Angular Distribution Measurements Research Articles

Angular Distribution of Bremsstrahlung Spectral Temperature Measured in a Full Dimension of ECR Ion Source Using NaI(TI) Detector

Measurement of angular distribution (AD) of the bremsstrahlung spectral temperature from a full dimension of the Electron Cyclotron Resonance Ion Source (ECRIS) along the beam axis is challenging. To overcome some challenges, this paper presents the AD of the bremsstrahlung spectral temperature measured in a full dimension of the ECRIS along the beam axis using data obtained from the Busan Center of Korea Basic Science Institute (KBSI). The bremsstrahlung spectral temperature from 28-GHz ECR Ion source at the KBSI was measured in six, three, and nine azimuthal angles at the injection, centre, and extraction sides of the ECRIS using three round type thallium-activated sodium iodide (NaI(TI)) scintillation detectors. Monte Carlo simulation based on the Geant4 software package was performed to take the geometrical acceptance and energy-dependent detection efficiency into account due to large non-uniformity in the material budget. True bremsstrahlung energy spectra from the 28-GHz ECR ion source were obtained using the inverse-matrix deconvolution method. The unfolding method was based on a full geometry of the Geant4 model of the ECRIS plasma. The results show that in all three measurement locations, the highest value of the spectral temperature was at an angle of 30∘ coincident with one of the maximum angles of the ECRIS plasma shape.

Evidence for Chiral Wobbler in Nuclei.

Three ΔI=1 bands with the πg_{9/2}⊗νg_{9/2} configuration have been identified in _{35}^{74}Br_{39}. Angular distribution, linear polarization, and lifetime measurements were performed to determine the multipolarity, type, mixing ratio, and absolute transition probability of the transitions. By comparing these experimental observations with the corresponding fingerprints and the quantum particle rotor model calculations, the second and third lowest bands are, respectively, suggested as the chiral partner and one-phonon wobbling excitation built on the yrast band. The evidence indicates the first chiral wobbler in nuclei.

Design and implementation of multispectral band gonioradiometer for ultraviolet light sources measurements

The aim of this study is to design a multispectral band gonioradiometer that can measure the distribution of irradiance from ultraviolet (UV) light sources using different band spectrum detectors. One detector is sensitive to UVA, while the other is sensitive to UVC. The gonioradiometer can also acquire signals from both detectors simultaneously, including the UVC/blue spectral band. The system is driven by software developed in LabVIEW, which allows for interactive front-panel user interfaces to record the signals. The uncertainty associated with the angular irradiance distribution measurements using the gonioradiometer system was evaluated to be approximately 2% for UVA, 2.4% for UVC, and less than 1.8% for blue light measurements (at k = 2).

Study of single-nucleon transfer reactions in the 18O+48Ti collision at 275 MeV

The study of single-nucleon transfer reactions for the 18O+48Ti system was pursued at the energy of 275 MeV as part of a more systematic study which is undertaken within the NUMEN and NURE experimental campaigns. The aim is to measure the complete set of available reaction network which are characterized by the same initial and final-state wavefunctions as the more suppressed double charge exchange reactions. Understanding the degree of competition between successive nucleon transfer and double charge exchange reactions is crucial for the description of the meson-exchange mechanism. In this respect, angular distribution measurements for one- and twonucleon transfer reactions for the 18O+48Ti system were carried out at theMAGNEX facility of INFN-LNS in Catania. An overview of the data analysis for the 48Ti(18O,19F)47Sc and 48Ti(18O,17O)49Ti reactions will be presented.

Measurement of yields and angular distributions of γ-quanta from the interaction of 14.1 MeV neutrons with oxygen, phosphorus, and sulfur* *Supported by RSCF (23-12-00239)

A study of the inelastic scattering of neutrons with an energy of MeV on the nuclei of oxygen, phosphorus, and sulfur was performed at the TANGRA facility at JINR (Dubna). The experiment aimed to refine existing data and obtain new data on the yields and angular distributions of γ-quanta emitted by the studied nuclei due to neutron-induced nuclear reactions using the tagged neutron method. Two types of detector systems were used to register γ-quanta. The γ-ray yields were measured using a high-purity germanium (HPGe) detector. The angular distributions of γ-rays were obtained using a system of 18 scintillation detectors based on bismuth germanite Bi Ge O (BGO) located around the sample. The performed experiments measured the yields of two transitions for the reaction of tagged neutrons with O, nine transitions for the reaction with P, and nine transitions for the reaction with S for the first time. The angular anisotropy of the γ-radiation accompanying the inelastic scattering of neutrons with an energy of MeV on P nuclei was also measured for the first time.

L-MM Auger electron emission from chlorinated organic molecules under proton impact: Angular distribution and total cross section measurement

We have measured the absolute cross section for L-MM Auger electron emission in chlorinated methanes and benzene chloride molecules in collision with keV energy protons. The measurements have been performed with four different chlorine containing organic molecules viz CCl4, CHCl3, CH2Cl2 and C6H5Cl. We have measured the angular distribution of chlorine L-MM Auger electrons at backward emission angles (90° – 150°). The angular distribution shows an isotropic character. We also studied the projectile energy dependence of the total L-MM Auger yield for proton energy ranging from 125 keV to 275 keV. Carbon K-LL Auger yield was also obtained in the same experiments.

Photodissociation dynamics of the ethyl radical via the Ã2A'(3s) state: H-atom product channels and ethylene product vibrational state distribution.

The photodissociation dynamics of jet-cooled ethyl radical (C2H5) via the Ã2A'(3s) states are studied in the wavelength region of 230-260nm using the high-n Rydberg H-atom time-of-flight (TOF) technique. The H + C2H4 product channels are reexamined using the H-atom TOF spectra and photofragment translational spectroscopy. A prompt H + C2H4(X̃1Ag) product channel is characterized by a repulsive translational energy release, anisotropic product angular distribution, and partially resolved vibrational state distribution of the C2H4(X̃1Ag) product. This fast dissociation is initiated from the 3s Rydberg state and proceeds via a H-bridged configuration directly to the H + C2H4(X̃1Ag) products. A statistical-like H + C2H4(X̃1Ag) product channel via unimolecular dissociation of the hot electronic ground-state ethyl (X̃2A') after internal conversion from the 3s Rydberg state is also examined, showing a modest translational energy release and isotropic angular distribution. An adiabatic H + excited triplet C2H4(ã3B1u) product channel (a minor channel) is identified by energy-dependent product angular distribution, showing a small translational energy release, anisotropic angular distribution, and significant internal excitation in the C2H4(ã3B1u) product. The dissociation times of the different product channels are evaluated using energy-dependent product angular distribution and pump-probe delay measurements. The prompt H + C2H4(X̃1Ag) product channel has a dissociation time scale of <10ps, and the upper bound of the dissociation time scale of the statistical-like H + C2H4(X̃1Ag) product channel is <5ns.

Recent results on the analysis of the 48Ti(18O, 20Ne)46Ca reaction at 275 MeV

The 18O+48Ti reaction was studied at the energy of 275 MeV for the first time under the NUMEN and NURE experimental campaigns with the aim of investigating the complete reaction network potentially involved in the 48Ti→48Ca double charge exchange transition. Understanding the degree of competition between successive nucleon transfer and double charge exchange reactions is crucial for the description of the meson exchange mechanism. Into this context, angular distribution measurements for one- and two-nucleon transfer reactions for the system 18O+48Ti were performed at the MAGNEX facility of INFN-LNS in Catania. An overview of the status of the analysis for the two-proton transfer reaction will be given.

Ozone Generation from a Germicidal Ultraviolet Lamp with Peak Emission at 222 nm.

Recent interest in commercial devices containing germicidal ultraviolet lamps with a peak emission wavelength at 222 nm (GUV222) has focused on mitigating virus transmission indoors while posing minimum risk to human tissue. However, 222 nm light can produce ozone (O3) in air. O3 is an undesirable component of indoor air because of health impacts from acute to chronic exposure and its ability to degrade indoor air quality through oxidation chemistry. In seven four-hour experiments we measured O3 produced from a single filtered GUV222 lamp in a 31.5 m3 stainless steel chamber. Using an emission model, we determined an O3 generation rate of 19.4 ppbv h-1 ± 0.3 ppbv h-1 (equivalent to 1.22 mg h-1 ± 0.02 mg h-1). We estimated the fluence rate from the lamp using two methods: (1) chemical actinometry using tetrachloroethylene (actinometry) and (2) geometric projection of the irradiance field from radial and angular distribution measurements of the GUV222 lamp fluence (irradiance). Using the estimated lamp fluence rates of 2.2 μW cm-2 (actinometry) and 3.2 μW cm-2 (irradiance) we predicted O3 production in our chamber within 20 % of the average measured mixing ratio. Future studies should evaluate the indoor air quality impacts of GUV222 technologies.

Predissociation dynamics of negative-ion resonances of H2 near 12 and 14.5 eV using the velocity slice imaging technique

Dissociative electron attachment is an important tool for investigating negative-ion resonances. We have studied the negative-ion resonances of ${\mathrm{H}}_{2}$ at 10 and 14 eV using the improved velocity slice imaging technique. We obtained modulations in the kinetic energy spectrum of ${\mathrm{H}}^{\ensuremath{-}}$ ions obtained at 12 and 14.5 eV electron energy, consistent with the earlier reported vibrational state contributions from the higher-lying bound resonances. We show that structures obtained at 12 eV are due to predissociation of the $C{\phantom{\rule{0.16em}{0ex}}}^{2}{\mathrm{\ensuremath{\Sigma}}}_{g}^{+}$ resonance consistent with the current understanding. However, based on our angular distribution measurements, we propose that the structures obtained at 14.5 eV are due to a predissociation of bound resonance of ${}^{2}{\mathrm{\ensuremath{\Sigma}}}_{g}^{+}$ symmetry as against ${\mathrm{\ensuremath{\Delta}}}_{g}$ that was proposed earlier. We also report that the bound ${}^{2}{\mathrm{\ensuremath{\Sigma}}}_{g}^{+}$ resonance contributes to the observed inversion symmetry breaking near 14 eV.

Compact 2D electron analyzer CoDELMA: Simultaneous wide reciprocal and real space analysis using wide-angle deceleration lens, CMA and projection lens

A compact wide-acceptance angle (around ± 50°) high-energy-resolution 2D electron analyzer CoDELMA (Compact DELMA) is proposed, constructed and tested. CoDELMA is composed of a recently-proposed variable-deceleration-ratio wide-acceptance-angle electrostatic lens (VD-WAAEL), a cylindrical mirror analyzer (CMA) and a projection lens. After a brief review of VD-WAAEL, the use of a plane grid in the lens is presented as a new design option, which allows keeping the focusing angle almost constant irrespective of the deceleration ratio. A detailed consideration is given to the combination of CMA and a projection lens, which allows simultaneous analysis of wide reciprocal ( ± 8°) and real space ( ± 5 mm) at the entrance of CMA. CoDELMA is the successor to the previously developed DELMA instrument including a concentric hemispherical analyzer. The whole system of CoDELMA becomes much more compact than that of DELMA owing to the use of VD-WAAEL and CMA, and this results in considerable reduction of the production cost. Results of test measurement of energy spectrum and angular distribution using an electron gun as an excitation source confirmed that the energy resolution and the acceptance angle are almost the same as the designed values.

Core-Level Photoelectron Angular Distributions at the Liquid-Vapor Interface.

ConspectusPhotoelectron spectroscopy (PES) is a powerful tool for the investigation of liquid-vapor interfaces, with applications in many fields from environmental chemistry to fundamental physics. Among the aspects that have been addressed with PES is the question of how molecules and ions arrange and distribute themselves within the interface, that is, the first few nanometers into solution. This information is of crucial importance, for instance, for atmospheric chemistry, to determine which species are exposed in what concentration to the gas-phase environment. Other topics of interest include the surface propensity of surfactants, their tendency for orientation and self-assembly, as well as ion double layers beneath the liquid-vapor interface. The chemical specificity and surface sensitivity of PES make it in principle well suited for this endeavor. Ideally, one would want to access complete atomic-density distributions along the surface normal, which, however, is difficult to achieve experimentally for reasons to be outlined in this Account. A major complication is the lack of accurate information on electron transport and scattering properties, especially in the kinetic-energy regime below 100 eV, a pre-requisite to retrieving the depth information contained in photoelectron signals.In this Account, we discuss the measurement of the photoelectron angular distributions (PADs) as a way to obtain depth information. Photoelectrons scatter with a certain probability when moving through the bulk liquid before being expelled into a vacuum. Elastic scattering changes the electron direction without a change in the electron kinetic energy, in contrast to inelastic scattering. Random elastic-scattering events usually lead to a reduction of the measured anisotropy as compared to the initial, that is, nascent PAD. This effect that would be considered parasitic when attempting to retrieve information on photoionization dynamics from nascent liquid-phase PADs can be turned into a powerful tool to access information on elastic scattering, and hence probing depth, by measuring core-level PADs. Core-level PADs are relatively unaffected by effects other than elastic scattering, such as orbital character changes due to solvation. By comparing a molecule's gas-phase angular anisotropy, assumed to represent the nascent PAD, with its liquid-phase anisotropy, one can estimate the magnitude of elastic versus inelastic scattering experienced by photoelectrons on their way to the surface from the site at which they were generated. Scattering events increase with increasing depth into solution, and thus it is possible to correlate the observed reduction in angular anisotropy with the depth below the surface along the surface normal.We will showcase this approach for a few examples. In particular, our recent works on surfactant molecules demonstrated that one can indeed probe atomic distances within these molecules with a high sensitivity of ∼1 Å resolution along the surface normal. We were also able to show that the anisotropy reduction scales linearly with the distance along the surface normal within certain limits. The limits and prospects of this technique are discussed at the end, with a focus on possible future applications, including depth profiling at solid-vapor interfaces.

The Neutron Scattering Cross Section and Angular Distribution Measurement Program at LANL

Neutron scattering cross sections and angular distributions are leading terms in descriptions of neutron transport through any system. Despite the fundamental importance of nuclear data on these quantities, significant gaps in understanding and lack of experimental data persist in heavier elements and down to lighter structural materials, such as iron and aluminum. Recent measurements on carbon have also shown definitive proof that the neutron angular distribution can change with respect to the emission angle of γ-rays from inelastic scattering, thereby complicating γ-tagged measurements of inelastic neutron scattering. In this work, we describe the emerging program at Los Alamos National Laboratory for measurements of neutron scattering cross sections and neutron, γ-ray, and correlated n-γ angular distributions utilizing liquid scintillator detectors and the Correlated Gamma-Neutron Array for Scattering (CoGNAC) of CLYC scintillators. Currently, these detectors are operated simultaneously with the in-progress array of CLYC detectors in an inverted position, and data analysis techniques are being developed to span scattering measurements from light nuclei up through actinides. Preliminary results for measurements on 12C, 27Al, and 56Fe are presented here with a description of the analysis methods applied and anticipated capabilities of the full-scale detection system.

Collision-induced atomic alignment of silver after [formula omitted] ionization by 10–50 keV electron impact: Influence of Coster–Kronig transition effect

This work reports atomic alignment of silver after L3-subshell ionization in collisions with electrons in energy range 10–50 keV, i.e., (3∼15)EL3, where EL3(=3.351 keV) is the binding energy of electrons in the L3-subshell. The characteristic spectra are measured at different emission angles from -40∘ to 40∘ intervals of 10∘. The angular dependence of X-ray emission is studied for Lα(L3→M4,5) and Lβ2(L3→N5) lines respectively, using a thin target. The anisotropy parameter β is determined from two angular distribution measurements of differential X-ray intensity ratios dI(Lα,θ)/dI(Lβ1,θ) and dI(Lβ2,θ)/dI(Lβ1,θ). This served to reduce the experimental uncertainties. For the derivation of the alignment factor A20 we took into account the Coster–Kronig (CK) correction factor κ, which allows for, CK transition probabilities fij among L-subshells. We found that the sign of A20 is mostly negative, and the influence of CK transition is significant for large alignment parameters. In addition, the experimental results are compared to theoretical predictions within the framework of Plane Wave Born Approximation (PWBA) and reasonable agreement is found in the energy range studied in the present work. Simultaneously, good scaling property of atomic alignment is demonstrated when we consider also previous experimental results. Our measurement extends the scaled velocity V (=vp/vt) to a range of 1∼4 for medium-Zt targets, and the results of atomic alignment can provide a fundamental testing ground for ionization models.

Development of THGEM-based Detectors for Nuclear Fission Studies

To optimize the exploration of Super Heavy Elements (SHE), the key challenge is to understand the dynamics of the fusion-fission through the measurements of mass and angular distribution of the fission fragments. For the detection of fission fragments, position sensitive Multi-Wire Proportional Counters are generally used due to their high gain, good temporal and position resolution. However, these detectors use fragile anode wires having a diameter of only 10 μm and therefore they are vulnerable. In the present work, a detector based on robust Thick Gaseous Electron Multiplier (THGEM) has been proposed. A numerical demonstration of THGEM-Multi Wire hybrid detector technology as a possible candidate for the new generation low-energy fission studies and their evaluation as a function of different possible geometric and electric configuration in low-pressure gas is discussed here.

Differential Measurement of Electron Ejection after Two-Photon Two-Electron Excitation of Helium.

We report the measurement of the photoelectron angular distribution of two-photon single-ionization near the 2p^{2} ^{1}D^{e} double-excitation resonance in helium, benchmarking the fundamental nonlinear interaction of two photons with two correlated electrons. This observation is enabled by the unique combination of intense extreme ultraviolet pulses, delivered at the high-repetition-rate free-electron laser in Hamburg (FLASH), ionizing a jet of cryogenically cooled helium atoms in a reaction microscope. The spectral structure of the intense self-amplified spontaneous emission free-electron laser pulses has been resolved on a single-shot level to allow for post selection of pulses, leading to an enhanced spectral resolution, and introducing a new experimental method. The measured angular distribution is directly compared to state-of-the-art theory based on multichannel quantum defect theory and the streamlined R-matrix method. These results and experimental methodology open a promising route for exploring fundamental interactions of few photons with few electrons in general.

Detection of correlated fission fragments with a twin Frisch-grid ionization chamber

Twin Frisch-grid ionization chambers (TFGICs) have been widely used in the measurement of total kinetic energy (TKE), angular distribution, mass, and charge of the correlated fission fragments. To study these correlated fission parameters, we have developed a TFGIC with a digital acquisition system for use at both the Chinese Mianyang research reactor (CMRR) and neutron science facility in the Institute of Nuclear Physics and Chemistry (INPC), as well as the China Spallation Neutron Source (CSNS). The distribution of the electric field was investigated with Garfield toolkit, the results showed that the ratio of the electric field of the collect region to the drift region (Ec /Ed ) must be greater than a critical value Z (1.78). An individual experiment, carried out with a compound alpha source (241Am and 243Am), was used to validate the preliminary performance of this detector. The effects of the electric field on the anode pulse height agreed well with the simulation results. Furthermore, the results also indicated that the energy resolution of (68.40 ± 1.07) keV at 5.39 MeV (243Am) and (69.67 ± 1.09) keV at 5.49 MeV (241Am) could be achieved. An initial in-beam fission experiment of 235U reaction with 14 MeV neutrons was also performed to test the setup, and the results showed that the reconstructed emission angle could achieve a resolution of 0.221 ± 0.002 on the difference of the cosines determined from both halves of TFGIC. The present work primarily reported the development of a TFGIC with a digital acquisition system in INPC.

Examination of nuclear chirality with a magnetic moment measurement of the I=9 isomeric state in Cs128

The $g$ factor of the isomeric $I={9}^{+}$ bandhead of the yrast states in $^{128}\mathrm{Cs}$ is obtained from the time differential perturbed angular distribution measurement performed with the electromagnet at IPN Orsay. An external magnetic field of 2.146 T at the target position was attained with GAMIPE reaction chamber surrounded by four high-purity germanium detectors, of which two were low-energy photon spectrometer type. The results are in accordance with $\ensuremath{\pi}{h}_{11/2}\ensuremath{\bigotimes}\ensuremath{\nu}{h}_{11/2}^{\ensuremath{-}1}\phantom{\rule{4pt}{0ex}}I={9}^{+}$ bandhead assignment and are discussed in the context of chiral interpretation of the $^{128}\mathrm{Cs}$ nucleus as a composition of the odd proton, odd neutron, and even-even core with their angular momentum vectors. The obtained $g$-factor value was compared with predictions of the particle-rotor model. The experimental $g$ factor corresponds to the nonchiral geometry of the isomeric bandhead. This observation indicates the existence of the chiral critical frequency in $^{128}\mathrm{Cs}$ and may explain the absence of the chiral doublet members for $I&lt;13\ensuremath{\hbar}$.

Measurement of angular and momentum distributions of charged particles within and around jets with the ATLAS detector

Studies of jet fragmentation in heavy-ion collisions can provide information about the mechanism of jet quenching inside the hot and dense QCD matter created in these collisions. These proceedings present results from measurements of charged particle yields within and around the jets in dijet, gamma+jet and Z+jet systems measured in $5.02$~TeV Pb+Pb and $pp$ collisions using the ATLAS detector at the LHC.

K-LL Auger electron angular distribution and absolute cross section measurement upon keV energy electron impact ionization of CH[formula omitted], N[formula omitted] and Ne

We report on the measurement of absolute cross sections and angular distribution of electron emission in the K-LL Auger region, upon electron impact ionization of molecular (CH4 and N2) and atomic (Ne) targets. Differential cross sections in the K-LL Auger energy range were measured at 6 keV and 8 keV impact energies. The angular distribution of the K-LL Auger yield is shown to be isotropic for all the three targets. Total K-LL Auger emission cross sections were estimated by integrating the measured differential cross sections over the entire energy and angular range. The estimated cross sections are in good agreement with the theoretical estimates.