Aerosol Optical Depth Measurements Research Articles

Examining UV Radiation Patterns in Relation to Particulate Matter and Atmospheric Conditions in Arid, Unclouded Skies

This study investigates the influences of air temperature (T), relative humidity (RH), wind speed (WS), clearance index (KT), particulate matter (PM) concentrations (PM10 and PM2.5), and aerosol optical depth (AOD) on ultraviolet (UV) radiation during clear skies in Riyadh, central Saudi Arabia. The observational dataset utilized in this study comprises global solar radiation (G), UVA radiation, AOD measurements, and PM concentrations. The data were collected from 2014 to 2015 at the King Abdulaziz City for Science and Technology (KACST) campus in Riyadh. Regression analyses were conducted to investigate the relationships between UV radiation and the considered variables. The methodology is based on the least square method and associated statistical tests. The findings of this study provide valuable insights into the impacts of meteorological variables and aerosols on UV radiation, contributing to the understanding of environmental and industrial applications in the Arabian Peninsula. The analyses showed that the strengths and magnitudes differed from one variable to another. No significant correlations between UVA radiation (315–400 nm) and hourly and daily values of PM2.5 were found. Moreover, no significant correlations were seen between daily values of the UVA radiation and RH and between the UVB (280–315 nm) and PM10. The rest of the correlations (between UV radiation and the PM10 and meteorological variables) were found to be significant. While WS, the ratio of the PM concentrations (PM2.5/PM10), KT, and T exhibited positive correlations with UV radiation, the rest of the variables had anti-correlations with UV radiation. The influences of T, WS, and RH on ambient PM concentrations during the considered period were taken into account, and it was found that the PM concentrations correlate, with different magnitudes and strengths, positively with T and negatively with RH and WS.

Local and Regional Diurnal Variability of Aerosol Properties Retrieved by DSCOVR/EPIC UV Algorithm

AbstractThe hour‐to‐hour variability of 388 nm aerosol optical depth (AOD) and single scattering albedo (SSA) derived from near UV observations by the Earth Polychromatic Imaging Camera (EPIC) on the Deep Space Climate Observatory has been evaluated at multiple locations around the world. AOD retrievals by the EPIC near UV algorithm (EPICAERUV) have been compared to ground based AOD measurements at 16 Aerosol Robotic Network (AERONET) stations representative of the most commonly observed aerosol types over geographic regions in three continents. Obtained results show that, in general, the EPICAERUV algorithm reproduces closely the hour‐to‐hour AOD variability reported by AERONET ground‐truth observations. Although most sites in the analysis show high correlation between the AOD hourly measurements by the ground‐based and space‐borne measuring techniques. Best algorithm performance is observed in the presence of carbonaceous and desert dust aerosols. The diurnal cycle of the retrieved SSA product was also analyzed. Although, a direct comparison of hourly EPICAERUV retrievals to equivalent ground‐based observations was not possible, the satellite result shows that diurnal SSA variability as large as 0.05 can be observed mostly associated with carbonaceous aerosols. EPICAERUV observed diurnal cycle of retrieved AOD on a regional basis was examined for the unusually active seasons of aerosol production of Saharan desert dust aerosols in 2020, and during the 2023 Canadian wildfires. Results presented in this study confirm the EPIC near UV aerosol product is well suited for observing diurnal variability of aerosols and, therefore, it is an important resource for climate and air quality studies.

Combined use of HYSPLIT model and MODIS aerosols optical depth to study the spatiotemporal circulation patterns of Saharan dust events over Central Europe

Mineral dust released from the desert region and transported into the atmosphere has a crucial impact on the Earth's climate system's biogeochemical cycle. It has serious adverse effects on human health. The Sahara is one of the world's dustiest areas. This investigation intends to uncover the underlying reasons for atmospheric dust dispersion throughout the year by tracking the dusttransport and deposition in Central Europe, focusing on arid areas of North Africa. In this paper, we use the GDAS (Global Data Assimilation System) archival meteorological database to compute the analytical forward trajectories and configure the particle concentrations using the HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) model. Besides, we investigate the synoptic meteorological conditions of acute Saharan dust episodes to determine the dynamic atmospheric system during their onset. The forward trajectories reveal the seasonality of wind-blown dust throughout the year. Dust storms are typically more prevalent in the spring, with a second peak in the Summer. As a result, particle transport takes various paths as the seasons and climatic conditions change. The most dust-laden masses, which reach high altitudes from the source areas, are often transported to Central Europe, where their seasonal distribution is relatively similar to that of the studied African region. However, the intensity and frequency of Saharan dust events (SDEs) have significantly changed in the previous decades, with an increased number of intense winter storms. According to the synoptic analysis, this variability is strongly linked to two factors. (1) The intensity and lifetime variation of the Mediterranean cyclones and (2) Climate change triggered lee-side (Sharav) cyclogenesis modified by the topographic complexity of Atlas. This study also confirmed the effectiveness of the HYSPLIT model in simulating atmospheric dust after comparing it with annual aerosol optical depth measurements from MODIS (Moderate-Resolution Imaging Spectroradiometer) data.

Satellite-based aerosol optical depth estimates over the continental U.S. during the 2020 wildfire season: Roles of smoke and land cover

Wildfires produce smoke that can affect an area >1000 times the burn extent, with far-reaching human health, ecologic, and economic impacts. Accurately estimating aerosol load within smoke plumes is therefore crucial for understanding and mitigating these impacts. We evaluated the effectiveness of the latest Collection 6.1 MODIS Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm in estimating aerosol optical depth (AOD) across the U.S. during the historic 2020 wildfire season. We compared satellite-based MAIAC AOD to ground-based AERONET AOD measurements during no-, light-, medium-, and heavy-smoke conditions identified using the Hazard Mapping System Fire and Smoke Product. This smoke product consists of maximum extent smoke polygons digitized by analysts using visible band imagery and classified according to smoke density. We also examined the strength of the correlations between satellite- and ground-based AOD for major land cover types under various smoke density levels. MAIAC performed well in estimating AOD during smoke-affected conditions. Correlations between MAIAC and AERONET AOD were strong for medium- (r = 0.91) and heavy-smoke (r = 0.90) density, and MAIAC estimates of AOD showed little bias relative to ground-based AERONET measurements (normalized mean bias = 3 % for medium, 5 % for heavy smoke). During two high AOD, heavy smoke episodes, MAIAC underestimated ground-based AERONET AOD under mixed aerosol (i.e., smoke and dust; median bias = −0.08) and overestimated AOD under smoke-dominated (median bias = 0.02) aerosol. MAIAC most overestimated ground-based AERONET AOD over barren land (mean NMB = 48 %). Our findings indicate that MODIS MAIAC can provide robust estimates of AOD as smoke density increases in coming years. Increased frequency of mixed aerosol and expansion of developed land could affect the performance of the MAIAC algorithm in the future, however, with implications for evaluating wildfire-associated health and welfare effects and air quality standards.

Novel use of an adapted ultraviolet double monochromator for measurements of global and direct irradiance, ozone, and aerosol

Abstract. A novel ultraviolet spectrometer has been developed and tested over 10 years at Lauder, New Zealand. The system, UV2, makes alternating measurements of the global and direct UV irradiance and can therefore be used to measure ozone and aerosol optical depth. After an analysis of the stability of UV2, these measurements, along with UV irradiance, are compared to relevant observations made by an additional UV spectrometer (UV4), a Dobson spectrophotometer (no. 072), and two radiometers measuring aerosol optical depth – a Prede sky radiometer and a Middleton Solar radiometer (SP02). UV2 irradiance is shown to be lower than UV4 by between 2.5 % and 3.5 %, with a standard deviation of a similar magnitude. Total column ozone values are shown to agree with Dobson spectrophotometer values with a mean bias of 2.57 Dobson units (DU) and standard deviation of 1.15 DU when using the direct sun measurements. Aerosol optical depth at 400–412 and 500 nm agrees to within 0.015 and is comparable to the difference between the reference radiometers. Further work is needed, particularly in the radiometric calibration at longer wavelengths, in order to determine if this instrument can supersede or enhance measurements made by the Dobson spectrophotometer or the aerosol radiometers.

Preliminary Retrieval and Validation of Aerosol Optical Depths from FY-4B Advanced Geostationary Radiation Imager Images

Fengyun-4B (FY-4B) is the latest Chinese next-generation geostationary meteorological satellite. The Advanced Geostationary Radiation Imager (AGRI) aboard FY-4B is equipped with 15 spectral bands, from visible to infrared, suitable for aerosol optical depth (AOD) retrieval. In this study, an overland AOD retrieval algorithm was developed for the FY-4B AGRI. Considering the large directional variation in the FY-4B AGRI reflectances, a bidirectional reflectance distribution function (BRDF) database was built, through which to estimate land surface reflectance/albedo. Seasonal aerosol models, based on four geographical regions in China, were developed between 2016 and 2022 using AERONET aerosol products, to improve their applicability to regional distribution differences and seasonal variations in aerosol types. AGRI AODs were retrieved using this new method over China from September 2022 to August 2023 and validated against ground-based measurements. The AGRI, Advanced Himawari Imager (AHI), and Moderate-Resolution Imaging Spectroradiometer (MODIS) official land aerosol products were also evaluated for comparison purposes. The results showed that the AGRI AOD retrievals were highly consistent with the AERONET AOD measurements, with a correlation coefficient (R) of 0.88, root mean square error (RMSE) of 0.14, and proportion that met an expected error (EE) of 65.04%. Intercomparisons between the AGRI AOD and other operational AOD products showed that the AGRI AOD retrievals achieved better performance results than the AGRI, AHI, and MODIS official AOD products. Moreover, the AGRI AOD retrievals showed high spatial integrity and stable performance at different times and regions, as well as under different aerosol loadings and characteristics. These results demonstrate the robustness of the new aerosol retrieval method and the potential of FY-4B AGRI measurements for the monitoring of aerosols with high accuracy and temporal resolutions.

Retrieval of Aerosol Optical Depth and FMF over East Asia from Directional Intensity and Polarization Measurements of PARASOL

The advantages of performing aerosol retrieval with multi-angle, multi-spectral photopolarimetric measurements over intensity-only measurements come from this technique’s sensitivity to aerosols’ microphysical properties, such as their particle size, shape, and complex refraction index. In this study, an extended LUT (Look Up Table) algorithm inherited from a previous work based on the assumption of surface reflectance spectral shape invariance is proposed and applied to PARASOL (Polarization and Anisotropy of Reflectances for Atmospheric Science coupled with Observations from a Lidar) measurements to retrieve aerosols’ optical properties including aerosol optical depth (AOD) and aerosol fine-mode fraction (FMF). Case studies conducted over East China for different aerosol scenes are investigated. A comparison between the retrieved AOD regional distribution and the corresponding MODIS (Moderate-resolution Imaging Spectroradiometer) C6 AOD products shows similar spatial distributions in the Jing-Jin-Ji (Beijing–Tianjin–Hebei, China’s mega city cluster) region. The PARASOL AOD retrievals were compared against the AOD measurements of seven AERONET (Aerosol Robotic Network) stations in China to evaluate the performance of the retrieval algorithm. In the fine-particle-dominated regions, lower RMSEs were found at Beijing and Hefei urban stations (0.16 and 0.18, respectively) compared to those at other fine-particle-dominated AERONET stations, which can be attributed to the assumption of surface reflectance spectral shape invariance that has significant advantages in separating the contribution of surface and aerosol scattering in urban areas. For the FMF validation, an RMSE of 0.23, a correlation of 0.57, and a bias of −0.01 were found. These results show that the algorithm performs reasonably in distinguishing the contribution of fine and coarse particles.

Fine and Coarse Dust Effects on Radiative Forcing, Mass Deposition, and Solar Devices Over the Middle East

AbstractIn desert regions like the Middle East, dust has a profound impact on the environment, climate, air quality, and solar devices. The size of dust particles determines the extent of these effects. Dust deposition (DD) measurements show that coarse dust particles with geometric radius r > 10 μm comprise most of the deposited mass. Still, these particles are not represented in the current models that are tuned to fit the observed aerosol optical depth (AOD). As a result, the existing models and reanalysis products underestimate DD and dust emission (DE) almost 3 times. This is the first study to constrain the dust simulations by both AOD and DD measurements to quantify the effect of coarse and fine dust using the WRF‐Chem model. We found that, on average, coarse dust contributes less than 10% to dust shortwave radiative forcing (RF) at the surface but comprises more than 70% of DE. Annual mean net RF over the Arabian Peninsula and regional seas locally reaches −25 W m−2. Airborne fine dust particles with radii r < 3 μm are mainly responsible for the significant dimming (5%–10%) of solar radiation, cooling the surface, and hampering solar energy production. However, dust mass deposition is primarily linked to coarse particles, decreasing the efficiency of photovoltaic panels by 2%–5% per day. Therefore, incorporating coarse dust in model simulations and data assimilation would improve the overall description of the dust mass balance and its impact on environmental systems and solar devices.

Study of Atmospheric Aerosols in The Bahamas Using Camera Lidar and Star Photometry Techniques

Aerosols, the tiny suspended particles in the atmosphere, are a widely studied topic around the world due to their effects on the Earth’s radiation budget, climate change, and human health. Knowledge of the spatial and temporal distribution of aerosols is essential to assess air pollution and predict potential climate change. This study measured aerosol optical depth (AOD) and altitude-dependent aerosol extinctions in Nassau, The Bahamas simultaneously using a camera-based imaging lidar (CLidar). The bistatic geometry of the setup which consisted of a wide-angle lens fitted to a charge-coupled device (CCD) camera, allowed for the measurement of extinctions at all altitudes at once without requiring expensive timing electronics common to lidars. A case study was conducted on November 5, 2018. The top of the boundary layer beyond which aerosol extinction was nearly zero was detected at ~ three km above sea level. Due to the excellent resolution of the CLidar at lower altitudes, variations of aerosol concentrations within the boundary layer are efficiently detected. Optical depth was measured using the same CLidar camera at the same time, utilising star photometry, and was found to be 0.043 ± 0.040. The value falls within the range of assumed values of AOD near the regions obtained from the Moderate Resolution Imaging Spectroradiometer (MODIS) Aqua satellite.

ANALYSIS OF AEROSOLS IN WEST AFRICA: MODELLING AND RADIATIVE FORCING

We studied the aerosol properties in Cinzana and Ilorin in West Africa using data of aerosols’ properties over the period 2000–2015 from MODIS (Moderate resolution Imaging Spectroradiometer). There has been limited report on the comparison between this two West African Stations. The time series modelling, prediction of aerosol parameters and the estimation of aerosol radiative forcing (ARF) were focused on. Statistical Package for the Social Sciences (SPSS) software was used for the modelling the monthly averaged measurements of aerosol optical depth at 550 nm (τ550), Angstrom exponent at 470 – 660 nm (α470-660), cloud fraction (Ncloud), fine mode fraction (FMF) and single scattering albedo at 470 nm (ωo) data over the two stations while the ARF values were calculated. The generated time series models are all good fit and the values are biased, both negatively and positively. The ARF of the two stations’ aerosol data shows value between 0.0 and -750.0 W/m2 for Ilorin and -10.0 to -200. 0 W/m2, which results mainly in cooling. Although there is a difference between ARF values in the two stations, both stations demonstrated clear seasonal variation with the rainy season having the least negative aerosol forcing. The results suggest that the aerosols are predominantly mineral dust, but those in Cinzana have more absorbing properties than those in Ilorin. Overall, the research shows that the modelled parameters can be utilized in lieu of the measured data and that the solar radiation received in this region has been attenuated at various degrees

Retrieving PM10 Surface Concentration from AERONET Aerosol Optical Depth: The Cairo and Delhi Megacities Case Studies

Large concentrations of air-suspended particulate matter (PM) in megacities represent an important health risk for their populations, but PM time series are often missing or too short to quantify the associated burden of diseases. In this study, we propose a model for retrieving the surface PM in Cairo (Egypt) and Delhi (India) from the automated measurements of aerosol optical depth (AOD), precipitable water (PW), and Angström exponent (AE) performed by the sunphotometers of the Aerosol Robotics Network (AERONET). For this we exploit the (1) synchronous measurements performed from 2010 to 2015 at the headquarters of the Egyptian Meteorological Authority and in 2009 at the Gual Pahari station (25 km south of Delhi) and (2) the ERA5 estimate of the planetary boundary layer height (H). The correlation between the surface PM10 and the AOD is primarily controlled by the variations of PW and secondarily by those of H: for similar surface PM10 concentrations, the AOD tends to be the largest in summer because of the hygroscopic enhancement of the mass extinction efficiency (σ) of the particles and their dilution in the more developed mixing layer. The variations of composition also play a significant role in Cairo. This effect, particularly marked in spring (coinciding with the dust season), can be parameterized as a linear function of AE. Finally, we show that the variations of the surface PM10 concentration at the two sites can be retrieved simply from those of the AOD, PW, AE and H. At the weekly temporal resolution, the agreement between the model and the observations is very good at the two locations (correlation coefficient > 0.81, relative mean absolute error < 15%). This validates indirectly the assumption made in the development of the model, namely that the aerosols are mostly confined to the mixing layer of the two megacities and not transported in the free atmosphere. Provided a few years of surface PM measurements are available, the methodology proposed in this study could be easily applied to any other AERONET station.

Spatial distribution of aerosols burden and evaluation of changes in aerosol optical depth using multi-approach observations in tropical region

Understanding of Aerosol optical depth (AOD) parameter is important for air quality assessment. This study aims to evaluate and validate AOD measurements from combine datasets to improve air quality for a period 2005–2020 using Aerosol Robotic Network (AERONET) at Ilorin site (8.320° N, 4.340° E) in Nigeria. AOD outputs from Community Atmosphere Model Version 6 with chemistry (CAM6-chem) at 1° horizontal resolution and Modern-Era Retrospective analysis for Research and Applications (MERRA-2) are investigated in addition to validation of two satellites AOD retrievals: Moderate Resolution Imaging Spectroradiometer (MODIS) and Multi-angle Imaging Spectroradiometer (MISR). Result of spatial distribution of AOD shows high values > 1 in the North and Western Sahara compared to Central Africa. Desert dust shows largest contribution in the North and Western Africa that is up to 2 magnitude larger than other aerosol types. Primary organic matter (POM) and secondary organic aerosols (SOAs) both presents high burdens with later been dominant at around 10° band, and black carbon (BC) largest burden (2.6 × 10 − 5 kgm − 2) is seen in the model from oil and gas exploration site in Nigeria. Inter-comparison of MERRA/MISR/MODIS and AERONET AOD using linear correlation of the seasonal dependence demonstrated high correlation (r = 0.864 − 0.973) subjected to Root Mean Square Error (RMSE = 0.069 − 0.211), suggesting good agreement between the datasets. When compared to seasonal mean maximum AERONET AOD value of 0.978 MERRA is ∼5%, MISR ∼28% and MODIS ∼29% lower with stronger correlations observed in the wet and pre-harmattan seasons. Similarly, MODEL AOD at 550 nm and dust burden were found to be ∼34% and ∼67% lower in context to AERONET AOD annual mean value of 0.627. Positive relationships that indicate an upward slope exist between all the computed datasets with moderate value of AERONET/CAM-chem spearman partial correlation, and MERRA/MODIS and MODIS/MISR showing strong and significant relationship with p-value less than 0.05. Low variance is observed with all measurements except in MERRA.

The impact of different aerosol layering conditions on the high-resolution MODIS/MAIAC AOD retrieval bias: The uncertainty analysis

The Eastern Mediterranean/Middle East (EMME) region belongs to one of the most polluted and vulnerable to climate change related areas in the world. To monitor these changes, comprehensive set of measurements need to be conducted. Ground-level monitoring sites provide continuous measurements, yet their spatial coverage in EMME is very limited. Satellite data largely expand spatial coverage, however, retrieval accuracy over arid regions with bright surface background, mixed with urban and industrial sources, remains challenging. In this study, we analyzed the agreement between aerosol optical depth (AOD) data from the Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm at 1-km spatial resolution and corresponding ground-based Aerosol Robotic Network (AERONET) measurements, using data from September 2019 to October 2022 in Tel Aviv, Israel. We identified all overestimation and underestimation MAIAC AOD measurements, relative to AERONET, and used multiwavelength polarization lidar observations of vertical aerosol profiles to characterize these conditions. Our findings suggest that under clear atmospheric conditions (AOD¡0.12), MAIAC overestimation prevails, while under dusty (AOD¿0.3), and partially cloudy conditions, MAIAC underestimation prevails. We found that dust component (high particle depolarization ratio, and low Angstrom exponent) is often presented in cases of underestimation, while a single layer overestimation cases typically related to anthropogenic pollution. The two-layers overestimation cases tend to have marine aerosols at the bottom and mixed pollution sources at the top. Our study highlights the importance of studying the different layering conditions that largely bias the MAIAC AOD retrieval accuracy. This knowledge is highly important since AOD is widely used as input variable in numerous modeling studies and air quality applications and rarely prepossessed for such a bias.

Operational AOD Retrieval at Subkilometer Resolution Using OceanSat‐2 OCM Over Land: SAER Algorithm, Uncertainties, Validation &amp; Inter‐Sensor Comparison

AbstractThe ocean color monitor (OCM) sensor onboard OceanSat‐2 is providing data in visible and near Infrared (NIR) bands. Due to the limited spectral coverage of OCM, the widely used dark‐target and deep‐blue aerosol algorithms cannot be adapted. Here, a new aerosol optical depth (AOD) retrieval algorithm for OCM (or similar sensors) over land, termed Space Applications Center AErosol Retrieval (SAER) is described. It utilizes two blue bands for the AOD inversion and, Red and NIR band to characterize the surface in visible bands without assuming red and NIR bands transparent to aerosols. Unlike the dark‐target algorithm, the SAER algorithm can retrieve AOD over bright arid and urban areas too. The uncertainty analysis of SAER suggests a theoretically expected error (EE) envelope of ±(0.06 + 0.26 × AOD) for typical retrieval conditions. OCM AOD over land is retrieved operationally for the first time over Indian and neighboring countries' landmass at the finest spatial resolution of 0.007°. The SAER algorithm is validated against in‐situ AOD measurements during the years 2016–2018 at 21 Aerosol Robotic Network stations located in south‐Asia. Overall validation using 1900 match‐up points shows correlations exceeding 0.8 with 74% of retrievals within EE. The retrievals over cropland, grassland, and mixed land cover types show high (low) correlation (bias), while over bright urban areas somewhat low (high) correlation (bias) is observed. Excluding monsoon season, OCM AOD retrievals show good performance over the year. The performance of MODerate Resolution Imaging Spectroradiometer dark‐target and OCM AOD, against common in‐situ, is close to each other. The study shows that OCM AOD can be used for air quality monitoring/modeling at high spatial resolution.

Footprint of the 2020 COVID-19 Lockdown on Column-Integrated Aerosol Parameters in Spain

The lockdown adopted in Spain to combat the global pandemic due to the coronavirus disease (COVID-19) led to a significant reduction in the emission of aerosols produced by road traffic and industry. This study aims to detect changes in column aerosols in Spain due to the COVID-19 lockdown. High-quality AErosol RObotic NETwork (AERONET) measurements of AOD (aerosol optical depth), AE (Ångström exponent) and SSA (single scattering albedo) over the period 2012–2020 are used for this purpose. Ten AERONET stations with available measurements during the lockdown and post-lockdown periods with a long previous data record are selected. The stations are well distributed throughout Spain, covering different areas and population densities. A comprehensive set of three statistical tests are applied to assess general changes in the dataset, the central tendency and low and high values for each parameter. The analyses are conducted for the 2020 lockdown and post-lockdown periods by comparing daily aerosol data with the measurements recorded for the same calendar days during the period 2012–2019. The results indicate a general increase in AOD during the lockdown and a decrease during the post-lockdown. While AE shows no overall behaviour, SSA is the parameter most sensitive to changes in anthropogenic contribution, with an overall significant increase in almost all the stations during both lockdown and post-lockdown periods. The study contributes to addressing the impact of the COVID-19 lockdown and provides methodologies to detect its footprint.

High-Resolution Aerosol Optical Depth Retrieval in Urban Areas Based on Sentinel-2

In this paper, an improved aerosol optical depth (AOD ) retrieval algorithm is proposed based on Sentinel-2 and AErosol RObotic NETwork (AERONET ) data. The surface reflectance for AOD retrieval was estimated from the image that had minimal aerosol contamination in a temporal window determined by AERONET data. Validation of the Sentinel-2 AOD retrievals was conducted against four Aerosol Robotic Network (AERONET ) sites located in Beijing. The results show that the Sentinel-2 AOD retrievals are highly consistent with the AERONET AOD measurements (R = 0.942), with 85.56% falling within the expected error. The mean absolute error and the root-mean-square error are 0.0688 and 0.0882, respectively. In addition, the AOD distribution map obtained by this algorithm well reflects the fine-spatial-resolution changes in AOD distribution. These results suggest that the improved high-resolution AOD retrieval algorithm is robust and has the potential advantage of retrieving high-resolution AOD over urban areas.

Generation of High Temporal Resolution Full-Coverage Aerosol Optical Depth Based on Remote Sensing and Reanalysis Data

Aerosol Optical Depth (AOD) is a crucial physical parameter used to measure the radiative and scattering properties of the atmosphere. Obtaining full-coverage AOD measurements is essential for a thorough understanding of its impact on climate and air quality. However, satellite-based AOD products can be affected by abnormal weather conditions and high reflectance surfaces, leading to gaps in spatial coverage. To address this issue, we propose a satellite-based AOD filling method based on hourly level-3 Himawari-8 AOD products. In this study, the optimal model with a mean bias error (MBE) less than 0.01 and a root-mean-square error (RMSE) less than 0.1 in most land cover types was selected to generate the full-coverage AOD. The generated full-coverage AOD was validated against in situ measurements from the AERONET sites and compared with the performance of Himawari-8 AOD and MERRA-2 AOD over the AERONET sites. The validation results indicate that the accuracy of full-coverage AOD is comparable to that of the Advanced Himawari Imager (AHI) AOD, and for other land cover types (excluding barren land), the accuracy of full-coverage AOD is superior to that of MERRA-2 AOD. To investigate the practical application of full-coverage AOD, we utilized it as an input parameter to perform radiative transfer simulations in northwestern and southern China. The validation results showed that the simulated at-sensor radiance based on full-coverage AOD was in good agreement with the at-sensor radiance observations from MODIS. These results indicate that complete and accurate measurements of AOD have considerable potential for application in the simulation of at-sensor radiance and other related topics.

Feasibility analysis of AERONET lunar AOD for nighttime particulate matter estimation

Several studies have attempted to estimate particulate matter (PM) concentrations using aerosol optical depth (AOD), based on AOD and PM relationships. Owing to the limited availability of nighttime AOD data, PM estimation studies using AOD have focused on daytime. Recently, the Aerosol Robotic Network (AERONET) produced nighttime AOD, called lunar AOD, providing an opportunity to estimate nighttime PM. Nighttime AOD measurements are particularly important as they help fill gaps in our understanding of aerosol variability and its impact on the atmosphere, as there are significant variations in AOD between day and night. In this study, the relationship between lunar AOD and PM was investigated using data from AERONET station, meteorological station, and air pollution station in Seoul Metropolitan area from May 2016 to December 2019, and then PM estimation model was developed covering both daytime and nighttime using random forest machine learning techniques. We have found the differences in the importance of variables affecting the AOD-PM relationship between day and night from the random forest model. The AOD-PM relationship in the daytime was more affected by time-related variables, such as the day of the year among the variables. The new model was developed using additional lunar AOD data to estimate continuous PM concentrations. The results have shown that the model based on lunar AOD data estimated well PM10 and PM2.5 with similar performance of model using solar AOD. The results imply the possibility of seamless near-surface PM concentration data on a large scale once satellites produce nighttime AOD data.

Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest

Abstract. The Amazon rainforest routinely experiences intense and long-lived biomass burning events that result in smoke plumes that cover vast regions. The spatial and temporal extent of the plumes and the complex pathways through which they interact with the atmosphere have proved challenging to measure for purposes of gaining a representative understanding of smoke impacts on the Amazonian atmosphere. In this study, we use multiple collocated satellite sensors on board AQUA and TERRA platforms to study the underlying smoke–cloud–radiation interactions during the diurnal cycle. An 18-year time series for both morning and afternoon overpasses is constructed, providing collocated measurements of aerosol optical depth (AOD; column-integrated aerosol extinction), cloud properties, top-of-atmosphere radiative fluxes, precipitation, and column water vapour content from independent sources. The long-term time series reduces the impact of interannual variability and provides robust evidence that smoke significantly modifies the Amazonian atmosphere. Low loadings of smoke (AOD ≤ 0.4) enhance convective activity, cloudiness, and precipitation, but higher loadings (AOD &gt; 0.4) strongly suppress afternoon convection and promote low-level cloud occurrence. Accumulated precipitation increases with convective activity but remains elevated under high smoke loadings, suggesting fewer but more intense convective cells. Contrasting morning and afternoon cloud responses to smoke are observed, in line with recent simulations. Observations of top-of-atmosphere radiative fluxes support the findings and show that the response of low-level cloud properties and cirrus coverage to smoke results in a pronounced and consistent increase in top-of-atmosphere outgoing radiation (cooling) of up to 50 W m−2 for an AOD perturbation of +1.0. The results demonstrate that smoke strongly modifies the atmosphere over the Amazon via widespread changes to the cloud field properties. Rapid adjustments work alongside instantaneous radiative effects to drive a stronger cooling effect from smoke than previously thought, whilst contrasting morning and afternoon responses of liquid and ice water paths highlight a potential method for constraining aerosol impacts on climate. Increased drought susceptibility, land use change, and deforestation will have important and widespread impacts on the region over the coming decades. Based on this analysis, we anticipate that further increases in anthropogenic fire activity will associated with an overall reduction in regional precipitation and a negative forcing (cooling) on the Earth's energy budget.

Ground-based measurements of cloud and aerosol optical depths in the UV-B at an urban tropical site

Cloud and aerosol optical depths (CODλ and AODλ respectively) at wavelength λ in the terrestrial atmosphere have been obtained from space and ground-based remote experiments. Generally, they are for the ultraviolet A (UV-A), visible, and infrared ranges of the electromagnetic spectrum. Despite the significant effects of the ultraviolet B (UV-B) on the biosphere, fewer optical depth studies have aimed at this range. The weaker irradiance of the solar UV-B in relation to the three other ranges, hampering UV-B direct Sun measurements through clouds and aerosol plumes, would be a reason for that. Nonetheless, for 16 months, CODλ and AODλ from ground-based measurements in the UV-B were obtained for an urban tropical site, where biomass burning aerosols are potential contributors in addition to anthropogenic pollutants and cumulus and stratus cloud genera as predominant cloud cover. CODλ and AODλ are drawn from the reduction of the optical depths of both ozone and molecular scattering (τO3λ and τMSλ respectively) from the atmospheric optical depth (τAtλ) obtained from Beer's Law. The daily averages of CODUV-B ranged from 0.205 to 1.101 ± 0.916 (1 standard deviation) for low and middle altitude clouds mainly, being the maximum CODUV-B ≈ 3.2. The daily averages of AODUV-B ranged from 0.09 ± 0.02 to 1.75 ± 0.07, being augmented by the presence of clouds.