Santa Quitéria, a city in northeastern Brazil, faces significant challenges in ensuring the availability of potable water due to its semi-arid climate and limited water resources. This study investigates the radiological quality of surface waters commonly used by the population for drinking and by animals for hydration. Water samples were collected from six different locations over a 25-month period, and the concentrations of naturally occurring radionuclides were measured using spectrophotometric analysis, total alpha, and gross beta counting. The mean activity concentrations of Unat, 226Ra, 210Pb, 232Th, and 228Ra were determined to be 9.89∙10−2, 5.35∙10−2, 5.86∙10−2, 6.89∙10−3, and 2.81∙10−3 Bq∙L−1, respectively. Statistical methods, such as cluster and factor analysis, were applied to understand the distribution patterns of these radionuclides. The study also estimated dose rates from radionuclide intake, with a maximum value of 108.5 µSv·y−1, and compared the results against dose limits set by relevant organizations. Furthermore, the risks of morbidity and mortality from radionuclide intake were assessed, revealing the need for optimization at one sampling point where the health risks exceeded intervention thresholds.
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