Atomic Quantum Memory Research Articles

Review of Biphoton Sources Based on the Double‐Λ$\Lambda$ Spontaneous Four‐Wave Mixing Process

AbstractThis review article focuses on biphoton sources based on the double‐ spontaneous four‐wave mixing (SFWM) process in laser‐cooled as well as room‐temperature or hot atomic ensembles. These biphoton sources have the advantage of providing stable frequencies, ultranarrow linewidths, and a tunability of the temporal biphoton width of more than one order of magnitude for high‐bandwidth applications. Therefore, the generated photons can be efficiently interfaced to, e.g., atomic quantum memories. In contrast, solid‐state biphoton sources typically require assistance by an optical cavity to operate at narrow linewidth that limits the tunability of the temporal width of the biphotons. Present state‐of‐the‐art double‐ SFWM biphoton sources can achieve one of the following results: a spectral linewidth of 50 kHz (290 kHz) or a temporal width of 13 (580 ns) with cold (hot) atoms, a detection rate of about 7 cps, and a generation rate of cps at a duty cycle of 0.4% or of cps in the steady state. The theoretical background of these biphoton sources, experimental implementations with cold and hot atoms, and progress over the years, will be illustrated.

Towards a realistic model for cavity-enhanced atomic frequency comb quantum memories

Atomic frequency comb (AFC) quantum memory is a favorable protocol in long distance quantum communication. Putting the AFC inside an asymmetric optical cavity enhances the storage efficiency but makes the measurement of the comb properties challenging. We develop a theoretical model for cavity-enhanced AFC quantum memory that includes the effects of dispersion, and show a close alignment of the model with our own experimental results. Providing semi-quantitative agreement for estimating the efficiency and a good description of how the efficiency changes as a function of detuning, it also captures certain qualitative features of the experimental reflectivity. For comparison, we show that a theoretical model without dispersion fails dramatically to predict the correct efficiencies. Our model is a step forward to accurately estimating the created comb properties, such as the optical depth inside the cavity, and so being able to make precise predictions of the performance of the prepared cavity-enhanced AFC quantum memory.

Deterministic storage and retrieval of telecom light from a quantum dot single-photon source interfaced with an atomic quantum memory.

A hybrid interface of solid-state single-photon sources and atomic quantum memories is a long sought-after goal in photonic quantum technologies. Here, we demonstrate deterministic storage and retrieval of light from a semiconductor quantum dot in an atomic ensemble quantum memory at telecommunications wavelengths. We store single photons from an indium arsenide quantum dot in a high-bandwidth rubidium vapor-based quantum memory, with a total internal memory efficiency of (12.9 ± 0.4)%. The signal-to-noise ratio of the retrieved light field is 18.2 ± 0.6, limited only by detector dark counts.

Stark control of solid-state quantum memory with spin-wave storage

Quantum memories for quantum communication need to be able to store photons for an extended time and then to release them on demand. This can be achieved in atomic frequency comb ensemble-based quantum memories by control pulses that transfer the excitation to and from long-lived spin states. However, such pulses can give rise to coherent and incoherent noise due to their interaction with the memory ensemble. In this paper, we experimentally demonstrate the ability to switch off the coherent noise from such control pulses during the echo emission in a spin-wave quantum memory, using the linear Stark effect in rare-earth-ion doped crystals. By applying an electric-field pulse, the echo emission was coherently switched off prior to the first spin transfer pulse, and the stored data pulse was restored only when both an optical recall pulse and a rephasing electrical pulse were applied, giving a high degree of control of both desired and undesired emissions. We estimate the effectiveness of this technique by turning off the free-induction decay of a narrow ensemble of ions. This technique can thus improve the noise performance of spin-wave storage at the single-photon level by quenching coherent optical radiation created by strong control pulses. The method demonstrated here represents a proof of principle that the spin-wave storage scheme can be combined with Stark control. The combined scheme serves as an addition to the toolbox of techniques that can be used to realize a full version of a quantum repeater. Published by the American Physical Society 2024

Single-Photon Synchronization with a Room-Temperature Atomic Quantum Memory.

Efficient synchronization of single photons that are compatible with narrow band atomic transitions is an outstanding challenge, which could prove essential for photonic quantum information processing. Here we report on the synchronization of independently generated single photons using a room-temperature atomic quantum memory. The photon source and the memory are interconnected by fibers and employ the same ladder-level atomic scheme. We store and retrieve the heralded single photons with end-to-end efficiency of η_{e2e}=25% and final antibunching of g_{h}^{(2)}=0.023. Our synchronization process results in an over tenfold increase in the photon-pair coincidence rate, reaching a rate of more than 1000 detected synchronized photon pairs per second. The indistinguishability of the synchronized photons is verified by a Hong-Ou-Mandel interference measurement.

Thermometry utilizing stored short-wavelength spin waves in cold atomic ensembles

Temperature, as a measure of thermal motion, is a significant parameter characterizing a cold atomic ensemble optical quantum memory. In a cold gas, storage lifetime strongly depends on its temperature and is associated with the spin wave decoherence. Here we experimentally demonstrate a new spin wave thermometry method relying on this direct dependence. The short-wavelength spin waves resulting from the counter-propagating configuration of the control and the probe laser beams make this thermometry highly suitable for probing in situ the atomic motion in elongated clouds as the ones used in quantum memories. Our technique is realized with comparable precision for memories that rely on electromagnetically induced transparency as well as far-detuned Raman storage.

Single-shot high-resolution identification of discrete frequency modes of single-photon-level optical pulses

Frequency-multiplexed quantum communication usually requires a single-shot identification of the frequency mode of a single photon . In this paper, we propose a scheme that can identify the frequency mode with high-resolution even for spontaneously emitted photons whose generation time is unknown, by combining the time-to-space and frequency-to-time mode mapping. We also demonstrate the mapping of the frequency mode (100 MHz intervals) to the temporal mode (435 ns intervals) for weak coherent pulses using atomic frequency combs. This frequency interval is close to the minimum frequency mode interval of the atomic frequency comb quantum memory with Pr3+ ion-doped Y2SiO5 crystal, and the proposed scheme has the potential to maximize the frequency multiplexing of the quantum repeater scheme with the memory.

Non-classical correlations over 1250 modes between telecom photons and 979-nm photons stored in 171Yb3+:Y2SiO5

Quantum repeaters based on heralded entanglement require quantum nodes that are able to generate multimode quantum correlations between memories and telecommunication photons. The communication rate scales linearly with the number of modes, yet highly multimode quantum storage remains challenging. In this work, we demonstrate an atomic frequency comb quantum memory with a time-domain mode capacity of 1250 modes and a bandwidth of 100 MHz. The memory is based on a Y2SiO5 crystal doped with 171Yb3+ ions, with a memory wavelength of 979 nm. The memory is interfaced with a source of non-degenerate photon pairs at 979 and 1550 nm, bandwidth-matched to the quantum memory. We obtain strong non-classical second-order cross correlations over all modes, for storage times of up to 25 μs. The telecommunication photons propagated through 5 km of fiber before the release of the memory photons, a key capability for quantum repeaters based on heralded entanglement and feed-forward operations. Building on this experiment should allow distribution of entanglement between remote quantum nodes, with enhanced rates owing to the high multimode capacity.

Postselected Entanglement between Two Atomic Ensembles Separated by 12.5km.

Quantum internet gives the promise of getting all quantum resources connected, and it will enable applications far beyond a localized scenario. A prototype is a network of quantum memories that are entangled and well separated. In this Letter, we report the establishment of postselected entanglement between two atomic quantum memories physically separated by 12.5km directly. We create atom-photon entanglement in one node and send the photon to a second node for storage via electromagnetically induced transparency. We harness low-loss transmission through a field-deployed fiber of 20.5km by making use of frequency down-conversion and up-conversion. The final memory-memory entanglement is verified to have a fidelity of 90% via retrieving to photons. Our experiment makes a significant step forward toward the realization of a practical metropolitan-scale quantum network.

Efficient quantum memory for photonic polarization qubits generated by cavity-enhanced spontaneous parametric downconversion.

Quantum memories, for storing then retrieving photonic quantum states on demand, are crucial components for scalable quantum technologies. Spontaneous parametric downconversion (SPDC) with a nonlinear crystal is the most widely used process for generating entangled photon pairs or heralded single photons. Despite the desirability of efficient quantum memories for SPDC-generated single photons, the storage and retrieval efficiencies achieved with this approach still fall below 50%, a threshold value for practical applications. Here, we report an efficiency of > 70% for the storage of heralded single photons generated by cavity-enhanced SPDC using atomic quantum memories based on electromagnetically induced transparency (EIT). In addition, we demonstrate the quantum memory for single-photon polarization qubits with a fidelity of ∼96%. This result paves the way towards the development of large-scale quantum networks.

Cavity-driven Rabi oscillations between Rydberg states of atoms trapped on a superconducting atom chip

Hybrid quantum systems involving cold atoms and microwave resonators can enable cavity-mediated infinite-range interactions between atomic spin systems and realize atomic quantum memories and transducers for microwave-to-optical conversion. To achieve strong coupling of atoms to on-chip microwave resonators, it was suggested to use atomic Rydberg states with strong electric-dipole transitions. Here we report on the experimental realization of coherent coupling of a Rydberg transition of ultracold atoms, trapped on an integrated superconducting atom chip, to the microwave field of an on-chip coplanar waveguide resonator. Close to the chip surface, stray electric fields lead to inhomogeneous Rydberg level shifts, which would hinder coherent interactions of atoms in a cloud with the Rydberg excitation lasers and the microwave cavity field. We, however, use optical excitation of a Rydberg state of atoms in a narrow layer with nearly constant electric field, which allows for resonant coupling of the atoms to the cavity microwave field on an appropriate Rydberg transition. We also achieve state-selective detection of the energetically close Rydberg states. We then observe and characterize cavity-driven Rabi oscillations between a pair of atomic Rydberg states. The residual damping of the oscillations is dominated by the spread of Rabi frequencies of atoms in different positions of the resonant cavity mode, as revealed by our model. Despite the technical challenges, our studies demonstrate the feasibility of coherent-state manipulation of Rydberg atoms interacting with superconducting circuits, paving the way for realization of capable hybrid quantum systems.

Quantum-Memory-Enhanced Preparation of Nonlocal Graph States.

Graph states are an important class of multipartite entangled states. Previous experimental generation of graph states and in particular the Greenberger-Horne-Zeilinger (GHZ) states in linear optics quantum information schemes is subjected to an exponential decay in efficiency versus the system size, which limits its large-scale applications in quantum networks. Here, we demonstrate an efficient scheme to prepare graph states with only a polynomial overhead using long-lived atomic quantum memories. We generate atom-photon entangled states in two atomic ensembles asynchronously, retrieve the stored atomic excitations only when both sides succeed, and further project them into a four-photon GHZ state. Wemeasure the fidelity of this GHZ state and further demonstrate its applications in the violation of Bell-type inequalities and in quantum cryptography. Our work demonstrates the prospect of efficient generation of multipartite entangled states in large-scale distributed systems with applications in quantum information processing and metrology.

Multicell Atomic Quantum Memory as a Hardware-Efficient Quantum Repeater Node

For scalable quantum communication and networks, a key step is to realize a quantum repeater node that can efficiently connect different segments of atom-photon entanglement using quantum memories. We report a compact and hardware-efficient realization of a quantum repeater node using a single atomic ensemble for multicell quantum memories. Millisecond lifetime is achieved for individual memory cells after suppressing the magnetic-field-induced inhomogeneous broadening and the atomic-motion-induced spin-wave dephasing. Based on these long-lived multicell memory cells, we achieve heralded asynchronous entanglement generation in two quantum repeater segments one after another and then an on-demand entanglement connection of these two repeater segments. As another application of the multicell atomic quantum memory, we further demonstrate storage and on-demand retrieval of heralded atomic spin-wave qubits by implementing a random access quantum memory with individual addressing capacity. This work provides a promising constituent for efficient realization of quantum repeaters for large-scale quantum networks.

Efficient and robust collective excitation transfer in a multimode quantum memory using modulated adiabatic pulses

Quantum memories are building blocks for a variety of quantum technologies. However, the collective transfer between optical excitations and spin-wave excitations determines the performance of the quantum memory. Here we propose a method for collective excitations transfer with high efficiency and fidelity in a multimode quantum memory. The pulse uses modulations of the control parameters to cancel the nonadiabatic transitions during the evolution. We demonstrate the universality of the control pulse by simulations for an atomic frequency comb spin-wave quantum memory. The protocol is robust to various experimental imperfections in the pulse amplitude and duration. The protocol also allows one to achieve high multiplexed storage at small cost on efficiency reduction. The protocol is particularly useful in retaining the phase coherence since the environment dissipation would decohere the system. These results pave a way for efficient and robust coherent manipulations in a multiplexed quantum memory.

Room-temperature single-photon source with near-millisecond built-in memory

Non-classical photon sources are a crucial resource for distributed quantum networks. Photons generated from matter systems with memory capability are particularly promising, as they can be integrated into a network where each source is used on-demand. Among all kinds of solid state and atomic quantum memories, room-temperature atomic vapours are especially attractive due to their robustness and potential scalability. To-date room-temperature photon sources have been limited either in their memory time or the purity of the photonic state. Here we demonstrate a single-photon source based on room-temperature memory. Following heralded loading of the memory, a single photon is retrieved from it after a variable storage time. The single-photon character of the retrieved field is validated by the strong suppression of the two-photon component with antibunching as low as {g}_{{rm{RR| W = 1}}}^{(2)}=0.20pm 0.07. Non-classical correlations between the heralding and the retrieved photons are maintained for up to {tau }_{{rm{NC}}}^{{mathcal{R}}}=(0.68pm 0.08) {rm{ms}}, more than two orders of magnitude longer than previously demonstrated with other room-temperature systems. Correlations sufficient for violating Bell inequalities exist for up to τBI = (0.15 ± 0.03) ms.

Entanglement distribution with wavevector-multiplexed quantum memory

Feasible distribution of quantum entanglement over long distances remains a fundamental step towards quantum secure communication and quantum network implementations. Quantum repeater nodes based on quantum memories promise to overcome exponential signal decay inherent to optical implementations of quantum communication. While performance of current quantum memories hinders their practical application, multimode solutions with multiplexing can offer tremendous increase in entanglement distribution rates. We propose to use a wavevector-multiplexed atomic quantum memory (WV-MUX-QM) as a fundamental block of a multiplexed quantum repeater architecture. We show the WV-MUX-QM platform to provide quasi-deterministic entanglement generation over extended distances, mitigating the fundamental issue of optical loss even with currently available quantum memory devices, and exceeding performance of repeaterless solutions as well as other repeater-based protocols such as temporal multiplexing. We establish the entangled-bit (ebit) rate per number of employed nodes as a practical figure of merit reflecting the cost-efficiency of larger inter-node distances.

Hybrid III-V diamond photonic platform for quantum nodes based on neutral silicon vacancy centers in diamond.

Integrating atomic quantum memories based on color centers in diamond with on-chip photonic devices would enable entanglement distribution over long distances. However, efforts towards integration have been challenging because color centers can be highly sensitive to their environment, and their properties degrade in nanofabricated structures. Here, we describe a heterogeneously integrated, on-chip, III-V diamond platform designed for neutral silicon vacancy (SiV0) centers in diamond that circumvents the need for etching the diamond substrate. Through evanescent coupling to SiV0 centers near the surface of diamond, the platform will enable Purcell enhancement of SiV0 emission and efficient frequency conversion to the telecommunication C-band. The proposed structures can be realized with readily available fabrication techniques.

Experimental demonstration of memory-enhanced scaling for entanglement connection of quantum repeater segments

The quantum repeater protocol is a promising approach to implement long-distance quantum communication and large-scale quantum networks. A key idea of the quantum repeater protocol is to use long-lived quantum memories to achieve efficient entanglement connection between different repeater segments with a polynomial scaling. Here we report an experiment which realizes efficient connection of two quantum repeater segments via on-demand entanglement swapping by the use of two atomic quantum memories with storage time of tens of milliseconds. With the memory enhancement, scaling-changing acceleration is demonstrated in the rate for a successful entanglement connection. The experimental realization of entanglement connection of two quantum repeater segments with an efficient memory-enhanced scaling demonstrates a key advantage of the quantum repeater protocol, which makes a cornerstone towards future large-scale quantum networks.

Temporal Wheeler\u2019s delayed-choice experiment based on cold atomic quantum memory

Nowadays the most intriguing features of wave-particle complementarity of single-photons are exemplified by the famous Wheeler’s delayed-choice experiment with linear optics, nuclear magnetic resonance, and integrated photonic device systems in the optical platform. Until now, the delayed-choice experiments are demonstrated by either massless photons or massive particles, such as atoms, however, there is no report demonstrating Wheeler’s ideas in a hybrid system which consists of photons and atoms simultaneously. Here, we demonstrate a Wheeler’s delayed-choice experiment in an interface of light and atomic memory, in which the cold atomic memory makes the heralded single-photon divided into a superposition of atomic collective excitation and leaked pulse, thus acting as memory-based beam-splitters. We observe the intermediate states between particle and wave behavior by changing the relative proportion of the quantum random number generator, the second memory efficiency, and the relative storage time of two memories. The reported results confirm Bohr’s view that it makes no sense to illustrate the wave-like or particle-like behavior of light and matter before the measurement happens, and are helpful for improving our comprehension of the complementarity principle under the interface of light-atom interaction.

Quantum Communication between Multiplexed Atomic Quantum Memories.

The use of multiplexed atomic quantum memories (MAQM) can significantly enhance the efficiency to establish entanglement in a quantum network. In the previous experiments, individual elements of a quantum network, such as the generation, storage, and transmission of quantum entanglement have been demonstrated separately. Here we report an experiment to show the compatibility and integration of these basic operations. Specifically, we generate photon-atom entanglement from any chosen pair of memory cells in a 6×5 MAQM, convert the spin-wave to time-bin photonic excitation after a controllable storage time, and then store and retrieve the photon in a second MAQM for another controllable storage time. The preservation of quantum information in this process is verified by measuring the state fidelity. We also demonstrate that higher dimension quantum states can be transferred between the two distant MAQMs.