Continuous-wave Terahertz Source Research Articles

Parasitic mixing in photomixers as continuous wave terahertz sources

We present observations of parasitic frequency components in the emission spectrum of typical photomixer sources for continuous wave (CW) terahertz generation. Broadband tunable photomixer systems are often used in combination with direct power detectors, e.g., for source and/or detector characterization. Here, spectral components besides the intended terahertz emission at the difference frequency of the two excitation lasers can significantly distort the measurement results. In this work, the appearance of parasitic mixing signals is observed in broadband measurements with a broadband antenna-coupled field-effect transistor as terahertz detector (TeraFET). The measurements reveal weaker spectral absorption features than expected and also a signal plateau towards higher frequencies, both strongly indicating a background in the detection signals. The photomixer emission is investigated in detail with a terahertz Fourier-transform infrared spectrometer (FTIR). We relate the observed parasitic frequency components with good quantitative agreement with the mode spectra of the semiconductor lasers. We also present one possible approach to overcome some of the issues, and we emphasize the importance of our findings to avoid distorted measurement results. To our knowledge, the essential aspect of parasitic mixing has so far been largely ignored in the literature where terahertz CW photomixer emitters are widely used for spectrally resolved measurements.

Full-Field Super-Resolution Terahertz Imaging Based on Rotating Coherent Scattering Microscopy

For decades, terahertz (THz) microscopic imaging has been limited by the resolution of the system due to the larger wavelength, the power of the source, and the equivalent noise power of the detector, so a lot of research has focused on single-point scanning imaging. With the development of hardware, full-field THz imaging based on high-power continuous-wave THz sources have been developed such as the direct intensity imaging method and lensless coherent imaging. In particular, the THz direct intensity imaging method requires no complicated computational reconstruction, while the high resolution, as a key issue, still needs to be improved. In this paper, the rotating coherent scattering microscopy was applied to THz imaging for the first time. Here, we designed and fabricated a hemisphere lens with high-resistance silicon. The tilted hemisphere lens transformed the incident divergent beam into a plane wave, and the total internal reflection occurred in the planar surface within the hemispherical lens, and generated evanescent waves in the rare medium. At the same time, the sample was placed very close to the plane of the hemispherical lens, so that the sample was illuminated by the evanescent waves. The scattered waves carried high frequency information to the far field, and thus through an objective, the super-resolution imaging was achieved along a single direction. Then, the hemispherical lens was rotated to obtain coherent scattering microscopic images under different evanescent wave illumination angles. Finally, the full-field super-resolution imaging results were obtained through incoherent superposition.

Lensless Fourier-transform terahertz digital holography for real-time full-field phase imaging

With the development of continuous-wave terahertz (THz) sources and array detectors, the pursuit of high-fidelity real-time imaging is receiving significant attention within the THz community. Here, we report a real-time full-field THz phase imaging approach based on lensless Fourier-transform THz digital holography. A triangular interferometric layout is proposed based on an oblique illumination of 2.52 THz radiation, which is different from other lensless holographic configurations at other frequencies. A spherical reference beam is generated by a reflective parabolic mirror with minor propagation loss. The complex-valued images are reconstructed using a single inverse Fourier transform of the hologram without complex calculation of the diffraction propagation. The experimental result for a Siemens star validates the lateral resolution of ∼ 346 μm in the diagonal direction. Sub-pixel image registration and image stitching algorithms are applied to enlarge the area of the reconstructed images. The dehydration process of an aquatic plant leaf (Hottonia inflata) is monitored for the first time, to the best of our knowledge, at the THz band. Rapid variations in water content and morphology are measured with a time interval of 0.6 s and a total time of 5 min from a series of reconstructed amplitude and phase images, respectively. The proposed method has the potential to become a powerful tool to investigate spontaneous phenomena at the THz band.

Review of photomixing continuous-wave terahertz systems and current application trends in terahertz domain

Within the last two decades, terahertz systems have become a well-established tool in scientific laboratories and industrial research and development departments. Unlike the methods of pulsed terahertz radiation that mainly rely on ultrafast optical technology, the technology behind continuous-wave terahertz sources and detectors has a long history involving many different types of technical schemes. The intent is to provide a brief review of the continuous-wave terahertz systems that are based on photomixing and current application trends in the field of terahertz technology.

Terahertz-based nanometrology: multispectral imaging of nanoparticles and nanoclusters in suspensions

Silica nanoparticles suspended in an organic solvent (nanosuspension) have been imaged and characterized via terahertz nanoscanning reconstructive three-dimension (3D) imaging technique. The size of individual silica nanoparticles in the suspension was quantified. In addition, the presence of nanoclusters along with their distribution in the suspension was visualized in 3D. It has also been qualitatively demonstrated that the volume fraction of solvent is significantly higher than that of the silica nanoparticles; an observation consistent with the composition of the nanosuspension in the present investigation. The measured size range of individual nanoparticles was found to be 10–12 nm, while the manufacturer’s specification indicates a nanoparticle size distribution in the range of 10 to 15 nm. However, a typical nanocluster size was determined to be 17.5 nm, thus indicating the presence of nanoparticles less than 10 nm. The nanometrology instrument used in this investigation was based on a dendrimer dipole excitation-based continuous wave terahertz source generating > 200 mW stable terahertz power.

Highly-efficient THz generation using nonlinear plasmonic metasurfaces

Nonlinear metasurfaces loaded with multi-quantum-well (MQW) heterostructures constitute a rapidly progressing class of optical devices that combine high nonlinear generation efficiency with an ultrathin profile. Here, we introduce and discuss terahertz (THz) difference-frequency generation (DFG) using MQW-based plasmonic metasurfaces and present a comprehensive theory for their rigorous electromagnetic analysis. We explicitly take into account complex phenomena associated with the local intensity saturation of intersubband transitions and identify fundamental upper-bounds for DFG conversion efficiency. Using this framework, we design and analyze a nonlinear DFG metasurface providing giant DFG nonlinear response and conversion efficiency up to 0.01% at 5.8 THz. Such metasurface can be used to generate 0.15 mW of THz power using pump intensities in the kW cm−2 range. We envision that such DFG metasurfaces can become a platform for uncooled, compact, and highly-efficient continuous-wave THz sources.

Terahertz Frequency Metrology for Spectroscopic Applications: a Review

We provide an overview on terahertz (THz) frequency metrology, starting from the nowadays available continuous wave THz sources, discussing their main features such as tunability, spectral purity, and frequency referencing to the primary frequency standards. A comparison on the achieved results in high-precision molecular spectroscopy is given and discussed, and finally, a special emphasis poses on the future developments of this upcoming field.

Low-threshold room-temperature continuous-wave operation of a terahertz difference-frequency quantum cascade laser source

The performance of a room-temperature continuous-wave (CW) terahertz source based on intracavity difference-frequency generation in a mid-infrared (λ ∼ 6.8 µm) quantum cascade laser with a dual-upper-state active region is reported. The fabricated buried heterostructure device, with a two-section buried distributed feedback grating, operates at two mid-infrared wavelengths and demonstrates a terahertz output of 2.92 THz with a very low threshold current density of 0.89 kA/cm2 in pulsed operation. Consequently, despite an epitaxial-side-up mounting configuration, the device achieves CW operation at room temperature in which a low CW threshold current density of 1.3 kA/cm2 is obtained.

Engineering and characterization of a packaged high-Tc superconducting terahertz source module

We present an effective engineering technique for compactly packaging high-Tc superconducting continuous-wave terahertz source modules. A terahertz-emitting device, which consists of stacks of intrinsic Josephson junctions in single crystalline Bi2Sr2CaCu2O, bias electrodes, a collimating lens, and other components, is packaged into a single finger-sized assembly. The rigid and stable structure used for the packaging guarantees physical and chemical stability with good thermal contact, and provides reproducible characteristics with a high yield rate. The coherent terahertz waves can be emitted from the back side of the base crystal without significant screening. The intuitive results obtained from the numerical simulation are consistent with the observed thermal properties. The modules are easy to use, and thus intended for all users unfamiliar with superconducting electronic devices.

Quad band Polarization Insensitive Millimeter Wave Frequency Selective Surface for Remote Sensing

A novel millimeter-wave frequency selective surface (FSS) is presented for demultiplexing four atmospheric remote sensing bands with varying bandwidth (3–20 GHz) and frequency separation (50–195 GHz). The unit cell (670 μm × 670 μm) is a circular metal mesh loaded with a monopole integrated concentric ring on a 175-μm-thick quartz substrate designed to reject 50–60 GHz (B1), 87–91 GHz (B 2), and 148–151 GHz (B3), and transmit 175–195 GHz (B4) for transverse electric (TE) and transverse magnetic (TM) polarizations at oblique incidence (25°−35 °). Transmission response of the cascaded FSS measured using a continuous-wave terahertz source showed insertion loss of 15 dB and higher in the reflection windows (B1, B2, and B3) and less than 0.5 dB in the transmission window (B4) for TE and TM polarizations at 30° incident angle.

Mode analysis and design of 0.3-THz Clinotron**Project supported by the National Natural Science Foundation of China (Grant No. 61231003).

To develop a high-power continuous-wave terahertz source, a Clinotron operating at 0.3 THz is investigated. Based on the analyses of field distribution and coupling impedance, the dispersion characteristic of a rectangular resonator is preliminarily studied. The effective way to select fundamental mode to interact with the electron beam is especially studied. Finally, the structure is optimized by particle-in-cell simulation, and the problems of manufacture tolerance, current density threshold, and heat dissipation during Clinotron’s operation are also discussed. The optimum device can work with a good performance under the conditions of 8 kV and 60 mA. With the generation of signal frequency at 315.89 GHz and output power at 12 W on average, this device shows great prospects in the application of terahertz waves.

A Methodology to Measure Input Power and Effective Area for Characterization of Direct THz Detectors

This paper presents a test setup and measurement methodology for the characterization of direct terahertz (THz) detectors. The detector under test is illuminated by a continuous wave THz source and its voltage response is measured using a lock-in amplifier. A reference detector is used to measure the input power density of the receiver antenna. The calculation of the effective area is done by measuring $E$ and $H$ plane radiation patterns of the receiver antenna. Several measurement techniques are shown in order to achieve a reliable characterization of the detector with different advantages and disadvantages. In addition, a setup modification is done for the removal of the electronically induced background noise due to the coupling of the signals through cables. Based on the measured input power, the performance parameters of an antenna-coupled field-effect transistor (FET)-based THz detector are measured and presented. This measurement methodology can also be used to characterize other direct THz detectors.

Room temperature continuous wave, monolithic tunable THz sources based on highly efficient mid-infrared quantum cascade lasers.

A compact, high power, room temperature continuous wave terahertz source emitting in a wide frequency range (ν ~ 1–5 THz) is of great importance to terahertz system development for applications in spectroscopy, communication, sensing, and imaging. Here, we present a strong-coupled strain-balanced quantum cascade laser design for efficient THz generation based on intracavity difference frequency generation. Room temperature continuous wave emission at 3.41 THz with a side-mode suppression ratio of 30 dB and output power up to 14 μW is achieved with a wall-plug efficiency about one order of magnitude higher than previous demonstrations. With this highly efficient design, continuous wave, single mode THz emissions with a wide frequency tuning range of 2.06–4.35 THz and an output power up to 4.2 μW are demonstrated at room temperature from two monolithic three-section sampled grating distributed feedback-distributed Bragg reflector lasers.

Real-Time Determination of Absolute Frequency in Continuous-Wave Terahertz Radiation with a Photocarrier Terahertz Frequency Comb Induced by an Unstabilized Femtosecond Laser

A practical method for the absolute frequency measurement of continuous-wave terahertz (CW-THz) radiation uses a photocarrier terahertz frequency comb (PC-THz comb) because of its ability to realize real-time, precise measurement without the need for cryogenic cooling. However, the requirement for precise stabilization of the repetition frequency (f rep) and/or use of dual femtosecond lasers hinders its practical use. In this article, based on the fact that an equal interval between PC-THz comb modes is always maintained regardless of the fluctuation in f rep, the PC-THz comb induced by an unstabilized laser was used to determine the absolute frequency f THz of CW-THz radiation. Using an f rep-free-running PC-THz comb, the f THz of the frequency-fixed or frequency-fluctuated active frequency multiplier chain CW-THz source was determined at a measurement rate of 10 Hz with a relative accuracy of 8.2 × 10−13 and a relative precision of 8.8 × 10−12 to a rubidium frequency standard. Furthermore, f THz was correctly determined even when fluctuating over a range of 20 GHz. The proposed method enables the use of any commercial femtosecond laser for the absolute frequency measurement of CW-THz radiation.

Terahertz Sub-Nanometer Sub-Surface Imaging of 2D Materials

Terahertz sub-surface imaging offers an effective solution for surface and 3D imaging because of minimal sample preparation requirements and its ability to “see” below the surface. Another important property is the ability to inspect on a layer-by layer basis via a non-contact route, non-destructive route. Terahertz 3D imager designed at Applied Research and Photonics (Harrisburg, PA) has been used to demonstrate reconstructive imaging with a resolution of less than a nanometer. Gridding with inverse distance to power equations has been described for 3D image formation. A continuous wave terahertz source derived from dendrimer dipole excitation has been used for reflection mode scanning in the three orthogonal directions. Both 2D and 3D images are generated for the analysis of silver iodide quantum dots’ size parameter. Layer by layer image analysis has been outlined. Graphical analysis was used for particle size and layer thickness determinations. The demonstrated results of quantum dot particle size checks well with those determined by TEM micrograph and powder X-ray diffraction analysis. The reported non-contact measurement system is expected to be useful for characterizing 2D and 3D naomaterials as well as for process development and/or quality inspection at the production line.

Frequency-tunable continuous-wave terahertz sources based on GaAs plasmonic photomixers

We present frequency-tunable, continuous-wave terahertz sources based on GaAs plasmonic photomixers, which offer high terahertz radiation power levels at 50% radiation duty cycle. The use of plasmonic contact electrodes enhances photomixer quantum efficiency while maintaining its ultrafast operation by concentrating a large number of photocarriers in close proximity to the device contact electrodes. Additionally, the relatively high thermal conductivity and high resistivity of GaAs allow operation under high optical pump power levels and long duty cycles without reaching the thermal breakdown limit of the photomixer. We experimentally demonstrate continuous-wave terahertz radiation with a radiation frequency tuning range of more than 2 THz and a record-high radiation power of 17 μW at 1 THz through plasmonic photomixers fabricated on a low temperature grown GaAs substrate at 50% radiation duty cycle.

Area dependence and influence of crystal inhomogeneity on superconducting properties of Bi2212 mesa structures

The rapid increase in applications of terahertz waves requires new techniques to obtain continuous wave terahertz sources. Mesa structures fabricated from high-Tc superconductor Bi2Sr2CaCu2O8+δ (Bi2212) single crystal have been observed as an intense, coherent, continuous electromagnetic wave source in the terahertz (THz) frequency region. However, in order to produce coherent radiation with high applicable power, we need large mesa structures that enter a collective electromagnetic state in which their oscillations are largely synchronized in phase. On the other hand, large mesa structures cause a heating problem. In this study, we report on the critical current density dependence of mesa area and the crystal inhomogeneity to understand heating problems in large area mesas for terahertz radiation. Since the doping dependence of Bi2212 is an important parameter, the as-grown Bi2212 crystals were heat-treated at various temperatures under vacuum conditions. We have fabricated triple mesa structures from Bi2212 single crystal using e-beam lithography and argon ion beam etching techniques with same area and with different area on the same chip. We investigated and compared characteristics of triple mesas which are on the same chip and next to each other. In this way, we searched the crystal inhomogeneity in triple mesa structures and studied the critical current density dependence of mesa area to obtain high emission power for the THz radiation. Our experimental results clearly show that the Josephson critical current density is decreasing when the area of mesa is increasing.

Real-time absolute frequency measurement of continuous-wave terahertz radiation based on dual terahertz combs of photocarriers with different frequency spacings.

Real-time measurement of the absolute frequency of continuous-wave terahertz (CW-THz) radiation is required for characterization and frequency calibration of practical CW-THz sources. We proposed a method for real-time monitoring of the absolute frequency of CW-THz radiation involving temporally parallel, i.e., simultaneous, measurement of two pairs of beat frequencies and laser repetition frequencies based on dual THz combs of photocarriers (PC-THz combs) with different frequency spacings. To demonstrate the method, THz-comb-referenced spectrum analyzers were constructed with a dual configuration based on dual femtosecond lasers. Regardless of the presence or absence of frequency control in the PC-THz combs, a frequency precision of 10(-11) was achieved at a measurement rate of 100 Hz. Furthermore, large fluctuation of the CW-THz frequencies, crossing several modes of the PC-THz combs, was correctly monitored in real time. The proposed method will be a powerful tool for the research and development of practical CW-THz sources, and other applications.

High-resolution reconstruction for terahertz imaging.

We present a high-resolution (HR) reconstruction model and algorithms for terahertz imaging, taking advantage of super-resolution methodology and algorithms. The algorithms used include projection onto a convex sets approach, iterative backprojection approach, Lucy-Richardson iteration, and 2D wavelet decomposition reconstruction. Using the first two HR reconstruction methods, we successfully obtain HR terahertz images with improved definition and lower noise from four low-resolution (LR) 22×24 terahertz images taken from our homemade THz-TDS system at the same experimental conditions with 1.0mm pixel. Using the last two HR reconstruction methods, we transform one relatively LR terahertz image to a HR terahertz image with decreased noise. This indicates potential application of HR reconstruction methods in terahertz imaging with pulsed and continuous wave terahertz sources.

Calorimetric measurement of absolute terahertz power at the sub-microwatt level

We developed a calorimeter for determining absolute terahertz (THz) power. The calorimeter is based on a DC substitution method using an isothermal temperature-control technique. A neutral-density optical filter glass was used as a volume absorber, and its THz absorption was evaluated by a time-domain spectrometer. Highly sensitive measurement of the absolute THz power was experimentally achieved in the range from the submicrowatt to microwatt level at room temperature. Power measurement of a continuous-wave THz source using a photomixer was demonstrated. This calorimeter is expected to demonstrate the traceability of THz power at a submicrowatt level.