The interrupted discrete waterjet (DWJ) offers advantages in surface treatment due to its exceptional load characteristics and high controllability. However, the surface characteristics of materials under controllable DWJ parameters have not been fully elucidated. This study delves into the surface morphology, roughness parameters, microhardness, residual stress, and distribution of crystal characteristics in both the depth and radial directions under 2400–36,000 impact cycles of DWJ through peening experiments and material characterization. The findings indicate that the surface morphology is influenced by high-frequency roughness components with limited impact cycles, while low-frequency waviness components gradually take precedence with more impact cycles. As impact cycles increase, certain roughness parameters such as Sq, S5p, S5v, and S10z initially rise until 21,600 cycles, after which they fluctuate within a specific range. Furthermore, DWJ peening leads to an increase in maximum hardness with impact cycles, with the depth of peak value transitioning from the surface layer to the subsurface. The residual compressive stress initially increases and then decreases with impact cycles. Under the experimental conditions, the maximum hardness reaches 268.1HV0.3, a 49.95 % increase from the original state, and the peak residual compressive stress reaches 297.7 MPa with a 310.2 % increase. As impact cycles continue to rise, a balance between material removal and surface hardening is achieved, resulting in the stabilization of maximum hardness and compressive stress as erosion strength grows. Following DWJ peening, there is an increase in the percentage of low-angle grain boundaries, along with enhanced grain refinement, increased geometrically necessary dislocation (GND) density, and the emergence of new phases. As the impact cycles increase, the effects of DWJ peening on crystal grains become more pronounced. Additionally, it has been observed that the lateral jetting influence extends further horizontally than in the depth direction of the incoming jet. It is considered that cyclic hardening and high strain rate effects (1.2 × 104) play significant roles in material hardening and failure.