Binary Bose Mixtures Research Articles

Anderson localization of elementary excitations in disordered binary Bose mixtures: Effects of the Lee-Huang-Yang quantum and thermal corrections

We investigate analytically and numerically the Anderson localization of quasiparticles in binary Bose mixtures in the presence of the Lee-Huang-Yang quantum and thermal corrections subjected to correlated disordered potentials. We calculate the density profiles, the Bogoliubov quasiparticle modes, and the localization length in both the mixture and droplet phases. We show that for one-dimensional speckle potentials, the peculiar interplay of disorder and the Lee-Huang-Yang fluctuations may enhance localization in one component while inducing delocalization in the other. Our results reveal also that thermal fluctuations lead to the emergence of two and multiple localization maxima. In the droplet state, our findings indicate that the Anderson localization of quasiparticles is weak in the flat-top region since its excitation modes are restricted to those below the particle-emission threshold. Published by the American Physical Society 2024

Attractive Solution of Binary Bose Mixtures: Liquid-Vapor Coexistence and Critical Point.

We study the thermodynamic behavior of attractive binary Bose mixtures using exact path-integral MonteCarlo methods. Our focus is on the regime of interspecies interactions where the ground state is in a self-bound liquid phase, stabilized by beyond mean-field effects. We calculate the isothermal curves in the pressure vs density plane for different values of the attraction strength and establish the extent of the coexistence region between liquid and vapor using the Maxwell construction. Notably, within the coexistence region, Bose-Einstein condensation occurs in a discontinuous way as the density jumps from the normal gas to the superfluid liquid phase. Furthermore, we determine the critical point where the line of first-order transition ends and investigate the behavior of the density discontinuity in its vicinity. We also point out that the density discontinuity at the transition could be observed in experiments of mixtures in traps.

Phase separation in binary Bose mixtures at finite temperature

We investigate the magnetic behavior of finite-temperature repulsive two-component Bose mixtures by means of exact path-integral Monte-Carlo simulations. Novel algorithms are implemented for the free energy and the chemical potential of the two components. Results on the magnetic susceptibility suggest that the conditions for phase separation are not modified from the zero temperature case. This contradicts previous predictions based on approximate theories. We also determine the temperature dependence of the chemical potential and the contact parameters for experimentally relevant balanced mixtures.

Discrete quantum droplets in one-dimensional binary Bose–Einstein condensates

We discuss the propagation and interaction of discrete quantum droplets in one-dimensional binary Bose mixtures by variationally and numerically solving the underlying generalized discrete Gross–Pitaevskii equation. Useful analytical expressions are obtained for the energy, the chemical potential, the density profile, and the droplet separation in the regime of a small droplet. We show that for weak lattice coupling, the stationary state of small droplets remains intact and does not display any special structures. An irregular dynamics is observed in both single and dual droplets with flat-top plateau in the limit of relatively strong coupling. Our results reveal also that two droplets interact weakly and cannot form a bound-state due to the intriguing interplay of the discreteness and quantum fluctuations.

Thermally induced local imbalance in repulsive binary Bose mixtures

Thermally induced local imbalance in repulsive binary Bose mixtures

Impurities in quasi-one-dimensional droplets of binary Bose mixtures

Impurities in quasi-one-dimensional droplets of binary Bose mixtures

Quantum Criticality of Liquid-Gas Transition in a Binary Bose Mixture.

Quantum liquid, in the form of a self-bound droplet, is stabilized by a subtle balance between the mean-field contribution and quantum fluctuations. While a liquid-gas transition is expected when such a balance is broken, it remains elusive whether liquid-gas critical points exist in the quantum regime. Here, we study the quantum criticality in a binary Bose mixture undergoing the liquid-gas transition. We show that, beyond a narrow stability window of the self-bound liquid, a liquid-gas coexistence persists, which eventually transits into a homogeneous mixture. Importantly, we identify two distinct critical points where the liquid-gas coexistence terminates. These critical points are characterized by rich critical behaviors in their vicinity, including divergent susceptibility, unique phonon-mode softening, and enhanced density correlations. The liquid-gas transition and the critical points can be readily explored in ultracold atoms confined to a box potential. Our work highlights the thermodynamic approach as a powerful tool in revealing the quantum liquid-gas criticality, and paves the way for further studies of critical phenomena in quantum liquids.

Spin conductivity spectrum and spin superfluidity in a binary Bose mixture

We investigate the spectrum of spin conductivity for a miscible two-component Bose-Einstein condensate (BEC) that exhibits spin superfluidity. By using the Bogoliubov theory, the regular part being the spin conductivity at finite ac frequency and the spin Drude weight characterizing the delta-function peak at zero frequency are analytically computed. We demonstrate that the spectrum exhibits a power-law behavior at low frequency, reflecting gapless density and spin modes specific to the binary BEC. At the phase transition points into immiscible and quantum-droplet states, the change in quasiparticle dispersion relations modifies the power law. In addition, the spin Drude weight becomes finite, indicating zero spin resistivity due to spin superfluidity. Our results also suggest that the Andreev-Bashkin drag density is accessible by measuring the spin conductivity spectrum.

Miscibility of dual-species Bose-Einstein condensates

<sec>The miscibility of quantum liquids is an interesting topic in many-body physics, which has been intensively investigated in <sup>3</sup>He-<sup>4</sup>He superfluids and the mixtures of ultracold atoms. In the context of dual species Bose-Einstein condensates, the mean-field description has been well established, according to which, the miscibility condition is density independent and determined only by the ratio of inter- and intra-species interaction strength. Recently, Nadion and Petrov proposed that [<ext-link ext-link-type="uri" xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="http://doi.org/10.1103/PhysRevLett.126.115301"><i>Phys. Rev. Lett.</i> <b>126</b> 115301</ext-link>], in the vicinity of the mixing-demixing threshold, quantum fluctuations play an important role to affect the equilibrium stability, and as a result, the partially miscible state emerges. This new phase of quantum matter opens up new perspectives to explore the beyond mean-field effect in ultracold atomic gases.</sec><sec>In this work, according to the equation of state taking the Lee-Huang-Yang correction into consideration, we investigate the ground state phase diagram of repulsive binary Bose mixtures in the interacting regime suffering a weak mean-field instability. Under the thermodynamic balance conditions, the phase boundaries between the immiscible state, partially miscible state and the homogenous state are determined. For the equal-mass case, these phase transitions only take place on condition that intra-species interactions are in an asymmetric form. In terms of interaction parameters, we explicitly derive analytical expressions of the phase boundaries, which are appropriate to describe the transitions in sufficiently dilute atomic gases. At the quantum critical point, where the partially miscible state terminates, the susceptibility tensor of the density response exhibits a divergent behavior. For the unequal-mass case, the beyond-mean-field equation of state cannot be written in a compact form, thus the determination of the phase boundaries is more involved. By expanding the Lee-Huang-Yang energy expression to the terms linear in the concentration of the minority species, we analytically obtain the threshold density for the partially miscible transition. We also propose a discriminant function, from which the configuration of the partially miscible state can be identified for the given mass ratio and interaction strength. Applications of these theoretical results to experimental systems, such as sodium, potassium, and rubidium gases, are presented.</sec>

Self-consistent theory of a homogeneous binary Bose mixture with strong repulsive interspecies interaction

Multicomponent quantum gases are ideal platforms to study fundamental phenomena arising from the mutual interaction between different constituents. Particularly, due to the repulsive interactions between two species, the system may exhibit a phase separation. We develop a mean-field-based theory for a two-component Bose mixture, which is equivalent to the Hartree-Fock-Bogoliubov approximation, and derive analytical expressions for the phase boundary and miscibility. The majority of existing theories, which are valid only for weakly interacting Bose gases, predict that the phase boundary is determined by the criterion $g_{ab}\leqslant\sqrt{g_{aa} g_{bb}}$ (where $g_{ab}$ is a coupling constant between the components $a$ and $b$). We show that in the Bose-Einstein-condensation phase ($T\leqslant T_c$) the system may remain in a stable and miscible phase also for larger values of $g_{ab}$, depending on the gas parameter $\gamma$ and temperature.

Spinor-induced instability of kinks, holes and quantum droplets

We address the existence and stability of one-dimensional (1D) holes and kinks and two-dimensional (2D) vortex-holes nested in extended binary Bose mixtures, which emerge in the presence of Lee–Huang–Yang (LHY) quantum corrections to the mean-field energy, along with self-bound quantum droplets. We consider both the symmetric system with equal intra-species scattering lengths and atomic masses, modeled by a single (scalar) LHY-corrected Gross–Pitaevskii equation (GPE), and the general asymmetric case with different intra-species scattering lengths, described by two coupled (spinor) GPEs. We found that in the symmetric setting, 1D and 2D holes can exist in a stable form within a range of chemical potentials that overlaps with that of self-bound quantum droplets, but that extends far beyond it. In this case, holes are found to be always stable in 1D and they transform into pairs of stable out-of-phase kinks at the critical chemical potential at which localized droplets turn into flat-top states, thereby revealing the connection between localized and extended nonlinear states. In contrast, we found that the spinor nature of the asymmetric systems may lead to instability of 1D holes, which tend to break into two gray states moving in the opposite directions. Remarkably, such instability arises due to spinor nature of the system and it affects only holes nested in extended modulationally-stable backgrounds, while localized quantum droplet families remain completely stable, even in the asymmetric case, while 1D holes remain stable only close to the point where they transform into pairs of kinks. We also found that symmetric systems allow fully stable 2D vortex-carrying single-charge states at moderate amplitudes, while unconventional instabilities appear also at high amplitudes. Symmetry also strongly inhibits instabilities for double-charge vortex-holes, which thus exhibit unexpectedly robust evolutions at low amplitudes.

Ultradilute Quantum Droplets in the Presence of Higher-Order Quantum Fluctuations

We investigate the effects of higher-order quantum fluctuations on the bulk properties of self-bound droplets in three-, two- and one-dimensional binary Bose mixtures using the Hartree–Fock–Bogoliubov theory. We calculate higher-order corrections to the equation of state of the droplet at both zero and finite temperatures. We show that our results for the ground-state energy are in a good agreement with recent quantum Monte Carlo simulations in any dimension. Our study extends to the finite temperature case where it is found that thermal fluctuations may destabilize the droplet state and eventually destroy it. In two dimensions, we reveal that the droplet occurs at temperatures well below the Berezinskii–Kosterlitz–Thouless transition temperature.

Finite-temperature spin dynamics of a two-dimensional Bose-Bose atomic mixture

We examine the role of thermal fluctuations in uniform two-dimensional binary Bose mixtures of dilute ultracold atomic gases. We use a mean-field Hartree-Fock theory to derive analytical predictions for the miscible-immiscible transition. A nontrivial result of this theory is that a fully miscible phase at $T=0$ may become unstable at $T\neq0$, as a consequence of a divergent behaviour in the spin susceptibility. We test this prediction by performing numerical simulations with the Stochastic (Projected) Gross-Pitaevskii equation, which includes beyond mean-field effects. We calculate the equilibrium configurations at different temperatures and interaction strengths and we simulate spin oscillations produced by a weak external perturbation. Despite some qualitative agreement, the comparison between the two theories shows that the mean-field approximation is not able to properly describe the behavior of the two-dimensional mixture near the miscible-immiscible transition, as thermal fluctuations smoothen all sharp features both in the phase diagram and in spin dynamics, except for temperature well below the critical temperature for superfluidity.

Ultradilute self-bound quantum droplets in Bose–Bose mixtures at finite temperature* *Project supported by the Australian Research Council’s (ARC) Discovery Program (Grant Nos. DE180100592 and DP190100815), (Grant No. DP180102018), and (Grant No. DP170104008).

We theoretically investigate the finite-temperature structure and collective excitations of a self-bound ultradilute Bose droplet in a flat space realized in a binary Bose mixture with attractive inter-species interactions on the verge of mean-field collapse. As the droplet formation relies critically on the repulsive force provided by Lee–Huang–Yang quantum fluctuations, which can be easily compensated by thermal fluctuations, we find a significant temperature effect in the density distribution and collective excitation spectrum of the Bose droplet. A finite-temperature phase diagram as a function of the number of particles is determined. We show that the critical number of particles at the droplet-to-gas transition increases dramatically with increasing temperature. Towards the bulk threshold temperature for thermally destabilizing an infinitely large droplet, we find that the excitation-forbidden, self-evaporation region in the excitation spectrum, predicted earlier by Petrov using a zero-temperature theory, shrinks and eventually disappears. All the collective excitations, including both surface modes and compressional bulk modes, become softened at the droplet-to-gas transition. The predicted temperature effects of a self-bound Bose droplet in this work could be difficult to measure experimentally due to the lack of efficient thermometry at low temperatures. However, these effects may already present in the current cold-atom experiments.

Thermodynamics of dilute Bose gases: Beyond mean-field theory for binary mixtures of Bose-Einstein condensates

We study the thermodynamic properties of binary Bose mixtures, by developing a beyond mean-field Popov theory which properly includes the effects of quantum and thermal fluctuations in both the density and spin channels. Results for key thermodynamic quantities, such as the isothermal compressibility and the magnetic susceptibility, are derived from a perturbative calculation of the grand-canonical potential. We find that thermal fluctuations can play a crucial role on the miscibility condition of a binary mixture, favoring phase separation at finite temperature even if the mixture is soluble at zero temperature, as already anticipated in a previous work [Ota et al., Phys. Rev. Lett. 123, 075301 (2019)]. We further investigate the miscibility condition for binary mixtures in the presence of asymmetry in the intra-species interactions, as well as in the masses of the two components. Furthermore, we discuss the superfluid behavior of the mixture and the temperature dependence of the Andreev-Bashkin effect.

Superfluidity and coherence in uniform dipolar binary Bose mixtures

We investigate the superfluidity and the coherence in dipolar binary Bose mixtures using the hydrodynamic approach. Useful analytical formulas for the excitation spectra, the first-order correlation function, the static structure factor, and the superfluid fraction are derived. We find that in the case of highly imbalanced mixture, the superfluidity can occur in the dilute component only at extremely low temperatures. The behavior of the first-order correlation function for both dipolar and nondipolar Bose mixtures is deeply analyzed. Then we face the two-dimensional case which encodes a non-trivial physics due to the roton modes.

Microscopic derivation of the extended Gross-Pitaevskii equation for quantum droplets in binary Bose mixtures

An ultradilute quantum droplet is a self-bound liquid-like state recently observed in ultracold Bose-Einstein condensates. In all previous theoretical studies, it is described by a phenomenological low-energy effective theory, termed as the extended Gross\textendash Pitaevskii equation. Here, we microscopically derive the Gross\textendash Pitaevskii equation for the condensate and also for a pairing field in an inhomogeneous quantum droplet realized by Bose-Bose mixtures with attractive inter-species interaction. We show that the inclusion of the pairing field is essential, in order to have a consistent description of the droplet state. We clarify that, the extended Gross\textendash Pitaevskii equation used earlier should be understood as the equation of motion for the pairing field, rather than the condensate. The fluctuations of the pairing field give rise to low-energy collective excitations of the droplet. We also present the Bogoliubov equations for gapless phonon modes and gapped modes due to pairing in real space, which characterizes single-particle-like excitations of the droplet. The equations of motion derived in this work for the condensate and the pairing field serve an ideal starting point to understand the structure and collective excitations of non-uniform ultradilute quantum droplets in on-going cold-atom experiments.

Microscopic pairing theory of a binary Bose mixture with interspecies attractions: Bosonic BEC-BCS crossover and ultradilute low-dimensional quantum droplets

Ultradilute quantum droplets are intriguing new state of matter, in which the attractive mean-field force can be balanced by the repulsive force from quantum fluctuations to avoid collapse. Here, we present a microscopic theory of ultradilute quantum droplets in three-, one- and two-dimensional two-component Bose-Bose mixtures, by generalizing the conventional Bogoliubov theory to include the bosonic pairing arising from the interspecies attraction. Our pairing theory is fully equivalent to a variational approach and hence gives an upper bound for the energy of quantum droplets. In three dimensions, we predict the existence of a strongly interacting Bose droplet at the crossover from Bose-Einstein condensates (BEC) to Bardeen--Cooper--Schrieffer (BCS) superfluids and map out the bosonic BEC-BCS crossover phase diagram. In one dimension, we find that the energy of the one-dimensional Bose droplet calculated by the pairing theory is in an excellent agreement with the latest diffusion Monte Carlo simulation {[}Phys. Rev. Lett. \textbf{122}, 105302 (2019){]}, for nearly all the interaction strengths at which quantum droplets exist. In two dimensions, we show that Bose droplets disappear and may turn into a soliton-like many-body bound state, when the interspecies attraction exceeds a critical value. Below the threshold, the pairing theory predicts more or less the same results as the Bogoliubov theory derived by Petrov and Astrakharchik {[}Phys. Rev. Lett. \textbf{117}, 100401 (2016){]}. The predicted energies from both theories are higher than the diffusion Monte Carlo results, due to the weak interspecies attraction and the increasingly important role played by the beyond-Bogoliubov-approximation effect in two dimensions.

Coupled superfluidity of binary Bose mixtures in two dimensions

We consider a two-component Bose gas in two dimensions at low temperature with short-range repulsive interaction. In the coexistence phase where both components are superfluid, inter-species interactions induce a nondissipative drag between the two superfluid flows (Andreev-Bashkin effect). We show that this behavior leads to a modification of the usual Berezinskii-Kosterlitz-Thouless (BKT) transition in two dimensions. We extend the renormalization of the superfluid densities at finite temperature using the renormalization group approach and find that the vortices of one component have a large influence on the superfluid properties of the other, mediated by the nondissipative drag. The extended BKT flow equations indicate that the occurrence of the vortex unbinding transition in one of the components can induce the breakdown of superfluidity also in the other, leading to a locking phenomenon for the critical temperatures of the two gases.

Fluctuations and quantum self-bound droplets in a dipolar Bose-Bose mixture

We systematically investigate the properties of three-dimensional dipolar binary Bose mixture at low temperatures. A set of coupled self-consistent equations of motion are derived for the two condensates. In the homogeneous case, useful analytical formulas for the condensate depletion, the anomalous density, the ground-state energy, and the equation of state are obtained. The theory is extended to the inhomogeneous case and the importance of the inhomogeneity is highlighted. Our results open up an avenue for studying dipolar mixture droplets. Impacts of the dipole-dipole interaction on the stability, density profiles, and the size of the self-bound droplet are deeply discussed. The finite-temperature behavior of such a state is also examined.