Dual-color Laser Research Articles

Unified framework for terahertz radiation from a single- or two-color plasma filament.

The plasma filament induced by photo-ionization in transparent media (e.g., air) is a competitive terahertz (THz) source, whose mechanism has been widely studied in two separate schemes, i.e., the one- or two-color femtosecond laser filamentation. However, the physical commonality of these two schemes is less explored currently, and a common theory is in urgent need. Here, we proposed the traveling-wave antenna (TWA) model applicable to both single- and dual-color laser fields, which successfully reproduced the reported far-field THz angular distribution/dispersion from different filament lengths with either a constant or a varied plasma density. This work paves the way toward a deeper understanding of the important laser-filament-based THz sources within the same theoretical framework.

Energy transfer assisted plasmonic random laser emission from polymer optical fiber

Here, we analyzed the effect of a donor molecule (Rh6G) on the random laser emission of an acceptor molecule (Rh640 perchlorate) coated on the surface of a polymer optical fiber. Due to the energy transfer mechanism, the random lasing threshold of Rh640 perchlorate was found to be reduced in the presence of Rh6G. Also, the emission spectrum of Rh640 perchlorate was blue-shifted with the addition of Rh6G. Meanwhile, there is an enhancement in the lasing threshold of Rh6G in the presence of Rh640 perchlorate. The present study demonstrates that by properly adjusting the concentrations of both donor and acceptor molecules, we can obtain a dual-color random laser emission from polymer optical fiber.

Passively synchronized dual-color soliton fiber laser based on single-walled carbon nanotubes

In this work, we propose a uniquely designed fiber laser to generate dual-color soliton molecules, which are stable bound states made up of solitons with different carrier frequencies, pulse widths and soliton energies. This fiber laser consists of two resonators, which are cascaded by a pair of wavelength division multiplexers (WDMs), and a single-walled carbon nanotube saturable absorber (SWCNT-SA) is placed in the common branch shared by two sub-cavities to achieve optical soliton mode-locking. The optical solitons generated by this laser have central wavelengths of 1530.43 nm and 1547.62 nm with pulse widths of 0.832 ps and 1.198 ps, respectively. The synchronous mode-locked operation of the two sub-cavities can be easily achieved by adjusting the optical delay line (DL) in one of the resonant cavities. When the synchronized state is reached, two solitons with different central wavelengths operate synchronously and stably at a consistent repetition frequency of ∼8.1505 MHz and dual-color soliton molecules are generated. The fiber laser has the advantages of simple structure and controllable generation of soliton molecules, which provide a new idea for the design of soliton molecule ultrafast fiber laser.

Ablation depth enhancement on a copper surface using a dual-color double-pulse femtosecond laser.

We investigate the femtosecond laser ablation of copper with a dual-color double-pulse femtosecond laser at the wavelengths of 515 nm and 1030 nm. By properly choosing the energy of the 515 nm pulse, the optical properties such as surface reflectivity and absorption coefficient on copper surface can be modified to increase the absorption of the subsequent 1030 nm pulse. The ablation depth of dual-color double-pulse laser is at least 50% higher than the total ablation depth of both the 515 nm and 1030 nm pulses, provided that the inter-pulse delay of the double-pulse laser is within the electron-phonon coupling time. The ablation depth enhancement on a copper surface using a dual-color double-pulse femtosecond laser is of significant interest for scientific research and industrial application.

A Novel Dual-wavelength, Dual-function Laser System for Presbyopia and Glaucoma Treatments

Purpose: To update the accommodation mechanisms and propose a dual-wavelength, dual-function laser system for presbyopia and glaucoma treatments.
 Study Design: Laser sclera softening (LSS) for increased accommodation of presbyopic eyes.
 Place and Duration of Study: New Taipei City, Taiwan, between Jan., 2023 and Feb., 2023.
 Methodology: Accommodation gain (AG) can be improved by: (i) thermal shrinkage of the scleral stroma and ciliary body, or (ii) softening of the scleral stroma (with temperature range of 700C to 900C), such that the the lens front and back curvature change (or lens thickening), leading to the thickening of ciliary body and its apex, and the increase of the space of ciliary body and lens equation (SCL), and the length of the posterior vitreal zonules (PVZ) increases.
 Results: A novel dual-color laser system having wavelength A and B, acting on the front-zone and back-zone of the sclera, respectively, where laser-A has a deep thermal penetration the sclera and ciliary body (CB) (0.5 to 1.0 mm); and laser-B has a shallow penetration depth in the sclera (0.3 to 0.5 mm), based on the optical property of the sclera. Laser-A (having a wavelength about0.8 to 0.98 um) leads to thermal shrinkage of the ciliary body such that the CLS is increased for accommodation gain which is much more effective than the prior art.
 Conclusion: The increase of AG can be achieved by scleral softening and ciliary body shrinkage which increase the SCL. A proposed novel dual-color laser system acting on the front-zone and back-zone of the sclera, respectively, could provide higher AG than that of single wavelength, or prior arts using scleral ablation. However, further clinical studies are required to justified the proposed novel system with predicted advantages and efficacy based on the optical properties of sclera.

Enhanced energy deposition and carrier generation in silicon induced by two-color intense femtosecond laser pulses

We theoretically investigate the optical energy absorption of crystalline silicon subject to dual-color femtosecond laser pulses, using the time-dependent density functional theory (TDDFT). We employ the modified Becke-Johnson (mBJ) exchange-correlation potential which reproduces the experimental direct bandgap energy $E_g$. We consider situations where the one color is in the ultraviolet (UV) range above $E_g$ and the other in the infrared (IR) range below it. The energy deposition is examined as a function of mixing ratio $\eta$ of the two colors with the total pulse energy conserved. Energy transfer from the laser pulse to the electronic system in silicon is dramatically enhanced by simultaneous dual-color irradiation and maximized at $\eta\sim 0.5$. Increased is the number of generated carriers, not the absorbed energy per carrier. The effect is more efficient for lower IR photon energy, or equivalently, larger vector-potential amplitude. As the underlying mechanism is identified the interplay between intraband electron motion in the {\it valence} band (before excitation) driven by the IR component and resonant valence-to-conduction interband excitation (carrier injection) induced by the UV component. The former increases excitable electrons which pass through the $k$ points of resonant transitions. The effect of different multiphoton absorption paths or intraband motion of carriers generated in the conduction band play a minor role.

Dual color, frequency, pulse duration and shape agile laser system for particle spectroscopy and manipulation.

A dual color, frequency and pulse duration agile laser system, capable of delivering laser pulses in arbitrary temporal profiles with ∼1 ns to ∼1 µs pulse duration, chirping rates of ∼27 MHz/ns with an achievable chirping range of several GHz across the pulse duration, and with energies ranging from a few nJ to hundreds of mJ per pulse has been developed. The flexibility and capability of this laser system provide a wide range of laser parameters that can be exploited to optimize operational conditions in various experiments ranging from laser diagnostics to spectroscopy and optical manipulation of matter. The developed system is successfully demonstrated to obtain coherent Rayleigh-Brillouin scattering (CRBS) in both single and dual color configuration, in an effort to expand the non-intrusive accessibility towards lower pressure regime for neutral gas and plasma diagnostics.

Tunable mode-locked Tm-doped fiber laser based upon cross-phase modulation.

We demonstrate the generation of soliton and dissipative soliton in an ultrafast thulium (Tm) doped fiber laser based upon cross-phase modulation (XPM) induced mode-locking. The mode-locking is realized by periodically modulating the 2-µm signal through XPM that is activated by an injected 1.5-µm pulsed laser. Such a mechanism enables the laser to be mode-locked in various operation regimes without any real or artificial saturable absorbers. Thanks to the XPM pulling effect, the wavelength of the Tm-doped fiber laser can be tuned by adjusting the repetition frequency of the 1.5-µm pulsed laser. The maximum tuning ranges achieved in this work for the soliton and dissipative soliton regimes are respectively 11 nm and 15 nm. The outcomes of this work not only provide a continuously and controllably wavelength-tunable ultrafast laser but also offer a passively synchronized dual-color fiber laser system, which is promised for many important applications such as Raman spectroscopy, nonlinear frequency conversion systems, and multi-color pump-probe systems.

Generation of broadband parabolic pulses based on a pre-chirper free, core-pumped nonlinear fiber amplifier for coherent anti-Stokes Raman imaging

We report the generation of parabolic pulses with broadband spectrum from a core-pumped Yb-doped fiber amplifier seeded by a dispersion managed fiber oscillator. The net cavity dispersion of Yb-doped oscillator was continuously changed from 0.074 to -0.170ps2, which enabled us to achieve dissipative soliton, stretched pulse and soliton mode-locking operations. Spectral evolution processes in the core-pumped nonlinear fiber amplifier seeded by various input solitons were investigated experimentally and theoretically. Our finding indicates that cavity dispersion of oscillator can be used to engineer the input pulse parameter for amplifier, thus forming a pre-chirper free fiber amplification structure. In the experiment, we obtained 410-mW parabolic pulses with spectral bandwidth up to 56 nm. In combination with a passively synchronized frequency-doubled Er-doped fiber laser, we have demonstrated coherent anti-Stokes Raman imaging. The compact dual-color fiber laser source may facilitate practical applications of nonlinear biomedical imaging beyond the laboratory environment.

An enhancement method of waveform simulation in dual-color laser field imaging based on Internet of Things

AbstractIn view of the fact that the existing methods are easy to be affected by nonlinear factors in the incident process of the light source, resulting in the received shock wave inconsistent with the reality and large calculation error, a two-color laser field imaging waveform simulation and enhancement method based on the Internet of things is proposed. According to the automatic transformation characteristics of augmented reality technology, the waveform simulation control process of two-color laser field imaging is constructed. The Gaussian distribution characteristics are used to analyze the target, the optical grid and double oscillation device are used to control the results, the spectrum Fourier transform is used to adjust the phase of the waveform, and finally the simulated modulated laser waveform is output. Through the comparison of laser waveform spectrum and peak value, the results show that this method is closest to the actual laser waveform, saves calculation time, and has good practical application effect.

High power supercontinuum generation by dual-color femtosecond laser pulses in fused silica

High power supercontinuum (SC) is generated by focusing 800 nm and 400 nm femtosecond laser pulses in fused silica with a microlens array. It is found that the spectrum of the SC is getting broader compared with the case of a single laser pulse, and the spectral energy density between the two fundamental laser wavelengths is getting significantly higher by optimizing the phase matching angle of the BBO. It exceeds μJ/nm over 490 nm range which is from 380 nm to 870 nm, overcoming the disadvantage of relative lower power in the ranges far from the fundamental wavelength.

An Optically Reconfigurable Förster Resonance Energy Transfer Process for Broadband Switchable Organic Single-Mode Microlasers

An Optically Reconfigurable Förster Resonance Energy Transfer Process for Broadband Switchable Organic Single-Mode Microlasers

Intensity-dependent self-induced dual-color laser phase modulation and its effect on terahertz generation

Powerful, broadband terahertz (THz) pulses and its application attract an exponential growth of interests. Dual-color laser filamentation in gases is one of the promising THz sources because of the scalability of the THz energy and wavelength with input parameters. But the additional phase induced by the nonlinearities associated with high intensities cannot be neglected because it may result in modulation of the THz waves. We investigate the influences of the infrared pump energy and air dispersion on the terahertz generation in dual-color laser filament. We observe that optimum dual-color laser relative phase of the THz generation undergoes a linear shift with increasing pump energy due to the intensity-induced refractive index change. This phase shift is verified by the spectral broadening of a two-color laser affected by the same mechanism. The result improves our understanding of the theoretical framework for a higher power THz source.

Dual-color plasmonic random lasers for speckle-free imaging

A dual-color plasmonic random laser under single-excitation is achieved in an ultrathin membrane doped with binary quantum dots and gold nanorods. The gold nanorods tune the luminescence lifetime and emission efficiency of quantum dots. Under single excitation, low-threshold random lasing is observed. Green random lasing at 547 nm is ‘turned on’ and red random lasing at 630 nm is greatly enhanced by the transversal and longitudinal surface plasmon resonance of the gold nanorods, respectively. Speckle-free color imaging is achieved by using the proposed dual-color random laser source. These properties would facilitate the development of random lasers in fields of illumination and imaging.

Enhanced laser wakefield acceleration using dual-color relativistic pulses

In a recent article by Li et al (2019 Sci. Adv. 5. eaav7940), experimental results from a dual-color laser wakefield acceleration (LWFA) were presented. In the present paper we, primarily, focus on detailed simulation studies of such a scheme in the self-injection and ionization injection regimes, respectively. The spatiotemporally-overlapped 30 fs dual-color laser pulses are at fundamental (FL, 800 nm, ‘red’) and second-harmonic (SH, 400 nm, ‘blue’) wavelengths. They are (a) co-propagating in an under-dense plasma, (b) relativistically intense (I > 1018 W cm−2) and (c) having relatively high-energy (multi-Joule, loose focusing) and low-energy (sub-Joule, tight focusing), respectively. The basic concept of the scheme is the fact that the depletion length (Lpd) for a relativistic laser pulse in an under-dense plasma has an inverse quadratic dependence on the laser wavelength (∝1/λ2). Here, first by using a single FL 77 TW/30 fs laser pulse to drive a LWFA, an electron beam was accelerated up to ∼400 MeV from a background plasma having an electron density of 1019 cm−3. Then, by driving the same LWFA by co-propagating ‘blue’ 7 TW/30 fs and ‘red’ 70 TW/30 fs laser pulses, the electron energy reached ∼700–800 MeV (maximum). The simulations confirm that in such a dual-color LWFA scheme, the role of the SH laser pulse is post-accelerating electrons after a rapid depletion of the FL laser pulse in the plasma. Furthermore, the SH pulse assists the ionization-injection of the electrons which is an additional benefit of the dual-color LWFA scheme.

Giant Enhancement of Air Lasing by Complete Population Inversion in N_{2}^{+}.

A fine manipulation of population transfer among molecular quantum levels is a key technology for control of molecular processes. When a light field intensity is increased to the TW-PW cm^{-2} level, it becomes possible to transfer a population to specific excited levels through nonlinear light-molecule interaction, but it has been a challenge to control the extent of the population transfer. We deplete the population in the X^{2}Σ_{g}^{+}(v=0) state of N_{2}^{+} almost completely by focusing a dual-color (800nm and 1.6 μm) intense femtosecond laser pulse in a nitrogen gas, and make the intensity of N_{2}^{+} lasing at 391nm enhanced by 5-6 orders of magnitude. By solving a time-dependent Schrödinger equation describing the population transfer among the three lowest electronic states of N_{2}^{+}, we reveal that the X^{2}Σ_{g}^{+}(v=0) population is depleted by the vibrational Raman excitation followed by the electronic excitation A^{2}Π_{u}(v=2,3,4)←X^{2}Σ_{g}^{+}(v=1)←X^{2}Σ_{g}^{+}(v=0), resulting in the excessive population inversion between the B^{2}Σ_{u}^{+}(v=0) and X^{2}Σ_{g}^{+}(v=0) states. Our results offer a promising route to efficient population transfer among vibrational and electronic levels of molecules by a precisely designed intense laser field.

Carbon nanotube-synchronized dual-color fiber laser for coherent anti-Stokes Raman scattering microscopy.

In this Letter, we present a passively synchronized dual-color fiber laser at 1.03 and 1.53 µm for coherent anti-Stokes Raman scattering (CARS) microscopy. This fiber laser consists of both Yb- and Er-doped laser cavities, combined by an ∼1.2m common branch with a single-walled carbon-nanotube-based saturable absorber. Stable passively synchronized mode-locked state is obtained within a total cavity length mismatch of 50 µm. We demonstrate the capability of the synchronized dual-color fiber laser for CARS spectroscopy in both low- and high-wavenumber regions, with a resolution of 6.6cm-1. Furthermore, a CARS image in the field of view 150×60µm2 of polystyrene at the Raman shift of 3041cm-1 has also been achieved. The results show the feasibility of our passively synchronized dual-color fiber laser to be employed as a stable and low-cost ultrafast laser source for CARS.

Rapid diagnosis and measurement of explosively formed projectiles based on high-quality sequential images.

The explosively formed projectile (EFP) is an important type of warhead technology. To verify and evaluate its design and performance, EFP testing is an essential procedure. This work applies a newly developed dual-color laser photographic system (DCLPS) to diagnose the EFP in a flight. The main concepts of the DCLPS and image measurement theory are introduced in detail. The states of the EFP in flight are recorded via experiments at the Nanshan Test Center. High-quality sequential images are obtained by the DCLPS, and the measured key parameters agree well with the simulation results. Test time is only a few minutes, and the measurement error is less than 10%. This work demonstrates the considerable capability of the DCLPS for rapid diagnosis and measurement of an ultrafast EFP, and its great potential in similar observation applications.

Experimental evidence for terahertz emission of continuum electrons in the dual-color laser field.

Terahertz (THz) wave generation (TWG) in a dual-color laser is investigated with joint measurements between THz and third-harmonic generation, where the relative phase delay of dual-color fields is determined in situ in sub-wavelength accuracy, allowing for the clarification of the TWG mechanism in a direct comparison with various theoretical predictions. The delay- and polarization-dependent experiment validates that the continuum-continuum transition within the escaped electron wavepacket in the single atom gives birth to THz emission, while the bound energetic level does not contribute to TWG. TWG from atoms and molecules would provide an all-optical, vacuum-free, and ultrafast tool to record the spatiotemporal evolution of tunneling electron wavepackets.

Nonlinear multimode interference-based dual-color mode-locked fiber laser

We present a dual-color-soliton fiber laser at two different wavebands by nonlinear multimode interference. A saturable absorber (SA) with single-mode-multimode (MMF)-single-mode fiber structure is placed in the common branch shared by two sub-cavities. Saturable absorption effects can be simultaneously satisfied at 1.5 and 2 µm at a proper length of the MMF. Dual-color solitons can still remain, even by slightly tuning the length of the MMF. The periodical characteristic of this SA provides a flexible choice of MMF length, making it simple for simultaneous mode locking (SML) at two separate wavebands in practice. Our approach not only paves the way for SML at two or more wavebands by the MMF but also could lead to significant applications in pump-probe spectroscopy.