Activity Of Natural Radionuclides Research Articles

Assessment of Natural Radioactive Nuclides in Different Herbal Remedies Consumed in Katsina Metropolis

The use of herbal remedies to treat various ailments is common practice in developing countries, but the formulation of these products is usually complex, hence, the need for thorough quality checks especially with possible health risks these could pose. The research aimed to assess the natural radioactive nuclides concentrations of herbal formulations sold in Katsina Metropolis and ascertain the radiological implications for humans. The activity concentration of natural radionuclides in the fifteen (15) herbal remedies commonly consumed in the Katsina metropolis. Results from the above table show the activity of natural radionuclides in 15 herbal remedy samples found in the Katsina metropolis. The activity concentration of 40K ranges from 1027.76+51.30, which was found to have the highest radioactivity in the G, and 51.77+2.60 was found to be lowest in K. In 238U which ranges from 72.78+7.67 in O and the lowest concentration of 1.65+0.23 in E then lastly followed by the activity concentration of 232Th activity concentration varies from 20.18+1.13 as the highest and the lowest in B with 1.26+-0.07.

Assessment of radioactive nuclides and heavy metals in soil and drink water in Lahij city, Yemen

This study was conducted in Lahij city, Yemen, to evaluate the concentrations and potential health risks of natural radioactive nuclides and heavy metals in soil and drinking water. A total of 21 soil samples and 17 water samples were collected from various locations. A high-purity germanium gamma detector HPGe was used to measure the concentrations of 40K, 232Th, and 226Ra in all samples, along with the concentrations of heavy metals. In soil samples, the average concentrations of 40K, 232Th, and 226Ra were 731.5, 30.7, and 28.16 Bq kg−1, respectively. While some samples showed higher than permissible levels for 226Ra and 232Th, the overall average remained within acceptable limits. However, 40K levels were almost twice the recommended global limits. In water samples, the average concentrations of these nuclides were 5.38, 0.73, and 0.66 Bq L−1, all within the global safety limits. Radiological risk assessments for soil indicated an average radium equivalent activity (Raeq) of 124.4 Bq kg−1, absorbed dose rate in air of 59.9 nGy h−1, annual effective dose rate of 0.07 mSv y−1, outdoor excess lifetime cancer risk (ELCR) of 0.26 × 10−3, and annual gonad equivalent dose (AGED) of 336.6 mSv y−1. Risk indices, including the activity concentration index (Iγ), external hazard index (Hex), and internal hazard index (Hin), averaged 0.48, 0.34, and 0.41, respectively, all below global limits except for AGED, which slightly exceeded the recommended level. For drinking water, the total ingestion dose was calculated for different age groups. The average doses for infants, children, and adults were 0.15, 0.27, and 0.19 mSv y−1, respectively. The doses for children and adults exceeded the permissible limits, while those for infants were within safe levels. Heavy metal concentrations were measured in all samples, and the Hazard Quotient (HQ) was calculated. In soil samples, HQ values for all metals >1, indicating potential health risks. In water samples, HQ values were also >1 for all metals except vanadium (V) and iron (Fe). To reduce the dangers associated with radioactive nuclides and heavy metals, regular monitoring and cleanup are crucial, and further research is needed to understand contamination sources and long-term health impacts.

RESEARCH OF THE POSSIBILITY OF USING CHP ASH IN THE PRODUCTION OF FIRED ASH GRAVEL

The article presents a comparative analysis of the characteristics of the dump ash of the Kyzylorda CHP hydraulic removal. A huge amount of ash, slag waste is collected in the dumps of the CHP, their accumulation in the dumps leads to a violation of the ecology of the environment. The issue of ash, slag waste disposal is an urgent problem. The use of ash and slag not only solves the issue of availability of raw materials, but also allows to improve the quality of products while reducing their cost. One of the valuable components of ash and slag waste is hydraulic removal ash. Hydraulic removal ash as a raw material can be used for the manufacture of artificial concrete aggregates (ash, agglomerate gravel, etc.). Studies were conducted to study the physico-chemical composition, determine the specific effective activity of natural radionuclides, loss during calcination of two types of hydraulic removal ash samples from Kyzylorda CHP (black and gray), which differ in sampling sites from ash dump. When studying the properties of the ash, X-Ray phase analysis was carried out, with the help of which the phase composition of the ash was determined. Work was carried out on the X-Ray phase analysis of ash, determination of the specific effective activity of natural radionuclides, calcination losses, which showed the possibility of using ash for the production of building materials. The conducted studies have confirmed the expediency of using the ash of the Kyzylorda thermal power plant in the production of fired ash gravel.

Natural radioactivity and heavy metal contamination in edible fish, shellfish and mollusks at the Bay of Bengal, Kuakata, Bangladesh

In this study, gamma activity concentrations, gross alpha and gross beta activity of natural radionuclides, and heavy metal concentrations were measured in eleven edible marine fish, four shellfish, two mollusks, and a common seaweed sample collected from a local sea fish market and sea beach area of the northern part of the Bay of Bengal, Kuakata, Bangladesh. Using HPGe gamma spectrometry, the activity concentrations of 238U, 232Th, and 40K were measured and found to be 19.7 ± 1.5 Bq/kg, 12.2 ± 0.9 Bq/kg, and 188 ± 15 Bq/kg, respectively, with the 232Th concentration surpassing that of 238U. The ZnS scintillation detector was used to assess the gross alpha and gross beta activity. The average gross alpha activity and gross beta activity were found to be 9.4 ± 1.4 Bq/kg and 26 ± 4 Bq/kg, respectively, with the latter attributed to beta emitting radionuclides's abundance. The activity concentrations of 238U, 232Th, and 40K in the analyzed samples varied in the order of Shellfish > Seaweed > Fish > Mollusks, Seaweed > Shellfish > Mollusks > Fish, and Seaweed > Shellfish > Fish > Mollusks. The annual effective dose due to consumption of analyzed seafood was found to be within the world limit of 2400 μSv/y recommended by UNSCEAR. The main contributor to the annual effective dose was 238U. The excess lifetime cancer risk (ELCR) results were below the permissible threshold of 10−3 for radiological risks. Furthermore, average concentrations of Zn and Mn were higher than WHO/FAO recommended values, and carcinogenic Pb, Cd, Cr, and Hg concentrations were below detection limits, according to heavy metal analysis performed by AAS. The average concentration of heavy metals in all of the seafood samples under investigation was in the order of Zn > Fe > Mn. The calculated hazard index (HI), target hazard quotient (THQ), and estimated daily intake (EDI) were compared to the permissible safety limits.

Review and statistical analysis of activity values reported for coastal sands worldwide

The activity of natural radionuclides is unevenly distributed across the Earth's crust, with certain areas exhibiting significantly higher levels than others, known as High Background Radiation Areas (HBRAs). This study presents a statistical analysis of reported activity values for coastal sands globally. Through this statistical analysis, costal sands were classified into four categories based on their activity levels, providing a standardized framework to compare the natural radioactivity of these sands. This classification is a valuable tool for identifying populations exposed to different radiation levels, which is essential for the study of stochastic effects. The study proposes thresholds to define HBRAs as regions with activity values exceeding 203 Bq/kg for 238U, 517 Bq/kg for 232Th, or 960 Bq/kg for 40K. Regions with lower values are classified as NonHBRAs. Further subdivision of these categories resulted in four distinct regions: NonHBRA−, NonHBRA+, HBRA−, and HBRA+. The activity values for these subdivisions are 92 Bq/kg and 2,903 Bq/kg for 238U, 94 Bq/kg and 7,230 Bq/kg for 232Th, and 901 Bq/kg and 2,298 Bq/kg for 40K. By calculating the external dose rates from the reported activity data, a threshold of 357 nGy/h was identified as the dose boundary separating NonHBRAs from HBRAs. The values for the subdivisions resulted 101 nGy/h and 3,867 nGy/h. The study also explores the content of these natural radionuclides in relation to their bearing minerals and discusses correlations between the reported activity values and the characteristics of the sands. Additionally, the activity of the anthropogenic radionuclide 137Cs (reported values ranging from the detection limit to 63 Bq/kg) is examined.

Оценка пространственно-временных изменений показателей радиоэкологического состояния почв зоны наблюдения Ростовской АЭС

The paper presents the results of a study of long-term (from 2003 to 2021) measurements of the specific activity of natural (226Ra, 232Th, 40K) radionuclides and artificial 137Cs in surface soil samples and soil profiles, including the dependence of the specific activity of radionuclides on some soil properties (content organic matter, pH level) in the observation zone of the Rostov NPP. In accordance with the requirements of radioecological monitoring, the study of the state of terrestrial ecosystems was carried out considering landscape-geochemical and climatic conditions in control plots with Haplic Kastanozems, Gleyic Kastanozems, Endosalic Kastanozems and Umbric Fluvisols soils laid out in the study region in 1999–2000 as part of pre-start monitoring of the Rostov NPP. It has been shown that there is a decrease in the specific activity of 226Ra in all studied soil types. A regular redistribution along the profile of artificial 137Cs in the Gleyic Kastanozems soil was revealed. There is no redistribution of natural radionuclides (226Ra, 232Th, 40K) in soil profiles over time. The minimum specific activity of radionuclides is recorded in Umbric Fluvisols soil located in the floodplain of the Don River. A linear dependence of the specific activity of 137Cs on pH and humus was established (r=0.62 and 0.88, respectively). Keywords: RADIOECOLOGICAL MONITORING, ROSTOV NPP, NATURAL AND ARTIFICIAL RADIONUCLIDES, ORGANIC MATTER, pH

PROPERTIES OF URBAN SOILS AFTER DECONTAMINATION MEASURES ON THE RADIOACTIVELY CONTAMINATED TERRITORY OF THE CITY OF ELEKTROSTAL

We studied morphological properties, pH, organic carbon content, and specific activity of 137Cs and natural radionuclides (40K, 226Ra, 232Th) in the upper horizons of soils in deactivated and slightly damaged areas of the city. The studies were carried out in the urban ecosystems of the city of Elektrostal (Moscow region) in 2019, i.e. 6 years after local precipitation of 137Cs due to a radiation incident. Morphological features of the upper horizons of urban soils were: brownish-gray color, light-loamy composition, small-lumpy and lumpy structure, inclusions of construction and household waste. In the upper horizons of urbiquasizems and urban soils, a low carbon content (less than 1%) with high coefficients of variation - were detected. In the studied urban soils, a wide range of water pH values was noted: from acidic (4,6-5,5) to highly alkaline (> 8,0) reaction. Correlation analysis showed that in the upper horizons of UR, the content of organic carbon was reduced and alkalinization of the soil environment was observed. The accumulative type of distribution of 137Cs was recorded for soil profiles of polluted urban ecosystems in which decontamination measures were not carried out. The profiles of urban soils that were subjected to decontamination revealed low values of the specific activity of 137Cs in surface bulk layers and maxima in buried contaminated horizons. In the bulk horizons of UR, which include a large amount of crushed stone, there is an increase in the specific activity of 226Ra. Some technogenic horizons UR and TCH, consisting mainly of quartz sand, are characterized by very low values of specific activities 226Ra and 40K. Correlations of chemical and radiation indicators in the profiles of urban soils reflect the different composition and properties of upper horizons formed as a result of excavation and decontamination work.

Measurement of Natural Radionuclide Activity in Soil Samples from Different Regions in Al-Hilla City, Iraq

Measurement of Natural Radionuclide Activity in Soil Samples from Different Regions in Al-Hilla City, Iraq

Accumulation of Technogenic and Natural Radionuclides in the Don Delta Sediments

The study of current sedimentation processes and radioactive contamination in the total area of the Don Delta is the research goal. The presented paper contains data analysis of radioecological and lithologic studies on bottom sediments, sampled in the northern part of the Don Delta in 2022. Based on the research results obtained, the authors provide the characteristics of the current conditions of sedimentation and specific activity of artificial and natural radionuclides in fluvial deposits, as well as indicate that similar in characteristics sandy-silty aleurites and sandy aleurite-clayish silts with inclusions of plant and shell detritus compose the bottom sediments of numerous braided channels. The authors determined the zonal accumulation character of both 137Cs technogenic and 226Ra, 40K, and 232Th natural radionuclides which conditions their accumulation and content increase from the lower delta to the upper delta areas. The velocity of currents in the braided channels (bayous) and related sedimentation conditions of suspended matter, as well as the lithotype of the bottom ground determine the indicated regularity. We assume that unlike 137Cs the distribution of natural radionuclides (40K, 226Ra, and 232Th) mainly depends on the mineral content of sediments entering the delta with the river runoff. Relatively low indices – on average ca. 9 Bq/kg of dry weight (d.w.) – characterise the current range of 137Cs radioisotope concentrations in the sediments of the Northern Don Delta. Such a level of specific activity is of no danger to the regional ecosystem.

Radioactivity estimation of baobab (Adonsonia digitata) in katsina metropolis, katsina state Nigeria

Radioactivity estimation of baobab plants was carried out in Katsina metropolis, Katsina State, Nigeria. Samples of soil, roots, and leaves were collected, prepared and analyzed to estimate the activity concentration of the natural radionuclides of U-238, Th-232, and K-40using NaI (TI) gamma ray spectrometry detector. The results obtained showed that the activity concentration ranged from 0.1 Bq/kg to 33.26 Bq/kg, 1.98 Bq/kg to 64.98 Bq/kg and 65.89 Bq/kg to 1009.69 Bq/kg with overall mean values of 11.35, 18.87 and 545.14 in Bq/kg for U-238, Th-232 and K-40 respectively. In order to assess the radiological parameters of the natural radioactivity; the radium equivalent activity (Raeq), an absorbed dose rate and the measured annual effective dose equivalent were calculated and lies in the ranges of 18.83 to 183.22 (Bq/kg), 9.07 to 85.90 nGy/h and 0.011 to 0.105 mSv/y respectively; mean values obtained are 87.20 Bq/kg, 40.55 nGy/h and 0.050 mSv/y respectively. However, the calculated values obtained for all the radiological parameters falls below the world acceptable limits of 370 Bq/kg for Raeq; 89 nGy/h for the absorbed dose rate and 1 mSv/y annual effective dose rate for the general public; for the annual effective dose due to ingestion or inhalation of NORMS in the soil, medicinal plants and food is 0.07 mSv/y and the value is within the acceptable limit of intake; external and internal hazard index were calculated and found to have values of 0.23 Bq/kg for Hex and 0.30 Bq/kg for Hin and are lower than unity set by ICRP. Base on the radiological hazards evaluations, there is no any health risk due to radiation from the natural sources in using the roots and leaves parts of baobab plants for any purposes in the study area. Moreover, the measured soil around the study area was found to be safe and will not pose any radiation exposure to the population. Hence, the research will serve as the baseline for detection of any future released activities of related natural radionuclides especially around the consumable plants. However, effort should be made to ensure that the radiological parameters of the study area are kept as low as reasonably achievable.

Geoinformation modeling of radioactive contamination of territories on the example of mines of the “ShidGSK” mining and processing plant

The aim of the study was to model the territorial distribution and statistical assessment of migration through the trophic chain of naturally occurring radionuclides released into the environment as a result of uranium ore mining. Statistical, geoinformation and experimental research methods were used in the study. Interpolation of the results of volumetric activity of natural radionuclides in environmental components and development of spatial models of their territorial distribution were performed using the ArcGIS software; statistical processing of modelling results and development of mathematical models of migration of natural radionuclides between environmental components were performed using ArcGIS Geostatistical Analyst software. The paper substantiates the choice of the method of geostatistical modelling of the territorial distribution of volumetric activity of natural radionuclides 234U, 238U, 210Po, 210Pb, 226Ra in soils and plants, which allows modelling the values of probabilistic indicators of radioecological contamination in the absence of a sufficient array of initial actual research results. Based on the analysis of the data obtained, the methodology of mathematical modelling of migration of natural radionuclides between soil and plant parts was further developed, which will facilitate consideration of the specifics of migration of natural radionuclides through the trophic chain and help in determining the level of radioecological hazard to the environment. The developed territorial models allow one to obtain stochastic data for their further analytical processing and visualizing radioecological hazard zones. Based on the developed models, zones of increased radioecological hazard within the existing sources of radioactive contamination were identified.

РАДИОЭКОЛОГИЧЕСКАЯ ОБСТАНОВКА В РАЙОНЕ ПЛОЩАДКИ УРАНОВОГО НАСЛЕДИЯ – ШАХТА «СТЕПНАЯ» (КАЛМЫКИЯ)

Purpose: To study the radio-ecological situation on the “uranium legacy” site of the former Stepnaya mine in the Republic of Kalmykia. Material and methods: To measure the ambient dose equivalent rate (ADER), the pedestrian gamma survey method was used using a portable spectrometric complex MKC-01A Multirad-M and dosimeter-radiometer MKC-AT6101c. The activity of gamma-emitting radionuclides in soil samples was measured using a stationary gamma spectrometer from CANBERRA. The activities of 210Po and 210Pb were measured using a radiometric installation UMF-2000 following their radiochemical separation from samples. Short-term measurements of activity concentration (AC) and equivalent equilibrium activity concentration (EEAC) of radon were carried out with an aerosol alpha radiometer for radon and thoron RAA-20P2 Poisk. Doses of radiation exposure to biological objects were estimated using dose coefficients provided by ICRP Publication 136 taking into account recommendations R52.18.820-2015. Results: Gamma ADER values at the mine site vary over the range from 0.1 to 0.36 µSv/h, and on 80 % of the area these values do not exceed the background value of 0.14 µSv/h. Along the road from the mine to Narta village the ADER values do not exceed background values with exception of the area around the dam, where in a local part of this area of about 300 m2 these values reach 0.49 µSv/h. The specific activities of natural radionuclides in the soil are below the criteria for classification as solid radioactive waste (SRW). Under the certain weather conditions, radon EEAC inside the buildings on the site reaches 13 kBq/m3, and on the territory 1-1.5 kBq/m3. Ecological risk for the terrestrial biological objects under consideration (grass, soil worm, snake and mouse-like rodents) does not exceed 0.025. Conclusions: The radiation situation at the Stepnaya mine site meets the requirements of SP LKP-91, which were in force until 2020. However, in order to transfer the facility to a local government body, reclamation work should be carried out in accordance with the Federal Law “On the Transfer of Lands or Land Plots from One Category to Another” dated December 21, 2004 No. 172-FZ and GOST R 59057— 2020 «Environmental Protection. Lands. General Requirements for Reclamation of Affected Lands». Doses of exposure to biological objects do not impact significantly on morbidity, reproduction and life expectancy of terrestrial biological objects.

Symkanych О.І., Коkhan О.P., Glukh О.S., Krch K.L., Lytvyn О.V., Svatiuk N.І., Butsyak І.V. MONITORING OF RADIONUCLIDE MIGRATION IN THE BOTTOM SEDIMENTS OF THE TISA BILA RIVER' SOURCE

The regularities of distribution, migration, and accumulation of natural gamma-active nuclides 40K, uranium 238U (214Pb, 214Bi), and thorium 232Th (212Pb, 212Bi, 228Ac, 208Tl) series, as well as man-made 137Cs in the sediments of the tributary of the Tysa River (Bila Tysa), have been established. It is shown that the total content of the studied radionuclides in the bottom sediments along the entire length of the Tysa River differs slightly and is proportional to the level of its siltation. And this largely depends on many factors, in particular - the intensity of radionuclide exchange processes between soil and water, the water content in the soil, organic substances, and the morphological features of the river. Fluctuations of the total specific activity of natural gamma-active radionuclides (excluding 40K) in sediments within the range of 195.5-293.9 Bq/kg were established. The highest content of these isotopes was determined at the confluence of the White and Black Tisza. Mapping of the studied territories according to the content of 40K and 137Cs has show that the area of accumulation of gamma-active nuclides is concentrated in the lower part of the river (the point of confluence of the White and Black Tisza), and the probable causes of this phenomenon were substantiated. The analysis of the degree of connection between the content of radionuclides (238U and 232Th, 40K and 137Cs series) and the territorial factor showed that for the majority of GAN there is a zonal distribution - in the bottom sediments of the river source.
 Keywords: radionuclides; gamma-active nuclides; radioecological monitoring; bottom deposits; migration; accumulation; Cs/K content; Tysa river.

Spatial distribution of 137Cs; 40K, 226Ra, 232Th in soils of Monchegorsk city (Murmansk region)

The purpose of the study was to establish the patterns of spatial distribution of radioactivity of technogenic 137Cs and natural radionuclides 232Th, 226Ra, 40K in urban soils of Monchegorsk. Location and time of the study. Soil samples, were collected in summer 2018 in the Monchegorsk city, Murmansk region, Russia. To study the specific activity of radiocesium and natural radionuclides, soil samples were taken from topsoil (0-5 cm) at 82 sites, including 68 sites within the city territory (urban soils) and 14 sites beyond the city limits in the subtorch areas strongly affected by the Severonickel factory. Similar studies of urban soils in Monchegorsk had not been carried out previously. Methods. During expeditionary work and laboratory research, soil, radiological, and mathematical and statistical methods were used. When carrying out gamma spectrometric measurements, radionuclides 137Cs, 226Ra, 232Th and 40K were determined on a low-background semiconductor gamma spectrometer ORTEC (USA) based on a high-purity coaxial germanium detector GEM10P4–70 (HPGe) with a SBS-75 pulse signal processor and Gamma-software. The resolution of the gamma spectrometer along the 1.33 MeV line (60Co) was 1.75 keV, and the relative efficiency was 15%. Calibration and quality control of gamma spectrometric measurements was carried out using volumetric activity measurements with 1-L Marinelli vessels of different densities (RITVERZ, Russia-Germany). Main results. The values of specific activity of radionuclides in soil samples were as following: in the technogenic 137Cs up to 31.3 Bq/kg and in the subtorch soils up to 63.4 Bq/kg. Specific activity of natural radionuclides in urban soils reached to 14.2 Bq/kg for 226Ra, whereas in the subtorch soils it reached 21.6 Bq/kg. The specific activity of 232Th in urban soils reached 18.3 Bq/kg, with 17 Bq/kg registered for the subtorch soils. As for 40K, its specific activity reached 498 Bq/kg in the urban soils and 317 Bq/kg. Conclusion. The gamma survey of the Monchegorsk territory did not reveal any anomaly in radiation. The dose rate of gamma radiation in the city does not exceed 0.074 μSv/hour, which is less than the values elsewhere in Russia, ranging from 0.04 to 0.20 μSv/hour. The obtained data about specific activity of technogenic 137Cs and natural radionuclides 232Th, 226Ra, 40K in the Monchegorsk soils are typical for the Murmansk region.

Изучение особенностей накопления искусственных и естественных радионуклидов в корнях лопуха большого Arctium lappa L.

The Voronezh region has traditionally been the most significant area for crop production and agriculture. However, the development of mineral resources, the implementation of chemical fertilisers in agriculture, and the consequences of the Chernobyl accident have highlighted the necessity to ensure the food industry has access to safe and effective plant raw materials. The use of low-quality plant raw materials and products derived from them represents a significant source of exposure to various ecotoxicants, including radionuclides, which can enter the human body. Objective: to examine the accumulation of the most significant artificial and natural radionuclides in the roots of a large burdock plant, harvested in different territories of the Voronezh region, with a view to determining the extent of the anthropogenic impact. Materials and methods. Under experimental conditions, the specific activity of the main long-lived artificial radioisotopes (cesium-137, strontium-90) and naturally occurring radionuclides (thorium-232, potassium-40, radium-226) on a spectrometer (RADEK MKGB-01 radiometer) was determined in samples of the upper layers of soils and roots of large burdock. Results. All of the studied samples of large burdock roots, which had been prepared in natural and artificial phytocenoses in the Voronezh region, met the existing radiation safety requirements (first group). With an increase in the specific activity of strontium-90, cesium-137, thorium-232, potassium-40, radium-226 in the soil, there was an accompanying increase in the specific activity of these radionuclides in the roots of a large burdock. Correlation analysis of the specific activity of artificial and natural radionuclides in the soil and roots of large burdock revealed a highly significant relationship between these numerical indicators, thereby confirming the predominant transposed pollution. Conclusion. The accumulation patterns in roots of large burdock, naturally occurring and anthropogenic radionuclides are described by mathematical dependencies, with an accuracy of approximation that is as high as possible.

Radiometric measurements at uranium mined-out sitesbefore their reclamation

The article presents the results of radiometric measurements of various indicators for objects at uranium mined-out sites before their reclamation: specific activity of natural radionuclides, total effective activity, specific alpha activity, pH value of water extract, exposure dose rate of gamma radiation, equivalent equilibrium volumetric activity of radon, content of long-lived radioactive aerosols in the air, and density of radon molasses. The results were compared with the regulatory requirements established for both the population and personnel. The article shows that the radiation indicators at a man-made object differ from the background values for natural objects, i.e., uranium mining is a source of radioactive pollution of the environmen.

Estimation of radioactivity in soil and drinking water samples from Northern Gulbarga District of Karnataka.

The gamma activity of the radionuclides238U, 232Th and 40K were measured in surface soil samples collected from 40 villages of Aland, Afzalpur, Ganaghapur and Kamalapur talukas of Northern Gulbarga district, Karnataka. The gamma activity of natural radionuclides were measured using 4" × 4" NaI (Tl) scintillation detector, the spectrum was analysed using a PC based 1k MCA (winTMCA 32 scinti SPEC) and the 222Rn activity concentrations in drinking water were determined by the Emanometry method. The activity of 238U, 232Th and 40K was found to be in the range from 14.3±0.3 to 64.5±6.1, 15.4±0.2 to 95.0±4.1 and 21±06 to 323±09 Bqkg-1, respectively. Outdoor AED from 0.023 to 0.07 mSvy-1 and all the radiological hazards indices were well within the safe limit. The 222Rn activity in ground water is found to vary from 1.11 to 66.6 Bql-1. The total annual effective doses due to 222Rn inhalation and ingestion range from 3.02 to 181.81μSvy-1, respectively, with an average value of 77.18μSvy-1.

Natural radioactivity measurements and evaluation of radiological hazards in the soil of an iron beneficiation plant in China

The specific activities of natural radionuclides, 232Th, 226Ra, and 40K, in a Chinese iron beneficiation plant and surrounding soil were analyzed with the high purity germanium gamma (HPGe) spectrometer in this study. Average specific activities of 238U, 232Th, 226Ra and 40K lower than the Chinese averages. To assess radiation impact, various indicators, radium equivalent index (Rae q), absorbed dose rate (DR), annual effective dose (AED), excess lifetime cancer risk (ELCR), external hazard index (Hex), internal hazard index (Hin) and activity utilization index (AUI), were calculated. Mean values were below international limits, indicating no significant health hazards for the local population. Statistical analyses, including skewness and kurtosis calculations, along with techniques like frequency distribution, Pearson's correlation analysis, box plots and cluster analysis, were applied to comprehensively assess distribution patterns and interrelationships among radiological parameters. In summary, there are no potential health hazards associated with the soil in the study region for people.

Soil-to-organic Sangyod rice grain transfer factors (TF values) of natural and anthropogenic radionuclides in Phatthalung province, Thailand

The specific activities of natural (40K 226Ra and 232Th) and anthropogenic (137Cs) radionuclides in paddy soil and organic Sangyod rice grain were measured and analyzed in this study with an aim to determine the soil-to-organic Sangyod rice grain transfer factors (TF values) of all required radionuclides in Don Pradu sub-district, Pak Phayun district in Phatthalung province in the south of Thailand. The high purity germanium (HPGe) detector and gamma-ray spectrometry analysis system which were installed and used in advanced laboratory at TINT were used to conduct experiments to measure and analyze of all required radionuclides in this research. The average concentrations of 40K 226Ra, 232Th, and 137Cs in paddy soil were found to have a value of 657.30 ± 23.03, 180.01 ± 4.39, 162.02 ± 3.84 and < 1.81 Bq/kg respectively while in organic Sangyod rice grain, their values were 24.11 ± 2.01, 0.28 ± 0.07, 0.17 ± 0.06 and 0.10 ± 0.03 Bq/kg respectively. For TF values were calculated and found to be 0.037, 0.002, 0.001, and 0.055 for 40K, 226Ra, 232Th, and 137Cs, respectively. Furthermore, four important radiological hazard indices which are gamma-absorbed dose rate (D), radium equivalent activity (Raeq), external hazard index (Hex) and annual external effective dose rate (AEDout) were also evaluated by using the average values of 40K, 226Ra and 232Th. In addition, by using the AEDout value, the excess lifetime cancer risk (ELCR (outdoor)) in paddy soil in the study area would be also studied, evaluated and presented. Moreover, the evaluated TF values of required radionuclides were higher than that reported by the International Atomic Energy Agency (IAEA) in 2010 but the values were much lower than those in the study in Malaysia.

Radiation risk assessment of quarry pit soil as construction material in Abeokuta, Nigeria: implications for environmental and public health

ABSTRACT Environmental and health risks posed by radionuclides in quarry pit soils are of great concern in environmental health monitoring. The current investigation was aimed at determining the natural radionuclide activity concentration (in Bq kg–1) of the understudied quarry pit granules used as construction materials. The collection and preparation of pit soil samples from Abeokuta quarry sites were done using standard methods, analysis of radiological parameters was carried out using hyperpure germanium (HPGe) spectrometer. Specific activity concentrations of 226Ra, 232Th, and 40K were measured. The values obtained were greater than the world weighted average of 35, 30, and 400 Bq kg–1 for 226Ra, 232Th, and 40K, respectively. The absorbed dose, the annual effective dose, and the radium equivalent were calculated and demonstrated significant values. The radionuclide content of the samples is relatively high and the use of pit soils as a building material, therefore, raises radiological concerns for dwellers in this area and requires periodic monitoring and undergoing a radiation protection program.