AlGaAs Nanoantennas Research Articles

Tuning nonlinear second-harmonic generation in AlGaAs nanoantennas via chalcogenide phase-change material

The ability to engineer nonlinear optical processes in all-dielectric nanostructures is both of fundamental interest and highly desirable for high-performance, robust, and miniaturized nonlinear optical devices. Herein, we propose a paradigm for the efficient tuning of a second-harmonic generation (SHG) process in dielectric nanoantennas by integrating with chalcogenide phase-change material. In a design with ${\mathrm{Ge}}_{2}{\mathrm{Sb}}_{2}{\mathrm{Te}}_{5}$ (GST) film sandwiched between the AlGaAs nanoantennas and ${\mathrm{AlO}}_{x}$ substrate, the nonlinear SHG signal from the AlGaAs nanoantennas can be boosted via the resonantly localized field induced by the optically induced Mie-type resonances, and further modulated by exploiting the GST amorphous-to-crystalline phase change in a nonvolatile, multilevel manner. The tuning strategy originates from the modulation of resonant conditions by changes in the refractive index of GST. With a thorough examination of tuning performances for different nanoantenna radii, a maximum modulation depth as high as $540%$ is numerically demonstrated. This work not only reveals the potential of GST in optical nonlinearity control, but also provides a promising strategy in smart designing of tunable and reconfigurable nonlinear optical devices, e.g., light emitters, modulators, and sensors.

From Fano to Quasi-BIC Resonances in Individual Dielectric Nanoantennas.

Sharp optical resonances in high-index dielectric nanostructures have recently attracted significant attention for their promising applications in nanophotonics. Fano resonances, as well as resonances associated with bound states in the continuum (BIC), have independently shown a great potential for applications in nanoscale lasers, sensors, and nonlinear optical devices. Here, we demonstrate experimentally a close connection between Fano and quasi-BIC resonances excited in individual dielectric nanoantennas. We analyze systematically the resonant response of AlGaAs nanoantennas pumped with a structured light in the near-infrared range. We trace a variation of the scattering spectrum that fully agrees with an analytical expression governed by a Fano parameter and observe directly a transition to a quasi-BIC resonance. Our results suggest a unified approach toward the analysis of sharp resonances in subwavelength nanostructures originating from strong coupling of optical modes that can provide high energy localization for enhanced light-matter interactions.

Vertical Second Harmonic Generation in Asymmetric Dielectric Nanoantennas

High-permittivity III-V semiconductor nanocavities have shown huge potential for enhanced nonlinear light-matter interactions at the nanoscale. In particular, Second Harmonic (SH) generation in AlGaAs nanoantennas can be extremely efficient; however, vertical emission is difficult to achieve, due to the zincblende χ <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">(2)</sup> tensor and epitaxially growth on (100) substrates. Here, we demonstrate that we can shape the second harmonic radiation pattern from a single AlGaAs nanostructure by exploiting a geometrical symmetry breaking optimization approach. The optimized design allows to redirect the SH signal toward the normal direction and to increase the SH power collection efficiency by 2 orders of magnitude in a small numerical aperture of 0.1 with respect to the symmetrical counterpart structure.

Enhanced second-harmonic generation from L-shaped AlGaAs nanoantennas

Nanostructured materials offer many advantages over bulk materials in nonlinear optical phenomena. For example, the subwavelength scale allows the neglect of phase-matching issues. The ability to control tight confinement and large resonant enhancement of electromagnetic fields also results in higher nonlinear frequency conversion efficiencies than bulk materials. Compared with plasmonic nanostructures, high-index dielectric nanostructures render larger mode volumes and show great promise for enhanced nonlinear optical processes. In this work, we present resonantly enhanced second-harmonic generation from L-shaped AlGaAs nanoantennas. By tuning the nanostructure thickness, arm length, and width, the overlap of resonances at fundamental and second-harmonic wavelengths can be achieved using any pump wavelength in a broad near-infrared spectral region. We predict SHG efficiency exceeding 4 × 10 − 3 with a pump intensity of 1 G W / c m 2 at two representative pump wavelengths of 1675 and 1800 nm. Our findings are valuable for applications involving all-dielectric nanoantennas, such as efficient sensing and single biomolecule tracking microscopy.

Resonant harmonic generation in AlGaAs nanoantennas probed by cylindrical vector beams.

We investigate second- and third-harmonic generation from individual AlGaAs nanoantennas using far-field mapping with radially- and azimuthally-polarized cylindrical vector beams. Due to the unique polarization structure of these beams, we are able to determine the crystal orientation of the nanoantenna in a single scanning map. Our method thus provides a novel and versatile optical tool to study the crystal properties of semiconductor nanoantennas. We also demonstrate the influence of cylindrical vector beam excitation on the resonant enhancement of second- and third-harmonic generation driven by electric and magnetic anapole-like modes, despite falling in the strong absorption regime of AlGaAs. In particular, we observe a greater nonlinear conversion efficiency from a single nanoantenna excited with a radially-polarized beam as compared to an azimuthally polarized cylindrical vector beam. The fundamental field of the radially-polarized beam strongly couples to the multipoles increasing the near-field enhancement of the nanoantenna. Our work introduces new ways to study individual nanostructures and to tailor the efficiencies of nonlinear phenomena at the nanoscale using non-conventional optical techniques.

Boosting Second Harmonic Radiation from AlGaAs Nanoantennas with Epsilon-Near-Zero Materials

Enhancing the second harmonic conversion efficiency at the nanoscale is a critical challenge in nonlinear optics. Here we propose the use of epsilon-near-zero materials to boost the nonlinear radiation in the far field. Here, a comparison of the second harmonic behavior of a cylindrical AlGaAs nanoantenna placed over different semi-infinite layers is presented. In particular, we observed that the second harmonic generation is strongly enhanced and redirected by the simultaneous presence of a resonance at the fundamental wavelength and a low-permittivity condition in the substrate at the harmonic wavelength. Our results pave the way for a novel approach to enhance optical nonlinearities at the nanoscale.

Nonlinear Goniometry by Second-Harmonic Generation in AlGaAs Nanoantennas

High-permittivity semiconductor nanoresonators have shown great potential for enhanced nonlinear light–matter interactions at the nanoscale due to the availability of a rich variety of resonances combined with low optical losses and a strong bulk nonlinearity. Second-harmonic generation in AlGaAs nanoantennas can be extremely efficient and exhibits a complex radiation pattern. However, the complexity of this far-field profile imposes severe constraints on practical applications and detection efficiency. In this work, we demonstrate, both experimentally and numerically, the control over the angular distribution of the second-harmonic radiation pattern from a monolithic AlGaAs-on-AlOx nanodisk by varying the polarization and the angle of incidence of the pump beam. By tuning the angle of incidence of a beam with s-polarized light from 0 to 45°, the detected second-harmonic signal is monotonically increased up to over an order of magnitude due to the strong dependence of the nonlinear radiation pattern on th...

Metal-dielectric hybrid nanoantennas for efficient frequency conversion at the anapole mode.

Background: Dielectric nanoantennas have recently emerged as an alternative solution to plasmonics for nonlinear light manipulation at the nanoscale, thanks to the magnetic and electric resonances, the strong nonlinearities, and the low ohmic losses characterizing high refractive-index materials in the visible/near-infrared (NIR) region of the spectrum. In this frame, AlGaAs nanoantennas demonstrated to be extremely efficient sources of second harmonic radiation. In particular, the nonlinear polarization of an optical system pumped at the anapole mode can be potentially boosted, due to both the strong dip in the scattering spectrum and the near-field enhancement, which are characteristic of this mode. Plasmonic nanostructures, on the other hand, remain the most promising solution to achieve strong local field confinement, especially in the NIR, where metals such as gold display relatively low losses.Results: We present a nonlinear hybrid antenna based on an AlGaAs nanopillar surrounded by a gold ring, which merges in a single platform the strong field confinement typically produced by plasmonic antennas with the high nonlinearity and low loss characteristics of dielectric nanoantennas. This platform allows enhancing the coupling of light to the nanopillar at coincidence with the anapole mode, hence boosting both second- and third-harmonic generation conversion efficiencies. More than one order of magnitude enhancement factors are measured for both processes with respect to the isolated structure.Conclusion: The present results reveal the possibility to achieve tuneable metamixers and higher resolution in nonlinear sensing and spectroscopy, by means of improved both pump coupling and emission efficiency due to the excitation of the anapole mode enhanced by the plasmonic nanoantenna.

Imaging Electric and Magnetic Modes and Their Hybridization in Single and Dimer AlGaAs Nanoantennas

AbstractAll‐dielectric nanoantennas enable the manipulation and confinement of light on the nanoscale through a variety of resonant excitations. Understanding and controlling the interactions among resonances at a level of individual nanoantennas is required for the development of appropriate design rules for their applications, especially with regard to nonlinear optics, where the nonlinear interaction depends on the resonant behavior in a superlinear manner. Here, cathodoluminescence imaging spectroscopy is used to experimentally investigate the electric and magnetic modes supported by single AlGaAs nanoantennas and their hybridization in a dimer configuration. An interplay is shown between the resonant modes of the nanostructures and interband emission of the semiconductor material, which contrasts with Si nanoantennas, where the bandgap effects are not significant. The measurements are in very good agreement with numerical simulations, which also provided further insight into the nature of the modes. The resonant modes of semiconductor nanoantennas are important for engineering linear and nonlinear metasurfaces, as well as for sensing applications and fluorescence control in nanophotonic environments.

Giant Nonlinear Response at the Nanoscale Driven by Bound States in the Continuum

Being motivated by the recent prediction of high-Q modes in subwavelength dielectric resonators inspired by bound states in the continuum (BIC), we study the second-harmonic generation from isolated subwavelength AlGaAs nanoantennas. We reveal that nonlinear effects at the nanoscale can be enhanced dramatically provided the resonator parameters are tuned to the BIC regime. We predict a record-high conversion efficiency for nanoscale resonators that exceeds by 2 orders of magnitude the conversion efficiency observed at the magnetic dipole Mie resonance, thus opening the way for highly efficient nonlinear metasurfaces and metadevices.

Nonlinear Optical Magnetism Revealed by Second-Harmonic Generation in Nanoantennas.

Nonlinear effects at the nanoscale are usually associated with the enhancement of electric fields in plasmonic structures. Recently emerged new platform for nanophotonics based on high-index dielectric nanoparticles utilizes optically induced magnetic response via multipolar Mie resonances and provides novel opportunities for nanoscale nonlinear optics. Here, we observe strong second-harmonic generation from AlGaAs nanoantennas driven by both electric and magnetic resonances. We distinguish experimentally the contribution of electric and magnetic nonlinear response by analyzing the structure of polarization states of vector beams in the second-harmonic radiation. We control continuously the transition between electric and magnetic nonlinearities by tuning polarization of the optical pump. Our results provide a direct observation of nonlinear optical magnetism through selective excitation of multipolar nonlinear modes in nanoantennas.

Controlling second-harmonic generation at the nanoscale with monolithic AlGaAs-on-AlOx antennas

We review recent achievements in the field of nanoscale nonlinear AlGaAs photonics based on all-dielectric optical antennas. After discussing the motivation and main technological challenges for the development of an AlGaAs monolithic platform for χ(2) nonlinear nanophotonics, we present numerical and experimental investigations of the second-order nonlinear response and physical reasons for high efficiency of second-order nonlinear interactions in the AlGaAs nano-antennas. In particular, we emphasize the role of the dipolar resonances at the fundamental frequency and the multipolar resonances at the second harmonic wavelength. We also discuss second-harmonic generation directionality and show possible strategies to engineer the radiation pattern of nonlinear antennas.

Nonlinear Generation of Vector Beams From AlGaAs Nanoantennas.

The quest for nanoscale light sources with designer radiation patterns and polarization has motivated the development of nanoantennas that interact strongly with the incoming light and are able to transform its frequency, radiation, and polarization patterns. Here, we demonstrate dielectric AlGaAs nanoantennas for efficient second harmonic generation, enabling the control of both directionality and polarization of nonlinear emission. This is enabled by specialized III-V semiconductor nanofabrication of high-quality AlGaAs nanostructures embedded in optically transparent low-index material, thus allowing for simultaneous forward and backward nonlinear emission. We show that the nanodisk AlGaAs antennas can emit second harmonic in preferential direction with a backward-to-forward ratio of up to five and can also generate complex vector polarization beams, including beams with radial polarization.

Enhanced second-harmonic generation from magnetic resonance in AlGaAs nanoantennas.

We designed AlGaAs-on-aluminium-oxide all-dielectric nanoantennas with magnetic dipole resonance at near-infrared wavelengths. These devices, shaped as cylinders of 400nm height and different radii, offer a few crucial advantages with respect to the silicon-on-insulator platform for operation around 1.55μm wavelength: absence of two-photon absorption, high χ((2)) nonlinearity, and the perspective of a monolithic integration with a laser. We analyzed volume χ((2)) nonlinear effects associated to a magnetic dipole resonance in these nanoantennas, and we predict second-harmonic generation exceeding 10(-3) efficiency with 1GW/cm(2) of pump intensity.