Combining the two advantages of mitigation of dependence on cement and natural sand resources and recycling waste concrete material, the utilization of recycled concrete powder (RCP) and recycled fine sand (RFS) to produce geopolymer concrete is of great value. However, the insufficient compressive strength and inherent brittleness of the existing RCP or RFS geopolymer concrete hampered its application. This paper aims to develop a high-performance engineered geopolymer composite (EGC) by maximizing the recycle amount of RCP and RFS. The effects of RCP and RFS on the physical, mechanical, and microscopic properties of EGC were investigated. The results indicated that, the less reactivity of RCP decreased the amount of gel products and compromised the strength development, while favored the multi-cracking behavior and the robust ductility. RFS showed a stronger interfacial bond with paste than quartz sand, compensating the degradation of strength driven by RCP and marginally affecting the tensile strain capacity. The developed EGC incorporating 50% RCP and 100% RFS possessed an 84 MPa compressive strength, 7.4 MPa tensile strength, and 8.1% tensile strain, which are at the highest level among the existing RCP or RFS geopolymer concretes. The main products included the coexistence of calcium aluminosilicate hydrate and alkali aluminosilicate (C(N)-A-S-H) gel and layered double hydroxide (LDH). The energy- and carbon-reduction were 16% and 57%, respectively, compared to the M45-ECC.The current findings prove the feasibility of utilizing high amounts of recycled materials to produce high value-added concrete.