ/cm2. The spectral peak is at about 0.2 THz, suitable for charged-particle manipulation.

Design of a contact grating setup for mJ-energy THz pulse generation by optical rectification

According to the recent calculations, more efficient THz pulse generation is possible using relief grating on the front surface of the generating LiNbO3 (LN) crystal for tilted-pulse-front-excitation rather than imaging the pump spot on a reflection grating into the LN crystal. Very recently, it was shown that—compared to a free-standing LN surface-relief grating—significantly higher diffraction efficiency can be reached if the grating profiles are filled with fused silica. Since realisation of such a setup is technically very challenging, in the present paper, we analyse the case where the input side of the LN grating is immersed into a refractive index matching liquid (RIML) instead of a solid material. Our results showed that the diffraction efficiency remains above 90 % for a refractive index ranging 1.45–1.60 of the applied RIML, and it is as high as 99 % for using the RIML for BK7. For this case, we carried out detailed calculations for various grating parameters. We propose a practical setup applying tilted input and slightly tilted output surfaces resulting in low losses and high diffraction efficiency for the pump. We conclude that a contact grating setup using BK7 RIML is suitable for producing THz pulses even in the mJ-energy range.

Efficient terahertz generation by optical rectification at 1035 nm

We demonstrate efficient generation of THz pulses by optical rectification of 1.03 um wavelength laser pulses in LiNbO3 using tilted pulse front excitation for velocity matching between the optical and THz fields. Pulse energies of 100 nJ with a spectral bandwidth of up to 2.5 THz were obtained at a pump energy of 400 uJ and 300 fs pulse duration. This conversion efficiency of 2.5x10(-4) was an order of magnitude higher than that obtained with collinear optical recitification in GaP, and far higher still than that measured using ZnTe in an optimized geometry. Using a simple model we demonstrate that two- and three-photon absorption strongly limit the THz generation efficiency at high pump fluences in ZnTe and GaP.

THz generation via optical rectification with ultrashort laser pulse focused to a line

We report on efficient THz pulse generation via optical rectification with femtosecond laser pulses focused to a line by a cylindrical lens. This configuration provides phase-matched conditions in the superluminal regime. 35 pJ THz pulses have been generated with this technique in a stoichiometric LiNbO3 crystal pumped by 2 μJ femtosecond laser pulses at room temperature. An unusual superquadratic rise of the THz pulse energy with the laser pulse energy has been observed at high laser energies. This extraordinary energy dependence of the THz generation efficiency is explained by self-focusing of the laser beam in the crystal. Z-scan measurements and comparison of the THz pulse spectra created with laser pulses having different energies confirm this interpretation.

Tunable THz pulse generation by optical rectification of ultrashort laser pulses with tilted pulse fronts

Optical rectification of ultrashort near-IR laser pulses with tilted pulse fronts and pulse energies of a few μJ in Mg-doped stoichiometric LiNbO3 cooled to low temperature is a powerful technique for efficient generation of THz pulses. The pulse energy critically depends on the Mg doping (necessary for preventing photorefractive damage) and can be easily increased by a factor of three if the MgO content is reduced. Pulse energies up to 400 pJ at repetition rates of 200 kHz and 3.4% quantum conversion efficiency are achieved at 77 K. At 10 K, changing the tilt angle of the pump pulse front results in continuous tuning of the frequency across the 1.0–4.4 THz range. The temporal pulse shapes measured by electro-optic sampling are in good agreement with the signal calculated by a simple theory. This model predicts tunability on a considerably broader range and narrower spectra even at room temperature if GaSe is used instead of LiNbO3. The advantages of the velocity matching technique utilizing tilted pulse fronts are analyzed in comparison with quasi-phase-matching in periodically poled LiNbO3 crystals. The first method provides a ten times higher pulse energy conversion efficiency.