Changes In Magnetic Structure Research Articles

Interlayer Interaction of Excitons and Magnons in Graphene/WS2/Néel‐Type Manganese Phosphorus Trichalcogenide Heterostructures

Abstract2D materials, particularly 2D semiconductors, and layered antiferromagnetic (AFM) compounds, exhibit rich light‐matter coupling phenomena in low‐dimensional systems. In this work, the occurrence of interlayer exciton–magnon coupling (EMC) is observed in Néel‐type AFM of MnPX3 (X = S or Se) and monolayer (1L) WS2 heterostructures. The energy of neutral exciton in 1L WS2 can be tuned by the adjacent AFM order, resulting in an additional energy shift of 10–14 meV. Furthermore, by filtering the photoluminescence spectrum with graphene and conducting magnetic measurements, the correlation is elucidated between the interlayer EMC and AFM transition process. In MnPS3, this coupling behavior exhibits sensitivity to the changes of magnetic structures, manifesting with a correlated length ξ of 8.34 Å at temperatures higher than Néel temperature (TN). The decoupling process in WS2/MnPS3 heterostructure below 50 K is originated from a weak out‐of‐plane ferromagnetic order, confirming the presence of an XY‐type magnetic phase transition in MnPS3 at sub‐TN temperature. This study provides a fundamental understanding of EMC and its potential applications in the integration of optical and magnetic devices.

Topological stability of spin textures in Si/Co-doped helimagnet FeGe

Element substitutions with magnetic or non-magnetic atoms are known to significantly impact the magnetic structure and related transport properties of magnets. To clarify the change of magnetic structure of B20-type magnets with element doping, we conduct real-space observations of spin textures and their temperature (T)-magnetic field (H) phase diagrams of a helimagnet FeGe with partially substituting Fe and Ge with Co and Si, respectively. The helical period (λ) changes dramatically by the element doping: λ increases by 147% to 103 nm in 30% Co-doped FeGe, whereas it decreases by around 70% to 49 nm in 30% Si-doped FeGe, compared to the λ =70 nm in FeGe. Upon applying the magnetic field normally to (001), (110), and (111) thin plates of both FeSi0.3Ge0.7 and Fe0.7Co0.3Ge, the hexagonal skyrmion crystal (SkX) state emerges. The magnetic phase diagrams observed through the real-space imaging reveal that (1) the SkX can extend to a larger T-H window by reducing the sample thickness or by cooling the sample under specific magnetic fields from temperatures above the transition temperature (TC ); (2) the stability of the SkX phase differs between Si-doped and Co-doped FeGe: the SkX phase is most unstable in the (111) FeSi0.3Ge0.7, while it remains robust in the (111) Fe0.7Co0.3Ge. These differences indicate distinct anisotropic behavior in FeGe with magnetic (Co) and non-magnetic-element (Si) dopants.

In-situ electric field-tailored exchange bias in the manganite/ferroelectric multiferroic heterostructures

The application of electric field-induced magnetic structure changes has significantly advanced nonvolatile data storage with ultralow energy consumption, as well as spintronics and quantum computing processes. In artificial perovskite oxide multiferroic structures composed of ferromagnetic and ferroelectric layers, the evolution of magnetic phases and ferroelectric domains often contribute to the magnetoelectric coupling. To fully understand the mechanisms behind electric field-induced changes in magnetic structures and enable the miniaturization of magnetoelectric devices, it is crucial to achieve local ferroelectric domain-triggered ferromagnetic evolution. In this study, we have fabricated La0.7Ca0.3MnO3/Pb(Zr0.52Ti0.48)O3 (LCMO/PZT) heterostructures, where the magnetic phase separation of LCMO and the ferroelectric domain of PZT can be modulated by substrates and piezoelectric force microscopy, respectively. Our experiments demonstrate that by switching the polarization states of PZT, we can observe electric field control of the magnetic exchange bias effect through changes in the phase separation of the LCMO layer. These results contribute to the development of magnetoelectric devices with enhanced properties and offer valuable insights for future design strategies.

Temperature- and magnetic field-induced magnetic structural changes in the Fe3Si/FeSi2 superlattice

Artificial lattices with semiconductor spacers are expected to exhibit changes in their magnetic structure owing to the control of their electronic states. The temperature (T) and magnetic-field (H ext) dependence of the in-plane magnetic structure of an [Fe3Si/FeSi2]20 superlattice with a nonmagnetic and semiconducting FeSi2 spacer layer is investigated using magnetization and polarized neutron reflectivity measurements. When H ext = 5 mT, nearly collinear antiferromagnetic (AF) structures are observed from 4 to 298 K. When H ext = 1 T, field-induced fan-like, noncollinear AF structures showing ferromagnetic components along H ext and transverse AF components are observed at low T.

Unveiling the Anomalous Hall Response of the Magnetic Structure Changes in the Epitaxial MnBi2Te4 Films.

Recently discovered as an intrinsic antiferromagnetic topological insulator, MnBi2Te4 has attracted tremendous research interest, as it provides an ideal platform to explore the interplay between topological and magnetic orders. MnBi2Te4 displays distinct exotic topological phases that are inextricably linked to the different magnetic structures of the material. In this study, we conducted electrical transport measurements and systematically investigated the anomalous Hall response of epitaxial MnBi2Te4 films when subjected to an external magnetic field sweep, revealing the different magnetic structures stemming from the interplay of applied fields and the material's intrinsic antiferromagnetic (AFM) ordering. Our results demonstrate that the nonsquare anomalous Hall loop is a consequence of the distinct reversal processes within individual septuple layers. These findings shed light on the intricate magnetic structures in MnBi2Te4 and related materials, offering insights into understanding their transport properties and facilitating the implementation of AFM topological electronics.

Magnetism and fermiology of kagome magnet YMn6Sn4Ge2

Kagome lattice magnets are an interesting class of materials as they can host topological properties in their magnetic and electronic structures. YMn6Sn6 is one such compound in which various exotic magnetic and electronic topological properties have been realized. Here, by means of a partial substitution of Sn with an isovalent and slightly smaller atom Ge, we demonstrate the sensitivity of such chemical substitution on the magnetic structure and its influence in the electronic properties. Magnetic structure of YMn6Sn4Ge2 determined by neutron diffraction reveals an incommensurate staggered magnetic spiral with a slightly larger spiral pitch than in YMn6Sn6. This change in magnetic structure influences the Fermi surface enhancing the out-of-plane conductivity. Such a sensitivity to the partial chemical substitution provides a great potential for engineering the magnetic phases and associated electronic properties not only in YMn6Sn6, but also in the large family of 166 rare-earth kagome magnet.

Effects of drawing and tension stress annealing on the structure and magnetic properties of Co-based amorphous wire

Cold drawing significantly improves the size uniformity of the amorphous wire, but leads to wire curling. Tensile stress annealing (TSA) is the key to regulating the straightness and magnetic properties of Co-based amorphous wires, but their intrinsic correlation is still unclear. Herein, the effects of TSA on the morphology, microstructure, soft magnetic properties and longitudinal driven giant magneto-impedance (LD-GMI) effect of cold drawn Co-based amorphous wires have been studied in detail. It was found that increasing tensile stress can effectively straighten the drawn amorphous wire, yet at the cost of decreasing fracture strength, increasing coercivity and deteriorating GMI effect. Furthermore, appropriate annealing can restore the magnetic properties of the TSA amorphous wire. The variation of magnetic properties is relative to the change of circular anisotropic field and magnetic domain structure.

Survival of fossil fields during the pre-main sequence evolution of intermediate-mass stars

Context. Chemically peculiar Ap and Bp stars host strong large-scale magnetic fields in the range of 200 G up to 30 kG, which are often considered to be the origin of fossil magnetic fields. Aims. We assess the evolution of such fossil fields during the star formation process and the pre-main sequence evolution of intermediate stars based on: fully convective models, models including a transition to a radiative protostar, and models with a radiative core. We also examine the implications of the interaction between the fossil field and the core dynamo. Methods. We employed analytic and semi-analytic calculations, combined with current observational constraints. Results. For fully convective models, we show that magnetic field decay via convection can be expected to be very efficient for realistic parameters of turbulent resistivities. Based on the observed magnetic field strength-density relation, as well as the expected amount of flux loss due to ambipolar diffusion, it appears unlikely that convection could be suppressed via strong enough magnetic fields. On the other hand, a transition from a convective to a radiative core could very naturally explain the survival of a significant amount of flux, along with the presence of a critical mass. We show that in some cases, the interaction of a fossil field with a core dynamo may further lead to changes in the surface magnetic field structure. Conclusions. In the future, it will be important to understand in more detail how the accretion rate evolves as a function of time during the formation of intermediate-mass protostars, including its impact on the protostellar structure. The latter may even allow us to derive quantitative predictions concerning the expected population of large scale magnetic fields in radiative stars.

Evolution of medium-range order and its correlation with magnetic nanodomains in Fe-Dy-B-Nb bulk metallic glasses

Fe-based metallic glasses are promising functional materials for advanced magnetism and sensor fields. Tailoring magnetic performance in amorphous materials requires a thorough knowledge of the correlation between structural disorder and magnetic order, which remains ambiguous. Two practical difficulties remain: the first is directly observing subtle magnetic structural changes on multiple scales, and the second is precisely regulating the various amorphous states. Here we propose a novel approach to tailor the amorphous structure through the liquid-liquid phase transition. In-situ synchrotron diffraction has unraveled a medium-range ordering process dominated by edge-sharing cluster connectivity during the liquid-liquid phase transition. Moreover, nanodomains with topological order have been found to exist in composition with liquid-liquid phase transition, manifesting as hexagonal patterns in small-angle neutron scattering profiles. The liquid-liquid phase transition can induce the nanodomains to be more locally ordered, generating stronger exchange interactions due to the reduced Fe–Fe bond length and the enhanced structural order, leading to the increment of saturation magnetization. Furthermore, the increased local heterogeneity at the medium-range scale enhances the magnetic anisotropy, promoting the permeability response under applied stress and leading to a better stress-impedance effect. These experimental results pave the way to tailor the magnetic structure and performance through the liquid-liquid phase transition.

Impact of Ge Doping on Structural and Magnetic Ordering in RMnxGa3 and R4Mn1-xGa12-yGey (R = Tb, Dy; x ≤ 0.25, y ≈ 1.0-3.3).

Single crystals of RMnxGa3 and their new quaternary derivatives R4Mn1-xGa12-yGey (R = Tb, Dy, x ≤ 0.25, y ≈ 1.0-3.3) were grown from a Ga flux. The compounds are derivatives of cubic RGa3 phases, with Mn atoms filling the Ga6 voids. RMnxGa3 formally adopts a cubic ABO3 perovskite structure, in which the presence of Mn atoms results in a shift of the neighboring Ga atoms from their ideal position. A partial substitution of Ga by Ge leads to a higher Mn content, resulting in structural ordering of the latter and the formation of the superstructure phases R4Mn1-xGa12-yGey, which can be formally described in the Y4PdGa12 structure type. The presence of Mn vacancies, which was observed for R = Tb, and Ga/Ge mixing lead to a noticeable deviation from the idealized structure. The compounds contain two magnetic sublattices: the R sublattice, which orders antiferromagnetically near 20 K, and the Mn sublattice, which orders ferromagnetically at TC = 125-225 K with the Ge doping resulting in higher TC. The two sublattices are not independent, as the Mn sublattice induces partial ferromagnetic ordering of the rare earth atoms below TC, at least for the Ge-doped phases. Near TN, both magnetic susceptibility and heat capacity reveal complex behavior, indicating changes in magnetic structures below TN.

Which Component of Solar Magnetic Field Drives the Evolution of Interplanetary Magnetic Field over the Solar Cycle?

The solar magnetic structure changes over the solar cycle. It has a dipole structure during solar minimum, where the open flux extends mainly from the polar regions into the interplanetary space. During maximum, a complex structure is formed with low-latitude active regions and weakened polar fields, resulting in spread open field regions. However, the components of the solar magnetic field that are responsible for long-term variations in the interplanetary magnetic field (IMF) are not clear, and the IMF strength estimated based on the solar magnetic field is known to be underestimated by a factor of 3–4 against the actual in situ observations (the open flux problem). To this end, we decomposed the coronal magnetic field into the components of the spherical harmonic function of degree and order (ℓ, m) using the potential field source surface model with synoptic maps from SDO/HMI for 2010–2021. As a result, we found that the IMF rapidly increased in 2014 December (7 months after the solar maximum), which coincided with the increase in the equatorial dipole, (ℓ, m) = (1, ±1), corresponding to the diffusion of active regions toward the poles and in the longitudinal direction. The IMF gradually decreased until 2019 December (solar minimum) and its variation corresponded to that of the nondipole component ℓ ≥ 2. Our results suggest that the understanding of the open flux problem may be improved by focusing on the equatorial dipole and the nondipole component and that the influence of the polar magnetic field is less significant.

Surface anisotropic magnetoresistance in the antiferromagnetic semiconductor CrSb2

We report on large anisotropic magnetoresistance (AMR) in surface states of an antiferromagnetic semiconductor $\mathrm{Cr}{\mathrm{Sb}}_{2}$. The low-temperature measurement of angle-dependent magnetoresistance (ADMR) is performed in high magnetic fields up to 24 T. At 1.4 K, where the surface conduction is dominant, ADMR exhibits clear twofold symmetry consistent with AMR due to magnetic-field-induced change of antiparallel magnetic structure. The AMR magnitude reaches 9.3% despite the small angle dependence of the net magnetic moments, suggesting strong spin-orbit interaction in the surface conduction layer.

Anomalous Hall effect in ferromagnetic LaCo2As2 and ferrimagnetic NdCo2As2

Abstract We conducted a comparative study of the magnetic and transport properties of single-crystalline LaCo2As2 and NdCo2As2. LaCo2As2 is a soft metallic ferromagnet which exhibits purely intrinsic anomalous Hall effect (AHE) due to Co-3d electrons. With Nd-4f electronic magnetism, ferrimagnetic NdCo2As2 manifests pronounced sign reversal and multiple hysteresis loops in temperature and field dependent magnetization, Hall resistivity and magnetoresistance, due to complicated magnetic structural changes. We reveal that the AHE for NdCo2As2 is stemming from the Co sub-lattice and deduce its phase diagram which includes magnetic compensation and two meta-magnetic phase transitions. The sensitivity of the Hall effect on the details of the magnetic structures in ferrimagnetic NdCo2As2 provides a unique opportunity to explore the magnetic interaction between 4f and 3d electrons and its impact on the electronic structure.

Influence of Cr-ion substitution on the magnetization and dielectric properties of the frustrated Ca3CoMnO6 compound

The Cr-doped Ca3CoMn1-xCrxO6 (x=0, 0.05, 0.1, 0.15) polycrystalline samples were prepared using a modified sol-gel method. The structural, magnetic and dielectric properties were systemically investigated. With increasing Cr3+-doping level, the partial Co2+ ions change to Co3+, leading to a decreased lattice volume. Correspondingly, the length of the short-range magnetic correlation is inhibited and a faster dynamic behavior in time dependent magnetization is found. At the benefit of the magnetic structural changes with the introduction of Cr3+ ions, the relaxor degree of the ferroelectric transition that induced by the exchange striction becomes lower, while the activation energy of the frozen polar-nanoregions increases. The replacement of Mn4+ by Cr3+ also leads to a reduced intra-chain antiferromagnetic coupling and the emergence of Co3+-Co3+ ferromagnetic interaction. As consequence, the Curie-Weiss temperature (θ) increases monotonously. The variation in dielectric permittivity with magnetic field confirms the existence of large magnetodielectric coupling in the Ca3CoMn1-xCrxO6 (0 ​≤ ​x ​≤ ​0.15) samples. Especially for the x ​= ​0.15 sample, the permittivity changes by about 7% under the magnetic field of H=4 ​T.

Significantly Enhanced Room-Temperature Ferromagnetism in Multiferroic EuFeO3-δ Thin Films.

Regulating the magnetic properties of multiferroics lays the foundation for their prospective application in spintronic devices. Single-phase multiferroics, such as rare-earth ferrites, are promising candidates; however, they typically exhibit weak magnetism at room temperature (RT). Here, we significantly boosted the RT ferromagnetism of a representative ferrite, EuFeO3, by oxygen defect engineering. Polarized neutron reflectometry and magnetometry measurements reveal that saturation magnetization reaches 0.04 μB/Fe, which is approximately 5 times higher than its bulk phase. Combining the annular bright-field images with theoretical assessment, we unravel the underlying mechanism for magnetic enhancement, in which the decrease in Fe-O-Fe bond angles caused by oxygen vacancies (VO) strengthens magnetic interactions and tilts Fe spins. Furthermore, the internal relationship between magnetism and VO was established by illustrating how the magnetic structure and magnitude change with VO configuration and concentration. Our strategy for regulating magnetic properties can be applied to numerous functional oxide materials.

Sign reversal in anomalous Hall effect at two Sn compositions in Mn4−xSnxN films on MgO(001) substrates

Rare-earth-free Mn4N has attracted increasing attention as a spintronic material thanks to its ferrimagnetism, perpendicular magnetic anisotropy, and controllability of magnetic properties by partial replacement of Mn atoms with other elements. Here, we grew ∼25-nm-thick Mn4−xSnxN epitaxial films (x = 0–1.4) on MgO(001) substrates by molecular beam epitaxy and investigated their lattice constants and magneto-transport properties. The ratio of the out-of-plane lattice constant c to the in-plane lattice constant a in the Mn4−xSnxN films, c/a, was less than 1 for x < 0.9, but it changed to more than 1 for x = 1.0. Amazingly, the sign of the anomalous Hall effect changed twice with increasing x. These results suggest that the magnetic structure of the Mn4−xSnxN films varies with Sn composition. Possible mechanisms of the magnetic structure change include magnetic compensation, ferrimagnetic–ferromagnetic phase transition, and the formation of noncollinear magnetic structures.

Magnetic Storms During the Space Age: Occurrence and Relation to Varying Solar Activity

AbstractWe study the occurrence of magnetic storms in space age (1957–2021) using Dst and Dxt indices. We find 2,526/2,743 magnetic storms in the Dxt/Dst index, out of which 45% are weak, 40% moderate, 12% intense and 3% major storms. Occurrence of storms in space age follows the slow decrease of sunspot activity and the related change in solar magnetic structure. We quantify the sunspot—coronal mass ejection (CME) storm relation in the five cycles of space age. We explain how the varying solar activity changes the structure of the heliospheric current sheet (HCS), and how this affects the high‐speed solar wind stream (HSS)/corotating interaction region (CIR) storms. Space age started with a record number of storms in 1957–1960, with roughly one storm per week. Solar polar fields attained their maximum in cycle 22, which led to an exceptionally thin HCS, and a space age record of large HSS/CIR storms in 1990s. In the minimum of cycle 23, for the only time in space age, CME storm occurrence reduced below that predicted by sunspots. Weak sunspot activity since cycle 23 has weakened solar polar fields and widened the HCS, which has decreased the occurrence of large and moderate HSS/CIR storms. Because of a wide HCS, the Earth has spent 50% of its time in slow solar wind since cycle 23. The wide HCS has also made large and moderate HSS/CIR storms occur in the early declining phase in recent cycles, while in the more active cycles 20–22 they occurred in the late declining phase.

Magnetism in PrMn0.6Fe0.4O3 compound

The magnetic structure of GdFeO3-type orthorhombically distorted PrMn0.6Fe0.4O3 compound was determined using the neutron powder diffraction experiment. The compound orders into the (Gx, 0, 0) antiferromagnetic structure and with magnetic propagation vector k = (0, 0, 0) in the temperature range TN (∼ 170 K) >T>35 K. Below 35 K the magnetic structure changes to canted antiferromagnetic, with k = (0, 0, 0) and with magnetic moments aligned into (0, Fy, Gz) pattern. Around 35 K there is a possibility of existence of short range magnetic correlations which are connected with rotation of magnetic moment from Gx to Gz and with appearing of ferromagnetic component along the b-axis.

Association of Number of Live Births With Electrocardiographic and Cardiac Structural Changes.

Background Pregnancy is a major life event unique to women and leads to significant hemodynamic, hormonal, and metabolic changes. The purpose of this study was to use the DHS (Dallas Heart Study), a multiethnic population-based cohort study of Dallas county adults, to evaluate the association between number of live births and cardiac magnetic resonance imaging and ECG parameters later in life. Methods and Results Women were included if they had data on self-reported live births and ECG or cardiac magnetic resonance imaging measurements. The 3014 women were stratified by number of live births: 0, 1, 2, 3, 4, and ≥5. Higher number of live births was associated with larger left ventricular (LV) end-diastolic volume (β, 1.31±0.41; P<0.01), LV end-systolic volume (β, 0.83±0.24; P<0.01), and LV mass (β, 1.13±0.49; P=0.02) and lower LV ejection fraction (β, -0.004±0.0014; P<0.01). Increasing parity was associated with longer PR intervals (β, 1.07±0.38; P<0.01). Subgroup analysis by race demonstrated that the association between number of live births and magnetic resonance imaging parameters (LV end-diastolic volume, LV end-systolic volume, and LV ejection fraction) only remained significant in Black women (P value for interaction <0.05). Conclusions Increasing number of live births was associated with electrocardiographic and cardiac structural changes in a multiethnic population. When stratified by race and ethnicity, magnetic resonance imaging structural changes only remained significant in Black participants. Whether these changes are pathologic and increase the risk of heart failure or arrhythmias in multiparous women warrants further investigation.

Giant and reversible electronic structure evolution in a magnetic topological material EuCd2As2

The electronic structure and the physical properties of quantum materials can be significantly altered by charge carrier doping and magnetic state transition. Here we report a discovery of a giant and reversible electronic structure evolution with doping in a magnetic topological material. By performing high-resolution angle-resolved photoemission measurements on EuCd2As2,we found that a huge amount of hole doping can be introduced into the sample surface due to surface absorption. The electronic structure exhibits a dramatic change with the hole doping which can not be described by a rigid band shift. Prominent band splitting is observed at high doping which corresponds to a doping-induced magnetic transition at low temperature (below -15 K) from an antiferromagnetic state to a ferromagnetic state. These results have established a detailed electronic phase diagram of EuCd2As2 where the electronic structure and the magnetic structure change systematically and dramatically with the doping level. They further suggest that the transport, magnetic and topological properties of EuCd2As2 can be greatly modified by doping. These work will stimulate further investigations to explore for new phenomena and properties in doping this magnetic topological material.