Continuous-wave Laser Operation Research Articles

Diode-Pumped Tunable Continuous Wave Laser Operation In Yb: NaY(WO4)2 Crystal

Diode-Pumped Tunable Continuous Wave Laser Operation In Yb: NaY(WO4)2 Crystal

Growth, spectroscopy properties, and laser operation of single crystal fiber: Nd3+-doped CNGG

Nd3+-doped calcium niobium gallium garnet single crystal fibers (Nd:CNGG SCFs) with varying Nd3+ concentrations were successfully grown using the laser-heated pedestal growth (LHPG) method. The study thoroughly examines the fundamental physical structure, optical properties, and laser characteristics of the as-grown Nd:CNGG SCFs. Results indicate that the Nd:CNGG SCF exhibits broader absorption and emission full width at half maximum (FWHM) compared to bulk single crystals. Moreover, pumped by a commercial 808 nm laser diode, continuous-wave laser operation at 1061 nm with a half-height width of 1.86 nm was achieved. The laser output power reached 1.04 W at an absorbed power of 7.46 W, with a slope efficiency of 25.4% relative to the absorbed pump power. These findings suggest that Nd:CNGG SCF holds promise as a practical and potent candidate for laser gain medium, offering significant research potential in the field of lasers.

Broadly tunable continuous-wave Tm,Ho:SrF2 and Tm,Ho:BaF2 lasers

We report on the first, to our knowledge, room-temperature continuous-wave laser operation of Tm3+,Ho3+-codoped barium and strontium fluoride crystals at ∼2.1 µm. The 3 at.% Tm, 0.5 at.% Ho:BaF2 laser generated 160 mW at 2073 nm with a slope efficiency of 31.0% and a laser threshold of 43 mW. The continuous wavelength tuning of this laser from 2010 to 2090 nm (tuning range, 80 nm) was demonstrated. The spectroscopic properties of Tm,Ho:SrF2 and Tm,Ho:BaF2 crystals were also determined, showing enhanced Tm3+ → Ho3+ energy transfer in rare-earth clusters. For Ho3+ ions in BaF2, the stimulated-emission cross section is 0.40 × 10−20 cm2 at 2044 nm, and the thermal equilibrium luminescence lifetime is as long as 14.1 ms.

Growth, Spectroscopic Characterization and Continuous-Wave Laser Operation of Er,Yb:GdMgB5O10Crystal

A transparent Er3+,Yb3+:GdMgB5O10 single crystal with dimensions up to 24 × 15 × 12 mm was grown successfully by the high-temperature solution growth on dipped seeds technique from K2Mo3O10-based solvent. The grown crystal was characterized using PXRD, DSC and ATR techniques. Differential scanning calorimetry measurements and SEM analysis of the heat-treated solids revealed Er,Yb:GdMgB5O10 to be an incongruent melting compound with an onset point of 1087 °C. The absorption edge of the Er,Yb:GMBO sample is located in the region of 245 nm, which approximates a value of 4.8 eV. Absorption and emission spectra, and luminescence kinetics, were studied. The energy transfer efficiency from ytterbium to erbium ions was determined. The laser operation in continuous-wave mode was realized and output characteristics were measured. The maximal output power of 0.15 W with a slope efficiency of 11% was obtained at 1568 nm.

Polarized, broadly tunable, 2.3 µm continuous-wave laser operation of Tm3+-vanadate crystals.

We report for the first time the polarized, broadly tunable, continuous-wave laser operation on the 3H4 → 3H5 transition in Tm3+-vanadate (Tm:REVO4, RE = Gd, Y, Lu) crystals. Continuous wavelength tunings with tuning widths of about 200 nm were achieved in π-polarization for both the Tm:GdVO4 and Tm:YVO4 crystals. To the best of our knowledge, these tuning widths are broader than most previously reported values for wavelength tunable 2.3 µm Tm lasers. Especially for σ-polarization, all the Tm:REVO4 lasers provide very smooth wavelength tuning curves around 2.3 µm. This work demonstrates the excellent broad wavelength tunability of the Tm:REVO4 crystals and their great potential for supporting the generation of ultrashort pulses from mode-locked lasers.

Crystal growth, polarized spectral properties, and 2.3 µm laser performance of Tm:LuVO4 crystal

We report on the Czochralski crystal growth, polarized optical spectroscopy, and the first continuous-wave laser operation of 1.5 at.% Tm:LuVO4 crystal on the 3H4 → 3H5 transition. The polarized absorption and stimulated-emission properties of Tm3+ ions in LuVO4 were revised and the crystal-field splitting of the Tm3+ multiplets was determined by low-temperature (12 K) spectroscopy. The maximum stimulated-emission cross-section for the 3H4 → 3H5 transition is 2.48 × 10−20 cm2 at 2363 nm for π-polarization corresponding to an emission bandwidth of 28 nm. Evidence of phonon-assisted emissions of Tm3+ ions above 2 µm is presented. The broadband emission properties of the Tm:LuVO4 crystal make it promising for ultrashort pulse generation. Additionally, pumped by a 796 nm fiber-coupled laser diode, the Tm:LuVO4 laser generated a Watt-level output power at 2279-2295 nm with a slope efficiency of 9.2% and linearly polarized emission (π-polarization).

Polarized spectral properties and 2.3 µm laser performance of the Tm:YVO4 crystal

The polarized spectral properties and ∼2.3 µm high-power continuous-wave laser operation of Tm3+-doped yttrium orthovanadate crystal (Tm:YVO4) are reported. For the 3H4 → 3H5 transition, the stimulated-emission cross-section σSE is 1.01 × 10−20 cm2 at 2276 nm corresponding to a large emission bandwidth of 52 nm (for π-polarization). Pumped by a 794 nm laser diode, the 1.5 at.% Tm:YVO4 laser delivered 5.52 W at 2.29 µm with a slope efficiency of 19.9%, a laser threshold of 8.70 W, and a linear laser polarization (π). The Tm laser operated on the cascade scheme (on the 3H4 → 3H5 and 3F4 → 3H6 transitions) which was mainly responsible for the observed high laser slope efficiency. We also report on the first passively Q-switched Tm:YVO4 laser at 2.3 µm by employing porous nano-grained cuprous selenide (PNG-Cu2Se) as a saturable absorber. The shortest pulse duration and the highest single pulse energy amounted to 706 ns and 3.65 µJ, respectively, corresponding to a pulse repetition rate of 62.8 kHz.

Growth, Spectroscopy, and Laser Performance of a 2.79 μm Er: YSGG Single Crystal Fibers.

Single crystal fibers combine the great specific surface area of fibers and the single crystal property of the bulk crystal which shows great potential for a high-power laser. For an Er-doped crystal, due to the fluorescence quenching at the 3 μm wavelength, high Er doping is necessary to increase the fluorescent up-conversion for the breaking limitation. However, a high Er doping concentration must lead to high heat accumulation, resulting in poor laser performance. Compared with an Er-doped bulk crystal, Er-doped SCF has the great potential to remove the heat in the crystal, and it is easy to obtain a high power. In this paper, Er: Y3Sc2Ga3O12 (Er: YSGG) single crystals were successfully grown using the micro-pulling-down method (μ-PD). Owing to the stably grown interface, the diameter of the crystal is 2 mm with a length up to 80 mm. Then, the measurements of Laue spots and Er3+ distribution indicated that our crystals have a high quality. Based on the as-prepared Er: YSGG SCF, the continuous-wave (CW) laser operations at 2794 nm were realized. The maximum output was 166 mW with a slope efficiency of up to 10.99%. These results show that Er: YSGG SCF is a suitable material for future high-power 3 μm laser operation.

Relevant parameters for laser surgery of soft tissue

In recent years, the laser has become an important tool in hospitals. Laser surgery in particular has many advantages. However, there is still a lack of the understanding of the influence of the relevant parameters for laser surgery. In order to fill this gap, the parameters pulse frequency, use of an exhaustion system, air cooling, laser power, laser scan speed, laser line energy and waiting time between cuts were analysed by ANOVA using inter-animal variation as a benchmark. The quality of the cuts was quantized by a previously published scoring system. A total of 1710 cuts were performed with a CO2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\ ext {CO}_2$$\\end{document} laser. Of the parameters investigated, laser power and scan speed have the strongest influence. Only the right combination of these two parameters allows good results. Other effects, such as the use of pulsed or continuous wave (CW) laser operation, or air cooling, show a small or negligible influence. By modulating only the laser power and scan speed, an almost perfect cut can be achieved with a CO2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\ ext {CO}_2$$\\end{document} laser, regardless of the external cooling used or the laser pulse duration or repetition rate from CW to nanosecond pulses.

Preparation, spectroscopic, thermal properties, and laser performances of ordered Nd3+: Ca3TaGa2.1Al0.9Si2O14 crystal

Langasite crystals with an ordered structure of space group P321 are well known for their excellent piezoelectric and nonlinear optics performance. In this paper, a novel Nd3+: Ca3TaGa2.1Al0.9Si2O14 (Nd: CTGAS) crystal with an ordered structure of space group P321 was successfully grown using the Czochralski method, which could be used as self-laser photoelastic modulators. The thermal behaviour, polarized spectroscopy, and fluorescence lifetime were characterized in detail, and excellent spectroscopic and laser properties were presented. The full width at half of the maximum (FWHM) of the 0.8 μm absorption band was 23.5 nm for σ-polarized and 15.3 nm for π-polarized. The emission spectra had inhomogeneous broadening; the maximum emission cross-section was 7.50 × 10−20 cm2 at 1065 nm with FWHM of 14.3 nm and 2.35 × 10−20 cm2 at 1346 nm with FWHM of 28.3 nm. The fluorescence lifetime at 1065 nm was 280.8 μs. The diode-pumped continuous-wave (CW) laser operation at 1.06 μm was achieved in Nd: CTGAS crystal, an output power of 1.77 W was obtained at the absorbed pump power of 5.5 W, the slope efficiency was 35.0 %, and the optical conversion efficiency was 32.2 %. A 1.35 μm CW laser operation with a slope efficiency of 12.0 % was realized in z-cut Nd: CTGAS crystal.

Growth, characterization, and efficient laser operation of Czochralski- and micro-pulling-down-grown Yb3+:YScO3 mixed sesquioxides

We report on the growth, spectroscopy and laser operation of Yb3+-doped mixed sesquioxide crystals. Various Yb3+-doped crystals with compositions close to (Y0.5Sc0.5)2O3 have been successfully grown by the Czochralski method and by the micro-pulling down (µ-PD) method. Our spectroscopic investigations reveal broadened stimulated emission and absorption cross-section spectra originating from the structural disorder of the mixed crystals. We find the peak wavelengths to shift by ∼1.6 nm between Y:Sc-ratios of 54:46 and 46:54 and confirm a linear relation of the peak position with the lattice constant of the host composition. In the laser experiments, we obtain highly efficient continuous-wave laser operation under pumping with an optically-pumped semiconductor laser (OPSL) at ∼975 nm, reaching slope efficiencies of up to 89% at optical-to-optical efficiencies exceeding 80% at laser wavelengths between 1037 nm and 1086 nm.

Efficient high-power 2.3 μm continuous-wave laser operation of diffusion-bonded composite YVO4/Tm:GdVO4 crystals

Abstract We reported on an efficient high-power continuous-wave laser operation on the 3H4 → 3H5 transition of Tm3+ ions in a diffusion-bonded composite YVO4/Tm:GdVO4 crystal. Pumped by a laser diode at 794 nm, a maximum output power of 7.5 W was obtained from a YVO4/Tm:GdVO4 laser at 2.29 μm, corresponding to a slope efficiency of 40.3% and exceeding the Stokes limit. To the best of our knowledge, this result represents the maximum power ever achieved from a Tm laser at 2.3 μm.

Kerr-lens mode-locked 49-fs Tm3+:YScO3 single-crystal laser at 2.1 µm.

We report on a continuous wave (CW) and Kerr-lens mode-locked (KLM) Tm3+:YScO3 single-crystal laser centered at 2.1 µm. Efficient CW laser operation with a maximum slope efficiency of 51% was achieved under in-band pumping by an Er:Yb fiber master oscillator power amplifier (MOPA). In KLM operation, pulses as short as 49 fs corresponding to seven optical cycles were achieved at a repetition rate of 96.7 MHz with an average output power of 126 mW. Such short pulse durations are enabled by the inhomogeneously broadened emission spectrum of Tm3+:YScO3 extending to above 2200 nm.

Evidence of Yb3+ band broadening and continuous wave laser operation in bismuth modified KY1-x-yBixYby(WO4)2 mixed single crystals

To increase the Yb3+ optical bandwidths in highly anisotropic β:KY(WO4)2 (KYW) type laser single crystals, the simultaneous contributions of the Bi3+ 6 s2 lone electron pair and Y3+/Bi3+ ionic radii mismatch is proposed. The top seeded solution growth method with K2W2O7 as solvent was used to grow Yb doped single crystals of the KY(WO4)2/KBi(WO4)2 (KYBiW) solid solution. Crystals obtained across the used KY1xBixW solid solution range show always the low temperature β phase, with the monoclinic C2/c crystalline structure, but important differences between the Y/Bi composition of the starting solute and that of the crystal grown are found. The incorporation of Y and Yb into the crystal is preferential, resulting in a low Bi segregation coefficient, SBi= 13%, on the KYW side but near SBi= 90% in the KBiW side (Yb is still strongly incorporated filling the remaining 10%). The saturation temperature of the melt decreases as the Bi concentration in the precursor KY1-x-yBixYby(WO4)2/K2W2O7 mixture increases. Evidence of optical absorption and photoluminescence broadening of the Yb3+ bands with Bi3+ incorporation is derived from 6 K and 300 K measurements. Laser operation of KY1-x-yBixYby(WO4)2 crystals is shown to be comparable to that of KY1−yYby(WO4)2 ones. Up to ≈ 0.5 W of output power is obtained pumping in continuous wave regime with a Ti sapphire laser with slope efficiency η ≈ 65% and pump threshold< 200 mW, which is within the usual performance of KYW:Yb crystals, but the spectral distribution of the laser output in KYBiW:Yb crystals is larger than that for KYW:Yb. This spectral broadening may help in the reduction of ultrashort (fs) laser pulse duration generated by modelocking.

UV-laser-diode-pumped visible Tb3+:LiLuF4 lasers.

We investigate the dependence of the visible laser performance of Tb3+:LiLuF3 (Tb:LLF) on the ultraviolet (UV) pumping wavelength and present the first, to the best of our knowledge, UV-laser-diode-pumped Tb3+-based laser. We find an onset of thermal effects already at moderate pump power for UV pump wavelengths with strong excited-state absorption (ESA), which vanishes at pump wavelengths with weak ESA. Pumping with a UV laser diode emitting at 378.5 nm enables continuous wave laser operation in a 3-mm short Tb3+(28 at.%):LLF crystal. Slope efficiencies of 36% at 542/544 nm and 17% at 587 nm are obtained with a minimum laser threshold as low as 4 mW.

Mid-infrared emission properties of erbium-doped fluorite-type crystals

We report on a comparative study of the spectroscopic properties and mid-infrared laser performance of five 5 at.% Er3+-doped fluorite-type crystals MF2, including parent compounds CaF2, SrF2, BaF2, and solid-solution (“mixed”) ones (Ca,Sr)F2 and (Sr,Ba)F2. In the M = Ca → Sr → Ba series, the host matrix phonon energy decreases, the absorption and mid-infrared emission spectra of Er3+ become narrower and more structured, and the luminescence lifetimes of the 4I11/2 and 4I13/2 Er3+ manifolds increase. The Er3+ transition probabilities were calculated using the Judd-Ofelt theory. In the “mixed” compounds, the Er3+ ions tend to reside in the larger / heavier cation environment. The low-temperature (12 K) spectroscopy evidences the presence of a single type of clusters at this doping level; the crystal-field splitting for Er3+ ions in clusters was determined. Continuous-wave low-threshold laser operation at ∼2.8 µm (the 4I11/2 → 4I13/2 transition) was achieved with all five Er3+:MF2 crystals. The maximum achieved laser slope efficiency was 37.9% (Er3+:CaF2), 23.5% (Er3+:SrF2) and 17.2% (Er3+:BaF2).

Tunable continuous-wave laser operation of Nd:YAG around 1.3 μm

A tunable continuous-wave (cw) Nd:YAG laser using a birefringent filter (BF) was performed at six different laser wavelengths of 1319, 1334, 1338, 1341, 1353 and 1356 nm based on the 4F3/2–4I13/2 transition. A highest output power of 4.64 W was achieved at an emission wavelength of 1319 nm with a slope efficiency of 29.8% with respect to the absorbed pump power. Moreover, by adjusting the rotation angle of the BF, a cw simultaneous dual-wavelength Nd:YAG laser operating at 1353 and 1356 nm was also demonstrated for the first time. At an absorbed pump power of 17.8 W, the maximum output power obtained at 1353 nm and 1356 nm is 262 mW and 520 mW, respectively.

Diode-pumped visible lasing in femtosecond-laser-written Pr:LiLuF4 waveguide.

In this Letter we report the realization of a femtosecond-laser-written diode-pumped Pr:LiLuF4 visible waveguide laser. The waveguide studied in this work consisted of a depressed-index cladding, whose design and fabrication were optimized to minimize the propagation loss. Laser emission has been achieved at 604 nm and 721 nm, with output power of 86 mW and 60 mW, respectively, and slope efficiencies of 16% and 14%. In addition, we obtained, for the first time in a praseodymium-based waveguide laser, stable continuous-wave laser operation at 698 nm (3 mW of output power and 0.46% of slope efficiency), corresponding to the wavelength necessary for the clock transition of the strontium-based atomic clock. The waveguide laser emission at this wavelength is mainly in the fundamental mode (i.e., the larger propagation constant mode) showing a nearly Gaussian intensity profile.

Efficient continuous-wave Tm,Ho:CaF2 laser at 2.1µm.

We report on the first, to the best of our knowledge, continuous-wave laser operation of a Tm3+,Ho3+-codoped calcium fluoride crystal at ∼2.1 µm. Tm,Ho:CaF2 crystals were grown by the Bridgman method, and their spectroscopic properties were studied. The stimulated-emission cross section for the 5I7 → 5I8 Ho3+ transition is 0.72 × 10-20 cm2 at 2025 nm, and the thermal equilibrium decay time is 11.0 ms. A 3 at. % Tm, 0.3 at. % Ho:CaF2 laser generated 737 mW at 2062-2088 nm with a slope efficiency of 28.0% and a laser threshold of 133 mW. Continuous wavelength tuning between 1985 and 2114 nm (tuning range: 129 nm) was demonstrated. The Tm,Ho:CaF2 crystals are promising for ultrashort pulse generation at ∼2 µm.

Cryogenic Tm:LiYF4 laser around 2 µm

We present the laser characteristics of a 5 at.% Tm:YLF crystal using a modular setup at cryogenic temperatures emitting around 2 µm. Continuous-wave laser operation was achieved by pumping the laser crystal using a Volume Bragg Grating-stabilized laser diode emitting at 793 nm. A maximum output power of 6.5 W was achieved at 80 K corresponding to a slope efficiency of 66.0% with respect to the absorbed power with excellent beam quality.