The orbital operation of spacecraft can excite the long-drawn and low-frequency vibration of the solar array, which is prone to affecting the task execution of the system. To address this issue, an envelope-based variable-gain control strategy is proposed to suppress vibration of the solar array using the reaction wheel (RW) actuator. The RW actuator is individually mounted on the solar array to provide reaction torque through the speed change of its rotor. The governing equation of motion of the solar array actuated by a RW actuator is deduced with the state space representation. The control relation between the measured bending moment and the rotational speed of the RW actuator with the constant-gain coefficient is firstly developed and demonstrated in numerical simulation. Changing the gain coefficient to be inversely proportional to the envelope function of vibration, a variable-gain control strategy is proposed to improve the damping effect of the RW actuator. Simulation results show that the vibration suppression performance of the RW actuator is improved compared to the constant-gain control. As the actual on-orbit natural frequency of the solar array is not always exactly known, the robustness of the control system is analyzed for the deviation between the estimated and the actual natural frequency values. The proposed variable-gain control is also experimentally verified using a simplified elastic plate model. Experimental results indicate that the vibration attenuation time is decreased to 29.1% and 50.22% compared to the uncontrolled and the constant-gain controlled states, respectively.