Circularly Polarized Research Articles

Chiral 3D Perovskite Formation Induced by Chiral Templates.

Chiral 3D perovskites pose challenges compared to lower-dimensional variants due to limited chiral organic cation options. Here, we present a universal and controlled method for synthesizing chiral 3D lead halide perovskites using organic amines or alcohols as chiral templates. Introducing these templates to PbCl2 in N,N-dimethylformamide (DMF) under acidic conditions induces the crystallization of R/S [DMA]PbCl3 (DMA = dimethylamine). The resulting structure aligns with the templates used, stemming from the helical Pb2Cl95- chain as verified by single-crystal X-ray diffraction. Furthermore, the chiral perovskite exhibits absorption and circular dichroism (CD) signals in the high-energy band, enabling the circularly polarized light (CPL) detection in the UV spectrum. A CPL detector constructed by this chiral perovskite demonstrates excellent performance, boasting an anisotropy factor for photocurrent (gIph) of 0.296. Our work not only introduces a novel and controllable method for crafting chiral perovskites but also opens new avenues for circularly polarized light detection.

Electrically reflectance-tunable circular polarization reflector based on thin polymer-stabilized cholesteric liquid crystals

This paper presents a reflectance-tunable circular polarization reflector that utilizes thin polymer-stabilized cholesteric nematic liquid crystals (PSCLCs) with negative anisotropy. The switching mechanism involves direct-current (DC) field-induced movement in the polymer network, which generates the mechanical force that causes a pitch-gradient helical structure and thus a distorted Bragg reflection. The pitch-gradient helical structure of the 5 μm-thick cells only allows for a limited number of pitch lengths, resulting in a decrease in reflectance at the designed Bragg reflectance and a reflectance tunable range determined by applying DC voltages. The PSCLCs reflecting red, green, and blue colors were measured for their reflectance tuning ability and circular polarization selectivity. A tunable polarization volume grating was fabricated using a PSCLC cell, and the ability of the grating to diffract light intensity was demonstrated.

Achievement splitting for topological states with pseudospin in phase modulation by using gyromagnetic photonic crystals

As we know, valley-Hall kink states or pseudospin helical edge states are excited by polarized-momentum-locking [left-handed circular polarization (LCP) and right-handed circular polarization (RCP)] because the valley-Hall kink modes or pseudospin polarized modes have intrinsic and local chirality, which is difficult for these states to achieve phase modulation. Here we theoretically design and study a compatible topological photonic system with coexistence of photonic quantum Hall phase and pseudospin Hall phase, which is composed of gyromagnetic photonic crystals with a deformed honeycomb lattice containing six cylinders. A typical kind of hybrid topological waveguide states with pseudospin-characteristic, magnetic field-dependent, and strong robustness against backscattering and perfect electric conductor (PEC) is realized in the present system. Furthermore, we re-design a structure with intersection-liked, achieve splitting for one-way pseudospin quantum Hall edge states by using phase modulation. Robustness of the one-way pseudospin-quantum Hall edge states in splitting has been demonstrated as well. Additionally, PEC inserted in transport channel brings optical path difference in waveguide transmission, which would influence splitting for hybrid topological waveguide states in phase difference modulation. This work not only provides a new way for manipulation (i.e., phase modulation) of hybrid topological waveguide states in compatible topological photonic system from distinct topological classes but also has potential in various applications, such as sensing, signal processing, and on-chip communications.

High-Gain Dual-Polarization Microstrip Antenna Based on Transmission Focusing Metasurface.

In this paper, a single-feed microstrip antenna (MA) equipped with a transmission-mode focusing metasurface (MS) is proposed to achieve dual-polarization capabilities and superior high-gain radiation performance. The original-feed MA comprises two distinct layers of coaxial-fed tangential patches, enabling it to emit a circular polarization (CP) wave with a gain of 3.5 dBic at 5.6 GHz and linear polarization (LP) radiation with a gain of 4 dBi at 13.7 GHz. To improve the performance of the single-feed MA, a dual-polarization transmission focusing MS is proposed and numerically substantiated. By positioning the originally designed MA at the focal point of the MS, we create a transmission-mode MS antenna system capable of achieving CP and LP radiations with the significantly higher gains of 12.9 dBic and 14.8 dBi at 5.6 GHz and 13.7 GHz, respectively. Measurements conducted on the fabricated dual-polarization focusing MS antenna closely align with the simulation results, validating the effectiveness of our approach. This work underscores the significant potential of dual-polarization high-speed data systems and offers a practical solution for enhancing antenna gains in contemporary wireless communication systems.

Recent Progress in Circularly Polarized Luminescent Materials Based on Cyclodextrins.

Circularly polarized luminescence (CPL) materials have been widely used in the fields of bioimaging, optoelectronic devices, and optical communications. The supramolecular interaction, involving harnessing non-covalent interactions between host and guest molecules to control their arrangements and assemblies, represents an advanced approach for facilitating the development of CPL materials and finely constructing and tuning the desired CPL properties. Cyclodextrins (CDs) are cyclic natural polysaccharides, which have also been ubiquitous in various fields such as molecular recognition, drug encapsulation, and catalyst separation. By adjusting the interactions between CDs and guest molecules precisely, composite materials with CPL properties can be facilely generated. This review aims to outline the design strategies and performance of CD-based CPL materials comprehensively and provides a detailed illustration of the interactions between host and guest molecules.

Broadband vortex beam generation by a reflective meta-surface based on a metal double-slit resonant ring

Recently, the meta-surface (MS) has emerged as a promising alternative method for generating vortex waves. At the same time, MS also faces the problem of a narrow bandwidth; in order to obtain a broad bandwidth, the MS unit cell structure becomes more and more complex, which will bring many inconveniences to the preparation process of MS devices. Therefore, we want to design a simple MS unit cell with a multi-frequency selection. In this paper, based on the principle of geometric phase, we design a simple reflective MS unit cell based on a metal double-slit resonant ring. We elaborate on the resonance mechanism of the MS unit cell. Under the normal incidence of circularly polarized (CP) waves, the reflection coefficient of the same polarization was greater than 85%. By rotating the orientation angle of the resonator on the MS unit cell, the continuous 2π phase coverage was satisfied in the frequency range of 0.52–1.1 THz, and the relative bandwidth becomes 71.6%. Based on this, we construct a vortex generator by using a 15×15 MS unit array. The right-handed circularly polarized (RCP) waves and left-handed circularly polarized (LCP) wave are separately incident on MS with topological charges of l=+1,+2,+3 under multiple resonant frequencies. The generated RCP vortex wave has topological charges of l=−1,−2,−3 and the generated LCP vortex wave has topological charges of l=+1,+2,+3. The numerical simulation results demonstrate that our designed MS, capable of achieving multiple resonance outcomes, can effectively operate in a multi-broadband mode and produce a wide-band vortex beam. In addition, we also calculate the pattern purity. Through theoretical analysis and numerical simulation, we prove that our designed MS can generate a broadband vortex wave.

Amplification of interlayer exciton emission in twisted WSe2/WSe2/MoSe2 heterotrilayers

Van der Waals heterostructures based on transition metal dichalcogenides exhibit physical properties that depend on their monolayer constituents’ twisting angle and stacking order. Particularly in type-II heterostructures, low-energy photoluminescence is dominated by interlayer excitons, resulting in low emission yields, which drastically hampers their optoelectronic applicability. This study reports on the photoluminescence quantum yield of heterostructures consisting of WSe2/WSe2/MoSe2 twisted layers. Our findings show that the additional WSe2 monolayer in the trilayer system enhances the low-energy photoluminescence by more than an order of magnitude depending on the WSe2/WSe2 twist-angle in comparison to their WSe2/MoSe2 heterobilayer counterpart. Furthermore, combining density functional theory calculations and extracted degree of circular polarization, we identify excitonic signatures arising from hybridized states that originate from the additional WSe2 layer. In addition to providing an additional understanding of hybridization effects in 2D semiconducting heterostructures, our findings provide a viable method to enhance emission in van der Waals heterostructures, relevant for studying the fundamental properties of excitons and enabling optoelectronic applications with high luminescence yield.

Programmable generation of counterrotating bicircular light pulses in the multi-terahertz frequency range

The manipulation of solid states using intense infrared or terahertz light fields is a pivotal area in contemporary ultrafast photonics research. While conventional circular polarization has been well explored, the potential of counterrotating bicircular light remains widely underexplored, despite growing interest in theory. In the mid-infrared or multi-terahertz region, experimental challenges lie in difficulties in stabilizing the relative phase between two-color lights and the lack of available polarization elements. Here, we successfully generated phase-stable counterrotating bicircular light pulses in the 14–39 THz frequency range circumventing the above problems. Employing spectral broadening, polarization pulse shaping with a spatial light modulator, and intra-pulse difference frequency generation leveraging a distinctive angular-momentum selection rule within the nonlinear crystal, we achieved direct conversion from near-infrared pulses into the designed counterrotating bicircular multi-terahertz pulses. Use of the spatial light modulator enables programmable control over the shape, orientation, rotational symmetry, and helicity of the bicircular light field trajectory. This advancement provides a novel pathway for the programmable manipulation of light fields, and marks a significant step toward understanding and harnessing the impact of tailored light fields on matter, particularly in the context of topological semimetals.

Terahertz polarization sensing for influenza A virus based on plasmonic metasurface

Terahertz metasurface sensors attract extensive attention for excellent characterisics. However, most existing sensing schemes overlooked the polarization state of electromagnetic waves. Here, we propose a plasmonic metasurface sensor based on the elliptical polarization state of reflected EM wave, which can be used for the sensing of influenza A virus. The sensor achieves the conversion from linear polarization to circular polarization within 1–3 THz. By analysing the electromagnetic field distributions of the resonances at 1.43 THz and 2.16 THz, it can be concluded that the polarization conversion originates from the magnetic dipole. Besides, the sensor can characterize the changes in the complex refractive index of the test sample based on the elliptical polarization state of the reflected wave. The electromagnetic response of the metasurface sensor shows an excellent linear relationship between the rotating direction angle of polarization ellipse and the extinction coefficient (k) of the complex RI of the analyte. Furthermore, we also demonstrate the feasibility of detecting three subtypes of Influenza A viruses (H1N1, H5N2, and H9N2) at 1.39 THz though the elliptical polarization state. This sensing approach does not rely on high-precision broadband scanning, providing an alternative perspective for THz biosensing.

Twisted Stacking Metasurface for Complete Amplitude and Phase Control of Circularly Polarized Terahertz Waves

AbstractTerahertz (THz) metasurfaces have emerged as a powerful tool for manipulating THz wavefronts, typically achieved by adjusting various geometric parameters. In this study, an approach is introduced by incorporating interlayer coupling into twisted stacking metasurface design to completely control the amplitude and phase of circularly polarized THz waves. By leveraging the interlayer coupling effect and the Pancharatnam–Berry phase, the study achieves efficient control over transmission phase and amplitude by simply adjusting the relative twist angle between paired C‐shaped split‐ring resonators. To validate the concept, a holographic metasurface is fabricated and characterized, providing experimental evidence of its THz wavefront manipulation capabilities. This design strategy presents a versatile and tunable solution for THz wave control, promising applications in a wide range of functional devices.

Scalar induced gravitational waves in chiral scalar–tensor theory of gravity

We study the scalar induced gravitational waves (SIGWs) from a chiral scalar–tensor theory of gravity. The parity-violating (PV) Lagrangian contains the Chern–Simons (CS) term and PV scalar–tensor terms, which are built of the quadratic Riemann tensor term and first-order derivatives of a scalar field. We consider SIGWs in two cases, in which the semi-analytic expression to calculate SIGWs can be obtained. Then, we calculate the fractional energy density of SIGWs with a monochromatic power spectrum for the curvature perturbation. We find that the SIGWs in chiral scalar–tensor gravity behave differently from those in GR before and after the peak frequency, which results in a large degree of circular polarization.

Highly efficient multifunctional metasurface integrating lens, prism, and wave plate

The miniaturization of optical systems is crucial for various applications, including compact augmented reality/virtual reality devices, microelectromechanical system sensors, ranging technologies, and microfabricated atomic clocks. However, reliance on bulky discrete optical elements has been a significant obstacle to achieving this miniaturization. This work introduces a highly efficient multifunctional metasurface (MFMS) that seamlessly integrates a lens, prism, and quarter-wave plate (QWP). This innovation allows simultaneous collimation, beam deflection, and polarization conversion within a singular thin element. Specifically, for the prism-QWP bifunctional integration, we achieved a high diffraction efficiency of 72.8% and a degree of circular polarization of −0.955 under exposure to linearly polarized light at a wavelength of 795 nm, proving its potential for ultracompact atomic clock applications. Moreover, the lens-prism-QWP trifunctional integration successfully showed diffraction-limited focusing performance with a numerical aperture of 0.4, which was sufficient to collimate a beam with a divergence angle of 20∘, corresponding to the light emitted from a standard vertical-cavity surface-emitting laser.

Pyro-Phototronic Effect Induced Circularly Polarized Light Detection with a Broadband Response.

Photopyroelectric-based circularly polarized light (CPL) detection, coupling the pyro-phototronic effect and chiroptical phenomena, has provided a promising platform for high-performance CPL detectors. However, as a novel detection strategy, photopyroelectric-based CPL detection is currently restricted by the short-wave optical response, underscoring the urgent need to extend its response range. Herein, visible-to-near-infrared CPL detection induced by the pyro-phototronic effect is first realized in chiral-polar perovskites. Specifically, chiral-polar multilayered perovskites (S-BPEA)2FAPb2I7 (1-S, S-BPEA = (S)-1-4-Bromophenylethylammonium, FA = formamidinium) with spontaneous polarization shows intrinsic pyroelectric and photopyroelectric performance. Strikingly, combining its merits of the pyro-phototronic effect and intrinsic wide-spectrum spin-selective effect, chiral multilayered 1-S presents efficient photopyroelectric-based broadband CPL detection performance spanning 405-785nm. This research first realizes photopyroelectric-based infrared CPL detection and also sheds light on developing high-performance broadband CPL detectors based on the pyro-phototronic effect in the fields of optics, optoelectronics, and spintronics.

Chirality-dependent topological edge states in photonic metacrystal.

Topological edge state, a unique mode for manipulating electromagnetic waves (EMs), has been extensively studied in both fundamental and applied physics. Up to now, the work on topological edge states has focused on manipulating linearly polarized waves. Here, we realize chirality-dependent topological edge states in one-dimensional photonic crystals (1DPCs) to manipulate circularly polarized waves. By introducing the magneto-electric coupling term (chirality), the degeneracy Dirac point (DP) is opened in PCs with symmetric unit cells. The topological properties of the upper and lower bands are different in the cases of left circularly polarized (LCP) and right circularly polarized (RCP) waves by calculating the Zak phase. Moreover, mapping explicitly 1D Maxwell's equations to the Dirac equation, we demonstrate that the introduction of chirality can lead to different topological properties of bandgaps for RCP and LCP waves. Based on this chirality-dependent topology, we can further realize chirality-dependent topological edge states in photonic heterostructures composed of two kinds of PCs. Finally, we propose a realistic structure for the chirality-dependent topological edge states by placing metallic helixes in host media. Our work provides a method for manipulating topological edge states for circularly polarized waves, which has a broad range of potential applications in designing optical devices including polarizers, filters, and sensors with robustness against disorder.

A Miniaturized Dual-Band Circularly Polarized Implantable Antenna for Use in Hemodialysis.

Hemodialysis is achieved by implanting a smart arteriovenous graft (AVG) to build a vascular pathway, but reliability and stability in data transmission cannot be guaranteed. To address this issue, a miniaturized dual-band circularly polarized implantable antenna operating at 1.4 GHz (for energy transmission) and 2.45 GHz (for wireless telemetry), implanted in a wireless arteriovenous graft monitoring device (WAGMD), has been designed. The antenna design incorporates a rectangular serpentine structure on the radiation surface to reduce its volume to 9.144 mm3. Furthermore, matching rectangular slots on the radiation surface and the ground plane enhance the antenna's circular polarization performance. The simulated effective 3 dB axial ratio (AR) bandwidths are 11.43% (1.4 GHz) and 12.65% (2.45 GHz). The simulated peak gains of the antenna are -19.55 dBi and -22.85 dBi at 1.4 GHz and 2.45 GHz, respectively. The designed antenna is implanted in a WAGMD both in the simulation and the experiment. The performance of the system is simulated in homogeneous human tissue models of skin, fat, and muscle layers, as well as a realistic adult male forearm model. The measurement results in a minced pork environment align closely with the simulation results.

Analysis of spiral antenna for enhancing antenna-plasma coupling impedance for SST-1 tokamak

Abstract A detailed characterization of a high-power radio frequency (RF) broadband circularly polarized two-arm spiral antenna is designed to operate within the frequency range of 0.1–1.0 GHz. The impedance matching network technique is introduced to optimize its performance. The traditional spiral antenna is excited by a vertical or horizontal balun, whereas the proposed design is directly fed by a coaxial cable featuring a planar feeding section specially optimized to achieve broadband input impedance matching. The spiral antenna is designed as per the steady-state superconducting tokamak (SST-1) port space constraints. The simulated efficiency of the RF power coupling with the hydrogen plasma is ∼70 %. Through simulation, it was evident that the proposed antenna exhibited inherent resonance at 0.5 GHz with a reflection coefficient of −27.94 dB and an axial ratio is 3.39 dB respectively. The obtained outcomes unequivocally demonstrate the circular polarization of the designed antenna. Overall, the findings support the enhancement of plasma heating and current drive techniques in fusion research.

Bidirectional triple-band truly incident angle insensitive polarization converter using graphene-based transmissive metasurface for terahertz frequency

Abstract The design and response of a triple-band linear-to-circular polarization converter (LTCPC) in the terahertz frequency regime using a graphene-based transmission-type metasurface have been studied numerically and analytically. The unit cell of the converter is constructed using lossy silicon dioxide (SiO2) with a relative permittivity of 3.9 as the substrate. And two similar layers of graphene-based sub-wavelength structures are used at the top and bottom of it. Multiband linear to circular polarization conversion is achieved from 0.74 THz to 0.98 THz, 1.70 THz to 2.33 THz, and 4.06 THz to 5.19 THz, i.e., about 28 %, 31 %, and 24 % fractional bandwidths, respectively. As the same metasurface configuration is used at the top and bottom layers of the transmission-type unit cell, it can be used as a bidirectional polarization converter with identical responses from both sides. The geometrical optimization of the unit cell is done, and an equivalent lumped parameter circuit model is also proposed for the same, considering analogous responses. Tunability over the operating frequency is achieved by varying the chemical potential and relaxation time of graphene. Moreover, due to the ultrathin width and special types of identical configuration of the metasurfaces, the response of the system remains excellent over a wide range of incident angle variations up to 80° angle of incidence.

Pair production in rotating electric fields via quantum kinetic equations: Resolving helicity states

We investigate the phenomenon of electron-positron pair production from vacuum in the presence of a strong electric field of circular polarization. By means of a nonperturbative approach based on the quantum kinetic equations (QKEs), we numerically calculate helicity-resolved momentum distributions of the particles produced and analyze the corresponding helicity asymmetry. It is demonstrated that the external rotating field tends to generate left-handed and right-handed particles traveling in opposite directions. Generic symmetry properties of the momentum spectra are examined analytically by means of the QKEs and also confirmed and illustrated by direct numerical computations. The helicity signatures revealed in our study are expected to provide a firmer basis for possible experimental investigations of the fundamental phenomenon of vacuum pair production in strong fields. Published by the American Physical Society 2024

Chiral Emission from Optical Metasurfaces and Metacavities

Chiral emission exhibiting a large degree of circular polarization (DCP) is important in diverse applications ranging from displays and optical storage to optical communication, bioimaging, and medical diagnostics. Although chiral luminescent materials can generate chiral emissions directly, they frequently suffer from either low DCP or low quantum efficiencies. Achieving high DCP and quantum efficiencies simultaneously remains extremely challenging. This review introduces an alternative approach to chiral emission. Chiral emission with large DCP can be readily achieved by combining conventional achiral emitters with chiral metasurfaces. Particularly, this article focuses on recent experimental and theoretical studies on perovskite metasurfaces and metacavities that employ achiral perovskite materials. First, chiral photoluminescence from extrinsic and intrinsic perovskite metasurfaces is explained together with theoretical discussions on metasurface design based on reciprocity and critical coupling. Chiral photoluminescence from other achiral materials is also explained. Subsequently, chiral electroluminescence from perovskite metacavities and other achiral materials is discussed. Finally, it is concluded with future perspectives. This review provides physical insights into how ideal chiral emission can be realized by optimizing the design of metasurfaces and metacavities. Compact chiral light sources with both near‐unity DCP and strong emission intensities can have far‐reaching consequences in a wide range of future applications.

A miniaturized dual wide‐band polarization reconfigurable antenna integrated with artificial magnetic conductor for next‐generation wireless applications

SummaryIn today's intricate wireless communication environment, ensuring system quality demands the use of a reliable and versatile antenna system. This research article introduces a polarization reconfigurable antenna integrated with a 4 × 4 Artificial Magnetic Conductor (AMC) surface. The AMC unit cell exhibits a triple‐band reflection phase response at 1.8GHz, 4.5GHz, and 5.5GHz, demonstrating double negative metamaterial behavior. The antenna features two distinct C‐shaped metal strips connected to two PIN diodes, enabling dynamic current distribution adjustment. Consequently, the proposed antenna offers three reconfigurable states, facilitating seamless switching between dual circular polarization (left and right‐hand circular polarization) and linear polarization. With a frequency coverage ranging from 1.29 to 2.52GHz and 3.59 to 6.15GHz, the antenna boasts a maximum axial ratio (AR) bandwidth of 31.96%. Additionally, it achieves a maximum peak gain of 5.5 dB and maintains front‐to‐back ratio (FBR) values exceeding 25 dB, while recording a minimum specific absorption rate (SAR) value of 0.1059 W/kg. The integration of the AMC surface ensures enhanced performance of the antenna. Experimental results from constructed prototypes closely align with simulation outcomes, validating the effectiveness of the proposed antenna. Consequently, this antenna holds significant promise for next‐generation wireless applications.