The spin-orbit interaction (SOI) offers a nonferromagnetic scheme to realize spin polarization through utilizing an electric field. Electrically tunable SOIs through electrostatic gates have been investigated; however, the relatively weak and volatile tunability limits their practical applications in spintronics. Here, we demonstrate the nonvolatile electric field control of the SOI via constructing ferroelectric Rashba architectures, i.e., two-dimensional ${\mathrm{Bi}}_{2}{\mathrm{O}}_{2}\mathrm{Se}/\mathrm{Pb}({\mathrm{Mg}}_{1/3}{\mathrm{Nb}}_{2/3}){\mathrm{O}}_{3}$-${\mathrm{PbTiO}}_{3}$ ferroelectric field-effect transistors. The experimentally observed weak antilocalization (WAL) cusp in ${\mathrm{Bi}}_{2}{\mathrm{O}}_{2}\mathrm{Se}$ films implies the Rashba-type SOI that arises from the asymmetric confinement potential. Significantly, taking advantage of the switchable ferroelectric polarization, the WAL-to-weak-localization-transition trend reveals the competition between spin relaxation and the dephasing process, and the variation of carrier density leads to a reversible and nonvolatile modulation of the spin-relaxation time and the spin-splitting energy of ${\mathrm{Bi}}_{2}{\mathrm{O}}_{2}\mathrm{Se}$ films by this ferroelectric gating. Our work provides a scheme to achieve nonvolatile control of the Rashba SOI with the utilization of ferroelectric remanent polarization.
Read full abstract