The Directed Energy Deposition (DED) method, which utilizes metal powder and a high-powder laser directed at specific locations on a substrate, is employed across various fields for repairing and refurbishing existing parts. In this study, two types of multi-materials were fabricated by depositing materials similar in alloy composition, and dissimilar, respectively, on an SCM440 substrate using the DED method. Unlike similar material, depositing the dissimilar material resulted in a recrystallized fine microstructure in the interlayer region, which enhanced the tensile properties of the multi-layer specimens. The yield strength, tensile strength, and elongation of the multi-layer specimen with similar material were 562 MPa, 787 MPa, and 14%, respectively, while those of the specimen with dissimilar material were significantly higher at 934 MPa, 1016 MPa, and 30%. These results demonstrate that using dissimilar materials, rather than identical or similar compositions, can improve the tensile properties when repairing and refurbishing parts made of SCM440 material.