Double Charge Exchange Research Articles

Measurement of the 116Sn(18O, 18Ne)116Cd double charge exchange reaction at 276 MeV

The measurement of the 116Sn(18O, 18Ne)116Cd double charge exchange reaction cross section at very forward angles was performed for the first time at INFN-LNS using the MAGNEX magnetic spectrometer. This study, carried out at 276 MeV beam energy, provides a cross section of 34 nb ([9, 44] nb at 95% confidence level), confirming the tiny values recently obtained for the same reaction in other nuclides. This result has a major impact on the forthcoming systematic investigation of 0νββ decay candidates carried out by the NUMEN project, since it allows to properly tailor future experiments with high-intensity beams. The ultimate goal of this exploration is to experimentally access information about nuclear matrix elements relevant to the 0νββ decay rate.

Creating negative ion beams from neutral gases using a negative hydrogen ion source

A typical method to produce negative ion beams uses alkali vapour as a medium for a double charge exchange to convert incident positive (1+) beams to negative (1-) beams. Alkali vapours pose a problem in ion production as they are flammable, explosive and cause vacuum surface contamination. Thus, it is advantageous to use non-metallic vapours for charge exchange as it will prevent hazards and the contamination of vacuum surfaces and targets in which the negative ion beams are incident upon. In this paper we will describe and demonstrate the process of creating negative ion beams by impinging a 15 keV to 30 keV beam from D-Pace's TRIUMF licenced H- volume-cusp ion source (1 mA to 15 mA) onto a volume of non-metallic neutral gas (X) resulting in a single or two-step charge exchange: H- + X → H + X- or H- + X → H + X + e → H + X-. The newly created X- ion beams will be accelerated by a (1 to 20) kV electrostatic accelerator and passed through a mass spectrometer system to separate the primary H- beam from the X- beam. The two gases studied are He and H2 and we will present the magnitude of the resultant beam currents after being separated from the incident H- beam by the mass spectrometer system.

Production of negative ion beams through charge transfer between negative hydrogen ion beams and non-metallic gases

Negative ion beam applications in tandem accelerators are used for nuclear research, environmental studies, materials analysis, medical treatments, and ion implantation in semiconductor devices. Conventional methods for generating negative ions for tandem accelerators rely on metallic vapors (typically alkali) for charge exchange, which pose challenges like contamination, electrical shorting and breakdowns, and maintenance issues. To address these drawbacks, this work explores an alternative approach to produce negative ions using a non-metallic charge exchange process. It involves directing negative hydrogen ions into neutral gases within a specially designed charge exchange cell equipped with an electrostatic accelerator. The method is applied to various gas targets, including He, H2 and O2, to accelerate and measure resulting negative ions. This innovative approach aims to mitigate contamination concerns associated with metallic vapor double-charge exchange methods and explore novel avenues for negative ion production through charge transfer. Any newly formed negative ion beam current conversion ratios from the incident H− beam will be reported as progress in this research.

Theory of Majorana-Type Heavy Ion Double Charge Exchange Reactions by Pion–Nucleon Isotensor Interactions

The theory of heavy ion double charge exchange (DCE) reactions proceeding by effective rank-2 isotensor interactions is presented. Virtual pion–nucleon charge exchange interactions are investigated as the source for induced isotensor interactions, giving rise to the Majorana DCE (MDCE) reaction mechanism. MDCE is of a generic character, proceeding through pairs of complementary (π±,π∓) reactions in the projectile and target nucleus. The dynamics of the elementary processes is discussed, where the excitation of pion–nucleon resonances are of central importance. Investigations of initial and final state ion–ion interactions show that these effects are acting as vertex renormalizations. In closure approximation, well justified by the finite pion mass, the second-order transition matrix elements reduce to pion potentials and effective two-body isotensor DCE interactions, giving rise also to two-body correlations in either of the participating nuclei. Connections to neutrinoless Majorana double beta decay (MDBD) are elucidated at various levels of the dynamics, from the underlying fundamental electro-weak and QCD scales to the physical scales of nuclear MDBD and MDCE physics. It is pointed out that heavy ion MDCE reactions may also proceed by competing electro-weak charge exchange processes, leading to lepton MDCE by electrons, positrons, and neutrinos.

Induced Isotensor Interactions in Heavy-Ion Double-Charge-Exchange Reactions and the Role of Initial and Final State Interactions

The role of initial state (ISI) and final state (FSI) ion–ion interactions in heavy-ion double-charge-exchange (DCE) reactions A(Z,N)→A(Z±2,N∓2) are studied for double single-charge-exchange (DSCE) reactions given by sequential actions of the isovector nucleon–nucleon (NN) T-matrix. In momentum representation, the second-order DSCE reaction amplitude is shown to be given in factorized form by projectile and target nuclear matrix elements and a reaction kernel containing ISI and FSI. Expanding the intermediate propagator in a Taylor series with respect to auxiliary energy allows us to perform the summation in the leading-order term over intermediate nuclear states in closure approximation. The nuclear matrix element attains a form given by the products of two-body interactions directly exciting the n2p−2 and p2n−2 DCE transitions in the projectile and the target nucleus, respectively. A surprising result is that the intermediate propagation induces correlations between the transition vertices, showing that DSCE reactions are a two-nucleon process that resembles a system of interacting spin–isospin dipoles. Transformation of the DSCE NN T-matrix interactions from the reaction theoretical t-channel form to the s-channel operator structure required for spectroscopic purposes is elaborated in detail, showing that, in general, a rich spectrum of spin scalar, spin vector and higher-rank spin tensor multipole transitions will contribute to a DSCE reaction. Similarities (and differences) to two-neutrino double-beta decay (DBD) are discussed. ISI/FSI distortion and absorption effects are illustrated in black sphere approximation and in an illustrative application to data.

Formal theory of heavy ion double charge exchange reactions

The theory of heavy ion double charge exchange (DCE) reactions A(Z, N) → A(Z ± 2, N ∓ 2) is recapitulated emphasizing the role of Double Single Charge Exchange (DSCE) and pion-nucleon Majorana DCE (MDCE) reactions. DSCE reactions are of second–order distorted wave character, mediated by isovector nucleon-nucleon (NN) interactions. The DSCE response functions resemble the nuclear matrix elements (NME) of 2ν2β decay. The MDCE process proceeds by a dynamically generated effective rank-2 isotensor interaction, defined by off–shell pion–nucleon DCE scattering. In closure approximation pion potentials and two–nucleon correlations are obtained, similar to the neutrino potentials and the intranuclear exchange of Majorana neutrinos in 0ν2β Majorana double beta decay (MDBD).

Modeling Double Charge Exchange processes occurring in Heavy Ion Reactions

Heavy ion induced double charge exchange reactions are treated as an incoherent sequence of two reactions driven by the exchange of charged mesons (double single charge exchange, DSCE). The process is described within a fully quantum mechanical distorted wave 2-step theory (2nd order DWBA). The DSCE reaction amplitudes are shown to be separable into superpositions of distortion factors, accounting for initial and final state ion-ion elastic interactions, and nuclear matrix elements (NMEs). Explicit expressions of projectile and target NMEs are derived within the QRPA theory. Reduction schemes for the DSCE transition form factors are described, analizing their momentum structure within the closure approximation. Formal analogies between the NMEs involved in DSCE reactions and in double beta decays are also pointed out. Results, obtained within this theoretical framework, are illustrated for the reaction 40Ca (18O, 18Ne)40Ar at 15.3 AMeV and compared to the data measured at INFN-LNS by the NUMEN Collaboration. Furthermore, preliminary results for reactions involving heavier systems, such as 76Se (18O, 18Ne)76Ge, are shown.

Heavy-ion induced double charge exchange reaction in a multi-channel approach: The research program of the NUMEN project

We give an updated view of the status and prospects of heavy-ion double charge exchange (HI-DCE) reaction studies performed at the Laboratori Nazionali del Sud of the Istituto Nazionale di Fisica Nucleare (INFN-LNS) in the context of the NUMEN project. The important role of HI-DCE for nuclear reaction, nuclear structure and double beta-decay investigations is outlined. A powerful way to scrutinize the nuclear response to HI-DCE is to consistently link it to the information extracted from the competing direct reactions pointing to a multi-channel description of the whole network of quasi-elastic processes. Indeed, these complementary studies are mandatory in order to minimize the systematic errors in the data analyses and build a many-facets and parameter-free representation of the systems under study.

New Interacting Boson Fermion-Fermion Model results

We present a new application of the Interacting Boson Model (IBM) and its extensions for describing double charge exchange reactions. The study of double charge exchange reactions induced by heavy ions involving candidate nuclei for neutrinoless double beta decay is a complex task carried out by the NUMEN collaboration. This investigation faces the intricacies of complex oddodd intermediate nuclei in sequential double charge exchange processes. We will offer a comprehensive description of heavy odd-odd nuclei using the Interacting Boson Fermion-Fermion Model (IBFFM). Additionally, we will outline the methodology for describing transfer operators within this framework. Finally, we will explore the potential applications of our results for describing double charge exchange reactions.

Nuclear Structure Aspects of DCX Reactions and β β Decay Transitions

The theory of Double Charge Exchange (DCX) reactions between nuclei requires both the description of the reaction mechanism, which consists of the exchange of nucleons between the target and the projectile, as well as the structure of the matrix elements of the operators which mediate the transitions. From the point of view of the nuclear structure theory it requires the use of microscopic models for light and heavy mass nuclei. The reaction sector requires the use of momentum-dependent operators. It has been argued that these matrix elements could be associated to decay channels like the neutrinoless nuclear double beta decay (0νββ)(DBD). The motivation related to this claim is the need to determine, as accurately as possible, the values of the matrix elements of operators responsible for 0νββ. We shall focus the attention on the possible relationship between DBD and DCX nuclear matrix elements, by studying the dependence of the participant operators upon the momentum.

Experimental and theoretical multichannel study of direct nuclear reactions: A tool to provide data driven information on neutrino-less double-beta decay

The search for neutrino-less double beta decay has attracted much interest in the last years due to the extraordinary consequences that could derive from its observation. In the view to provide experimental information on the nuclear matrix elements involved in the expression of neutrino-less double beta decay half-life, the NUMEN project is measuring cross-sections of double charge exchange and other quasi-elastic nuclear reactions using the MAGNEX magnetic spectrometer. In particular, the newly proposed multichannel approach, applied both to the experimental and theoretical analysis, will be discussed.

Recent results on the analysis of the 18O+48Ti collision at 275 MeV: Single charge exchange reaction

The present work is inherent to the NUMEN project that aims at providing data-driven information for the nuclear matrix elements of the neutrinoless double beta decay through the study of heavy-ion induced double charge exchange reactions. This is a formidable task since during a nuclear collision, the same final states may be populated through various reaction mechanisms. In this respect, understanding the degree of competition between successive nucleon transfer and charge exchange reactions is crucial for the proper description of the meson-exchange mechanism. To this purpose, the reaction dynamics in the 18O+48Ti collision were sought by measuring a plethora of reaction channels under the same experimental conditions. The 48Ti was chosen as target since it is the daughter nucleus of 48Ca in double beta decay. The relevant experiment was performed at the MAGNEX facility of INFN-LNS in Catania. In this contribution, the status of the analysis for the 48Ti(18O,18F)48Sc single charge exchange reaction will be presented.

Study of single-nucleon transfer reactions in the 18O+48Ti collision at 275 MeV

The study of single-nucleon transfer reactions for the 18O+48Ti system was pursued at the energy of 275 MeV as part of a more systematic study which is undertaken within the NUMEN and NURE experimental campaigns. The aim is to measure the complete set of available reaction network which are characterized by the same initial and final-state wavefunctions as the more suppressed double charge exchange reactions. Understanding the degree of competition between successive nucleon transfer and double charge exchange reactions is crucial for the description of the meson-exchange mechanism. In this respect, angular distribution measurements for one- and twonucleon transfer reactions for the 18O+48Ti system were carried out at theMAGNEX facility of INFN-LNS in Catania. An overview of the data analysis for the 48Ti(18O,19F)47Sc and 48Ti(18O,17O)49Ti reactions will be presented.

Quantum-mechanical four-body versus semi-classical three-body theories for double charge exchange in collisions of fast alpha particles with helium targets

AbstractWithin the two-channel distorted wave second-order perturbative theoretical formalism, we study capture of both electrons from helium-like targets by heavy nuclei as projectiles at intermediate and high impact energies. The emphasis is on the four-body single-double scattering (SDS-4B) method and the three-body continuum distorted wave impact parameter method (CDW-3B-IPM). The SDS-4B method deals with the full quantum-mechanical correlative dynamics of all the four interactively participating particles (two electrons, two nuclei). The CDW-3B-IPM is a semi-classical three-body independent particle model (one electron, two nuclei), using a combinatorial calculus to describe double capture by a product of two uncorrelated probabilities, integrated over impact parameters. Both theories share a common feature in having altogether two electronic full Coulomb continuum wave functions. One such function is centered on the projectile nucleus in the entrance channel, whereas the other is centered on the target nucleus in the exit channel. These two methods satisfy the correct initial and final Coulomb boundary conditions in the asymptotic region of scattering, at infinitely large inter-particle separations. Yet, it is presently demonstrated that most of the available experimental data on total cross sections for the double capture from helium by alpha particles distinctly favor the SDS-4B method. This is especially true at intermediate energies. Such energies are critically important in versatile applications under the general umbrella of ion transport in matter, including thermonuclear fusion (plasma physics) and ion therapy (medicine).

A multi–channel study of the 20Ne + 130Te system within the NUMEN project

The NUMEN project aims to measure specific reaction cross sections to provide experimentally driven information about nuclear matrix elements of interest in the context of neutrinoless double beta decay (0νββ). In particular, it was proposed to use heavy – ion induced double charge exchange reactions as tools towards the determination of information on the nuclear matrix elements of 0νββ, strongly motivated by a number of similarities between the two processes. To this extent, the 20Ne + 130Te system was experimentally investigated in a multi-channel approach by measuring the complete net of reactions channels, namely double charge exchange, single charge exchange, elastic and inelastic scattering, one – and two – nucleon transfer reactions, characterized by the same initial projectile and target nuclei. The goal of the study is to fully characterize the properties of the nuclear wavefunctions entering in the 0νββ decay nuclear matrix elements. The experimental setup, the data reduction and some of the obtained results for the 20Ne + 130Te system will be presented and discussed.

Response of G-NUMEN LaBr3(Ce) Detectors to High Counting Rates

The G-NUMEN array is the future gamma spectrometer of the NUMEN experiment (nuclear matrix element for neutrinoless double beta decay), to be installed around the object point of the MAGNEX magnetic spectrometer at the INFN-LNS laboratory. This project aims to explore double-charge exchange (DCE) reactions in order to obtain crucial information about neutrinoless double beta decay (0νββ). The primary objective of the G-NUMEN array is to detect the gamma rays emitted from the de-excitation of the excited states that are populated via DCE reactions with a good energy resolution and detection efficiency, amidst a background composed of the transitions from competing reaction channels with far higher cross sections. To achieve this, G-NUMEN signals will be processed in coincidence with those generated by the detection of reaction ejectiles by the MAGNEX focal plane detector (FPD). Under the expected experimental conditions, G-NUMEN detectors will operate at high counting rates, of the order of hundreds of kHz per detector, while maintaining excellent energy and timing resolutions. The complete array will consist of over 100 LaBr3(Ce) scintillators. Initial tests were conducted on the first detectors of the array, allowing for the determination of their performance at high rates.

Recent results on the analysis of the 48Ti(18O, 20Ne)46Ca reaction at 275 MeV

The 18O+48Ti reaction was studied at the energy of 275 MeV for the first time under the NUMEN and NURE experimental campaigns with the aim of investigating the complete reaction network potentially involved in the 48Ti→48Ca double charge exchange transition. Understanding the degree of competition between successive nucleon transfer and double charge exchange reactions is crucial for the description of the meson exchange mechanism. Into this context, angular distribution measurements for one- and two-nucleon transfer reactions for the system 18O+48Ti were performed at the MAGNEX facility of INFN-LNS in Catania. An overview of the status of the analysis for the two-proton transfer reaction will be given.

Double charge-exchange reactions for the nuclear matrix elements of neutrinoless double beta decay

Double charge exchange (DCE) reactions induced by heavy ions are crucial tools to access information relevant for neutrinoless double beta decay nuclear matrix elements. In this context the NUMEN project aims to investigate, for each system of interest, the DCE reaction channel together with the whole set of reactions promoted by the same projectile/target interaction in the same experimental conditions and within the same theoretical framework.

New high intensity Heavy - Ion beams @ INFN-LNS: NUMEN project status and perspective

The upgrade project POTLNS to produce high-intensity beams has already started at INFN- Laboratori Nazionali del Sud in Catania (Italy). The POTLNS project was triggered by the NUMEN physics case that aims to provide experimental information on the Nuclear Matrix Elements (NMEs) that enter in the expression of the neutrino-less double beta (0νββ) decay half-life. The tools proposed by NUMEN project are the cross-section measurements of nuclear Double Charge Exchange (DCE) reactions. The search for 0νββ decay is currently a key topic in physics, due to its possible wide implications for nuclear physics, particle physics and cosmology: the NUMEN project could provide a crucial contribution in this search.

Experimental and theoretical multi-channel study of direct nuclear reactions: a tool to provide data driven information on the 76Ge neutrino-less double-beta decay

The study of heavy-ions induced double charge-exchange (HI-DCE) nuclear reactions is a promising way to access data-driven information on neutrino-less double-beta decay nuclear matrix elements. In the following, particular attention is given to the (18O,18Ne) and (20Ne,20O) HI-DCE reactions as tools for β + β + and β − β − decays, respectively. The experiments are performed in Catania at the Laboratori Nazionali del Sud of the Istituto Nazionale di Fisica Nucleare (INFN-LNS). The MAGNEX magnetic spectrometer is used to momentum analyse the ejectiles of a large network of nuclear reactions. New preliminary experimental data for the 76Se(18O,18F)76As and 76Ge(20Ne,20F)76As single charge exchange (SCE) and for the 76Se(18O,18Ne)76Ge and 76Ge(20Ne,20O)76Se DCE nuclear reactions were also investigated.