Coplanar Grid CdZnTe Detectors Research Articles

Design and study of a coplanar grid array CdZnTe detector for improved spatial resolution

Coplanar grid (CPG) CdZnTe detectors have been used as gamma-ray spectrometers for years. Comparing with pixelated CdZnTe detectors, CPG CdZnTe detectors have either no or poor spatial resolution, which directly limits its use in imaging applications. To address the issue, a 2×2 CPG array CdZnTe detector with dimensions of 7×7×5mm3 was fabricated. Each of the CPG pairs in the detector was moderately shrunk in size and precisely designed to improve the spatial resolution while maintaining good energy resolution, considering the charge loss at the surface between the strips of each CPG pairs. Preliminary measurements were demonstrated at an energy resolution of 2.7–3.9% for the four CPG pairs using 662keV gamma rays and with a spatial resolution of 3.3mm, which is the best spatial resolution ever achieved for CPG CdZnTe detectors. The results reveal that the CPG CdZnTe detector can also be applied to imaging applications at a substantially higher spatial resolution.

Pulse-shape discrimination of surface events in CdZnTe detectors for the COBRA experiment

Events near the cathode and anode surfaces of a coplanar grid CdZnTe detector are identifiable by means of the interaction depth information encoded in the signal amplitudes. However, the amplitudes cannot be used to identify events near the lateral surfaces. In this paper a method is described to identify lateral surface events by means of their pulse shapes. Such identification allows for discrimination of surface alpha particle interactions from more penetrating forms of radiation, which is particularly important for rare event searches. The effectiveness of the presented technique in suppressing backgrounds due to alpha contamination in the search for neutrinoless double beta decay with the COBRA experiment is demonstrated.

Analytical model for event reconstruction in coplanar grid CdZnTe detectors

Coplanar-grid (CPG) particle detectors were designed for materials such as CdZnTe (CZT) in which charge carriers of only one sign have acceptable transport properties. The presence of two independent anode signals allows for a reconstruction of deposited energy based on the difference between the two signals, and a reconstruction of the interaction depth based on the ratio of the amplitudes of the sum and difference of the signals. Energy resolution is greatly improved by modifying the difference signal with an empirically determined weighting factor to correct for the effects of electron trapping. This paper introduces a modified interaction depth reconstruction formula which corrects for electron trapping utilizing the same weighting factor used for energy reconstruction. The improvement of this depth reconstruction over simpler formulas is demonstrated. Further corrections due to the contribution of hole transport to the signals are discussed.

Performance of a Large Volume 20<formula formulatype="inline"> <tex Notation="TeX">$\times$</tex></formula>20<formula formulatype="inline"><tex Notation="TeX">$\times$</tex> </formula>15 mm<formula formulatype="inline"><tex Notation="TeX">$^{3}$</tex></formula> CPG Detector

Large-volume CdZnTe (CZT) single crystals with electron lifetimes exceeding 10 μs recently became available commercially for making large effective area gamma-ray arrays. However, significant variations were observed in the performance of detectors made from such arrays. We evaluated the spectroscopic performance of such a large-volume, 20 × 20 × 15 mm3, coplanar-grid (CPG) CdZnTe detector, intended for use in a handheld radioisotope-identifier, which unexpectedly showed a poor spectral performance with an energy resolution of 3.5-4% FWHM measured with 662-keV gamma-rays. To understand the factors affecting its performance, we applied several characterization techniques, viz., white X-ray diffraction topography measurements, IR microscopy, and micron-spatial resolution X-ray mapping. They allowed us to identify major crystal defects in the device that limit its energy resolution and detection efficiency.

Synchrotron radiation studies of spectral response features caused by Te inclusions in a large volume coplanar grid CdZnTe detector

We report preliminary results from a synchrotron radiation study of Te inclusions in a large volume single crystal CdZnTe (CZT) coplanar-grid detector. The experiment was carried out by probing individual inclusions with highly collimated monochromatic X- and γ-ray beams. It was found that for shallow X-ray interaction depths, the effect of an inclusion on measured energy loss spectra is to introduce a ∼10% shift in the peak centroid energy towards lower channel numbers. The total efficiency is however not affected, showing that the net result of inclusions is a reduction in the Charge Collection Efficiency (CCE). For deeper interaction depths, the energy-loss spectra shows the emergence of two distinct peaks, both downshifted in channel number. We note that the observed spectral behaviour shows strong similarities with that reported in semiconductors, which exhibit polarization effects, suggesting that the underlying mechanism is common.

True coincidence-summing corrections for the coincident γ-rays measured with coplanar grid CdZnTe detectors

In this study, true coincidence-summing (TCS) correction factors have been measured for the sources (22)Na, (60)Co, (133)Ba and (152)Eu by use of three large volume coplanar grid CdZnTe (acronym: CZT) detectors. In case of a close-in detection geometry, two different TCS calculation algorithms were used to compute the required TCS correction factors. Both of the algorithms are based on the measured total-to-peak (TTP) ratio and full-energy peak (FEP) efficiency values that were obtained using almost "single" energy and coincidence-free nuclides. The results for TCS correction factors obtained by two different algorithms were agreeable to each other. The obtained TCS factors were ranged from about 7% to 30.5% in a 2250 mm(3) CZT detector when a close counting geometry was used. For other two detectors with a volume of 1000 and 1687.5mm(3), the resulted TCS correction factors were relatively smaller and varied between about 0.1% and 20% at the close counting geometry condition. Therefore, the results indicate that there is a need for the estimation of TCS corrections in CZT detectors, especially when their crystal volumes are greater than 1cm(3) and these detectors are used in the case of a close-in detection geometry.

Detecting multi-hit events in a CdZnTe coplanar grid detector using pulse shape analysis: A method for improving background rejection in the COBRA [formula omitted] experiment

A number of experiments are underway to search for a rare form of radioactivity, neutrinoless double beta decay, as a measurement of the half-life would enable the neutrino mass to be determined. The COBRA collaboration [1,2] (Zuber, 2001; Dawson, 2009) employs CdZnTe detectors in such a search. This paper describes techniques using pulse shape analysis for identifying two-centre events in a coplanar grid CdZnTe detector. This enables Compton scatter events to be identified and so suppressing the background present within the COBRA detectors.

Evaluation of CdZnTe as neutron detector around medical accelerators

The operation of electron linear accelerators (LINACs) and cyclotrons can produce a mixed gamma-neutron field composed of energetic neutrons coming directly from the source and scattered lower energy neutrons. The thermal neutron detection properties of a non-moderated coplanar-grid CdZnTe (CZT) gamma-ray detector close to an 18 MV electron LINAC and an 18 MeV proton cyclotron producing the radioisotope (18)F for positron emission tomography are investigated. The two accelerators are operated at conditions producing similar thermal neutron fluence rates of the order of 10(4) cm(-2) s(-1) at the measurement locations. The counting efficiency of the CZT detector using the prompt 558 keV photopeak following (113)Cd thermal neutron capture is evaluated and a good neutron detection performance is found at the two installations.

Feasibility and design of a solid state gamma-ray detector

For conventional radiation detectors fabricated from compound semi-conductors, the wide disparity between the transport properties of the electron and holes, means that detector performances are limited by the carrier with the poorest mobility-lifetime product (μτ). Finite drift lengths introduce an energy dependent depth term into the charge collection process, which effectively limit maximum detection volume to tens of mm3 – entirely unsuitable for the detection of gamma-rays. The recent introduction of the coplanar-grid charge-sensing techniques has overcome this problem by essentially discarding the carrier with the poorest transport properties, thus permitting high spectral resolution and high detection efficiency. For example, energy resolutions of 2% full-width half-maximum at 662 keV have been demonstrated with coplanar-grid CdZnTe detectors of volumes up to 2 cm3. Further improvements in detector performance and yield are being pursued through refinements in electrode design and material quality. Because coplanar-grid CdZnTe detectors can operate at room temperature, they are ideally suited for applications requiring portability, small size, or low power consumption such as planetary space missions. Other potential applications include well logging, medical diagnostics, and gamma-ray astronomy. We discuss the feasibility and design of a solid state gamma-ray detector based on CdZnTe and compare its performance to a large volume Ge detector. As will be shown, a significant improvement can be made if T1Br is used as the detection medium.

Performance Comparison of a Large Volume CZT Semiconductor Detector and a LaBr$_3$(Ce) Scintillator Detector

The development of portable nuclear instrumentation demands compact high sensitivity detectors operated at room temperature. The sensitivity of these detectors mainly depends on two parameters: absolute efficiency and energy resolution. In order to provide high efficiency, large volumes are needed. For semiconductor detectors able to operate at room temperature, the largest effective volumes with acceptable resolution are achieved with CdZnTe coplanar-grid and pixel detectors. On the other hand, new scintillation materials were recently developed with spectrometric capabilities only reachable some years ago with semiconductors. In this work we compare the performance of two state of the art detectors of different technologies with a relative large volume: a coplanar-grid CdZnTe detector with dimensions 15 mmtimes15 mmtimes10 mm and a LaBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> (Ce) crystal with volume 18 mmtimes18 mmtimes30 mm. The CdZnTe crystal was made by Yinnel Tech (USA) and the detector was manufactured by BSI (Latvia). The LaBr <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</sub> (Ce) scintillator was grown and encapsulated by Saint-Gobain (France). The energy resolution for the CZT detector is 2.05% FWHM at 662 keV. The resolution for the scintillator at this energy was near 3%. The total efficiency was studied in a setup with calibrated point sources. The experimental spectra were compared with Monte-Carlo simulations performed with Geant4. The implications of the results of this comparison are discussed in the context of the practical use of these units

Hard X- and γ-ray measurements with a large volume coplanar grid CdZnTe detector

The recent introduction of coplanar grid techniques has led to resurgence in interest in developing large volume compound semiconductor detectors that have a reasonable γ-ray response but also good spectroscopic resolution. We report the results of a series of hard X- and γ-ray measurements on a large 15×15 mm2, 10 mm thick CdZnTe coplanar grid detector. The measurements were carried out at the HASYLAB and ESRF synchrotron radiation facilities using highly monochromatic pencil beams across the energy range 20–800 keV. Additional full-area measurements were carried out using radioactive sources. All measurements were carried out at room temperature. The measured energy resolution under full-area illumination was 8 and 12 keV FWHM at 59.95 and 662 keV, respectively. Under pencil beam illumination, the measured resolutions were essentially the same. The detector energy response function was found to be linear over the energy range 20–1400 keV with an average rms nonlinearity of 1.4%, consistent with statistics. The spatial uniformity of the detector was evaluated at 30, 60 and 180 keV by raster scanning a 20×20 μm2 monoenergetic X-ray beam across the active area. Apart from a few localized areas, the detector response was found to uniform at the few percent level, consistent with statistics. At 180 keV, the nonuniformity in the energy response due to the grids was estimated to be at the 0.7% level.

Synchrotron radiation response characterization of coplanar grid CZT detectors

Commercial 15/spl times/15/spl times/7.5 mm/sup 3/ coplanar grid CdZnTe detectors were studied on the micron-scale using a collimated high-energy X-ray beam provided by Brookhaven's National Synchrotron Light Source. This powerful tool enables simultaneous studies of detector response uniformity, electronic properties of the material, and effects related to the device's contact pattern and electric field distribution. The availability of a front-end Application Specific Integrated Circuit, developed at Brookhaven's Instrumentation Division, providing low noise amplification of grids and cathode signals, corresponding timing signal and adjustable relative gain, allowed to correlate performance mapping and fluctuations in collected charge. We observed the effect of the strip contacts comprising the coplanar grids on the energy resolution of the coplanar-grid device.

Investigation of the asymmetric characteristics and temperature effects of CdZnTe detectors

The results of our newest depth sensing coplanar grid CdZnTe detectors will be discussed. These detectors, which utilize the third-generation coplanar anode design, were fabricated by Baltic Scientific Instruments, Ltd., using crystals acquired from Yinnel Tech, Inc., having dimensions of 1.5 cm /spl times/1.5cm/spl times/ 0.9 cm and 1.5 cm /spl times/ 1.5cm /spl times/ 0.95 cm. Employing various compensation techniques, an energy resolution of about 1.7% full width at half maximum (FWHM) was achieved for 662-keV gamma rays. We observed that the spectral performance was highly dependent upon the biasing orientation of the detector. The /spl mu//sub e//spl tau//sub e/ product for one of the crystals was measured and it was found to be a high value of 1.13 /spl times/ 10/sup -2/ cm/sup 2//V. A study of the spectroscopic performance of CdZnTe for reduced temperature operation was implemented and we observed degraded performance for temperatures below 0/spl deg/C and a complete loss of spectral information at -30/spl deg/C.

Characteristics of depth-sensing coplanar grid CdZnTe detectors

The latest depth-sensing coplanar grid CdZnTe detectors have been tested. Two of these have dimensions 1.5×1.5×1.0 cm 3 and one is a cylindrical detector with 1.5 cm diameter and 1.0 cm length, all of them using the third-generation coplanar anode design. Energy resolutions of 2.0% and 2.4% FWHM at 662 keV γ-ray energies were obtained. Detector performance has been observed experimentally as a function of depth of the γ-ray interaction, and as a function of radial position near the anode surface. The measured results show the improvement of the third-generation anode design. Material uniformity of CdZnTe crystals manufactured by eV Products have been directly observed and compared on two 1.5×1.5×1.0 cm 3 detectors.

Recent developments in semiconductor gamma-ray detectors

The successful development of lithium-drifted Ge detectors in the 1960s marked the beginning of the significant use of semiconductor crystals for direct detection and spectroscopy of gamma-rays. In the 1970s, high-purity Ge became available, which enabled the production of complex detectors and multi-detector systems. In the following decades, the technology of semiconductor gamma-ray detectors continued to advance, with significant developments not only in Ge detectors but also in Si detectors and room-temperature compound-semiconductor detectors. In recent years, our group at Lawrence Berkeley National Laboratory has developed a variety of gamma-ray detectors based on these semiconductor materials. Examples include Ge strip detectors, lithium-drifted Si strip detectors, and coplanar-grid CdZnTe detectors. These advances provide new capabilities in the measurement of gamma-rays, such as the ability to perform imaging and the realization of highly compact spectroscopy systems.

Factors affecting energy resolution of coplanar-grid CdZnTe detectors

Coplanar-grid CdZnTe detectors have been under development for the past 10 years as room-temperature gamma-ray spectrometers, and they are being produced for use in a number of applications. Despite the improvements in detector active volume and spectral response that have been achieved with the coplanar-grid technique, the full potential of such detectors is still far from being realized. There exist a number of material, device, and electronics factors that limit detector performance and yield. Some of the major factors are identified and examined in terms of their origins and the magnitude of their effects on energy resolution.

Effect of differential bias on the transport of electrons in coplanar grid CdZnTe detectors

Segmented and pixilated electrode structures are used to compensate for poor hole transport in CdZnTe devices used for gamma-ray spectrometry and imaging. Efforts to model these structures have focused primarily on geometric effects; however, device performance also depends on the physical properties of the bulk and surface material, as well as the electrodes. In this paper, we describe experiments to characterize the electric field near the anode of a coplanar grid detector. The experiment is contrasted with a calculation that is based on an assumption commonly used to reduce the computational effort required to determine internal electric fields. Explanations for differences between the calculation and the experiment are proposed.

Simultaneous ballistic deficit immunity and resilience to parallel noise sources: A new pulse shaping technique

A new and different time-variant pulse processing system has been developed based on a simple CR-RC filter and two analog switches. The new pulse processing technique combines both ballistic deficit immunity and resilience to parallel noise without a significant compromise to the low energy resolution, generally considered a mutually exclusive requirement. The filter is realized by combining two different pulse shaping techniques. One of the techniques creates a low rate of curvature at the pulse peak, which reduces ballistic deficit, while the second technique increases the tolerance to low-frequency noise by modifying the noise history. Several experimental measurements are presented, including tests on a coplanar grid CdZnTe detector. Improvements on both the resolution and line shape are shown for the 662 keV line of /sup 137/Cs.

Multi-element, large-volume CdZnTe detectors

Many applications using gamma rays, such as the determination of the elemental composition of planetary bodies, require the detection of gamma rays in the energy range 100 keV–10 MeV in a light, compact, room-temperature system. The photopeak efficiency of a single CdZnTe detector is limited because the volume currently available is limited to about 3.4 cm 3. To achieve adequate efficiency, we have combined the signals from several large-volume, coplanar-grid CdZnTe detectors. At low energy, the signals are summed without requiring coincidence; at high energy, multi-fold coincidence is required to suppress the Compton continuum. To minimize noise, a signal from a single detector is only included in the sum if it exceeds a threshold set just above the noise. We describe the electronics, the single detectors, their packaging in thin-walled boxes, and the resulting spectra. The energy resolution for the combined spectrum is only slightly worse than the resolution of the single detectors. The effectiveness of the Compton suppression depends on the spectrum. The photopeak efficiency of the multi-element detector when the signals are summed without requiring coincidence is approximately the sum of the photopeak efficiencies of the single detectors, whereas the photopeak efficiency with Compton suppression is a more complicated function of the incident gamma-ray energy. These results indicate that a 27-element (3×3×3) array of 15 mm×15 mm×15 mm single detector elements can provide good gamma-ray data for planetary bodies and terrestrial applications requiring high-efficiency, good-resolution portable instruments.

Coplanar-grid CdZnTe detector with three-dimensional position sensitivity

A three-dimensional position-sensitive coplanar-grid detector design for use with compound semiconductors is described. This detector design maintains the advantage of a coplanar-grid detector in which good energy resolution can be obtained from materials with poor charge transport. Position readout in two dimensions is accomplished using proximity-sensing electrodes adjacent to the electron-collecting grid electrode of the detector. Additionally, depth information is obtained by taking the ratio of the amplitudes of the collecting grid signal and the cathode signal. Experimental results from a prototype CdZnTe detector are presented.