Desert Dust Sources Research Articles

Contribution of black carbon and desert dust to aerosol absorption in the atmosphere of the Eastern Arabian Peninsula

Discriminating the absorption coefficients of aerosol mineral dust and black carbon (BC) in different aerosol size fractions is a challenge because of BC's large mass absorption cross-section compared to dust. Ambient aerosol wavelength dependent absorption coefficients (babs) in supermicron and submicron size fractions were determined with a high time resolution. The measurements were performed simultaneously using identical systems at an urban and a regional background site in Qatar. At each site, measurements were taken by co-located Aethalometers, one with a virtual impactor (VI) and the other with a PM1 cyclone to respectively collect super-micron-enhanced and submicron fractions. The combined measurement of aerosol absorption and scattering coefficients enabled the particles to be classified based on their optical properties' wavelength dependence. The classification reveals the presence of BC internally/externally mixed with different aerosols. Helium ion microscopy images provided information concerning the extent of mineral dust in the submicron fraction. The determination of absorption coefficients during dust storms and non-dust periods was used to establish the absorption Ångström exponent for dust and BC. Non-parametric wind regression, potential source contribution function and back-trajectory analysis reveal major regional sources of desert dust associated with north-westerly winds and a minor local dust contribution. In contrast, major BC sources found locally were associated with south-westerly winds with a smaller contribution made by offshore emissions transported by north-easterly and easterly winds. The use of a pair of Aethalometers with VI and PM1 inlets separates contributions of BC and dust to the aerosol absorption coefficient.

Effect of spatial and temporal “drought legacy” on dust sources in adjacent ecoregions

AbstractDrought affects the occurrence and intensity of aeolian dust events in many ecoregions. This study investigated the effects of “drought legacy” (the cumulative temporal persistence of drought's consequences on the earth system) on dust generation, a topic which had not previously been evaluated. We investigated the potential dust/drought legacy relationship in the USA's Southern Great Plains and Chihuahuan Desert ecoregions over 14 years, including the 2011–2012 extreme drought, at spatial distances up to 100 km around dust point sources and for up to 5 years' drought history. At every temporal and spatial scale, drought levels associated with dust initiation points in the two ecoregions were significantly different. Chihuahuan Desert dust sources concentrated in areas of severe to extreme drought, while those in the Southern Great Plains, which experiences greater land use, spanned wider ranges of drought conditions. At short temporal scales of drought (1 week and 1 year), dust initiation in the Chihuahuan Desert was associated strongly with severe to exceptional drought conditions at all spatial extents, while Southern Great Plains dust sources were linked to lower drought intensities. For longer drought histories (the past 2 and 5 years), Chihuahuan Desert dust sources were connected with moderate to severe drought, while Southern Great Plains dust sources were linked to moderate drought, at all spatial extents. Drought's legacies, extending over multiple years and kilometer scales, are shown to have roles in subsequent dust events at regional scales, though they can be regionally modulated by land use practices and ecosystem characteristics.

Machine learning-driven scenario-based models for predicting desert dust sources in central playas of Iran

Monitoring and controlling dust sources under climate changes and developing suitable prediction approaches is very important, since they have direct impacts on the environment and human health. The current study was performed with the aim of predicting the dust emission of Yazd province, located in the central playas of Iran, by combining a machine learning ensemble model and the global climate model IPSL-CM6A-LR. The key variables of dust emission including physiographic characteristics, climatic variables and human factors were mapped in order to model occurrence data against background data. After removing 15 autocorrelated points, from 120 pixels located in dust sources, 75 % and 25 % of them were randomly selected as training and test datasets, respectively. To evaluate modeling, in addition to sensitivity, specificity, TSS and Kappa indices, the Partial ROC approach was used. For the final mapping of land susceptibility to dust emission, individual models based on the weighted average of AUCratio values were used to create the ensemble model. The relative importance of dust emission controlling factors was obtained with the consensus of seven machine learning models: distance to dirt roads, altitude, distance to mines and mean temperature of driest quarter. MARS outperformed the other individual models, so that it showed no significant difference with the ensemble model at the thresholds of E = 10 and E = 5 (p-value < 0.05). Statistical analysis of the ensemble model with AUCratio equal to 1.933 showed that currently 28.56 percent of the province, is prone to dust emission and it will increase linearly in the future for scenarios SSP1-2.6 and SSP5-8.5. In both time periods (2041–2070 and 2071–2100), dust emissions will be higher under the SSP5-8.5 scenario compared to the SSP1-2.6 scenario. The results can be used by policymakers for the sustainable management of deserts and thus reduce the impacts of dust on current and future ecosystem health.

Saharan dust induces NLRP3-dependent inflammatory cytokines in an alveolar air-liquid interface co-culture model

BackgroundEpidemiological studies have related desert dust events to increased respiratory morbidity and mortality. Although the Sahara is the largest source of desert dust, Saharan dust (SD) has been barely examined in toxicological studies. Here, we aimed to assess the NLRP3 inflammasome-caspase-1-pathway-dependent pro-inflammatory potency of SD in comparison to crystalline silica (DQ12 quartz) in an advanced air-liquid interface (ALI) co-culture model. Therefore, we exposed ALI co-cultures of alveolar epithelial A549 cells and macrophage-like differentiated THP-1 cells to 10, 21, and 31 µg/cm² SD and DQ12 for 24 h using a Vitrocell Cloud system. Additionally, we exposed ALI co-cultures containing caspase (CASP)1−/− and NLRP3−/− THP-1 cells to SD.ResultsCharacterization of nebulized DQ12 and SD revealed that over 90% of agglomerates of both dusts were smaller than 2.5 μm. Characterization of the ALI co-culture model revealed that it produced surfactant protein C and that THP-1 cells remained viable at the ALI. Moreover, wild type, CASP1−/−, and NLRP3−/− THP-1 cells had comparable levels of the surface receptors cluster of differentiation 14 (CD14), toll-like receptor 2 (TLR2), and TLR4. Exposing ALI co-cultures to non-cytotoxic doses of DQ12 and SD did not induce oxidative stress marker gene expression. SD but not DQ12 upregulated gene expressions of interleukin 1 Beta (IL1B), IL6, and IL8 as well as releases of IL-1β, IL-6, IL-8, and tumor necrosis factor α (TNFα). Exposing wild type, CASP1−/−, and NLRP3−/− co-cultures to SD induced IL1B gene expression in all co-cultures whereas IL-1β release was only induced in wild type co-cultures. In CASP1−/− and NLRP3−/− co-cultures, IL-6, IL-8, and TNFα releases were also reduced.ConclusionsSince surfactants can decrease the toxicity of poorly soluble particles, the higher potency of SD than DQ12 in this surfactant-producing ALI model emphasizes the importance of readily soluble SD components such as microbial compounds. The higher potency of SD than DQ12 also renders SD a potential alternative particulate positive control for studies addressing acute inflammatory effects. The high pro-inflammatory potency depending on NLRP3, CASP-1, and IL-1β suggests that SD causes acute lung injury which may explain desert dust event-related increased respiratory morbidity and mortality.

From desert dust to ongoing soil formation in the mountainous areas of the south Levant

Mediterranean soils of the south Levant have been investigated and described during the past several decades, especially brown-reddish mountain soils, but certain issues, such as the role of desert dust as a parent material, remain unresolved. This study aims to quantify the role of desert dust in the formation of the mountain soils of the south Levant area, examine the environmental factors that affect the soil formation processes, and evaluate their time of formation. This is done by sampling and analyzing soil sites along two west-east transects across the Judea and Samaria mountains that encompass the transition from the Mediterranean to the semiarid climate. The new database includes the bulk mineralogical and chemical compositions of major oxides and trace elements, particle size distributions, and basic soil’s parameters. Although the range of calcite content in the soils studied is large (>1 % to 60 %), all soil types have similar grain size distributions of three modes: 45–55 μm mode within the coarse silt fraction, 20–25 μm mode within the fine silt fraction, and a clay mode. Local (Jerusalem) dust, collected near the sampled soils, is distinguished from desert dust by a lower quartz content and lower concentrations of SiO2, TiO2, Th, and Zr, suggesting that the local dust is a mixture of remote desert dust and local sources. The soils on the eastern side of the Judean Mountains, under a semiarid climate, are dominated by the coarse silt mode, and their compositions reflect a higher contribution of desert dust and weaker pedogenic processes. The pedogenic formation of smectites turns the clay fraction into the main grain size mode in the leached soils of the western side, under higher precipitation and denser vegetation. The almost identical compositions found for two adjacent soils on limestone and on chert demonstrate that dust is almost the exclusive parent material for soils presently forming on hard sedimentary rocks. This, other chemical parameters, and additional field observations indicate no relation between soils and bedrock or visible karstic activity at present. Accordingly, soil formation in the mountainous areas of the south Levant is a result of ongoing dust accumulation and transformation since the last major erosion event in the early Holocene.

Effects of Desert Dust and Sandstorms on Human Health: A Scoping Review.

Desert dust and sandstorms are recurring environmental phenomena that are reported to produce serious health risks worldwide. This scoping review was conducted to identify the most likely health effects of desert dust and sandstorms and the methods used to characterize desert dust exposure from the existing epidemiological literature. We systematically searched PubMed/MEDLINE, Web of Science, and Scopus to identify studies that reported the effects of desert dust and sandstorms on human health. Search terms referred to desert dust or sandstorm exposure, names of major deserts, and health outcomes. Health effects were cross-tabulated with study design variables (e.g., epidemiological design and methods to quantify dust exposure), desert dust source, health outcomes and conditions. We identified 204 studies that met the inclusion criteria for the scoping review. More than half of the studies (52.9%) used a time-series study design. However, we found a substantial variation in the methods used to identify and quantify desert dust exposure. The binary metric of dust exposure was more frequently used than the continuous metric for all desert dust source locations. Most studies (84.8%) reported significant associations between desert dust and adverse health effects, mainly for respiratory and cardiovascular mortality and morbidity causes. Although there is a large body of evidence on the health effects of desert dust and sandstorms, the existing epidemiological studies have significant limitations related to exposure measurement and statistical analysis that potentially contribute to inconsistencies in determining the effect of desert dust on human health.

Modeling coarse and giant desert dust particles

Abstract. Dust particles larger than 20 µm in diameter have been regularly observed to remain airborne during long-range transport. In this work, we modify the parameterization of the mineral dust cycle in the GOCART-AFWA dust scheme of WRFV4.2.1 to also include such coarse and giant particles, and we further discuss the underlying misrepresented physical mechanisms which hamper the model in reproducing adequately the transport of the coarse and giant mineral particles. The initial particle size distribution is constrained by observations over desert dust sources. Furthermore, the Stokes drag coefficient has been updated to account for realistic dust particle sizes (Re &lt; 105). The new code was applied to simulate dust transport over Cabo Verde in August 2015 (AER-D campaign). Model results are evaluated against airborne dust measurements and the CALIPSO-LIVAS pure dust product. The results show that the modeled lifetimes of the coarser particles are shorter than those observed. Several sensitivity runs are performed by reducing artificially the particles' settling velocities in order to compensate underrepresented mechanisms, such as the non-spherical aerodynamics, in the relevant parameterization schemes. Our simulations reveal that particles with diameters of 5.5–17 and 40–100 µm are better represented under the assumption of an 80 % reduction in the settling velocity (UR80), while particles with sizes ranging between 17 and 40 µm are better represented in a 60 % reduction in settling velocity (UR60) scenario. The overall statistical analysis indicates that the best agreement with airborne in situ measurements downwind (Cabo Verde) is achieved with a 40 % reduction in settling velocity (UR40). Moreover, the UR80 experiment improves the representation of the vertical structure of the dust layers as those are captured by the CALIPSO-LIVAS vertically resolved pure dust observations. The current study highlights the necessity of upgrading the existing model parameterization schemes of the dust life-cycle components towards improving the assessment of the dust-related impacts within the Earth–atmosphere system.

The “Weekend Effect” in Lightning Activity during Winter Thunderstorms over the Tel-Aviv, Israel, Metropolitan Area

We report the analysis of nine winter seasons (December, January, February (DJF)) aerosol and lightning data over the Tel-Aviv metropolitan area, Israel’s largest and densest urban region. Hourly averaged aerosol concentrations (PM2.5 and PM10) were obtained from 27 automatic air quality stations operated by the Ministry for Environmental Protection. Lightning data obtained from the Israeli Lightning Detection Network (ILDN) and by the Earth Network Total Lightning Network (ENTLN) for four overlapping seasons showed an irregular pattern, with lower activity during Sunday–Tuesday, and maximum activity on Wednesday and Thursday, but also on Saturday, when less pollution was present. The accepted explanation for the weekend effect is that increased amounts of particles tend to prolong the lifetime of storms and their total lightning amounts and change their intracloud/cloud-to-ground flash ratios. However, our results suggest that lightning is not directly related to the level of ambient pollution, but likely depends on the synergistic effects of desert dust and urban pollution particles in the area that affect the electrical structure of winter thunderstorms. Since the source of desert dust is independent of any regularity that can be attributed to anthropogenic activity (e.g., increased levels of pollution due to the traffic-load in Tel-Aviv), it obscures any weekend–weekday patterns that are often detected in other large metropolitan areas.

Short-term effects of exposure to particulate matter concentrations originating from desert dust on mortality in Athens, Greece

Background &amp;#x26; Aim: Evidence on the independent associations of source-specific particulate matter (PM) exposures with health outcomes is limited. Our aim was to investigate the effects of short-term exposure to PM&amp;#x2264; 10&amp;#x3bc;m (PM10) concentrations originating from windblown desert dust and local sources on mortality. Methods: We investigated the effect of exposure to total PM10 concentrations, as well as estimated concentrations originating from desert dust and other sources on total mortality, between the years 2010-2019. We used Poisson regression models to estimate the association between PM10 from different sources, also controlling for possible confounding by season, meteorology, day of the week and holiday effect. Results: During the 10-year study period, 35% of days were affected by desert dust (desert dust PM10&amp;#x3e; 0&amp;#x3bc;g/m3). An increment of 10&amp;#x3bc;g/m3 in total PM10 concentrations was associated with a 0.52% (lag 0–1, 95% confidence interval (CI): 0.21, 0.83%) increase in natural mortality. When mutually adjusting non-desert and desert dust PM10 concentrations, a 10&amp;#x3bc;g/m3 increase in non-desert was associated with a 0.45% (95% CI: 0.07% to 0.84%) increase in natural mortality. On the other hand, the effect of desert PM10 (lag 0-1 days) concentrations was non-significant (0.59%; 95% CI: -0.53% to 1.72%). Conclusions: Our findings support the hypothesis that daily exposure to traffic-related particles have more toxic effects, compared to ones originating from windblown desert dust, in Athens, Greece leading to increased mortality.

Compositional data analysis (CoDA) as a tool to evaluate a new low-cost settling-based PM10 sampling head in a desert dust source region

Abstract. This paper presents a new sampling head design and the method used to evaluate it. The elemental composition of aerosols collected by two different sampling devices in a semi-arid region of Tunisia is compared by means of compositional perturbation vectors and biplots. This set of underused mathematical tools belongs to a family of statistics created specifically to deal with compositional data. The two sampling devices operate at a flow rate in the range of 1 m3 h−1, with a cut-off diameter of 10 µm. The first device is a low-cost laboratory-made system, where the largest particles are removed by gravitational settling in a vertical tube. This new system will be compared to the second device, a brand-new standard commercial PM10 sampling head, where size segregation is achieved by particle impaction on a metal surface. A total of 44 elements (including rare earth elements, REEs, together with Al, As, Ba, Be, Ca, Cd, Co, Cr, Cu, Fe, K, Li, Mg, Mn, Mo, Na, Ni, P, Pb, Rb, S, Sc, Se, Sr, Ti, Tl, U, V, Zn, and Zr) were analysed in 16 paired samples, collected during a 2-week field campaign in Tunisian dry lands, close to source areas, with high levels of large particles. The contrasting meteorological conditions encountered during the field campaign allowed a broad range of aerosol compositions to be collected, with very different aerosol mass concentrations. The compositional data analysis (CoDA) tools show that no compositional differences were observed between samples collected simultaneously by the two devices. The mass concentration of the particles collected was estimated through chemical analysis. Results for the two sampling devices were very similar to those obtained from an online aerosol weighing system, TEOM (tapered element oscillating microbalance), installed next to them. These results suggest that the commercial PM10 impactor head can therefore be replaced by the decanter, without any measurable bias, for the determination of chemical composition and for further assessment of PM10 concentrations in source regions.

Earth, Wind, Fire, and Pollution: Aerosol Nutrient Sources and Impacts on Ocean Biogeochemistry.

A key Earth system science question is the role of atmospheric deposition in supplying vital nutrients to the phytoplankton that form the base of marine food webs. Industrial and vehicular pollution, wildfires, volcanoes, biogenic debris, and desert dust all carry nutrients within their plumes throughout the globe. In remote ocean ecosystems, aerosol deposition represents an essential new source of nutrients for primary production. The large spatiotemporal variability in aerosols from myriad sources combined with the differential responses of marine biota to changing fluxes makes it crucially important to understand where, when, and how much nutrients from the atmosphere enter marine ecosystems. This review brings together existing literature, experimental evidence of impacts, and new atmospheric nutrient observations that can be compared with atmospheric and ocean biogeochemistry modeling. We evaluate the contribution and spatiotemporal variability of nutrient-bearing aerosols from desert dust, wildfire, volcanic, and anthropogenic sources, including the organic component, deposition fluxes, and oceanic impacts.

Towards understanding the characteristics of new particle formation in the Eastern Mediterranean

Abstract. To quantify the contribution of new particle formation (NPF) to ultrafine particle number and cloud condensation nuclei (CCN) budgets, one has to understand the mechanisms that govern NPF in different environments and its temporal extent. Here, we study NPF in Cyprus, an Eastern Mediterranean country located at the crossroads of three continents and affected by diverse air masses originating from continental, maritime, and desert-dust source areas. We performed 1-year continuous measurements of aerosol particles down to ∼ 1 nm in diameter for the first time in the Eastern Mediterranean and Middle East (EMME) region. These measurements were complemented with trace gas data, meteorological variables, and retroplume analysis. We show that NPF is a very frequent phenomenon at this site and has higher frequencies of occurrence during spring and autumn. NPF events were both of local and regional origin, and the local events occurred frequently during the month with the lowest NPF frequency. Some NPF events exhibited multiple onsets, while others exhibited apparent particle shrinkage in size. Additionally, NPF events were observed during the nighttime and during episodes of high desert-dust loadings. Particle formation rates and growth rates were comparable to those in urban environments, although our site is a rural one. Meteorological variables and trace gases played a role in explaining the intra-monthly variability of NPF events, but they did not explain why summer months had the least NPF frequency. Similarly, pre-existing aerosol loading did not explain the observed seasonality. The months with the least NPF frequency were associated with higher H2SO4 concentrations but lower NO2 concentrations, which is an indicator of anthropogenic influence. Air masses arriving from the Middle East were not observed during these months, which could suggest that precursor vapors important for nucleation and growth are transported to our site from the Middle East. Further comprehensive measurements of precursor vapors are required to prove this hypothesis.

The EMIT mission information yield for mineral dust radiative forcing

The net direct radiative effect of mineral dust is a large uncertainty in global radiative forcing. To address this challenge, NASA's Earth Mineral dust source InvesTigation (EMIT) will map the surface mineralogy of Earth's desert dust source regions, constraining the composition of mineral dust aerosol for use in Earth system models (ESMs). This mission foreshadows multiple future global spectroscopic investigations for which coupling with ESMs will play a critical role. Planning such experiments requires a methodology for assessing the impact of uncertain remote observations on ESM accuracy. We design and implement an end-to-end simulation of the EMIT mission, leveraging Bayesian statistical methods and Monte Carlo sampling to analyze uncertainties in the retrieval and processing of EMIT data products. Special focus is placed on those uncertainties caused by atmospheric water vapor and aerosol loading conditions likely to be encountered by EMIT. We apply these results to a single-column configuration of the Community Earth System Model (CESM), revealing the potential impact of EMIT observations on radiative forcing estimates. We show that EMIT data stand to significantly reduce uncertainty in estimates of the dust direct radiative forcing attributable to uncertainties in surface mineralogies that are input to ESMs, and that the information gain for radiative forcing comes predominantly from better constraining iron oxides, which dominate the shortwave radiative effects of aerosol dust.

Influence of sampling approaches on physical and geochemical analysis of aeolian dust in source regions

The characterisation of mineral dust at emission sources is essential for quantifying the wider-scale environmental impacts dust has, as well as improving its incorporation in modelling. Methods of sampling sediments at these source areas for the purposes of dust characterisation are varied and can produce different representations of emitted dust. This study systematically compared dust characterisations from three established approaches for estimating dust emission potential, namely: Big Spring Number Eight (BSNE) traps, a Portable In-situ Wind Erosion Laboratory (PI-SWERL) wind tunnel, and bulk surface sampling, at a known Namib Desert dust source. Individual particle analysis by auto-SEM (QEMSCAN) allowed comparison of size, shape, mineralogy and elemental composition at micrometre-scale for samples from the three approaches. BSNE samples consisted of a lower proportion of fine sediment (<20 µm particle diameter) than PI-SWERL-derived samples, with this performance possibly influenced by atmospheric humidity. In comparison, PI-SWERL characterised the dust with relatively fewer particles between 63 and 100 µm, a fraction that was more evident in both the BSNE-derived and surface sediments. The reduced representation of this coarser fraction resulted in appreciable differences in particle shape and mineralogic characteristics compared to BSNE and surface-derived samples. The different representations by the three methods return variable dust characteristics at source across fundamental properties of particle size, shape and mineralogy. Awareness of the different representations of dust caused by sampling technique remains essential for the appropriate physical and geochemical characterisation of aeolian dust and highlights how standardised techniques are important for meaningful comparisons, while methods to achieve accurate characterisation remain a priority for the discipline.

Are the phosphate oxygen isotopes of Saharan dust a robust tracer of atmospheric P source?

Abstract Aeolian dust is a significant source of phosphorus (P) in various ecosystems. The Saharan desert is the major dust source on earth and it contributes atmospheric P to terrestrial ecosystems which often depend on these inputs. Since estimations on the contribution of dust to the atmospheric P cycle vary between studies, accurate estimations on the aerosol-P inputs to ecosystems can be enhanced by an identification method for dust from the other atmospheric P sources. In the current study, we explored the use of the oxygen stable isotopes in phosphate, δ18OP, as a marker for desert dust P. To characterize the δ18OP in Saharan dust, we analyzed atmospheric particles sampled in Puerto Rico, which has good exposure in summer to African dust with little exposure to wildfires, local, or anthropogenic influence on atmospheric inputs. Additionally, to evaluate possible isotopic fractionations in desert dust sources, which could affect the soil δ18OP before transport, we analyzed the δ18OP in Israeli desert soils that served as an analog. Saharan dust storms sampled at Puerto Rico were found to have δ18OP values of 22.5 ± 0.3‰ in the resin fraction (which represents labile inorganic P), similar to previously reported values of Saharan dust sampled in Israel. The data from Israel desert soils demonstrated that biological activity in desert crusts can have a small effect (with a maximum difference of 3.3‰ between the topsoil and the subsoil) on the δ18OP of desert soils, mainly when developed soil crust is present, as a result of intracellular isotopic equilibration between oxygen in phosphate and soil water. However, biological crusts are not considered a major dust source. Additionally, Saharan dust sampled in Israel and in Puerto Rico had a δ18OP similar to apatite minerals derived from sedimentary phosphorites. Thus, we suggest the dust source had little or no biological activity. Furthermore, the δ18OP in Saharan dust was distinctive from other atmospheric P sources, such as pollen and wildfire ash, and as a result, the δ18OP can be used to distinguish between these atmospheric P main sources.

Modeling the biogeochemical impact of atmospheric phosphate deposition from desert dust and combustion sources to the Mediterranean Sea

Abstract. Daily modeled fields of phosphate deposition to the Mediterranean from natural dust, anthropogenic combustion and wildfires were used to assess the effect of this external nutrient on marine biogeochemistry. The ocean model used is a high-resolution (1∕12°) regional coupled dynamical–biogeochemical model of the Mediterranean Sea (NEMO-MED12/PISCES). The input fields of phosphorus are for 2005, which are the only available daily resolved deposition fields from the global atmospheric chemical transport model LMDz-INCA. Traditionally, dust has been suggested to be the main atmospheric source of phosphorus, but the LMDz-INCA model suggests that combustion is dominant over natural dust as an atmospheric source of phosphate (PO4, the bioavailable form of phosphorus in seawater) for the Mediterranean Sea. According to the atmospheric transport model, phosphate deposition from combustion (Pcomb) brings on average 40.5×10−6 mol PO4 m−2 yr−1 over the entire Mediterranean Sea for the year 2005 and is the primary source over the northern part (e.g., 101×10−6 mol PO4 m−2 yr−1 from combustion deposited in 2005 over the north Adriatic against 12.4×10−6 from dust). Lithogenic dust brings 17.2×10−6 mol PO4 m−2 yr−1 on average over the Mediterranean Sea in 2005 and is the primary source of atmospheric phosphate to the southern Mediterranean Basin in our simulations (e.g., 31.8×10−6 mol PO4 m−2 yr−1 from dust deposited in 2005 on average over the south Ionian basin against 12.4×10−6 from combustion). The evaluation of monthly averaged deposition flux variability of Pdust and Pcomb for the 1997–2012 period indicates that these conclusions may hold true for different years. We examine separately the two atmospheric phosphate sources and their respective flux variability and evaluate their impacts on marine surface biogeochemistry (phosphate concentration, chlorophyll a, primary production). The impacts of the different phosphate deposition sources on the biogeochemistry of the Mediterranean are found localized, seasonally varying and small, but yet statistically significant. Differences in the geographical deposition patterns between phosphate from dust and from combustion will cause contrasted and significant changes in the biogeochemistry of the basin. We contrast the effects of combustion in the northern basin (Pcomb deposition effects are found to be 10 times more important in the northern Adriatic, close to the main source region) to the effects of dust in the southern basin. These different phosphorus sources should therefore be accounted for in modeling studies.

Atmospheric Ice‐Nucleating Particles in the Dusty Tropical Atlantic

AbstractDesert dust is one of the most important atmospheric ice‐nucleating aerosol species around the globe. However, there have been very few measurements of ice‐nucleating particle (INP) concentrations in dusty air close to desert sources. In this study we report the concentration of INPs in dust laden air over the tropical Atlantic within a few days' transport of one of the world's most important atmospheric sources of desert dust, the Sahara. These measurements were performed as part of the Ice in Clouds Experiment‐Dust campaign based in Cape Verde, during August 2015. INP concentrations active in the immersion mode, determined using a droplet‐on‐filter technique, ranged from around 102 m−3 at −12°C to around 105 m−3 at −23°C. There is about 2 orders of magnitude variability in INP concentration for a particular temperature, which is determined largely by the variability in atmospheric dust loading. These measurements were made at altitudes from 30 to 3,500 m in air containing a range of dust loadings. The ice active site density (ns) for desert dust dominated aerosol derived from our measurements agrees with several laboratory‐based parameterizations for ice nucleation by desert dust within 1 to 2 orders of magnitude. The small variability in ns values determined from our measurements (within about 1 order of magnitude) is striking given that the back trajectory analysis suggests that the sources of dust were geographically diverse. This is consistent with previous work, which indicates that desert dust's ice‐nucleating activity is only weakly dependent on source.

The effect of mineral dust transport on PM10 concentrations and physical properties in Istanbul during 2007–2014

Mineral dust is the most significant source of natural particulate matter. In urban regions, where >50% of the world population is currently living, local emissions of particulate matter are further aggravated by mineral dust loadings from deserts. The megacity of Istanbul is located in an area sensitive to local pollution due to transportation (i.e., private cars, public transportation, aircrafts, ships, heavy diesel trucks, etc.), industrial emissions, residential heating, and long-range transport from Europe, Asia, and deserts. In this work, the effect of desert dust transport on PM10 concentrations and physical properties was investigated for the period of 2007–2014 in the touristic area of Aksaray, Istanbul. The Dust Regional Atmospheric Model (DREAM8b) was used to predict dust loading in Istanbul during dust transport events. Variations on surface PM10 concentrations were investigated according to seasons and during dust transport events. Cluster analysis of air mass backward trajectories was useful to understand frequency analysis and air mass trajectory dependence of PM10 concentrations on dust loadings. The effect of desert dust transport on aerosol optical depths was also investigated. It was observed that PM10 concentrations exceeded the air quality standard of 50μgm−3 50% of the time during the study period. The largest number of exceedances in air quality standard occurred during the spring and winter seasons. Approximately 40–60% of the dust loading occurs during the spring. Desert dust and non-desert dust sources contribute to 22–72% and 48–81% of the ground-level PM10 concentrations in Aksaray, Istanbul during the study period. Averaged AOD observed during dust transport events in spring and summer ranged 0.35–0.55. Cluster analysis resolved over 82% the variability of individual air mass backward trajectories into 5 clusters. Overall, air masses arriving to Istanbul at 500m are equally distributed into northern (52%) and southern (48%). Frequency analysis of PM10 concentrations with mean air mass backward trajectories showed that PM10 from local anthropogenic sources may be enhanced by long-range transport from the African Desert, Asian Desert, Arabian Peninsula, Russia, and Ukraine. The work presented here provides the first integrated assessment for evaluation of occurrence and quantification of the effect of dust transport to ground-level PM10 concentrations in Istanbul, which is helpful for human health prevention and implementation of air quality control measures.

Desert dust hazards: A global review

Dust storms originate in many of the world’s drylands and frequently present hazards to human society, both within the drylands themselves but also outside drylands due to long-range transport of aeolian sediments. Major sources of desert dust include the Sahara, the Middle East, central and eastern Asia, and parts of Australia, but dust-raising occurs all across the global drylands and, on occasion, beyond. Dust storms occur throughout the year and they vary in frequency and intensity over a number of timescales. Long-range transport of desert dust typically takes place along seasonal transport paths. Desert dust hazards are here reviewed according to the three phases of the wind erosion system: where dust is entrained, during the transport phase, and on deposition. This paper presents a synthesis of these hazards. It draws on empirical examples in physical geography, medical geology and geomorphology to discuss case studies from all over the world and in various fields. These include accelerated soil erosion in agricultural zones – where dust storms represent a severe form of accelerated soil erosion – the health effects of air pollution caused by desert aerosols via their physical, chemical and biological properties, transport accidents caused by poor visibility during desert dust events, and impacts on electricity generation and distribution. Given the importance of desert dust as a hazard to human societies, it is surprising to note that there have been relatively few attempts to assess their impact in economic terms. Existing studies in this regard are also reviewed, but the wide range of impacts discussed in this paper indicates that desert dust storms deserve more attention in this respect.

Variations in dust-related PM10 emission from an arid land due to surface composition and topsoil disturbance

Aeolian (wind) erosion is most common in arid regions. The resulted emission of PM10 (particulate matter that is smaller than 10 μm in diameter) from the soil has many environmental and socioeconomic consequences such as soil degradation and air pollution. Topsoil resistance to aeolian transport highly depends on the surface composition. The study aim was to examine variations in PM10 fluxes in a desert-dust source due to surface composition and topsoil disturbance. Aeolian field experiments using a boundary layer wind tunnel alongside soil composition analysis were integrated in this study. The results show variations in PM10 fluxes (ranging from 9.5 to 524.6 mg m−2 min−1) in the studied area. Higher wind velocity increased significantly the PM10 fluxes in all surface compositions. A short-term natural disturbance caused changes in the aggregate soil distribution (ASD) and increased significantly PM10 emissions. Considering that PM10 contains clays, organic matter, and absorbed elements, the recorded PM10 fluxes are indicative of the potential soil loss and degradation by wind erosion in such resource-limited ecosystems. The findings have implications in modeling dust emission from a source area with complex surfaces.