cntTSP is a flow visualization technique that combines temperature-sensitive paint (TSP) and carbon nanotube (CNT). TSP is a sprayable temperature sensor, and CNT is used as a thin inner electric heater for the TSP. The cntTSP technique allows the visualization of the movement of the boundary layer transition on a moving airfoil. In this study, cntTSP was applied to a pitch-oscillating airfoil in a low-speed wind tunnel. Three methods were compared as methods for detecting the boundary layer transition position. The transition position was successfully evaluated using a heat transfer coefficient that was calculated by the surface temperature. Moreover, at a high-reduced frequency, the detected transition positions were different between the pitching-up and pitching-down procedure. Moreover, we observed a hysteresis loop of the transition position.