Atomic Spin Ensembles Research Articles

Graph states of atomic ensembles engineered by photon-mediated entanglement

Graph states are a broad family of entangled quantum states, each defined by a graph composed of edges representing the correlations between subsystems. Such states constitute versatile resources for quantum computation and quantum-enhanced measurement. Their generation and engineering require a high level of control over entanglement. Here we report on the generation of continuous-variable graph states of atomic spin ensembles, which form the nodes of the graph. We program the entanglement structure encoded in the graph edges by combining global photon-mediated interactions in an optical cavity with local spin rotations. By tuning the entanglement between two subsystems, we either localize correlations within each subsystem or enable Einstein–Podolsky–Rosen steering—a strong form of entanglement that enables the extraction of precise information from one subsystem through measurements on the other. We further engineer a four-mode square graph state, highlighting the flexibility of our approach. Our method is scalable to larger and more complex graphs, laying groundwork for measurement-based quantum computation and advanced protocols in quantum metrology.

Precise Determination of Magnetic Gradient Relaxation of Coupled Atomic Spin Ensemble in Spin-Exchange Relaxation-Free Co-Magnetometer

Inside a spin-exchange relaxation-free (SERF) co-magnetometer with a high-pressure buffer gas atomic cell, the magnetic field gradient causes the decoherence of atomic spins to produce magnetic-field gradient relaxation. This paper presents a new method for the accurate measurement of magnetic field gradient relaxation of alkali metal atoms and inert atoms of strongly coupled spin systems under triaxial magnetic field gradients in the K-Rb-21Ne co-magnetometer. The magnetic field gradient relaxation of alkali metal atoms is measured using a step magnetic field modulation method, and the magnetic field gradient relaxation of inert atoms is measured using a combined free induction decay and spin growth method. The method does not require the use of large background magnetic fields and RF fields to maintain the atoms in the SERF state, does not require additional optics, and is not affected by the pumping or detecting of optical power. A kinetic model that considers a large electron-equivalent magnetic field was designed and a gradient relaxation model was developed. The quadratic coefficients of the experimentally measured gradient relaxation curves fit the theoretical model well over the range of the applied magnetic field gradients, confirming the validity of the proposed method.

Ultrasensitive Optical Rotation Detection With Closed-Loop Suppression of Spin Polarization Error

Optical rotation detection system (ORDS) utilizing quantum nondemolition (QND) measurement methods is widely applied in the field of quantum metrology and quantum information. However, the sensitivity of ORDS is limited by the uncertainty from optical-couple noise during the measurement of the atomic spin ensemble. In this study, we specifically analyze the mechanism of optical-couple noise caused by the fluctuations of probe light’s polarization in the modulated ORDS with a new model established to describe atomic spin precession in this particular condition. It is discovered that transverse electron-spin polarization errors are generated by the residual probe photon spin polarization in the ORDS, which results in extra coupling magnetic noise. In order to suppress this noise, a novel in situ method is proposed that the resultant electron-spin errors are reduced by a specifically designed closed-loop system. The results are verified through the ORDS in a co-magnetometer. After zeroing the extra probe photon spin polarization, an angular sensitivity better than <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$1 \times 10 ^{\mathrm {-8}}$ </tex-math></inline-formula> rad/Hz <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$^{\mathrm {1/2}}$ </tex-math></inline-formula> is achieved for frequencies higher than 5 Hz, demonstrating a probe background noise of 0.26 fT/Hz <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$^{\mathrm {1/2}}$ </tex-math></inline-formula> @14.5 Hz, approaching electronic noise and photon shot noise (PSN). With closed-loop control, the optical rotation bias instability is promoted by 4.2 times (from 107.9 to <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$25.7 \mu $ </tex-math></inline-formula> rad/h), and the angular noise of the ORDS is reduced by 2.4 times at 1–100 Hz. The measurement uncertainty of the realized ORDS nears the standard quantum limit, paving the road for long-term ultrasensitive measurements for new physics explorations.

Magnon-atom-optical photon entanglement via the microwave photon-mediated Raman interaction.

We show that it is possible to generate magnon-atom-optical photon tripartite entanglement via the microwave photon-mediated Raman interaction. Magnons in a macroscopic ferromagnet and optical photons in a cavity are induced into a Raman interaction with an atomic spin ensemble when a microwave field couples the magnons to one Raman wing. The controllable magnon-atom entanglement, magnon-optical photon entanglement, and even genuine magnon-atom-optical photon tripartite entanglement can be generated simultaneously. In addition, these bipartite and tripartite entanglements are robust against the environment temperature. Our scheme paves the way for exploring a quantum interface bridging the microwave and optical domains, and may provide a promising building block for hybrid quantum networks.

Transverse light-shift in a spin-exchange relaxation-free co-magnetometer: measurement, decoupling, and suppression.

The transverse light-shift can induce non-negligible polarization error in the output signal of spin-exchange relaxation-free (SERF) co-magnetometer. In this paper, a novel method for rapid measurement of transverse light-shift based on the error of steady-state response of co-magnetometer is proposed firstly, then the sources of transverse light-shift in a compact SERF co-magnetometer is modeled and analyzed from three aspects: the non-ideal linear polarization of probe laser, the circular dichroism of the atomic spin ensembles, and the stress-induced birefringence effect of the cell wall. Furthermore, the decoupling and suppression methods of transverse light-shift based on a degree of circular polarization (DOCP) regulation scheme is presented, to realize the decoupling measurement of the transverse light-shift introduced by the whole co-magnetometer cell, and cancel it out with the non-ideal linear polarization of the probe laser. Eventually, the DOCP regulation scheme suggested in this paper achieves more than a 67% suppression ratio in transverse light-shift, and the short- and long-term performance of SERF co-magnetometer are improved due to the reduction of the coupling effect between the probe laser power and transverse field. Moreover, the measurement, decoupling and suppression methods provided in this paper also have the potential to be applied to other atomic sensors, such as the SERF magnetometers and nuclear spin co-magnetometers.

Atomic Spin Polarization Controllability Analysis: A Novel Controllability Determination Method for Spin-Exchange Relaxation-Free Co-Magnetometers

This paper investigates the atomic spin polarization controllability of spin-exchange relaxation-free co-magnetometers (SERFCMs). This is the first work in the field of controllability analysis for the atomic spin ensembles systems, whose dynamic behaviors of spin polarization are described by the Bloch equations. Based on the Bloch equations, a state-space model of the atomic spin polarization for SERFCM is first established, which belongs to a particular class of nonlinear systems. For this class of nonlinear systems, a novel determination method for the global state controllability is proposed and proved. Then, this method is implemented in the process of controllability analysis on the atomic spin polarization of an actual SERFCM. Moreover, a theoretically feasible and reasonable solution of the control input is proposed under some physical constraints, with whose limitation of realistic conditions, the controller design can be accomplished more practically and more exactly. Finally, the simulation results demonstrate the feasibility and validation of the proposed controllability determination method.

Analysis and suppression of the misalignment error for the pumping laser in the atomic comagnetometer.

The misalignment error of the pumping laser in the atomic comagnetometer (ACM) dramatically diminishes the efficiency of the optical pumping process (characterized by the polarization of the hybrid atomic spin ensembles containing electron spins and nuclear spins) and deteriorates the performance of the ACM (characterized by the Allan standard deviation). In this work, a steady-state response model considering the misalignment error of the pumping laser is established and an in-situ evaluation method for this error is proposed. Based on the evaluation method, the influence of this misalignment error on the pumping efficiency and the performance of the ACM is quantitatively analyzed. Furthermore, a pumping laser alignment method based on the second harmonic of a single-beam magnetometer is then proposed, whose effectiveness is verified by experiments. The experimental results show that compared to the original ACM with the severely misaligned pumping laser, the polarization of the hybrid atomic spin ensembles of the ACM with the pumping laser aligned by the proposed method is increased by about 19%, and the corresponding Allan variance at 100s is reduced by about 40%.

Beating standard quantum limit via two-axis magnetic susceptibility measurement

We report a metrology scheme which measures the magnetic susceptibility of an atomic spin ensemble along the x and z directions and produces parameter estimation with precision beating the standard quantum limit. The atomic ensemble is initialized via one-axis spin squeezing with optimized squeezing time and parameter ϕ (to be estimated) assumed as uniformly distributed between 0 and 2π while fixed in each estimation. One estimation of ϕ can be produced with every two magnetic susceptibility data measured along the two axes respectively, which has an imprecision scaling (1.43 ± 0.02)/N 0.687±0.003 with respect to the number N of the atomic spins. The measurement scheme is easy to implement and is robust against the measurement fluctuation caused by environment noise and measurement defects.

Noisy atomic magnetometry in real time

Continuously monitored atomic spin-ensembles allow, in principle, for real-time sensing of external magnetic fields beyond classical limits. Within the linear-Gaussian regime, thanks to the phenomenon of measurement-induced spin-squeezing, they attain a quantum-enhanced scaling of sensitivity both as a function of time, t, and the number of atoms involved, N. In our work, we rigorously study how such conclusions based on Kalman filtering methods change when inevitable imperfections are taken into account: in the form of collective noise, as well as stochastic fluctuations of the field in time. We prove that even an infinitesimal amount of noise disallows the error to be arbitrarily diminished by simply increasing N, and forces it to eventually follow a classical-like behaviour in t. However, we also demonstrate that, ‘thanks’ to the presence of noise, in most regimes the model based on a homodyne-like continuous measurement actually achieves the ultimate sensitivity allowed by the decoherence, yielding then the optimal quantum-enhancement. We are able to do so by constructing a noise-induced lower bound on the error that stems from a general method of classically simulating a noisy quantum evolution, during which the stochastic parameter to be estimated—here, the magnetic field—is encoded. The method naturally extends to schemes beyond the linear-Gaussian regime, in particular, also to ones involving feedback or active control.

In-SituEvaluation of Low-Frequency Magnetic Field Fluctuation in an Atomic Comagnetometer

This paper investigates a novel method for the in-situ evaluation of the low-frequency magnetic field fluctuation in an atomic comagnetometer (ACM). An in-situ magnetic field measurement model is first established for the hybrid atomic spin ensembles in the ACM based on the simplified Bloch equations. Then, the ACM is transformed into an in-situ magnetometer by employing a large longitudinal magnetic field and a transversal alternating current (AC) magnetic field, respectively. This in-situ magnetometer is sensitive to the magnetic field fluctuation along the detection laser direction according to the established measurement model and can realize the magnetic field measurement sensitivity of 88fT/Hz <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">1/2</sup> at 0.1Hz. Finally, the low-frequency magnetic field fluctuation is evaluated with this in-situ magnetometer, whose influence on the stability of the ACM is also analyzed by the Allan variance method. The experimental results show that the contribution of the magnetic field fluctuation along the detection laser direction to the stability of the ACM is about 0.0068 deg/h, which means that the magnetic field error still has a non-negligible effect on the stability of the system. This new in-situ magnetic field measurement method has the advantages of simple operation and no need to replace the atomic vapor cell, which provides an effective means of the magnetic field error evaluation for the ACM.

Enhancing Associative Memory Recall and Storage Capacity Using Confocal Cavity QED

We introduce a near-term experimental platform for realizing an associative memory. It can simultaneously store many memories by using spinful bosons coupled to a degenerate multimode optical cavity. The associative memory is realized by a confocal cavity QED neural network, with the cavity modes serving as the synapses, connecting a network of superradiant atomic spin ensembles, which serve as the neurons. Memories are encoded in the connectivity matrix between the spins, and can be accessed through the input and output of patterns of light. Each aspect of the scheme is based on recently demonstrated technology using a confocal cavity and Bose-condensed atoms. Our scheme has two conceptually novel elements. First, it introduces a new form of random spin system that interpolates between a ferromagnetic and a spin-glass regime as a physical parameter is tuned---the positions of ensembles within the cavity. Second, and more importantly, the spins relax via deterministic steepest-descent dynamics, rather than Glauber dynamics. We show that this nonequilibrium quantum-optical scheme has significant advantages for associative memory over Glauber dynamics: These dynamics can enhance the network's ability to store and recall memories beyond that of the standard Hopfield model. Surprisingly, the cavity QED dynamics can retrieve memories even when the system is in the spin glass phase. Thus, the experimental platform provides a novel physical instantiation of associative memories and spin glasses as well as provides an unusual form of relaxational dynamics that is conducive to memory recall even in regimes where it was thought to be impossible.

A Real-Time Digital Receiver for Correlation Measurements in Atomic Systems

We present the development and characterization of a generic, reconfigurable, low-cost ($<$ 350 USD) software-defined digital receiver system (DRS) for temporal correlation measurements in atomic spin ensembles. We demonstrate the use of the DRS as a component of a high resolution magnetometer. Digital receiver based fast Fourier transform spectrometers (FFTS) are generally superior in performance in terms of signal-to-noise ratio (SNR) compared to traditional swept-frequency spectrum analyzers (SFSA). In applications where the signals being analyzed are very narrow band in frequency domain, recording them at high speeds over a reduced bandwidth provides flexibility to study them for longer periods. We have built the DRS on the STEMLab 125-14 FPGA platform and it has two different modes of operation: FFT Spectrometer and real time raw voltage recording mode. We evaluate its performance by using it in atomic spin noise spectroscopy (SNS). We demonstrate that the SNR is improved by more than one order of magnitude with the FFTS as compared to that of the commercial SFSA. We also highlight that with this DRS operating in the triggered data acquisition mode one can achieve spin noise (SN) signal with high SNR in a recording time window as low as 100 msec. We make use of this feature to perform time resolved high-resolution magnetometry. While the receiver was initially developed for SNS experiments, it can be easily used for other atomic, molecular and optical (AMO) physics experiments as well.

Transverse optical pumping of spin states

Optical pumping is an efficient method for initializing and maintaining atomic spin ensembles in a well-defined quantum spin state. Standard optical pumping methods orient the spins by transferring photonic angular momentum to spin polarization. Generally the spins are oriented along the propagation direction of the light due to selection rules of the dipole interaction. Here we present and experimentally demonstrate that by modulating the light polarization, angular momentum perpendicular to the optical axis can be transferred efficiently to cesium vapor. The transverse pumping scheme employs transversely oriented dark states, allowing for control of the trajectory of the spins on the Bloch sphere. This new mechanism is suitable and potentially beneficial for diverse applications, particularly in quantum metrology.

Overcoming the Standard Quantum Limit in Gravitational Wave Detectors Using Spin Systems with a Negative Effective Mass.

Quantum backaction (QBA) of a measurement limits the precision of observation of the motion of a free mass. This profound effect, dubbed the "Heisenberg microscope" in the early days of quantum mechanics, leads to the standard quantum limit (SQL) stemming from the balance between the measurement sensitivity and the QBA. We consider the measurement of motion of a free mass performed in a quantum reference frame with an effective negative mass which is not limited by QBA. As a result, the disturbance on the motion of a free mass can be measured beyond the SQL. QBA-limited detection of motion for a free mass is extremely challenging, but there are devices where this effect is expected to play an essential role, namely, gravitational wave detectors (GWDs) such as LIGO and Virgo. Recent reports on the observations of gravitational waves have opened new horizons in cosmology and astrophysics. We present a general idea and a detailed numerical analysis for QBA-evading measurement of the gravitational wave effect on the GWD mirrors, which can be considered free masses under relevant conditions. The measurement is performed by two entangled beams of light, probing the GWD and an auxiliary atomic spin ensemble, respectively. The latter plays the role of a free negative mass. We show that under realistic conditions the sensitivity of the GWD in m/sqrt[Hz] can be increased by 6dB over the entire frequency band of interest.

Simultaneous tracking of spin angle and amplitude beyond classical limits.

Measurement of spin precession is central to extreme sensing in physics,1,2 geophysics,3 chemistry,4 nanotechnology5 and neuroscience,6 and underlies powerful magnetic resonance spectroscopies.7 Because there is no spin-angle operator, any measurement of spin precession is necessarily indirect, e.g., inferred from spin projectors Fα at different times. Such projectors do not commute, and thus quantum measurement back-action (QMBA) necessarily enters the spin measurement record, introducing errors and limiting sensitivity. Here we show how to reduce this disturbance below the classical limit for N spins, by directing the QMBA almost entirely into an unmeasured spin component. This generates a planar squeezed state8 which, because spins obey non-Heisenberg uncertainty relations,9,10 allows simultaneous precise knowledge of spin angle and amplitude. We use high-dynamic-range optical quantum non-demolition measurements11–13 applied to a precessing magnetic spin ensemble, to demonstrate spin tracking with steady-state angular sensitivity 2.9 dB beyond the standard quantum limit, simultaneous with amplitude sensitivity 7.0 dB beyond Poisson statistics.14 This method for the first time surpasses classical limits in non-commuting observables, and enables orders-of-magnitude sensitivity boosts for state-of-the-art sensing15–18 and spectroscopy.19,20

Nonclassical-state generation in macroscopic systems via hybrid discrete-continuous quantum measurements

Non-classical state generation is an important component throughout experimental quantum science for quantum information applications and probing the fundamentals of physics. Here, we investigate permutations of quantum non-demolition quadrature measurements and single quanta addition/subtraction to prepare quantum superposition states in bosonic systems. The performance of each permutation is quantified and compared using several different non-classicality criteria including Wigner negativity, non-classical depth, and optimal fidelity with a coherent state superposition. We also compare the performance of our protocol using squeezing instead of a quadrature measurement and find that the purification provided by the quadrature measurement can significantly increase the non-classicality generated. Our approach is ideally suited for implementation in light-matter systems such as quantum optomechanics and atomic spin ensembles, and offers considerable robustness to initial thermal occupation.

Feedback cooling of an atomic spin ensemble.

We apply entropy removal by measurement and feedback to a cold atomic spin ensemble. Using quantum nondemolition probing by Faraday rotation measurement, and feedback by weak optical pumping, we drive the initially random collective spin variable F toward the origin F=0. We use input-output relations and ensemble quantum noise models to describe this quantum control process and identify an optimal two-round control procedure. We observe 12 dB of spin noise reduction, or a factor-of-63 reduction in phase-space volume. The method offers a nonthermal route to generation of exotic entangled states in ultracold gases, including macroscopic singlet states and strongly correlated states of quantum lattice gases.

Entanglement-enhanced probing of a delicate material system

Quantum metrology1 uses entanglement2,3,4,5 and other quantum effects6 to improve the sensitivity of demanding measurements7,8,9. Probing of delicate systems demands high sensitivity from limited probe energy and has motivated the field's key benchmark—the standard quantum limit10. Here we report the first entanglement-enhanced measurement of a delicate material system. We non-destructively probe an atomic spin ensemble by means of near-resonant Faraday rotation, a measurement that is limited by probe-induced scattering in quantum-memory and spin-squeezing applications6,11,12,13. We use narrowband, atom-resonant NOON states to beat the standard quantum limit of sensitivity by more than five standard deviations, both on a per-photon and per-damage basis. This demonstrates quantum enhancement with fully realistic loss and noise, including variable-loss effects14,15,16. The experiment opens the way to ultra-gentle probing of single atoms17, single molecules18, quantum gases19 and living cells20.

Evading Quantum Mechanics: Engineering a Classical Subsystem within a Quantum Environment

Quantum mechanics is potentially advantageous for certain information-processing tasks, but its probabilistic nature and requirement of measurement back action often limit the precision of conventional classical information-processing devices, such as sensors and atomic clocks. Here we show that by engineering the dynamics of coupled quantum systems, it is possible to construct a subsystem that evades the measurement back action of quantum mechanics, at all times of interest, and obeys any classical dynamics, linear or nonlinear, that we choose. We call such a system a quantum-mechanics-free subsystem (QMFS). All of the observables of a QMFS are quantum-nondemolition (QND) observables; moreover, they are dynamical QND observables, thus demolishing the widely held belief that QND observables are constants of motion. QMFSs point to a new strategy for designing classical information-processing devices in regimes where quantum noise is detrimental, unifying previous approaches that employ QND observables, back-action evasion, and quantum noise cancellation. Potential applications include gravitational-wave detection, optomechanical force sensing, atomic magnetometry, and classical computing. Demonstrations of dynamical QMFSs include the generation of broad-band squeezed light for use in interferometric gravitational-wave detection, experiments using entangled atomic spin ensembles, and implementations of the quantum Toffoli gate.

Certified quantum non-demolition measurement of material systems

An extensive debate on quantum non-demolition (QND) measurement, reviewed in Grangier et al (1998 Nature396 537), finds that true QND measurements must have both non-classical state-preparation capability and non-classical information-damage tradeoff. Existing figures of merit for these non-classicality criteria require direct measurement of the signal variable and are thus difficult to apply to optically-probed material systems. Here we describe a method to demonstrate both criteria without need for to direct signal measurements. Using a covariance matrix formalism and a general noise model, we compute meter observables for QND measurement triples, which suffice to compute all QND figures of merit. The result will allow certified QND measurement of atomic spin ensembles using existing techniques.