Photon Bunching Research Articles

Realization of one-dimensional anyons with arbitrary statistical phase.

Low-dimensional quantum systems can host anyons, particles with exchange statistics that are neither bosonic nor fermionic. However, the physics of anyons in one dimension remains largely unexplored. In this work, we realize Abelian anyons in one dimension with arbitrary exchange statistics using ultracold atoms in an optical lattice, where we engineer the statistical phase through a density-dependent Peierls phase. We explore the dynamical behavior of two anyons undergoing quantum walks and observe the anyonic Hanbury Brown-Twiss effect as well as the formation of bound states without on-site interactions. Once interactions are introduced, we observe spatially asymmetric transport in contrast to the symmetric dynamics of bosons and fermions. Our work forms the foundation for exploring the many-body behavior of one-dimensional anyons.

Coherent Coupling of a Diamond Tin-Vacancy Center to a Tunable Open Microcavity

Efficient coupling of optically active qubits to optical cavities is a key challenge for solid-state-based quantum optics experiments and future quantum technologies. Here we present a quantum photonic interface based on a single tin-vacancy center in a micrometer-thin diamond membrane coupled to a tunable open microcavity. We use the full tunability of the microcavity to selectively address individual tin-vacancy centers within the cavity mode volume. Purcell enhancement of the tin-vacancy center optical transition is evidenced both by optical excited state lifetime reduction and by optical linewidth broadening. As the emitter selectively reflects the single-photon component of the incident light, the coupled emitter-cavity system exhibits strong quantum nonlinear behavior. On resonance, we observe a transmission dip of 50% for low incident photon number per Purcell-reduced excited state lifetime, while the dip disappears as the emitter is saturated with higher photon number. Moreover, we demonstrate that the emitter strongly modifies the photon statistics of the transmitted light by observing photon bunching. This work establishes a versatile and tunable platform for advanced quantum optics experiments and proof-of-principle demonstrations on quantum networking with solid-state qubits. Published by the American Physical Society 2024

Two photons everywhere.

We discuss two-photon physics, taking for illustration the particular but topical case of resonance fluorescence. We show that the basic concepts of interferences and correlations provide at the two-photon level an independent and drastically different picture than at the one-photon level, with landscapes of correlations that reveal various processes by spanning over all the possible frequencies at which the system can emit. Such landscapes typically present lines of photon bunching and circles of antibunching. The theoretical edifice to account for these features rests on two pillars: (i) a theory of frequency-resolved photon correlations and (ii) admixing classical and quantum fields. While experimental efforts have been to date concentrated on correlations between spectral peaks, strong correlations exist between photons emitted away from the peaks, which are accessible only through multi-photon observables. These could be exploited for both fundamental understanding of quantum-optical processes as well as applications by harnessing these unsuspected resources. This article is part of the theme issue 'Celebrating the 15th anniversary of the Royal Society Newton International Fellowship'.

Emission dynamics of optically driven aluminum nitride quantum emitters

Aluminum nitride is a technologically important wide band-gap semiconductor which has been shown to host bright quantum emitters. We use photon emission correlation spectroscopy (PECS), time-resolved photoluminescence (TRPL), and state-population dynamic simulations to probe the dynamics of emission under continuous wave (CW) and pulsed optical excitation. We infer that there are at least four dark shelving states, which govern the TRPL, bunching, and saturation of the optical transition. We study in detail the emission dynamics of two quantum emitters (QEs) with differing power-dependent shelving processes, hypothesized to result from charge ionization and recombination. These results demonstrate that photon bunching caused by shelving the system in a dark state inherently limits the saturation rate of the photon source. In emitters where increasing optical power deshelves the dark states, we observe an increased photon emission intensity. Published by the American Physical Society 2024

The Intermode Polariton Parametric Scattering Laser in a Strong Coupled Microcavity Via Two-Photon Absorption.

Exciton-polaritons, hybrid quasiparticles from the strong coupling of excitons and cavity photons in semiconductor microcavities, offer a platform for exploring quantum coherence and nonlinear optical properties. The unique polariton parametric scattering (PPS) laser is of interest for its potential in quantum technologies and nonlinear devices. However, direct resonant excitation of polaritons in strong-coupling microcavities is challenging. This study proposes an innovative two-photon absorption (TPA) pump mechanism to address this. We observe TPA-driven PPS lasing in a strongly coupled microcavity at room temperature. High K-value exciton injections promote coherent stimulated emission of polariton scattering through intermode channels. Angle-resolved spectra confirm a TPA process, showing evolution from pump-state to signal-state. Hanbury Brown-Twiss measurement of second-order correlation g2(τ) of signal state indicates a phase transition from a classical thermal state to a quantum coherent state. Theoretical modeling provides insights into the physical mechanisms of PPS. Our work advances nonlinear phenomena exploration in strongly coupled light-matter systems, contributing to quantum polaritonics and nonlinear optics.

Photon discerner: adaptive quantum optical sensing near the shot noise limit

Photon statistics of an optical field can be used for quantum optical sensing in low light level scenarios free of bulky optical components. However, photon-number-resolving detection to unravel the photon statistics is challenging. Here, we propose a novel detection approach, that we call ‘photon discerning’, which uses adaptive photon thresholding for photon statistical estimation without recording exact photon numbers. Our photon discerner is motivated by the field of neural networks where tunable thresholds have proven efficient for information extraction in machine learning tasks. The photon discerner maximizes Fisher information per photon by iteratively choosing the optimal threshold in real-time to approach the shot noise limit. Our proposed scheme of adaptive photon thresholding leads to unique remote-sensing applications of quantum degree of linear polarization camera and quantum LiDAR. We investigate optimal thresholds and show that the optimal photon threshold can be counter-intuitive (not equal to 1) even for weak signals (mean photon number much less than 1), due to the photon bunching effect. We also put forth a superconducting nanowire realization of the photon discerner which can be experimentally implemented in the near-term. We show that the adaptivity of our photon discerner enables it to beat realistic photon-number-resolving detectors with limited photon-number resolution in certain applications. Our work suggests a new class of detectors for information-theory driven, compact, and learning-based quantum optical sensing.

Polarization-engineered photon statistics and its tomography via optomagnonic interaction.

Cavity optomagnonics has received considerable research interest in recent years, due to the coherent magnetic Brillioun light scattering in the ferromagnetic material. Here, we theoretically propose and numerically verify a feasible scheme for the full polarization tomography on photon statistics in an optomagnonic whispering-gallery-mode microresonator system in the weak-coupling regime. By performing the polarization pre- and post-selections to manipulate the polarization states of the input and output photons, we find that the rich sub- and super-Poissonian photon statistics can be selectively generated, thanks to quantum interferences. In the parameter space of phase delay, the evolution from photon bunching to antibunching indicates the change from phase to amplitude squeezing. Our obtained result has potential applications in tunable quantum polarized light sources based on the cavity optomagnonic platform in micro-nano scale. It also offers a deeper understanding for full quantum cavity optomagnonics.

Squeezing and bunching of photons of coherent light interacting with two quantum anharmonic oscillators coupled through the angular momentum

Squeezing and bunching of photons of coherent light interacting with two quantum anharmonic oscillators coupled through the angular momentum

Diffusion-Dominated Luminescence Dynamics of CsPbBr3 Studied Using Cathodoluminescence and Microphotoluminescence Spectroscopy.

Time-resolved or time-correlation measurements using cathodoluminescence (CL) reveal the electronic and optical properties of semiconductors, such as their carrier lifetimes, at the nanoscale. However, halide perovskites, which are promising optoelectronic materials, exhibit significantly different decay dynamics in their CL and photoluminescence (PL). We conducted time-correlation CL measurements of CsPbBr3 using Hanbury Brown-Twiss interferometry and compared them with time-resolved PL. The measured CL decay time was on the order of subnanoseconds and was faster than PL decay at an excited carrier density of 2.1 × 1018 cm-3. Our experiment and analytical model revealed the CL dynamics induced by individual electron incidences, which are characterized by highly localized carrier generation followed by a rapid decrease in carrier density due to diffusion. This carrier diffusion can play a dominant role in the CL decay time for undoped semiconductors, in general, when the diffusion dynamics are faster than the carrier recombination.

Two-dimensional control of a biphoton joint spectrum.

Control over the joint spectral amplitude of a photon pair has proved highly desirable for many quantum applications, since it contains the spectral quantum correlations, and has crucial effects on the indistinguishability of photons, as well as promising emerging applications involving complex quantum functions and frequency encoding of qudits. Until today, this has been achieved by engineering a single degree of freedom, either by custom poling nonlinear crystal or by shaping the pump pulse. We present a combined approach where two degrees of freedom, the phase-matching function, and the pump spectrum, are controlled. This approach enables the two-dimensional control of the joint spectral amplitude, generating a variety of spectrally encoded quantum states - including frequency uncorrelated states, frequency-bin Bell states, and biphoton qudit states. In addition, the joint spectral amplitude is controlled by photon bunching and anti-bunching, reflecting the symmetry of the phase-matching function.

Photon noise correlations in millimeter-wave telescopes.

Many modern millimeter and submillimeter ("mm-wave") telescopes for astronomy are deploying more detectors by increasing the detector pixel density and, with the rise of lithographed detector architectures and high-throughput readout techniques, it is becoming increasingly practical to overfill the focal plane. However, when the pixel pitch p p i x is small compared to the product of the wavelength λ and the focal ratio F, or p p i x ≲1.2F λ, the Bose term of the photon noise correlates between neighboring detector pixels due to the Hanbury Brown and Twiss (HBT) effect. When this HBT effect is non-negligible, the array-averaged sensitivity scales with the detector count N det less favorably than the uncorrelated limit of Ndet-1/2. In this paper, we present a general prescription to calculate this HBT correlation based on a quantum optics formalism and extend it to polarization-sensitive detectors. We then estimate the impact of HBT correlations on the sensitivity of a model mm-wave telescope and discuss the implications for a focal plane design.

Scintillation and cherenkov photon counting detectors with analog silicon photomultipliers for TOF-PET

Objective. Standard signal processing approaches for scintillation detectors in positron emission tomography (PET) derive accurate estimates for 511 keV photon time of interaction and energy imparted to the detection media from aggregate characteristics of electronic pulse shapes. The ultimate realization of a scintillation detector for PET is one that provides a unique timestamp and position for each detected scintillation photon. Detectors with these capabilities enable advanced concepts for three-dimensional (3D) position and time of interaction estimation with methods that exploit the spatiotemporal arrival time kinetics of individual scintillation photons. Approach. In this work, we show that taking into consideration the temporal photon emission density of a scintillator, the channel density of an analog silicon photomultiplier (SiPM) array, and employing fast electronic readout with digital signal processing, a detector that counts and timestamps scintillation photons can be realized. To demonstrate this approach, a prototype detector was constructed, comprising multichannel electronic readout for a bismuth germanate (BGO) scintillator coupled to an SiPM array. Main Results. In proof-of-concept measurements with this detector, we were able to count and provide unique timestamps for 66% of all optical photons, where the remaining 34% (two-or-more-photon pulses) are also independently counted, but each photon bunch shares a common timestamp. We show this detector concept can implement 3D positioning of 511 keV photon interactions and thereby enable corrections for time of interaction estimators. The detector achieved 17.6% energy resolution at 511 keV and 237 ± 10 ps full-width-at-half-maximum coincidence time resolution (CTR) (fast spectral component) versus a reference detector. We outline the methodology, readout, and approach for achieving this detector capability in first-ever, proof-of-concept measurements for scintillation photon counting detector with analog silicon photomultipliers. Significance. The presented detector concept is a promising design for large area, high sensitivity TOF-PET detector modules that can implement advanced event positioning and time of interaction estimators, which could push state-of-the-art performance.

Squeezed correlations of bosons with nonzero widths for expanding sources

We explore the squeezed back-to-back correlation (SBBC) and investigate how the squeezing effect influences the Hanbury-Brown–Twiss (HBT) interferometry using an expanding Gaussian source with nonzero width. The SBBC and HBT of D0 and ϕ mesons with finite in-medium widths are studied. The expanding flow of the source may enhance the SBBC strength of D0D¯0 and ϕϕ in the low momentum region but suppress the SBBC in the larger momentum region. The squeezing effect suppresses the influence of flow on the HBT radii, which is significant for two identical bosons with large pair momentum or with large mass. Due to the squeezing effect, the relationship between the HBT radii and the pair momentum exhibits nonflow behavior for the D0D0 pair. Likewise, nonflow behavior also appears in the HBT radii of ϕϕ with large pair momentum. This phenomenon may bring new insights for studying the squeezing effect. Published by the American Physical Society 2024

Analysis of photon bunching in coherent cathodoluminescence

Analysis of photon bunching in coherent cathodoluminescence

Second-Order Temporal Coherence of Polariton Lasers Based on an Atomically Thin Crystal in a Microcavity.

Bosonic condensation and lasing of exciton polaritons in microcavities is a fascinating solid-state phenomenon. It provides a versatile platform to study out-of-equilibrium many-body physics and has recently appeared at the forefront of quantum technologies. Here, we study the photon statistics via the second-order temporal correlation function of polariton lasing emerging from an optical microcavity with an embedded atomically thin MoSe_{2} crystal. Furthermore, we investigate the macroscopic polariton phase transition for varying excitation powers and temperatures. The lower-polariton exhibits photon bunching below the threshold, implying a dominant thermal distribution of the emission, while above the threshold, the second-order correlation transits towards unity, which evidences the formation of a coherent state. Our findings are in agreement with a microscopic numerical model, which explicitly includes scattering with phonons on the quantum level.

Investigation of the generalised Wigner–Dunkl harmonic oscillator and its coherent states

This study investigates the quantum mechanics of the harmonic oscillator in the presence of the Generalised-Wigner–Dunkl formalism based on creation and annihilation operators, which include also the reflection operator. We provide explicit results on the spectral properties of the Hamiltonian and an explicit form of the quantum propagator. Deformed coherent states are introduced and their non-classical properties such as photon statistics, Mandel parameter, and bunching or anti-bunching effect are studied.

Noise-induced dynamics and photon statistics in bimodal quantum-dot micropillar lasers

Emission characteristics of quantum-dot micropillar lasers (QDMLs) are located at the intersection of nanophotonics and nonlinear dynamics, which provides an ideal platform for studying the optical interface between classical and quantum systems. In this work, a noise-induced bimodal QDML with orthogonal dual-mode outputs is modeled, and nonlinear dynamics, stochastic mode jumping and quantum statistics with the variation of stochastic noise intensity are investigated. Noise-induced effects lead to the emergence of two intensity bifurcation points for the strong and the weak mode, and the maximum output power of the strong mode becomes larger as the noise intensity increases. The anti-correlation of the two modes reaches the maximum at the second intensity bifurcation point. The dual-mode stochastic jumping frequency and effective bandwidth can exceed 100 GHz and 30 GHz under the noise-induced effect. Moreover, the noise-induced photon correlations of both modes simultaneously exhibit super-thermal bunching effects () in the low injection current region. The -value of the strong mode can reach over 6 in the high injection current region. Photon bunching () of both modes is observed over a wide range of noise intensities and injection currents. In the presence of the noise-induced effect, the photon number distribution of the strong or the weak mode is a mixture of Bose–Einstein and Poisson distributions. As the noise intensity increases, the photon number distribution of the strong mode is dominated by the Bose–Einstein distribution, and the proportion of the Poisson distribution is increased in the high injection current region, while that of the weak mode is reduced. Our results contribute to the development preparation of super-bunching quantum integrated light sources for improving the spatiotemporal resolution of quantum sensing measurements and enhancing the security of optical communication.

Nonreciprocal unconventional photon blockade in atom-cavity with χ(2) nonlinear medium

In this paper, we show that the photon blockade (PB) can be observed in a nonreciprocal way with a driven spinning atom-cavity coupled filled with [Formula: see text] nonlinear medium. We analytically derive the optimal conditions for strong photon antibunching, which are in good agreement with those obtained by numerical simulations. Under the weak driving condition, we discuss the physical origins of the nonreciprocal unconventional photon blockade (UPB), which originates from the destructive quantum interference between different paths from the ground state to two-photon states by driving the device from the left side. While the quantum interference paths are broken when the device is driven from the right side, which leads to the occurrence of the photon bunching. Moreover in the opposite direction of driving the device, we also observe another nonreciprocal UPB effect, which can occur by generating bunching and antibunching effects via driving the device from the left and right sides under the derived optimal conditions, respectively. Finally, we cannot observe the nonreciprocal UPB phenomenon with the large cavity decay compared to the atomic spontaneous emission rate (or the bad cavity limit), and give the physical reason behind it. Possible experimental implementation for this scheme is presented.

Hanbury Brown-Twiss approach for imaging through a dynamic scattering medium.

The Hanbury Brown-Twiss approach, associated with the correlation of intensity fluctuations at two different points in a wave field, unveils fundamental aspects of light. Here, we propose and experimentally demonstrate an imaging and phase recovery technique through a dynamic scattering medium using the Hanbury Brown-Twiss approach. A detailed theoretical basis is presented and verified by experimental demonstrations. To validate the application of the proposed technique, the randomness of the dynamically scattered light is exploited using temporal ergodicity for evaluating the correlation of intensity fluctuations and consequently applying it in the reconstruction of the object hidden behind the dynamic diffuser.

Boson bunching is not maximized by indistinguishable particles

Boson bunching is among the most remarkable features of quantum physics. A celebrated example in optics is the Hong–Ou–Mandel effect, where the bunching of two photons arises from a destructive quantum interference between the trajectories where they both either cross a beamsplitter or are reflected. This effect takes its roots in the indistinguishability of identical photons. Hence, it is generally admitted—and experimentally verified—that bunching vanishes as soon as photons can be distinguished, for example, when they occupy distinct time bins or have different polarizations. Here we disprove this alleged straightforward link between indistinguishability and bunching by exploiting a recent finding in the theory of matrix permanents. We exhibit a family of optical circuits such that the bunching of photons into two modes can be substantially boosted by making them partially distinguishable via an appropriate polarization pattern. This boosting effect is already visible in a seven-photon interferometric process, making the observation of this phenomenon within reach of current photonic technology. This unexpected behaviour questions our understanding of multiparticle interference in the grey zone between indistinguishable bosons and classical particles. A common belief about boson bunching—fully indistinguishable bosons exhibit the utmost bunching—is theoretically disproved with seven photons of distinct polarization in a seven-mode interferometric process. Enhanced bunching could thus be observed with partially distinguishable photons.